Готові списки джерел за темами / Ultrafast Raman Spectroscopy

Добірка наукової літератури з теми "Ultrafast Raman Spectroscopy"

Автор: Grafiati
Опубліковано: 6 вересня 2023

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Статті в журналах з теми "Ultrafast Raman Spectroscopy"

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Umapathy, Siva, Adithya Lakshmanna, and Babita Mallick. "Ultrafast Raman loss spectroscopy." Journal of Raman Spectroscopy 40, no. 3 (March 2009): 235–37. http://dx.doi.org/10.1002/jrs.2199.

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2

Keller, Emily L., Nathaniel C. Brandt, Alyssa A. Cassabaum, and Renee R. Frontiera. "Ultrafast surface-enhanced Raman spectroscopy." Analyst 140, no. 15 (2015): 4922–31. http://dx.doi.org/10.1039/c5an00869g.

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3

Lindley, Matthew, Kotaro Hiramatsu, Hayate Nomoto, Fukashi Shibata, Tsuyoshi Takeshita, Shigeyuki Kawano, and Keisuke Goda. "Ultrafast Simultaneous Raman-Fluorescence Spectroscopy." Analytical Chemistry 91, no. 24 (November 27, 2019): 15563–69. http://dx.doi.org/10.1021/acs.analchem.9b03563.

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Qiu, Xueqiong, Xiuting Li, Kai Niu, and Soo-Y. Lee. "Inverse Raman bands in ultrafast Raman loss spectroscopy." Journal of Chemical Physics 135, no. 16 (October 28, 2011): 164502. http://dx.doi.org/10.1063/1.3653940.

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5

Suemoto, Tohru, Koichiro Tanaka, and Hideyuki Ohtake. "Ultrafast electronic raman spectroscopy in semiconductors." Progress in Crystal Growth and Characterization of Materials 33, no. 1-3 (January 1996): 57–63. http://dx.doi.org/10.1016/0960-8974(96)83613-8.

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Gruenke, Natalie L., M. Fernanda Cardinal, Michael O. McAnally, Renee R. Frontiera, George C. Schatz, and Richard P. Van Duyne. "Ultrafast and nonlinear surface-enhanced Raman spectroscopy." Chemical Society Reviews 45, no. 8 (2016): 2263–90. http://dx.doi.org/10.1039/c5cs00763a.

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RAI, N. K., A. Y. LAKSHMANNA, V. V. NAMBOODIRI, and S. UMAPATHY. "Basic principles of ultrafast Raman loss spectroscopy#." Journal of Chemical Sciences 124, no. 1 (January 2012): 177–86. http://dx.doi.org/10.1007/s12039-012-0214-8.

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Petrich, J. W., and J. L. Martin. "Ultrafast absorption and Raman spectroscopy of hemeproteins." Chemical Physics 131, no. 1 (March 1989): 31–47. http://dx.doi.org/10.1016/0301-0104(89)87079-x.

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Ferrante, Carino, Alessandra Virga, Lara Benfatto, Miles Martinati, Domenico De Fazio, Ugo Sassi, Claudia Fasolato, et al. "Raman spectroscopy of graphene under ultrafast laser excitation." EPJ Web of Conferences 205 (2019): 05003. http://dx.doi.org/10.1051/epjconf/201920505003.

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Анотація:
The out-of-equilibrium Raman response of graphene is addressed by pulsed laser excitation. Phonon spectrum is rationalized by revisiting the electron-phonon picture in the light of a transient broadening of the Dirac cone.
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Rohringer, Nina. "X-ray Raman scattering: a building block for nonlinear spectroscopy." Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences 377, no. 2145 (April 2019): 20170471. http://dx.doi.org/10.1098/rsta.2017.0471.

