Дисертації з теми "Covalent Interactions"
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Yang, Lixu. "Non-covalent interactions in solution." Thesis, University of Edinburgh, 2013. http://hdl.handle.net/1842/8097.
Повний текст джерелаCockroft, Scott L. "Understanding non-covalent interactions." Thesis, University of Sheffield, 2006. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.434497.
Повний текст джерелаBayach, Imene. "Non-covalent interactions in natural products." Thesis, Limoges, 2014. http://www.theses.fr/2014LIMO0050/document.
Повний текст джерелаNatural polyphenols form non-covalent complexes in which π-stacking and H-bonding play a key stabilizing role. The dispersion-corrected DFT calculations have paved the way towards reliable description of aggregation processes of natural products. In this work, these methods are applied at i) understanding of stereo- and regio-selective oligostilbenoids biosynthesis; ii) predicting natural antioxidant aggregation within lipid bilayer membrane, which may allow rationalizing the synergism of vitamin E, vitamin C and polyphenols in their antioxidant action; and iii) modulating optical properties of chalcone derivatives
Hubbard, Thomas A. "Non-covalent interactions in lubricant chemistry." Thesis, University of Edinburgh, 2015. http://hdl.handle.net/1842/15935.
Повний текст джерелаSIRTORI, F. RICCARDI. "STUDY OF COVALENT AND NON COVALENT INTERACTIONS OF BIOPOLYMER BY MASS SPECTROMETRY." Doctoral thesis, Università degli Studi di Milano, 2010. http://hdl.handle.net/2434/150205.
Повний текст джерелаComí, Bonachí Marc. "Biobased polyurethanes with tunable properties through covalent and non-covalent approaches." Doctoral thesis, Universitat Rovira i Virgili, 2017. http://hdl.handle.net/10803/454764.
Повний текст джерелаEsta tesis está dirigida específicamente al desarrollo de poliuretanos (PU)s funcionalizados en la cadena lateral (FPU)s, sintetizados a partir de dioles funcionales que provienen de ácidos grasos y dos diisocianats diferentes; el diisocianato de isoforona (IPDI) y el diisocianato de hexametileno (HDI). Estos nuevos FPUs presentan una amina terciaria y grupos alquilo, alilo, propargilo o la combinación de éstos en posiciones de cadena lateral. Posteriormente los FPUs se modifican mediante dos mecanismos de post-polimerización basados en enlaces covalentes o en enlaces no covalentes.En el primer caso, se llevan a cabo una serie de reacciones fotoiniciadas de acoplamiento tiol-eno/ino entre el grupo alilo y propargilo que presentan los FPUs (formados a partir de IPDI), y tioglicerol. Los hidroxi-PUs obtenidos, exhiben una mejora de su carácter hidrófilo. Alternativamente, los FPUs que contienen sólo una amina terciaria como grupo funcional situado en la cadena lateral del PU, se mezclan con diferentes ácidos carboxílicos mediante una reacción de ácido base. Los PUs supramoleculares resultantes (SPU)s se caracterizan por espectroscopia para verificar la presencia de enlaces iónicos de hidrógeno que unen las cadenas de PU formando interacciones físicas. Además, se demuestra la correlación existente entre la estructura química y las propiedades térmicas y mecánicas de los materiales sintetizados. Estos materiales presentan prometedoras propiedades adaptativas. Por ejemplo, resaltan las buenas propiedades de regeneración y reciclaje/remodelación, debidas al carácter reversible de las interacciones físicas. Adicionalmente, estos elastómeros poseen una inherente capacidad de autorautorreparación, que en términos prácticos se podría ver como una mejora de su sostenibilidad. Finalmente, se sintetizan redes de PU que tienen un doble carácter estructural mediante enlaces iónicos de hidrógeno dinámicos y entrecruzamientos covalentes. La variación de la densidad de entrecruzamiento covalente introducido para cada una de estas redes produce un ajuste sistemático de las propiedades mecánicas y la sensibilidad del material al calor. Esta preparación demuestra una vía simple y eficaz para la fabricación de poliuretanos multifuncionales.
