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Littérature scientifique sur le sujet « Spin polarized STM/STS »

Auteur : Grafiati
Publié le 9 mars 2023
Mis à jour le 10 mars 2023

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Articles de revues sur le sujet "Spin polarized STM/STS"

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HAZE, Masahiro, Yasuo YOSHIDA et Yukio HASEGAWA. « Spin Polarized STM/STS on Mn Thin Films on W(110) Using a Bulk Cr Tip ». Hyomen Kagaku 36, no 8 (2015) : 403–7. http://dx.doi.org/10.1380/jsssj.36.403.

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Safari, Mohammad Reza, Frank Matthes, Karl-Heinz Ernst, Daniel E. Bürgler et Claus M. Schneider. « Deposition of Chiral Heptahelicene Molecules on Ferromagnetic Co and Fe Thin-Film Substrates ». Nanomaterials 12, no 19 (21 septembre 2022) : 3281. http://dx.doi.org/10.3390/nano12193281.

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The discovery of chirality-induced spin selectivity (CISS), resulting from an interaction between the electron spin and handedness of chiral molecules, has sparked interest in surface-adsorbed chiral molecules due to potential applications in spintronics, enantioseparation, and enantioselective chemical or biological processes. We study the deposition of chiral heptahelicene by sublimation under ultra-high vacuum onto bare Cu(111), Co bilayer nanoislands on Cu(111), and Fe bilayers on W(110) by low-temperature spin-polarized scanning tunneling microscopy/spectroscopy (STM/STS). In all cases, the molecules remain intact and adsorb with the proximal phenanthrene group aligned parallel to the surface. Three degenerate in-plane orientations on Cu(111) and Co(111), reflecting substrate symmetry, and only two on Fe(110), i.e., fewer than symmetry permits, indicate a specific adsorption site for each substrate. Heptahelicene physisorbs on Cu(111) but chemisorbs on Co(111) and Fe(110) bilayers, which nevertheless remain for the sub-monolayer coverage ferromagnetic and magnetized out-of-plane. We are able to determine the handedness of individual molecules chemisorbed on Fe(110) and Co(111), as previously reported for less reactive Cu(111). The demonstrated deposition control and STM/STS imaging capabilities for heptahelicene on Co/Cu(111) and Fe/W(110) substrate systems lay the foundation for studying CISS in ultra-high vacuum and on the microscopic level of single molecules in controlled atomic configurations.
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YAMADA, Toyokazu, et Tadashi MIZOGUCHI. « Spin-polarized Scanning Tunneling Microscopy/Spectroscopy and Quantitative Analysis Studied on Mn(001) ». Hyomen Kagaku 26, no 1 (2005) : 2–10. http://dx.doi.org/10.1380/jsssj.26.2.

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Mukasa, K., K. Sueoka, H. Hasegawa, Y. Tazuke et K. Hayakawa. « Spin-polarized STM and its family ». Materials Science and Engineering : B 31, no 1-2 (avril 1995) : 69–76. http://dx.doi.org/10.1016/0921-5107(94)08016-x.

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Khitrov, Greg. « Simultaneous Spin and Structure Maps by Spin-Polarized STM ». MRS Bulletin 28, no 1 (janvier 2003) : 4. http://dx.doi.org/10.1557/mrs2003.3.

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Seridonio, A. C., F. M. Souza et I. A. Shelykh. « Spin-polarized STM for a Kondo adatom ». Journal of Physics : Condensed Matter 21, no 9 (29 janvier 2009) : 095003. http://dx.doi.org/10.1088/0953-8984/21/9/095003.

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YAMADA, Toyo Kazu. « How to Get Molecular Spin-Polarization Using Spin-Polarized STM ». Hyomen Kagaku 36, no 7 (2015) : 375–81. http://dx.doi.org/10.1380/jsssj.36.375.

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Kubetzka, A., O. Pietzsch, M. Bode, R. Ravlić et R. Wiesendanger. « Spin-Polarized STM Investigation of Magnetic Domain Walls ». Acta Physica Polonica A 104, no 3-4 (septembre 2003) : 259–68. http://dx.doi.org/10.12693/aphyspola.104.259.