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Анотація:
Ultraintense X-ray free-electron laser pulses of attosecond duration can enable new nonlinear X-ray spectroscopic techniques to observe coherent electronic motion. The simplest nonlinear X-ray spectroscopic concept is based on stimulated electronic X-ray Raman scattering. We present a snapshot of recent experimental achievements, paving the way towards the goal of realizing nonlinear X-ray spectroscopy. In particular, we review the first proof-of-principle experiments, demonstrating stimulated X-ray emission and scattering in atomic gases in the soft X-ray regime and first results of stimulated hard X-ray emission spectroscopy on transition metal complexes. We critically asses the challenges that have to be overcome for future successful implementation of nonlinear coherent X-ray Raman spectroscopy. This article is part of the theme issue ‘Measurement of ultrafast electronic and structural dynamics with X-rays’.
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Дисертації з теми "Ultrafast Raman Spectroscopy"

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Pestov, Dmitry Sergeyevich. "Detection of bacterial endospores by means of ultrafast coherent raman spectroscopy." Texas A&M University, 2008. http://hdl.handle.net/1969.1/85958.

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This work is devoted to formulation and development of a laser spectroscopic technique for rapid detection of biohazards, such as Bacillus anthracis spores. Coherent anti-Stokes Raman scattering (CARS) is used as an underlying process for active retrieval of species-specific characteristics of an analyte. Vibrational modes of constituent molecules are Raman-excited by a pair of ultrashort, femtosecond laser pulses, and then probed through inelastic scattering of a third, time-delayed laser field. We first employ the already known time-resolved CARS technique. We apply it to the spectroscopy of easy-to-handle methanol-water mixtures, and then continue building our expertise on solutions of dipicolinic acid (DPA) and its salts, which happen to be marker molecules for bacterial spores. Various acquisition schemes are evaluated, and the preference is given to multi-channel frequency-resolved detection, when the whole CARS spectrum is recorded as a function of the probe pulse delay. We demonstrate a simple detection algorithm that manages to differentiate DPA solution from common interferents. We investigate experimentally the advantages and disadvantages of near-resonant probing of the excited molecular coherence, and finally observe the indicative backscattered CARS signal from DPA and NaDPA powders. The possibility of selective Raman excitation via pulse shaping of the preparation pulses is also demonstrated. The analysis of time-resolved CARS experiments on powders and B. subtilis spores, a harmless surrogate for B. anthracis, facilitates the formulation of a new approach, where we take full advantage of the multi-channel frequency-resolved acquisition and spectrally discriminate the Raman-resonant CARS signal from the background due to other instantaneous four-wave mixing (FWM) processes. Using narrowband probing, we decrease the magnitude of the nonresonant FWM, which is further suppressed by the timing of the laser pulses. The devised technique, referred to as hybrid CARS, leads to a single-shot detection of as few as 104 bacterial spores, bringing CARS spectroscopy to the forefront of potential candidates for real-time biohazard detection. It also gives promise to many other applications of CARS, hindered so far by the presence of the overwhelming nonresonant FWM background, mentioned above.
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Rohrdanz, Mary A. "Intermolecular communication via lattice phonons, probed by ultrafast spectroscopy /." view abstract or download file of text, 2005. http://wwwlib.umi.com/cr/uoregon/fullcit?p3190543.

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Анотація:
Thesis (Ph. D.)--University of Oregon, 2005.
Typescript. Includes vita and abstract. Includes bibliographical references (leaves 79-80). Also available for download via the World Wide Web; free to University of Oregon users.
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Barlow, Aaron M. "Spectral Distortions & Enhancements In Coherent Anti-Stokes Raman Scattering Hyperspectroscopy." Thesis, Université d'Ottawa / University of Ottawa, 2015. http://hdl.handle.net/10393/32388.

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Coherent anti-Stokes Raman scattering microscopy is a versatile technique for label-free imaging and spectroscopy of systems of biophysical interest. Due to the coherent nature of the generated signals, CARS images and spectra can often be difficult to interpret. In this thesis, we document how distortions and enhancements can be produced in CARS hyperspectroscopy as a result of the instrument, geometrical optical effects, or unique molecular states, and discuss how these effects may be suppressed or exploited in various CARS applications.
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Odhner, Johanan. "INVESTIGATIONS OF TEMPORAL RESHAPING DURING FILAMENTARY PROPAGATION WITH APPLICATION TO IMPULSIVE RAMAN SPECTROSCOPY." Diss., Temple University Libraries, 2012. http://cdm16002.contentdm.oclc.org/cdm/ref/collection/p245801coll10/id/196129.