This Thesis is addressed to the development of side-chain functionalized polyurethanes (FPU)s, with enhanced properties, made from fatty acid-based functional diols and two different diisocyanates; isophorone diisocyanate (IPDI) and hexamethylene diisocyanate (HDI). The novel FPUs present tertiary amine and alkyl, allyl, propargyl moieties or the combination of these, as side-chain positions groups. The FPUs were further modified via two post-polymerization mechanisms based on covalent or non-covalent bonds. In the first case, photoinitiated thiol-ene/yne coupling reaction between allyl, propargyl-functionalized PUs (based on IPDI) and thioglycerol was carried out. Obtained hydroxyl-PUs exhibit different thermal and mechanical properties in comparison with precursor PUs. Moreover, the incorporation of hydroxyl groups leads to PUs with enhanced hydrophilicity. Alternatively, the FPU (based on IPDI) containing only tertiary amine pendant group was mixed with different carboxylic acids in an acid-base reaction. Supramolecular ionic PUs were characterized by spectroscopic tools to verify the presence of ionic hydrogen bond as ionic interaction. Correlation between structure and thermal and mechanical properties was demonstrated. Samples show rapid thermal reversibility and recyclability thanks to the reversible bonds. In addition, elastomeric supramolecular PUs networks were prepared from HDI and aminodiol. The resulting materials exhibit some promising adaptive material properties such as effective energy dissipation upon deformation through unzipping the ionic hydrogen bonding network, combined with good shape-regeneration property and recycling/reshaping capability arising from their recoverable nature. More importantly, the resulting biobased elastomers possess the inherent self-healing ability, which can be seen as an upgrade of their sustainability.A novel thermo-reversible network is constructed by the thiol-ene functionalized polyurethane via dynamic ionic hydrogen bonds and covalent cross-links. By varying the covalent cross-linking density, the mechanical properties and the stimuli-responsive behaviour can be systematically tuned. This synthesis demonstrates a simple and effective pathway to fabricate multifunctional polyurethanes with desired functions.
Mati, Ioulia. "Molecular torsion balances for quantifying non-covalent interactions." Thesis, University of Edinburgh, 2013. http://hdl.handle.net/1842/7610.
Повний текст джерелаBenevelli, Francesca. "Solid-state NMR characterisation of non-covalent interactions." Thesis, University of Cambridge, 2002. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.620286.
Повний текст джерелаAbuajwa, Wissam. "Non-covalent interactions of C60 fullerene and its derivatives." Thesis, University of Nottingham, 2012. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.588068.
Повний текст джерелаAdam, Catherine. "Molecular balances for measuring non-covalent interactions in solution." Thesis, University of Edinburgh, 2015. http://hdl.handle.net/1842/16466.
Повний текст джерелаGao, Yunyi. "Solution Behaviors of Macroions Driven by Non-covalent Interactions." University of Akron / OhioLINK, 2018. http://rave.ohiolink.edu/etdc/view?acc_num=akron1509897811144406.
Повний текст джерелаMADDIS, D. DE. "HIGH RESOLUTION MASS SPECTROMETRIC STRATEGIES IN DRUG DISCOVERY FOR THE INVESTIGATION OF COVALENT AND NON-COVALENT INTERACTIONS." Doctoral thesis, Università degli Studi di Milano, 2014. http://hdl.handle.net/2434/232398.
Повний текст джерелаVivas, de Meftahi Marina. "Compatibility of polymers through H-bonding interactions and covalent crosslinks." Thesis, University of Ottawa (Canada), 1988. http://hdl.handle.net/10393/5190.
Повний текст джерелаArendorf, J. R. T. "A study of some non-covalent functional group π interactions". Thesis, University College London (University of London), 2011. http://discovery.ucl.ac.uk/1334083/.
Повний текст джерелаMoïse, Joelle. "A study of some non-covalent functional group-arene interactions." Thesis, University College London (University of London), 2006. http://discovery.ucl.ac.uk/1445699/.
Повний текст джерелаAnderson, Emily Baird. "Synthesis and Non-Covalent Interactions of Novel Phosphonium-Containing Polymers." Diss., Virginia Tech, 2010. http://hdl.handle.net/10919/28849.
Повний текст джерелаPh. D.