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YAMADA, Toyo Kazu. « Spin-Polarized STM Overview and Issues for Next Developments ». Journal of the Vacuum Society of Japan 60, no 5 (2017) : 159–64. http://dx.doi.org/10.3131/jvsj2.60.159.

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Wieser, R., T. Stapelfeldt, E. Y. Vedmedenko et R. Wiesendanger. « Manipulation of domain walls using a spin-polarized STM ». EPL (Europhysics Letters) 97, no 1 (1 janvier 2012) : 17009. http://dx.doi.org/10.1209/0295-5075/97/17009.

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Thèses sur le sujet "Spin polarized STM/STS"

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ACHILLI, SIMONA. « Spectral properties of adsorbates on metal surfaces via the embedding method ». Doctoral thesis, Università degli Studi di Milano-Bicocca, 2010. http://hdl.handle.net/10281/10827.

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Adsorbates on metal surfaces have attracted recently the scientific interest both from a fundamental point of view (quantum confinement) and in perspective of application in technology. In particular the electronic properties of such reduced symmetry systems are strictly related to their low dimensionality. An accurate theoretical description of their spectral properties has necessarily to deal with the absence of periodicity that characterizes these systems in one (thin films) or more (adatoms) directions. The embedding method allows to overcome this drawback considering a really infinite system both on vacuum and bulk side. In this thesis the ab initio spectral properties of single adatoms (alkali-metal atom and Ba) on Cu(111) and thin overlayers (K/Cu(111), Bi/Cu(100), O/Fe(100)) are analyzed, also in comparison with experimental results. The capabilities of the theoretical method adopted allow to evidence the role of the substrate band structure on the adsorbates induced electronic states. In particular the aspects related to the resonant charge transfer from the adsorbate's states to the bulk continuum are analyzed. This process represents an elastic decay channel for the surface electronic states and contributes to the elastic lifetime, that we can estimate according to the description of a continuous substrate band structure. The results presented for single adatoms evidence the blockade effect that a surface projected energy gap of the substrate produces on the resonant charge transfer. On the other hand the results relative to the overlayer allows to analyze the complex hybridization mechanism between surface features and substrate states in different points of the surface Brillouin zone. In addition the theoretical description of the electronic properties of overlayers on metal surfaces is devoted in this thesis also to the simulation of experimental findings, namely STM and STS images and photoemission spectra, showing the predictive character of the theoretical approach used.
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Holl, Christian [Verfasser], Markus [Akademischer Betreuer] Morgenstern et Samir [Akademischer Betreuer] Lounis. « High frequency STM and spin polarized STM on magnetic vortices / Christian Holl ; Markus Morgenstern, Samir Lounis ». Aachen : Universitätsbibliothek der RWTH Aachen, 2018. http://d-nb.info/1192217926/34.

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Wang, Kangkang. « Atomic Imaging and Spin Mapping of Magnetic Nitride Surfaces ». Ohio University / OhioLINK, 2011. http://rave.ohiolink.edu/etdc/view?acc_num=ohiou1313500678.

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Verlhac, Benjamin. « Atomic-scale spin-sensing with a single molecule at the apex of a scanning tunneling microscope ». Thesis, Strasbourg, 2019. http://www.theses.fr/2019STRAE007/document.

