Статті в журналах з теми "Coherent spectroscopy"

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1

Carton, W. R. S. "Coherent atomic spectroscopy." Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 31, no. 1-2 (April 1988): 93–101. http://dx.doi.org/10.1016/0168-583x(88)90400-4.

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2

Kim, Young L., Yang Liu, Vladimir M. Turzhitsky, Hemant K. Roy, Ramesh K. Wali, and Vadim Backman. "Coherent backscattering spectroscopy." Optics Letters 29, no. 16 (August 13, 2004): 1906. http://dx.doi.org/10.1364/ol.29.001906.

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3

Chen, Peter C. "An Introduction to Coherent Multidimensional Spectroscopy." Applied Spectroscopy 70, no. 12 (December 2016): 1937–51. http://dx.doi.org/10.1177/0003702816669730.

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Coherent multidimensional spectroscopy is a field that has drawn much attention as an optical analogue to multidimensional nuclear magnetic resonance imaging. Coherent multidimensional spectroscopic techniques produce spectra that show the magnitude of an optical signal as a function of two or more pulsed laser frequencies. Spectra can be collected in either the frequency or the time domain. In addition to improving resolution and overcoming spectral congestion, coherent multidimensional spectroscopy provides the ability to investigate and conduct studies based upon the relationship between different peaks. The purpose of this paper is to provide a general introduction to the area of coherent multidimensional spectroscopy, to provide a brief overview of current experimental approaches, and to discuss some emerging developments in this relatively young field.
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4

Dawlaty, Jahan M., Akihito Ishizaki, Arijit K. De, and Graham R. Fleming. "Microscopic quantum coherence in a photosynthetic-light-harvesting antenna." Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences 370, no. 1972 (August 13, 2012): 3672–91. http://dx.doi.org/10.1098/rsta.2011.0207.

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We briefly review the coherent quantum beats observed in recent two-dimensional electronic spectroscopy experiments in a photosynthetic-light-harvesting antenna. We emphasize that the decay of the quantum beats in these experiments is limited by ensemble averaging. The in vivo dynamics of energy transport depends upon the local fluctuations of a single photosynthetic complex during the energy transfer time (a few picoseconds). Recent analyses suggest that it remains possible that the quantum-coherent motion may be robust under individual realizations of the environment-induced fluctuations contrary to intuition obtained from condensed phase spectroscopic measurements and reduced density matrices. This result indicates that the decay of the observed quantum coherence can be understood as ensemble dephasing. We propose a fluorescence-detected single-molecule experiment with phase-locked excitation pulses to investigate the coherent dynamics at the level of a single molecule without hindrance by ensemble averaging. We discuss the advantages and limitations of this method. We report our initial results on bulk fluorescence-detected coherent spectroscopy of the Fenna–Mathews–Olson complex.
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5

Wright, John C. "Multiresonant Coherent Multidimensional Spectroscopy." Annual Review of Physical Chemistry 62, no. 1 (May 5, 2011): 209–30. http://dx.doi.org/10.1146/annurev-physchem-032210-103551.

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6

Cundiff, Steven T., and Shaul Mukamel. "Optical multidimensional coherent spectroscopy." Physics Today 66, no. 7 (July 2013): 44–49. http://dx.doi.org/10.1063/pt.3.2047.

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7

Tarasek, Matthew R., David J. Goldfarb, and James G. Kempf. "Coherent NMR Stark spectroscopy." Journal of Magnetic Resonance 214 (January 2012): 346–51. http://dx.doi.org/10.1016/j.jmr.2011.11.018.

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8

Mukamel, Shaul, Yoshitaka Tanimura, and Peter Hamm. "Coherent Multidimensional Optical Spectroscopy." Accounts of Chemical Research 42, no. 9 (September 15, 2009): 1207–9. http://dx.doi.org/10.1021/ar900227m.

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9

Zadkov, Viktor N., P. V. Kozlov, S. A. Losev, and V. A. Pavlov. "Coherent shock-wave spectroscopy." Soviet Journal of Quantum Electronics 18, no. 1 (January 31, 1988): 77–81. http://dx.doi.org/10.1070/qe1988v018n01abeh010590.

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10

Wright, John C. "Coherent multidimensional vibrational spectroscopy." International Reviews in Physical Chemistry 21, no. 2 (April 2002): 185–255. http://dx.doi.org/10.1080/01442350210124506.

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11

Cundiff, Steven T. "Coherent spectroscopy of semiconductors." Optics Express 16, no. 7 (March 20, 2008): 4639. http://dx.doi.org/10.1364/oe.16.004639.