ZHOU, JING. "Understanding the Non-Covalent Interactions in Macroions and Hybrid Macromolecules." University of Akron / OhioLINK, 2016. http://rave.ohiolink.edu/etdc/view?acc_num=akron1447426152.
Повний текст джерелаMark, Kevin J. "Studies of non-covalent myoglobin interactions by electrospray ionization mass spectrometry." Thesis, University of British Columbia, 2006. http://hdl.handle.net/2429/30947.
Повний текст джерелаScience, Faculty of
Chemistry, Department of
Graduate
Sundqvist, Gustav. "Studies of non-covalent interactions using nano-electrospray ionization mass spectrometry." Licentiate thesis, Stockholm : Tekniska högsk, 2004. http://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-336.
Повний текст джерелаKennedy, Matthew R. "Non-covalent interactions and their role in biological and catalytic chemistry." Diss., Georgia Institute of Technology, 2014. http://hdl.handle.net/1853/53044.
Повний текст джерелаZhou, Min. "Understanding non-covalent interactions : cooperativity in ligand binding and enzyme catalysis." Thesis, University of Cambridge, 2005. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.615013.
Повний текст джерелаJu, Lin. "Non-Covalent Interactions in Polymeric Materials: From Ionomers to Polymer Blends." Diss., Virginia Tech, 2019. http://hdl.handle.net/10919/102651.
Повний текст джерелаDoctor of Philosophy
Mather, Brian Douglas. "Non-Covalent Interactions in Block Copolymers Synthesized via Living Polymerization Techniques." Diss., Virginia Tech, 2007. http://hdl.handle.net/10919/27068.
Повний текст джерелаPh. D.
Davis, Holly. "Harnessing non-covalent interactions to control regioselectivity in the functionalisation of arene C-H bonds." Thesis, University of Cambridge, 2018. https://www.repository.cam.ac.uk/handle/1810/277900.
Повний текст джерелаAtilio, Anzellotti I. "Study Of Covalent And Non-Covalent Interactions In Ternary Systems Involving: Metal/DNA-RNA/Protein, Where Metal = Platinum(II), Palladium(II)." VCU Scholars Compass, 2007. http://scholarscompass.vcu.edu/etd/1164.
Повний текст джерелаPearcy, Adam C. "Non-covalent and covalent interactions between phenylacetylene and quinoline radical cations with polar and non-polar molecules in the gas phase." VCU Scholars Compass, 2019. https://scholarscompass.vcu.edu/etd/5990.
Повний текст джерелаArmentano, Antonio. "Non-covalent interactions in molecular clusters : competition between π- and H-bonding". Thesis, University of Manchester, 2010. https://www.research.manchester.ac.uk/portal/en/theses/noncovalent-interactions-in-molecular-clusters-competition-between-pie-and-hbonding(b07b38a8-9f0f-40d2-be8c-4e6c8341e8d6).html.
Повний текст джерелаHughes, Robert Murray Waters Marcey L. "Non-covalent interactions in [beta]-hairpin peptides and small molecule model systems." Chapel Hill, N.C. : University of North Carolina at Chapel Hill, 2007. http://dc.lib.unc.edu/u?/etd,807.
Повний текст джерелаTitle from electronic title page (viewed Dec. 18, 2007). "... in partial fulfillment of the requirements for the degree of Doctor of Philosophy in the Department of Chemistry." Discipline: Chemistry; Department/School: Chemistry. On t.p., [beta] is the Greek letter.
McCammon, Margaret Gallacher. "Non-covalent interactions in multi-subunit protein assemblies : a mass spectrometry investigation." Thesis, University of Oxford, 2001. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.393604.
Повний текст джерелаTong, Xin. "Non-covalent interactions in aromatic molecules and clusters : studies by laser spectroscopy." Thesis, University of York, 2005. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.423680.
Повний текст джерелаBerg, Lotta. "Exploring non-covalent interactions between drug-like molecules and the protein acetylcholinesterase." Doctoral thesis, Umeå universitet, Kemiska institutionen, 2017. http://urn.kb.se/resolve?urn=urn:nbn:se:umu:diva-129900.
Повний текст джерелаLee, Eun-ju. "The study of molecular assemblies formed via non-covalent interactions between calixarenes /." free to MU campus, to others for purchase, 2003. http://wwwlib.umi.com/cr/mo/fullcit?p1418042.