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Анотація:
Chemistry
Ph.D.
Femtosecond laser filamentation in gaseous media is a new source of broadband, ultrashort radiation that has the potential for application to many fields of research. In this dissertation filamentation is studied with a view to understanding the underlying physics governing the formation and propagation dynamics of filamentation, as well as to developing a method for vibrational spectroscopy based on the filament-induced impulsive vibrational excitation of molecules in the filamentation region. In pursuit of a better understanding of the underlying physical processes driving filamentation, the development of a new method for characterizing high intensity ultrashort laser pulses is presented, wherein two laser beams generate a transient grating in a noble gas, causing the pulse undergoing filamentation to diffract from the grating. Measuring the spectrum as a function of time delay between the filament and probe beams generates a spectrogram that can be inverted to recover the spectral and temporal phase and amplitude of the filamentary pulse. This technique enables measurement of the filamentary pulse in its native environment, offering a window into the pulse dynamics as a function of propagation distance. The intrinsic pulse shortening observed during filamentation leads to the impulsive excitation of molecular vibrations, which can be used to understand the dynamics of filamentation as well. Combined measurements of the longitudinally-resolved filament Raman spectrum, power spectrum, and fluorescence intensity confirm the propagation dynamics inferred from pulse measurements and show that filamentation provides a viable route to impulsive vibrational spectroscopy at remote distances from the laser source. The technique is applied to thermometry in air and in flames, and an analytical expression is derived to describe the short-time dynamics of the rovibrational wave-packet dispersion experienced by diatomic molecules in the wave of the filament. It is found that no energy is initially partitioned into the distribution of rovibrational states during the filamentation process. Filament-assisted impulsive stimulated Raman spectroscopy of more complex systems is also performed, showing that filament-assisted vibrational measurements can be used as an analytical tool for gas phase measurements and has potential for use as a method for standoff detection. Finally, a study of the nonlinear optical mechanisms driving the filamentation process is conducted using spectrally-resolved pump-probe measurements of the transient birefringence of air. Comparison to two proposed theories shows that a newly described effect, ionization grating-induced birefringence, is largely responsible for saturation and sign inversion of the birefringence at 400 nm and 800 nm, while the magnitude of contributions described by a competing theory that relies on negative terms in the power series expansion of the bound electron response remain undetermined.
Temple University--Theses
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Wachsmann-Hogiu, Sebastian. "Vibronic coupling and ultrafast electron transfer studied by picosecond time resolved resonance Raman and CARS spectroscopy." Doctoral thesis, [S.l. : s.n.], 2000. http://deposit.ddb.de/cgi-bin/dokserv?idn=960830898.

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Zoubir, Arnaud. "TOWARDS DIRECT WRITING OF 3-D PHOTONIC CIRCUITS USING ULTRAFAST LASERS." Master's thesis, University of Central Florida, 2004. http://digital.library.ucf.edu/cdm/ref/collection/ETD/id/3907.

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Анотація:
The advent of ultrafast lasers has enabled micromachining schemes that cannot be achieved by other current techniques. Laser direct writing has emerged as one of the possible routes for fabrication of optical waveguides in transparent materials. In this thesis, the advantages and limitations of this technique are explored. Two extended-cavity ultrafast lasers were built and characterized as the laser sources for this study, with improved performance over existing systems. Waveguides are fabricated in oxide glass, chalcogenide glass, and polymers, these being the three major classes of materials for the telecommunication industry. Standard waveguide metrology is performed on the fabricated waveguides, including refractive index profiling and mode analysis. Furthermore, a finite-difference beam propagation method for wave propagation in 3D-waveguides is proposed. The photo-structural modifications underlying the changes in the material optical properties after exposure are investigated. The highly nonlinear processes of the light/matter interaction during the writing process are described using a free electron model. UV/visible absorption spectroscopy, photoluminescence spectroscopy and Raman spectroscopy are used to assess the changes occurring at the atomic level. Finally, the impact of laser direct writing on nonlinear waveguide applications is discussed.
Ph.D.
Other
Optics and Photonics
Optics
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7

Alexeev, Evgeny. "Hot-carrier luminescence in graphene." Thesis, University of Exeter, 2015. http://hdl.handle.net/10871/18231.