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12

Sassaroli, Angelo, Kristen Tgavalekos, and Sergio Fantini. "The meaning of “coherent” and its quantification in coherent hemodynamics spectroscopy." Journal of Innovative Optical Health Sciences 11, no. 06 (November 2018): 1850036. http://dx.doi.org/10.1142/s1793545818500360.

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We have recently introduced a new technique, coherent hemodynamics spectroscopy (CHS), which aims at characterizing a specific kind of tissue hemodynamics that feature a high level of covariation with a given physiological quantity. In this study, we carry out a detailed analysis of the significance of coherence and phase synchronization between oscillations of arterial blood pressure (ABP) and total hemoglobin concentration ([Hbt]), measured with near-infrared spectroscopy (NIRS) during a typical protocol for CHS, based on a cyclic thigh cuff occlusion and release. Even though CHS is based on a linear time invariant model between ABP (input) and NIRS measurands (outputs), for practical reasons in a typical CHS protocol, we induce finite “groups” of ABP oscillations, in which each group is characterized by a different frequency. For this reason, ABP (input) and NIRS measurands (output) are not stationary processes, and we have used wavelet coherence and phase synchronization index (PSI), as a metric of coherence and phase synchronization, respectively. PSI was calculated by using both the wavelet cross spectrum and the Hilbert transform. We have also used linear coherence (which requires stationary process) for comparison with wavelet coherence. The method of surrogate data is used to find critical values for the significance of covariation between ABP and [Hbt]. Because we have found similar critical values for wavelet coherence and PSI by using five of the most used methods of surrogate data, we propose to use the data-independent Gaussian random numbers (GRNs), for CHS. By using wavelet coherence and wavelet cross spectrum, and GRNs as surrogate data, we have found the same results for the significance of coherence and phase synchronization between ABP and [Hbt]: on a total set of 20 periods of cuff oscillations, we have found 17 coherent oscillations and 17 phase synchronous oscillations. Phase synchronization assessed with Hilbert transform yielded similar results with 14 phase synchronous oscillations. Linear coherence and wavelet coherence overall yielded similar number of significant values. We discuss possible reasons for this result. Despite the similarity of linear and wavelet coherence, we argue that wavelet coherence is preferable, especially if one wants to use baseline spontaneous oscillations, in which phase locking and coherence between signals might be only temporary.
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13

Smallwood, Christopher L., and Steven T. Cundiff. "Coherent Spectroscopy: Multidimensional Coherent Spectroscopy of Semiconductors (Laser Photonics Rev. 12(12)/2018)." Laser & Photonics Reviews 12, no. 12 (December 2018): 1870052. http://dx.doi.org/10.1002/lpor.201870052.

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14

Bartels, Randy A., Dan Oron, and Hervé Rigneault. "Low frequency coherent Raman spectroscopy." Journal of Physics: Photonics 3, no. 4 (September 13, 2021): 042004. http://dx.doi.org/10.1088/2515-7647/ac1cd7.

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15

Dostál, Jakub. "Nonresonant coherent two-dimensional spectroscopy." Spectrochimica Acta Part A: Molecular and Biomolecular Spectroscopy 267 (February 2022): 120441. http://dx.doi.org/10.1016/j.saa.2021.120441.

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16

Tas, Guray, Selezion A. Hambir, Jens Franken, David E. Hare, and Dana D. Dlott. "Coherent Raman spectroscopy of nanoshocks." Journal of Applied Physics 82, no. 3 (August 1997): 1080–87. http://dx.doi.org/10.1063/1.365874.

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17

Ogilvie, Jennifer P., Meng Cui, Dmitry Pestov, Alexei V. Sokolov, and Marlan O. Scully. "Time-delayed coherent Raman spectroscopy." Molecular Physics 106, no. 2-4 (February 2008): 587–94. http://dx.doi.org/10.1080/00268970801961005.

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18

SCHRÖTTER, H. W., and J. P. BOQUILLON. "COHERENT RAMAN SPECTROSCOPY IN GASES." Le Journal de Physique Colloques 48, no. C7 (December 1987): C7–707—C7–710. http://dx.doi.org/10.1051/jphyscol:19877174.

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19

Lomsadze, Bachana, and Steven T. Cundiff. "Tri-Comb Multidimensional Coherent Spectroscopy." IEEE Photonics Technology Letters 31, no. 23 (December 1, 2019): 1886–89. http://dx.doi.org/10.1109/lpt.2019.2948342.

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20

Cho, Minhaeng. "Coherent Two-Dimensional Optical Spectroscopy." Chemical Reviews 108, no. 4 (April 2008): 1331–418. http://dx.doi.org/10.1021/cr078377b.