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L’étude présentée dans ce manuscrit s’inscrit dans le domaine du magnétisme de surface, qui a connu de grands développements ces dernières années grâce au microscope à effet tunnel (STM). Elle a pour but de montrer qu’une molécule simple, le nickelocène [Ni(C5H5)2], peut être attachée au sommet d’une pointe STM afin de produire une pointe-sonde magnétique, qui, dans le cadre de l’imagerie magnétique, présente des avantages indéniables comparés à des pointes conventionnelles. À la différence d’autres systèmes moléculaires étudiés avec le STM, nous montrons que les propriétés magnétiques du nickelocène en phase gazeuse sont préservées en présence d’un métal, même lorsque la molécule est attachée au sommet d’une pointe STM. Nous présentons trois résultats marquants avec cette pointe-sonde moléculaire: 1) Nous montrons que l’on peut contrôler le spin du nickelocène, activant à souhait un effet Kondo ; 2) Nous produisons à l’aide du courant tunnel des excitations entre les états de spin du nickelocène, que nous pouvons aisément identifier au travers de la conductance moléculaire. Ces états sont sensibles à toute perturbation magnétique extérieure au nickelocène; 3) Au travers de ces excitations, nous sondons alors le magnétisme de surface. Nous montrons qu’en couplant magnétiquement la pointe-sonde moléculaire avec des atomes, soit isolés soit dans une surface ferromagnétique, nous pouvons mesurer leur polarisation de spin, ainsi que le couplage d’échange nickelocène-atome. Ce dernier permet d’obtenir un contraste magnétique en imagerie STM à l’échelle atomique
The study presented in this manuscript is part of the field of surface magnetism, which has undergone major developments in recent years thanks to the scanning tunneling microscope (STM). It aims to show that a single molecule, nickelocene [Ni(C5H5)2], can be attached to the tip of a STM to produce a magnetic probe-tip, which, in the context of magnetic imaging, has undeniable advantages compared to conventional tips. Unlike other molecular systems studied with STM, we show that the magnetic properties of nickelocene in the gas phase are preserved in the presence of a metal, even when the molecule is attached to the tip of a STM. We present three remarkable results with this molecular probe-tip: 1) We show that we can control the spin of nickelocene, activating at will a Kondo effect; 2) We monitor the spin states of nickelocene by producing electrically-driven excitations, which we can easily identify through the molecular conductance. These states are sensitive to the magnetic environment surrounding nickelocene; 3) We use these states to probe surface magnetism. We show that by magnetically coupling the molecular probe tip with single atoms, either isolated or in a ferromagnetic surface, we can measure their spin polarization, as well as the nickelocene-atom exchange coupling. By monitoring this coupling it is possible to obtain a magnetic contrast in the STM images with atomic-scale resolution
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Scheffler, Martha. « Microscopic tunneling experiments on atomic impurities in graphene and on magnetic thin films ». Doctoral thesis, Saechsische Landesbibliothek- Staats- und Universitaetsbibliothek Dresden, 2015. http://nbn-resolving.de/urn:nbn:de:bsz:14-qucosa-174831.

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This thesis presents investigations on hydrogenated graphene by scanning tunneling microscopy and spectroscopy (STM/STS) as well as the implementation of spin-polarized STM. Preparation processes for a magnetic standard sample and spin-sensitive chromium tips are developed. The measurements on graphene reveal specific hydrogen adsorption sites in low coverage and the formation of a pattern at higher coverage. Both is found to be in agreement with previous predictions and calculations. Upon hydrogenation, an impurity midgap state emerges in the density of states which is measured directly for the first time. Complementing angle resolved photoemission experiments confirm that this state is dispersionless over the whole Brillouin zone. A routine is developed to prepare the standard sample system of ultra-thin iron films on tungsten (Fe/W(110)). Investigations on this system confirm the magnetic properties known from literature, including the presence of a spin spiral, and prove that it is well suited for the characterization of spin-polarized tips. Different approaches for the preparation of tips from the antiferromagnetic material chromium are tested. Among these, a promising new method is presented: The coating of crystalline chromium tips with fresh chromium material suggests reproducibility of the tip characteristics. The performance of the produced tips in STM measurements is excellent in regard to a fixed spin-polarization, high resolution and stability. Especially, a recovery of the tip magnetization direction proposed in this thesis makes this new preparation method superior to all processes yielding antiferromagnetic tips reported so far
Inhalt der vorliegenden Arbeit sind Untersuchungen von hydogeniertem Graphen mittels Rastertunnelmikroskopie und -spektroskopie (RTM/RTS) sowie die Einführung spin-polarisierter RTM. Im Rahmen dessen wurden Präparationsprozesse für magnetische Standardproben und spin-sensitive Chrom-Spitzen entwickelt. Die Messungen an Graphen zeigen spezifische Wasserstoff-Adsorptionsstellen bei geringer Bedeckung und die Ausbildung eines Musters bei höherer Bedeckung, jeweils in Übereinstimmung mit Vorhersagen und Berechnungen. Der durch Hydrogenierung entstehende Störstellenzustand in der Bandlücke der Zustandsdichte wurde zum ersten Mal direkt gemessen. Ergänzende winkelaufgelöste Photoelektronenspektroskopieexperimente bestätigen, dass dieser Zustand in der gesamten Brillouinzone dispersionsfrei ist. Ein Verfahren zur Herstellung magnetischer Standardproben aus ultradünnen Eisenfilmen auf Wolfram (Fe/W(110)) wurde entwickelt. RTM-Untersuchungen an diesem System bestätigen die bereits aus der Literatur bekannten magnetischen Eigenschaften, insbesondere das Vorhandensein einer Spinspirale. Damit ist Fe/W(110) hervorragend geeignet für die Charakterisierung spin-polarisierter Spitzen. Verschiedene Ansätze, die zur Herstellung von Spitzen aus dem antiferromagnetischen Material Chrom verfolgt wurden, werden präsentiert, darunter auch eine vielversprechende neue Methode: Das Aufwachsen eines frischen Chromfilms auf kristalline Spitzen desselben Materials verspricht eine Reproduzierbarkeit von Spitzeneigenschaften. Der Einsatz von so hergestellten Spitzen in RTMMessungen ist geprägt von einer festgelegten Spin-Polarisation, hohem Auflösungsvermögen und Stabilität. Insbesondere die mögliche Reproduzierbarkeit der Magnetisierungsrichtung, die in dieser Arbeit diskutiert wird, macht diese Methode allen bisher berichteten Herstellungprozessen antiferromagnetischer Spitzen überlegen
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Aluru, Rama K. P. « Spectroscopic imaging STM study of the interplay between magnetism and superconductivity in iron-based superconductors ». Thesis, University of St Andrews, 2017. http://hdl.handle.net/10023/12048.