Повний текст джерелаBosc, Denis G. "The catalytic subunits of protein kinase CK2, expression, covalent modification, and regulatory interactions." Thesis, National Library of Canada = Bibliothèque nationale du Canada, 1999. http://www.collectionscanada.ca/obj/s4/f2/dsk2/ftp03/NQ35040.pdf.
Повний текст джерелаUllrich, Susanne. "Conformers and non-covalent interactions studied by laser spectroscopies and Ab initio calculations." Thesis, University of York, 2001. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.247030.
Повний текст джерелаWilliams, Christopher M. "Computational Development of Trimetallic Cyclotrimers for Gas-Filtration Applications through Non-Covalent Interactions." Thesis, University of North Texas, 2019. https://digital.library.unt.edu/ark:/67531/metadc1609127/.
Повний текст джерелаWu, Xing. "Exploitation of noncovalent/dynamic covalent interactions in sensing, self-assembly and membrane transport." Thesis, University of Southampton, 2016. https://eprints.soton.ac.uk/398005/.
Повний текст джерелаPekkanen, Allison Marie. "Non-Covalent Interactions in the Design and Performance of Macromolecules for Biological Technologies." Diss., Virginia Tech, 2017. http://hdl.handle.net/10919/86521.
Повний текст джерелаPh. D.
Dominelli, Whiteley Nicholas. "Hydrogen-bonding and halogen-arene interactions." Thesis, University of Edinburgh, 2017. http://hdl.handle.net/1842/28824.
Повний текст джерелаPascoe, Dominic James. "Orbital interactions." Thesis, University of Edinburgh, 2018. http://hdl.handle.net/1842/33196.
Повний текст джерелаBrahim, Bessem. "Etude de la stabilité des interactions ioniques en phase gazeuse : application aux complexes biologiques." Phd thesis, Université Pierre et Marie Curie - Paris VI, 2014. http://tel.archives-ouvertes.fr/tel-00978816.
Повний текст джерелаHornblower, Breton. "The alpha-hemolysin nanopore as an analytical device to probe non-covalent molecular interactions /." Diss., Digital Dissertations Database. Restricted to UC campuses, 2006. http://uclibs.org/PID/11984.
Повний текст джерелаLemaiÌ‚tre, Vincent J. "Non-covalent interactions in biomolecules studied by ¹â·O NMR and MD simulations." Thesis, University of Oxford, 2004. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.414230.
Повний текст джерелаNkrumah, Anna. "Design, Synthesis, and Characterization of Dynamic Metallo-Supramolecular Polymers Stabilized by Non-Covalent Interactions." Ohio University Honors Tutorial College / OhioLINK, 2013. http://rave.ohiolink.edu/etdc/view?acc_num=ouhonors1369141489.
Повний текст джерелаLv, Dingding <1992>. "Non-covalent interactions in weakly bound molecular complexes: a high-resolution rotational spectroscopy study." Doctoral thesis, Alma Mater Studiorum - Università di Bologna, 2022. http://amsdottorato.unibo.it/10095/7/Dingding%20Lv%20Thesis%202022-03-21.pdf.
Повний текст джерелаMotley, Tanieka L. "Terahertz spectroscopy and molecular modeling of molecules connected by a network of non-covalent interactions." Related electronic resource: Current Research at SU : database of SU dissertations, recent titles available full text, 2009. http://wwwlib.umi.com/cr/syr/main.
Повний текст джерелаBuckwalter, Daniel James. "Non-covalent Intermolecular Interactions in Polymer Design: Segmented Copolymers to Non-viral Gene Delivery Vectors." Diss., Virginia Tech, 2013. http://hdl.handle.net/10919/50926.