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21

Gundogdu, Kenan, Katherine W. Stone, Daniel B. Turner, and Keith A. Nelson. "Multidimensional coherent spectroscopy made easy." Chemical Physics 341, no. 1-3 (November 2007): 89–94. http://dx.doi.org/10.1016/j.chemphys.2007.06.027.

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22

Meijer, Gerard, Maarten G. H. Boogaarts, Rienk T. Jongma, David H. Parker, and Alec M. Wodtke. "Coherent cavity ring down spectroscopy." Chemical Physics Letters 217, no. 1-2 (January 1994): 112–16. http://dx.doi.org/10.1016/0009-2614(93)e1361-j.

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23

Cundiff, Steven T. "Optical three dimensional coherent spectroscopy." Phys. Chem. Chem. Phys. 16, no. 18 (2014): 8193–200. http://dx.doi.org/10.1039/c4cp00176a.

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24

Rubano, A., D. Paparo, F. Miletto Granozio, U. Scotti di Uccio, and L. Marrucci. "Coherent Raman spectroscopy of YBa_2Cu_3O_7." Optics Express 16, no. 12 (June 4, 2008): 9054. http://dx.doi.org/10.1364/oe.16.009054.

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25

Chen, Peter C. "High Resolution Coherent 2D Spectroscopy." Journal of Physical Chemistry A 114, no. 43 (November 4, 2010): 11365–75. http://dx.doi.org/10.1021/jp102401s.

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26

Smallwood, Christopher L., and Steven T. Cundiff. "Multidimensional Coherent Spectroscopy of Semiconductors." Laser & Photonics Reviews 12, no. 12 (November 8, 2018): 1800171. http://dx.doi.org/10.1002/lpor.201800171.

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27

Melnikov, L. A., V. L. Derbov, I. M. Umansky, and S. I. Vinitsky. "Coherent laser spectroscopy of ¯pHe+." Hyperfine Interactions 101-102, no. 1 (December 1996): 471–77. http://dx.doi.org/10.1007/bf02227658.

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28

Felker, Peter M., and Gregory V. Hartland. "Fourier transform coherent Raman spectroscopy." Chemical Physics Letters 134, no. 6 (March 1987): 503–6. http://dx.doi.org/10.1016/0009-2614(87)87182-8.

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29

Kobayashi, Yuki, and Stephen R. Leone. "Characterizing coherences in chemical dynamics with attosecond time-resolved x-ray absorption spectroscopy." Journal of Chemical Physics 157, no. 18 (November 14, 2022): 180901. http://dx.doi.org/10.1063/5.0119942.

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Coherence can drive wave-like motion of electrons and nuclei in photoexcited systems, which can yield fast and efficient ways to exert materials’ functionalities beyond the thermodynamic limit. The search for coherent phenomena has been a central topic in chemical physics although their direct characterization is often elusive. Here, we highlight recent advances in time-resolved x-ray absorption spectroscopy (tr-XAS) to investigate coherent phenomena, especially those that utilize the eminent light source of isolated attosecond pulses. The unparalleled time and state sensitivities of tr-XAS in tandem with the unique element specificity render the method suitable to study valence electronic dynamics in a wide variety of materials. The latest studies have demonstrated the capabilities of tr-XAS to characterize coupled electronic–structural coherence in small molecules and coherent light–matter interactions of core-excited excitons in solids. We address current opportunities and challenges in the exploration of coherent phenomena, with potential applications for energy- and bio-related systems, potential crossings, strongly driven solids, and quantum materials. With the ongoing developments in both theory and light sources, tr-XAS holds great promise for revealing the role of coherences in chemical dynamics.
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30

Jiang, Shicheng, and Konstantin Dorfman. "Detecting electronic coherences by time-domain high-harmonic spectroscopy." Proceedings of the National Academy of Sciences 117, no. 18 (April 16, 2020): 9776–81. http://dx.doi.org/10.1073/pnas.1919360117.