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In this thesis, the effect of the sample properties on the characteristics of the hot carrier luminescence in graphene is investigated. The present work focuses on the two main issues described below. The first issue is the modification effects of near-infrared pulsed laser excitation on graphene. For excitation fluences several orders of magnitude lower than the optical damage threshold, the interaction with ultrafast laser pulses is found to cause a stable change in the properties of graphene. This photomodification also results in a decrease of the hot photoluminescence intensity. The detailed analysis shows that ultrafast photoexcitation leads to an increase in the local level of hole doping, as well as a change in the mechanical strain. The variation of doping and strain are linked with the enhanced adsorption of atmospheric oxygen caused by the distortion of the graphene surface. These findings demonstrate that ultrashort pulsed excitation can be invasive even if a relatively low laser power is used. Secondly, the variation of the hot photoluminescence intensity with the increasing charge carrier density in graphene is investigated. The electro-optical measurements performed using graphene field-effect transistors show a strong dependence of the photoluminescence intensity on the intrinsic carrier concentration. The emission intensity has a maximum value in undoped graphene and decreases with the increasing doping level. The theoretical calculations performed using a refined two-temperature model suggest that the reduction of the photoluminescence intensity is caused by an increase in the hot carrier relaxation rate. The modification of the carrier relaxation dynamics caused by photoinduced doping is probed directly using the two-pulse correlation measurements. The discovered sensitivity of the hot photoluminescence to the intrinsic carrier concentration can be utilised for spatially-resolved measurements of the Fermi level position in graphene samples, offering an advantage in resolution and speed.
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8

Cunning, Benjamin V. "An Exploration in Nano-Carbons: Bulk Graphene, Ultrafast Physics, Carbon-Nanotubes." Thesis, Griffith University, 2013. http://hdl.handle.net/10072/367408.

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Carbon nanomaterials encompass the newly discovered allotropes of carbon with at least one of its spatial dimensions on the order of a few nanometers. The physical properties of these nanomaterials differ substantially from the bulk carbon allotropes such as graphite and diamond. Of these nanomaterials, single-walled carbon nanotubes (SWNTs) and graphene have illicited much of the attention owing to their unique and attractive electronic, optical, thermal, and mechanical properties which have found numerous applications in emerging technologies. Raman spectroscopy is an invaluable technique in the characterisation of these materials as it allows for both a rapid and non-destructive analysis of these nanomaterials. We examined a number of methodologies for the synthesis of “bulk” quantities of graphene, and using Raman spectroscopy, analysed these samples to critically assess their crystalline quality, finding that many of the bulk methods produce material which could be considered as amorphous, rather than crystalline, having crystalline domain sizes less than a few nanometers. An important finding, as many of graphene’s unique properties are severely attenuated with increasing defects. Using these findings, we utilised the non-linear optical properties of graphene, namely its property of saturable absorption (wherby its light absorption decreases with increasing light intensitiy), to create saturable absorber mirrors (SAMs) which are used in the mode-locking of lasers creating pulses of light on the order femtoseconds with very high peak power. We developed graphene SAMs from the bulk synthetic methods which we found to have good crystalline quality and attempted to use them to passively mode-lock an Er:fiber laser operating at t 1560 nm. We successfully mode-locked the laser with graphene produced from the ultrasound induced exfoliation of graphite generating pules of sub-200 fs duration with low nonsaturable loss, and large modulation depths allowing use in low-gain lasers.
Thesis (PhD Doctorate)
Doctor of Philosophy (PhD)
School of Biomolecular and Physical Sciences
Science, Environment, Engineering and Technology
Full Text
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Dantas, Willian Francisco Cordeiro 1989. "Análise de Franck-Condon para pireno suportado em filmes poliméricos e estudo comparativo entre as espectroscopias Raman nos domínios da frequência e do tempo." [s.n.], 2015. http://repositorio.unicamp.br/jspui/handle/REPOSIP/249162.