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The discovery of high-temperature superconductivity in 1986 in copper-oxide materials have opened up new avenues to investigate new families of quantum materials that were previously not known. Understanding the mechanism of superconductivity in high-T[sub]c superconductors has been an important research theme in condensed matter physics, as it is believed to be essential to realize the next generation engineered materials that become superconducting at room temperature. Discovered in 2006, iron based superconductors are a new addition to the family of high-T[sub]c superconductors, these materials exhibit several interesting properties and show some vivid similarities with cuprates and other families of high-temperature superconductors. In this thesis, I will present the spin-polarized scanning tunneling microscopy (SPSTM) study carried out on the parent compound of iron chalcogenide high temperature superconductor Fe[sub](1+y)Te to investigate the bi-collinear antiferromagnetic order. Magnetic tips in this work are prepared using a novel preparation technique by picking up excess iron atoms and clusters of FeTe from the surface of the sample. Next, I will present the SP-STM results obtained in the spin glass phase of Fe[sub](1+y)SeₓTe₁₋ₓ visualizing the interplay between the short ranged bi-directional bi-collinear antiferromagnetic order and superconductivity at the atomic scale. In this thesis, I will also present the scanning tunneling microscopy and spectroscopy (STM/STS) study of the native and engineered defect bound states in the iron-pnictide superconductor LiFeAs. This study addresses the pairing symmetry of the superconducting order parameter and understanding of dip-hump features seen in STM spectra outside the superconducting gap in iron pnictide superconductor LiFeAs.
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Ma, Yingqiao. « A Two-dimensional Semiconducting GaN-based Ferromagnetic Monolayer ». Ohio University / OhioLINK, 2018. http://rave.ohiolink.edu/etdc/view?acc_num=ohiou1541513207541646.

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Lin, Wenzhi. « Growth and Scanning Tunneling Microscopy Studies of Magnetic Films on Semiconductors and Development of Molecular Beam Epitaxy/Pulsed Laser Deposition and Cryogenic Spin-Polarized Scanning Tunneling Microscopy System ». Ohio University / OhioLINK, 2011. http://rave.ohiolink.edu/etdc/view?acc_num=ohiou1304610814.

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Sojka, Antonín. « Nízkoteplotní rastrovací tunelová mikroskopie ». Master's thesis, Vysoké učení technické v Brně. Fakulta strojního inženýrství, 2017. http://www.nusl.cz/ntk/nusl-320160.