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Ultrafast spectroscopy is capable of monitoring electronic and vibrational states. For electronic states a few eV apart, an X-ray laser source is required. We propose an alternative method based on the time-domain high-order harmonic spectroscopy where a coherent superposition of the electronic states is first prepared by the strong optical laser pulse. The coherent dynamics can then be probed by the higher-order harmonics generated by the delayed probe pulse. The high nonlinearity typically modeled by the three-step mechanism introduced by Lewenstein and Corkum can serve as a recipe for generation of the coherent excitation with broad bandwidth. The main advantage of the method is that only optical (non–X-ray) lasers are needed. A semiperturbative model based on the Liouville space superoperator approach is developed for the bookkeeping of the different orders of the nonlinear response for the high-order harmonic generation using multiple pulses. Coherence between bound electronic states is monitored in the harmonic spectra from both first- and second-order responses.
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31

Nakanishi, S., H. Itoh, T. Fuji, T. Kashiwagi, N. Tsurumachi, M. Furuichi, H. Nakatsuka, and M. Kamada. "Application of synchrotron radiation to ultrafast spectroscopy." Journal of Synchrotron Radiation 5, no. 3 (May 1, 1998): 1072–74. http://dx.doi.org/10.1107/s0909049597014805.

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A novel application of synchrotron radiation to ultrafast optical spectroscopy is demonstrated. The application is based on the short coherence time of broadband synchrotron radiation and employs a conventional interferometer. From a detailed study of the coherence of synchrotron radiation, it is shown that the coherent interference between two synchrotron radiation beams, split from a single beam, can provide ultimate time resolution down to a few femtoseconds. Experimental results of ultrafast spectroscopy using broadband synchrotron radiation are presented; these include free-induction decay and photon echoes in the visible and ultraviolet regions.
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32

Rohringer, Nina. "X-ray Raman scattering: a building block for nonlinear spectroscopy." Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences 377, no. 2145 (April 2019): 20170471. http://dx.doi.org/10.1098/rsta.2017.0471.

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Ultraintense X-ray free-electron laser pulses of attosecond duration can enable new nonlinear X-ray spectroscopic techniques to observe coherent electronic motion. The simplest nonlinear X-ray spectroscopic concept is based on stimulated electronic X-ray Raman scattering. We present a snapshot of recent experimental achievements, paving the way towards the goal of realizing nonlinear X-ray spectroscopy. In particular, we review the first proof-of-principle experiments, demonstrating stimulated X-ray emission and scattering in atomic gases in the soft X-ray regime and first results of stimulated hard X-ray emission spectroscopy on transition metal complexes. We critically asses the challenges that have to be overcome for future successful implementation of nonlinear coherent X-ray Raman spectroscopy. This article is part of the theme issue ‘Measurement of ultrafast electronic and structural dynamics with X-rays’.
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33

Lee, Sooheyong, Eric C. Landahl, and Wojciech Roseker. "Special Issue on Trends in Sub-Microsecond X-ray Science with Coherent Beams." Applied Sciences 12, no. 18 (September 11, 2022): 9127. http://dx.doi.org/10.3390/app12189127.

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Large increases in synchrotron brightness have brought notable breakthroughs in measurement techniques that exploit transverse coherence, such as X-ray photon correlation spectroscopy (XPCS), coherent diffraction imaging (CDI), diffraction microscopy, and ptychography [...]
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34

Novelli, Fabio, Jonathan O. Tollerud, Dharmalingam Prabhakaran, and Jeffrey A. Davis. "Persistent coherence of quantum superpositions in an optimally doped cuprate revealed by 2D spectroscopy." Science Advances 6, no. 9 (February 2020): eaaw9932. http://dx.doi.org/10.1126/sciadv.aaw9932.

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Quantum materials displaying intriguing magnetic and electronic properties could be key to the development of future technologies. However, it is poorly understood how the macroscopic behavior emerges in complex materials with strong electronic correlations. While measurements of the dynamics of excited electronic populations have been able to give some insight, they have largely neglected the intricate dynamics of quantum coherence. Here, we apply multidimensional coherent spectroscopy to a prototypical cuprate and report unprecedented coherent dynamics persisting for ~500 fs, originating directly from the quantum superposition of optically excited states separated by 20 to 60 meV. These results reveal that the states in this energy range are correlated with the optically excited states at ~1.5 eV and point to nontrivial interactions between quantum many-body states on the different energy scales. In revealing these dynamics and correlations, we demonstrate that multidimensional coherent spectroscopy can interrogate complex quantum materials in unprecedented ways.
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35

Haug, Hartmut. "Quantum Coherence in Ultrafast Semiconductor Spectroscopy." Journal of Nonlinear Optical Physics & Materials 07, no. 02 (June 1998): 227–39. http://dx.doi.org/10.1142/s0218863598000193.