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Анотація:
Orientador: René Alfonso Nome Silva
Dissertação (mestrado) - Universidade Estadual de Campinas, Instituto de Química
Made available in DSpace on 2018-08-27T06:54:35Z (GMT). No. of bitstreams: 1 Dantas_WillianFranciscoCordeiro_M.pdf: 2446830 bytes, checksum: a6ef77a86d65956736e20e7c5e22ff59 (MD5) Previous issue date: 2015
Resumo: A espectroscopia vibracional de femtossegundos da vizinhança é ideal para caracterizar os movimentos moleculares da vizinhança acoplados com o sistema eletrônico captador de luz. No caso dos movimentos nucleares intramoleculares, isto pode ser realizado tanto por infravermelho quanto por Raman, ambos de femtossegundos. No caso de movimentos intermoleculares, a dinâmica de femtossegundos somente pode ser caracterizada com experimento Raman coerente, e, por essa razão, é importante sabermos qual é o comportamento do clorofórmio em um experimento de femtossegundo. Dessa forma, pode-se realizar a comparação entre os dados experimentais e teóricos e concluir se o comportamento observado experimentalmente é o mesmo que o esperado. Este trabalho explora a análise de Franck-Condon para os espectros de emissão do pireno com dependência da temperatura. Assume-se que uma progressão vibrônica de bandas no formato de Lorenzianas pode representar o formato das bandas de emissão do fluoróforo. Consequentemente, é possível obter alguns parâmetros, como a largura de linha das bandas obtidas, as intensidades relativas dos picos observados (valores que são utilizados para encontrar os fatores de Huang-Rhys), a variação do comprimento de onda de emissão com o aumento da temperatura e a área integrada dos espectros
Abstract: The femtosecond vibrational spectroscopy of the neighborhood is ideal to characterize the molecular movements of the neighborhood coupled with the electronics pickup light. In the case of intra-molecular nuclear movements, this can be accomplished either by infrared and Raman both femtosecond. In the case of intermolecular movements, the dynamics of femtosecond can only be characterized with coherent Raman experiment, and so it is important to know the behavior of chloroform in a femtosecond experiment. Thus, it is possible to make a comparison between experimental and theoretical data and conclude that the observed experimentally is the same behavior expected. This work explores the Franck-Condon analysis for the emission spectra of pyrene in dependence on temperature. It is assumed that a vibronic bands in the progression Lorenzianas shape may represent the format of fluorophore emission bands. Consequently, it is possible to obtain some parameters such as the line width of the bands obtained, the relative intensities of the observed peaks (values that are used to find the Huang-Rhys factors), the variation of emission wavelength with increasing temperature and the integrated area of the spectra
Mestrado
Físico-Química
Mestre em Química
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10

Challa, Jagannadha Reddy. "Electronic and Vibrational Dynamics of Heme Model Compounds-An Ultrafast Spectroscopic Study." Case Western Reserve University School of Graduate Studies / OhioLINK, 2007. http://rave.ohiolink.edu/etdc/view?acc_num=case1181323422.

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Книги з теми "Ultrafast Raman Spectroscopy"

1

D, Fayer Michael, ed. Ultrafast infrared and raman spectroscopy. New York: Marcel Dekker, 2001.

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2

Milne, Christopher Jackson. Diffractive-optics based fifth-order Raman spectroscopy of ultrafast liquid dynamics. Ottawa: National Library of Canada, 2001.

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3

Fayer, M. D. Ultrafast Infrared and Raman Spectroscopy. Taylor & Francis Group, 2001.

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Fayer. Ultrafast Infrared and Raman Spectroscopy. Taylor & Francis Group, 2001.

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Fayer. Ultrafast Infrared and Raman Spectroscopy. Taylor & Francis Group, 2001.

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Fayer. Ultrafast Infrared and Raman Spectroscopy. Taylor & Francis Group, 2001.

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Fayer. Ultrafast Infrared and Raman Spectroscopy. Taylor & Francis Group, 2001.

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8

Fayer. Ultrafast Infrared and Raman Spectroscopy. Taylor & Francis Group, 2001.

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9

Fayer, Michael D. Ultrafast Infrared and Raman Spectroscopy (Practical Spectroscopy). CRC, 2001.