Повний текст джерелаAmide containing segmented copolymers relies heavily on hydrogen bonding intermolecular interactions for physical crosslinking to impart the necessary microphase separated morphology responsible for a copolymers physical properties. Amide containing hard segments are composed of various chemical structures from crystalline aramids to amorphous alkyl amides with each structure possessing unique intermolecular interactions. Variations to either of the copolymer segments alters the copolymers physical properties allowing for tuning of a copolymers properties for a particular application. The synthetic strategies, structure-property relationships, and physical properties of amide containing segmented copolymers are thoroughly reported in the literature. Each class of segmented copolymer that contain amide hydrogen bonding groups exhibits a wide range of tunable properties desirable for many applications. The segmented copolymers discussed here include poly(ether-block-amide)s, poly(ether ester amide)s, poly(ester amide)s, poly(oxamide)s, PDMS polyamides, and polyamides containing urethane, urea, or imide groups.
The structure-property relationships (SPR) of poly(oxamide) segmented copolymers is not well understood with only one report currently found in literature. The effects of oxamide spacing in the hard segment and molecular weight of the soft segments in PDMS poly(oxamide) segmented copolymers demonstrated the changes in physical properties associated with minor structural variations. The optically clear PDMS poly(oxamide) copolymers possessed good mechanical properties after bulk polymerization of ethyl oxalate terminated PDMS oligomers with alkyl diamines or varied length. FTIR spectroscopy experiments revealed an ordered hydrogen bonding carbonyl stretching band for each copolymer and as the spacing between oxamide groups increased, the temperature at which the hard segment order was disrupted decreased. The increased spacing between oxamide groups also led to a decrease in the flow temperature observed with dynamic mechanical analysis. Copolymer tensile properties decrease with increased oxamide spacing as well as the hysteresis. The structure-property investigations of PDMS poly(oxamide) segmented copolymers showed that the shortest oxamide spacing resulted in materials with optimal mechanical properties.
A new class of non-chain extended segmented copolymers that contained both urea and oxamide hydrogen bonding groups in the hard segment were synthesized. PDMS poly(urea oxamide) (PDMS-UOx) copolymers displayed thermoplastic elastomer behavior with enhanced physical properties compared to PDMS polyurea (PDMS-U) controls. Synthesis of a difunctional oxamic hydrazide terminated PDMS oligomer through a two-step end capping procedure with diethyl oxalate and hydrazine proved highly efficient. Solution polymerization of the oxamic hydrazide PDMS oligomers with HMDI afforded the desired PDMS-UOx segmented copolymer, which yielded optically clear, tough elastomeric films. Dynamic mechanical analysis showed a large temperature insensitive rubbery plateau that extended up to 186 ÚC for PDMS-UOx copolymers and demonstrated increased rubbery plateau ranges of up to 120 ÚC when compared to the respective PDMS-U control. The increase in thermomechanical properties with the presence of oxamide groups in the hard segment was due to the increased hydrogen bonding, which resulted in a higher degree of microphase separation. DMA, SAXS, and AFM confirmed better phase separation of the PDMS-UOx copolymers compared to PDMS-U controls and DSC and WAXD verified the amorphous character of PDMS-UOx. Oxamide incorporation showed a profound effect on the physical properties of PDMS-UOx copolymers compared to the controls and demonstrated promise for potential commercial applications.
Two novel segmented copolymers based on a poly(propylene glycol) (PPG) that contained two or three oxamide groups in the hard segment were synthesized. Synthesis of non-chain extended PPG poly(trioxamide) (PPG-TriOx) and PPG poly(urea oxamide) (PPG-UOx) segmented copolymers utilized the two-step end-capping procedure with diethyl oxalate and hydrazine then subsequent polymerization with oxalyl chloride or HMDI, respectively. The physical properties of the PPG-TriOx and PPG-UOx copolymers were compared to those of PPG poly(urea) (PPG-U) and poly(oxamide) (PPG-Ox) copolymers. FTIR studies suggested the presence of an ordered hydrogen bonded hard segment for PGG-TriOx and PPG-Ox copolymers with PPG-TriOx possessing a lower energy ordered hydrogen bonding structure. PPG-UOx copolymers exhibited a larger rubbery plateau and higher moduli compared to PPG-U copolymers and also a dramatic increase in the tensile properties with the increased hydrogen bonding. The described copolymers provided a good example of the utility of this new step-growth polymerization chemistry for producing segmented copolymers with strong hydrogen bonding capabilities.