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Coherent optical phenomena such as the optical Stark effect, Rabi flopping, photon echo and quantum beating which are well-known in atomic spectroscopy can also be observed in semiconductors by using femtosecond laser pulses. On these short time scales, the quantum coherence of the optical excitations in the solid do not only influence the optical properties but change at the same time the relaxation and dephasing kinetics. The quasi-classical Boltzmann kinetics has to be replaced by quantum kinetics. Coherence leads to the appearance of memory in the scattering integrals. For femtosecond four-wave mixing and pump-and-probe spectroscopy the use of quantum kinetics for LO-phonon and for carrier-carrier scattering will be reviewed.
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36

Volpato, Andrea, and Elisabetta Collini. "Time-frequency methods for coherent spectroscopy." Optics Express 23, no. 15 (July 23, 2015): 20040. http://dx.doi.org/10.1364/oe.23.020040.

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37

Fleisher, Adam J., David A. Long, Zachary D. Reed, Joseph T. Hodges, and David F. Plusquellic. "Coherent cavity-enhanced dual-comb spectroscopy." Optics Express 24, no. 10 (May 4, 2016): 10424. http://dx.doi.org/10.1364/oe.24.010424.

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38

Steven, T. Cundiff, and Bachana Lomsadze. "Frequency comb-based multidimensional coherent spectroscopy." EPJ Web of Conferences 205 (2019): 03017. http://dx.doi.org/10.1051/epjconf/201920503017.

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We present multidimensional coherent spectroscopy that utilizes frequency combs and multi-heterodyne detection. We demonstrate its capability to measure collective hyperfine resonances in atomic vapor induced by long-range dipole-dipole interactions.
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39

Tian, P. "Femtosecond Phase-Coherent Two-Dimensional Spectroscopy." Science 300, no. 5625 (June 6, 2003): 1553–55. http://dx.doi.org/10.1126/science.1083433.

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40

Reppert, Mike, and Paul Brumer. "Classical coherent two-dimensional vibrational spectroscopy." Journal of Chemical Physics 148, no. 6 (February 14, 2018): 064101. http://dx.doi.org/10.1063/1.5017985.

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41

Newbury, Nathan R., Ian Coddington, and William Swann. "Sensitivity of coherent dual-comb spectroscopy." Optics Express 18, no. 8 (March 31, 2010): 7929. http://dx.doi.org/10.1364/oe.18.007929.

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42

Goetz, Sebastian, Donghai Li, Verena Kolb, Jens Pflaum, and Tobias Brixner. "Coherent two-dimensional fluorescence micro-spectroscopy." Optics Express 26, no. 4 (February 6, 2018): 3915. http://dx.doi.org/10.1364/oe.26.003915.

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43

Grübel, Gerhard, and Federico Zontone. "Correlation spectroscopy with coherent X-rays." Journal of Alloys and Compounds 362, no. 1-2 (January 2004): 3–11. http://dx.doi.org/10.1016/s0925-8388(03)00555-3.

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44

McIlrath, T. J., Keith D. Bonin, and D. G. Cooper. "High-resolution coherent extreme-ultraviolet spectroscopy." Journal of the Optical Society of America B 4, no. 4 (April 1, 1987): 588. http://dx.doi.org/10.1364/josab.4.000588.

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45

Harel, Elad. "Four-dimensional coherent electronic Raman spectroscopy." Journal of Chemical Physics 146, no. 15 (April 21, 2017): 154201. http://dx.doi.org/10.1063/1.4979485.

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46

Chen, Peter C., Candace C. Joyner, Sheena T. Patrick, Rebecca M. Royster, and Leigha L. Ingham. "Gas Chromatography−Multiplex Coherent Raman Spectroscopy." Analytical Chemistry 75, no. 13 (July 2003): 3066–72. http://dx.doi.org/10.1021/ac0207123.

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47

Masumoto, Yasuaki. "Coherent spectroscopy of semiconductor quantum dots." Journal of Luminescence 100, no. 1-4 (December 2002): 191–208. http://dx.doi.org/10.1016/s0022-2313(02)00444-1.

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48

Wynands, R., and A. Nagel. "Precision spectroscopy with coherent dark states." Applied Physics B: Lasers and Optics 68, no. 1 (January 1, 1999): 1–25. http://dx.doi.org/10.1007/s003400050581.

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49

Hopkins, G. A., M. Maroncelli, J. W. Nibler, and T. R. Dyke. "Coherent raman spectroscopy of HCN complexes." Chemical Physics Letters 114, no. 1 (February 1985): 97–102. http://dx.doi.org/10.1016/0009-2614(85)85063-6.

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Auston, D. H., and K. P. Cheung. "Coherent time-domain far-infrared spectroscopy." Journal of the Optical Society of America B 2, no. 4 (April 1, 1985): 606. http://dx.doi.org/10.1364/josab.2.000606.

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