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10

Kubarych, Kevin Joel. Heterodyne detected fifth-order Raman spectroscopy of ultrafast liquid dyamics. 2003, 2003.

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Частини книг з теми "Ultrafast Raman Spectroscopy"

1

Zinth, W., and W. Kaiser. "Ultrafast Coherent Raman Spectroscopy." In Springer Proceedings in Physics, 166–74. Berlin, Heidelberg: Springer Berlin Heidelberg, 1987. http://dx.doi.org/10.1007/978-3-642-72758-0_12.

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2

Milne, C. J., Y. L. Li, T. l. C. Jansen, L. Huang, and R. J. D. Miller. "Fifth-order Raman spectroscopy: Liquid benzene." In Ultrafast Phenomena XV, 297–99. Berlin, Heidelberg: Springer Berlin Heidelberg, 2007. http://dx.doi.org/10.1007/978-3-540-68781-8_96.

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3

Graener, H., R. Zürl, and M. Hofmann. "Spontaneous Raman Scattering with Picosecond Pulses." In Ultrafast Processes in Spectroscopy, 101–4. Boston, MA: Springer US, 1996. http://dx.doi.org/10.1007/978-1-4615-5897-2_22.

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4

Kulagin, I. A., and T. Usmanov. "Essentially Transient Raman Amplification in Excited Medium." In Ultrafast Processes in Spectroscopy, 383–86. Boston, MA: Springer US, 1996. http://dx.doi.org/10.1007/978-1-4615-5897-2_86.

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5

Khalil, M., O. Golonzka, N. Demirdoven, and A. Tokrnakoff. "Phase-sensitive detection for polarizationselective femtosecond Raman spectroscopy." In Ultrafast Phenomena XII, 545–47. Berlin, Heidelberg: Springer Berlin Heidelberg, 2001. http://dx.doi.org/10.1007/978-3-642-56546-5_160.

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6

Tanaka, Satoshi, and Shaul Mukamel. "Coherent Femtosecond X-ray Raman Spectroscopy of Molecules." In Ultrafast Phenomena XIII, 63–65. Berlin, Heidelberg: Springer Berlin Heidelberg, 2003. http://dx.doi.org/10.1007/978-3-642-59319-2_19.

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Morrissey, F. X., and S. L. Dexheimer. "Vibrational spectroscopy of nonlinear excitations via excited-state resonant impulsive Raman spectroscopy." In Ultrafast Phenomena XV, 240–42. Berlin, Heidelberg: Springer Berlin Heidelberg, 2007. http://dx.doi.org/10.1007/978-3-540-68781-8_77.

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Klebniczki, J., J. Seres, and J. Hebling. "Resonance Raman Scattering of Laser Dyes in a Travelling Wave Amplifier." In Ultrafast Processes in Spectroscopy, 397–400. Boston, MA: Springer US, 1996. http://dx.doi.org/10.1007/978-1-4615-5897-2_90.

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Paskover, Yuri, and Yehiam Prior. "Single-Shot Time Resolved Coherent Anti-Stokes Raman Spectroscopy." In Ultrafast Phenomena XV, 353–55. Berlin, Heidelberg: Springer Berlin Heidelberg, 2007. http://dx.doi.org/10.1007/978-3-540-68781-8_114.

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Kelley, Anne Myers, and Lian C. T. Shoute. "Resonance Hyper-Raman Spectroscopy of Organic Nonlinear Optical Chromophores." In Ultrafast Phenomena XV, 519–21. Berlin, Heidelberg: Springer Berlin Heidelberg, 2007. http://dx.doi.org/10.1007/978-3-540-68781-8_168.

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Тези доповідей конференцій з теми "Ultrafast Raman Spectroscopy"

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Mier, L., Y. Min, E. O. Danilov, A. J. Epstein, T. L. Gustafson, P. M. Champion, and L. D. Ziegler. "Ultrafast Vibrational Spectroscopy of Perylene Diimide Complexes." In XXII INTERNATIONAL CONFERENCE ON RAMAN SPECTROSCOPY. AIP, 2010. http://dx.doi.org/10.1063/1.3482517.