Non-viral nucleic acid delivery has become a hot field in the past 15 years due to increased safety, compared to viral vectors, and ability to synthetically alter the material properties. Altering a synthetic non-viral delivery vector allows for custom tailoring of a delivery vector for various therapeutic applications depending on the target disease. The types of non-viral delivery vectors are diverse, however the lack of understanding of the endocytic mechanisms, endosomal escape, and nucleic acid trafficking is not well understood. This lack of understanding into these complex processes limits the effective design of non-viral nucleic acid delivery vehicles to take advantage of the cellular machinery, as in the case of viral vectors.
Mechanisms for cellular internalization of polymer-nucleic acid complexes are important for the future design of nucleic acid delivery vehicles. It is well known that the mammalian cell surface is covered with glycosaminoglycans (GAG) that carry a negative charge. In an effort to probe the effect of GAG charge density on the affinity of cationic poly(glcoamidoamine) (PGAA)-pDNA complexes, quartz crystal microbalance was employed to measure the mass of GAGs that associated with a polyplex monolayer. Affinity of six different GAGs that varied in the charge density were measured for polyplexes formed with poly(galactaramidopentaethylenetetramine) (G4) cationic polymers and pDNA. Results showed that the affinity of GAGs for G4 polyplexes was not completely dependent on the electrostatic interactions indicating that other factors contribute to the GAG-polyplex interactions. The results provided some insight into the interactions of polyplexes with cell surface GAGs and the role they play in cellular internalization.
Two adamantane terminated polymers were investigated to study the non-covalent inclusion complexation with click cluster non-viral nucleic acid delivery vehicles for passive targeting of the click cluster-pDNA complexes (polyplex). Incorporation of adamantyl terminated poly(ethylene glycol) (Ad-PEG) and poly(2-deoxy-2-methacrylamido glucopyranose) (Ad-pMAG) polymers into the polyplex formulation revealed increased colloidal stability under physiological salt concentrations. Ad-pMAG polyplexes resulted in lower cellular uptake for HeLa cells and not two glioblastoma cell lines indicating the pMAG corona imparts some cell line specificity to the polyplexes. Ad-pMAG provided favorable biological properties when incorporated into the polyplexes as well as increased polyplex physical properties.
Ph. D.
Haso, Fadi. "The Effect of Specific Non-Covalent Interactions on The Assembly Behavior of Macroions in Solution." University of Akron / OhioLINK, 2016. http://rave.ohiolink.edu/etdc/view?acc_num=akron1444937090.
Повний текст джерелаWerlé, Christophe. "Experimental and theoretical study of non-covalent interactions in organometallic chemistry : the concept of hemichelation." Thesis, Strasbourg, 2014. http://www.theses.fr/2014STRAF032/document.
Повний текст джерелаThe present manuscript will present a rational method of synthesis, characterization, determination of the electronic structure and dynamic behaviour of solution-persistent, and formally unsaturated binuclear Cr(0)-M complexes (with M= Pd(II), Pt(II) or Rh(I)). This new class of complexes constitutes rare examples of persistent coordinatively unsaturated 14-electrons complexes, whose cohesion stems essentially from a compensation of insufficient donor/acceptor Cr-M bonding by non-covalent interactions of preponderant attractive Coulombic nature. By taking advantage of the ambiphilic character of a heteroditopic ligand capable of chelating a metal centre through covalent and noncovalent bonds, truly coordination-unsaturated complexes can be synthesized in a manageable form. We propose to name “Hemichelation” the half-covalent/half noncovalent bonding-relationship between the ambiphilic heteroditopic ligand and the electron-unsaturated metallic centre
Le, Thien Anh [Verfasser], Bernd [Gutachter] Engels, and Volker [Gutachter] Engel. "Theoretical investigations of proton transfer and interactions or reactions of covalent and non-covalent inhibitors in different proteins / Thien Anh Le ; Gutachter: Bernd Engels, Volker Engel." Würzburg : Universität Würzburg, 2020. http://d-nb.info/1219429864/34.
Повний текст джерелаChivers, Claire Elizabeth. "Investigating high-affinity non-covalent protein-ligand interaction via variants of streptavidin." Thesis, University of Oxford, 2011. http://ora.ox.ac.uk/objects/uuid:631c65ed-08d9-484e-a8df-309a4c95df45.
Повний текст джерела