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2

Kapteyn, Henry, Margaret Murnane, P. M. Champion, and L. D. Ziegler. "Molecular Dynamics Probed by Ultrafast Coherent X-Rays." In XXII INTERNATIONAL CONFERENCE ON RAMAN SPECTROSCOPY. AIP, 2010. http://dx.doi.org/10.1063/1.3482307.

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3

Milne, C. J., Y. L. Li, T. l. C. Jansen, L. Huang, and R. J. D. Miller. "Fifth-order Raman spectroscopy: Liquid benzene." In International Conference on Ultrafast Phenomena. Washington, D.C.: OSA, 2006. http://dx.doi.org/10.1364/up.2006.mi17.

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4

Palese, S., J. T. Buontempo, Y. Tanimura, S. Mukamel, R. J. D. Miller, and W. T. Lotshaw. "Femtosecond Two-Dimensional Raman Spectroscopy of Liquid Water." In International Conference on Ultrafast Phenomena. Washington, D.C.: Optica Publishing Group, 1994. http://dx.doi.org/10.1364/up.1994.wc.21.

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Анотація:
Critical to the understanding of condensed phase reaction dynamics is the understanding of a solvent's response to and influence on the system dynamics. Although models of a solvent's vibrational and orientational dynamics can be tested against infrared and Raman studies of the neat solvent, thus far this has not proven fruitful because the influence of nuclear dynamics on infrared absorption, optical Kerr effect, spontaneous Raman and CARS spectra is usually masked by inhomogeneous broadening. However, valuable information about the solvent nuclear dynamics can be extracted from nonlinear spectroscopies such as infrared and Raman echoes. Using the formalism of Tanimura and Mukamel,1 we have calculated the 3rd, 5th, and 7th order Raman spectra for liquid water employing a multimode Brownian oscillator model to represent the water modes. This model is expected to be appropriate for liquid water because it accounts for nuclear dynamics occurring on a finite time scale, extrapolating continuously between the limiting cases of homogeneous and inhomogeneous nuclear dephasing.
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5

Kliewer, Christopher. "Coherent Raman imaging for combustion sensing." In Ultrafast Nonlinear Imaging and Spectroscopy IV, edited by Zhiwen Liu. SPIE, 2018. http://dx.doi.org/10.1117/12.2239333.

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6

Mallick, Babita, Siva Umapathy, P. M. Champion та L. D. Ziegler. "Ultrafast Raman Loss Study of Excited State Evolution of α -terthiophene". У XXII INTERNATIONAL CONFERENCE ON RAMAN SPECTROSCOPY. AIP, 2010. http://dx.doi.org/10.1063/1.3482625.

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7

Potma, Eric O., and John Kenison. "Coherent Raman scattering at interfaces (Conference Presentation)." In Ultrafast Nonlinear Imaging and Spectroscopy VI, edited by Zhiwen Liu, Demetri Psaltis, and Kebin Shi. SPIE, 2018. http://dx.doi.org/10.1117/12.2322636.

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8

Cocking, Alexander, Corey Janisch, Steven H. Huang, Lan Yang, and Zhiwen Liu. "Raman sensing in optical microresonantors (Conference Presentation)." In Ultrafast Nonlinear Imaging and Spectroscopy IV, edited by Zhiwen Liu. SPIE, 2016. http://dx.doi.org/10.1117/12.2238347.

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9

Shi, Lingyan. "Raman imaging of metabolic activities in brain." In Ultrafast Nonlinear Imaging and Spectroscopy VIII, edited by Zhiwen Liu, Demetri Psaltis, and Kebin Shi. SPIE, 2020. http://dx.doi.org/10.1117/12.2571112.

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10

Bartels, Randy A., Sandro Heuke, Siddharth Sivankutty, Camille Scotté, Patrick Stockton, Anne Sentenac, and Hervé Rigneault. "Spatial frequency spontaneous and nonlinear Raman microscopy." In Ultrafast Nonlinear Imaging and Spectroscopy VIII, edited by Zhiwen Liu, Demetri Psaltis, and Kebin Shi. SPIE, 2020. http://dx.doi.org/10.1117/12.2571276.

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