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The diploma thesis is divided into two main parts. The first part describes the production of chrome and cobalt tips for SP-STM with subsequent testing of chrome tips on the Fe-Ir system (111). Furthermore, the first results from the growth studies of niobium on iridium(111) are presented. In the second part is described in detail the experimental LT-STM microscope of the Faculty of Physical Engineering. The chapter deals with the development of the microscope and its testing on a HOPG sample under atmospheric and vacuum conditions. The chapter describes the biggest problems which were solved when the microscope was puting into operation state. The second part also introduces the design of a new vacuum transport system, which consists of a tip and sample transport pallet. At the end of the second part is described the testing of cooling systems for LT-STM and the design of their modifications.
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Ye, Ruei-Wun, et 葉瑞文. « Fabrication of magnetic tips for spin-polarized STM by using electrochemical etching method ». Thesis, 2010. http://ndltd.ncl.edu.tw/handle/06728504061350488014.

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碩士
國立嘉義大學
光電暨固態電子研究所
98
In this thesis, we developed an improved electrochemical etching method combined with the automatic power cut-off system for the reproducible fabrication of sharp ferromagnetic tips used in spin polarized scanning tunneling microscopy (SP-STM). By using the automatic power cut-off circuit system, it can cut off power in time to avoid over-etching the apex of the tip. After testing different DC voltages for the circuit of electrochemical etching system, a sharp Ni tip with a lowest aspect ratio can be obtained at 8V DC voltage. We also studied different kinds of electrolytes and various concentrations of electrolytes for electrochemical etching of nickel probe, it was found that etching results of HCl solution are better than those of the KCl solution. Moreover, the best etching result of nickel tip was obtained by using the concentration of HCl at 1.5 M. In addition, a plastic cube of 1.33 g is attached to the end of an immersed nickel wire, this leads to a sharp nickel tip with an apex size about 100nm and the reproducible rate better than 40%. Finally, the tip apex was etched in HF (40~48%) for 20 seconds, this not only removes the oxide but also improves the tip shape and reduces the curvature radius of Ni tip.
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Chapitres de livres sur le sujet "Spin polarized STM/STS"

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Yamada, Toyo Kazu. « Spin Polarization of Single Organic Molecule Using Spin-Polarized STM ». Dans Molecular Architectonics, 381–97. Cham : Springer International Publishing, 2017. http://dx.doi.org/10.1007/978-3-319-57096-9_15.

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Chen, C. Julian. « Tip Treatment ». Dans Introduction to Scanning Tunneling Microscopy, 343–58. Oxford University Press, 2021. http://dx.doi.org/10.1093/oso/9780198856559.003.0014.

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This chapter discusses various methods for tip treatment. First, a general discussion about the experimental facts of STM and AFM tips is presented, which points to the subtleties and significance of the last few atoms at the tip apex. The standard method of making an STM tip is the electrochemical etching of a tungsten wire. The experimental procedure is described in detail. The study of the tip using field-ion microscopy is outlined. The tungsten tips freshly made from electrochemical etching often do not provide atomic resolution. Ex-situ and in-situ tip treatments are necessary. Several ex-situ tip treatment methods are described, inducing annealing, field evaporation, and annealing with a field. In-situ tip treatment method such as high-field treatment and controlled collision are described. Then, tip treatment for electrochemical STM is described. Tip treatment methods for spin-polarized STM are described. Finally, tip functionalization, especially with Xe atom and CO molecule, is described.
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Chen, C. Julian. « Atomic-Scale Imaging ». Dans Introduction to Scanning Tunneling Microscopy, 187–234. Oxford University Press, 2021. http://dx.doi.org/10.1093/oso/9780198856559.003.0007.

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This chapter discusses the imaging mechanism of STM and AFM at the atomic scale. Experimental facts show that at atomic resolution, tip electronic states play a key role. Analytic theoretical treatments provide quantitative explanation of the effect of the tip electronic states. On transition-metal tips, first-principle studies unanimously show that d-type tip electronic states dominate the Fermi-level DOS. First-principle studies of the combined tip-sample systems show that for both STM and AFM, the p- and d-type tip electronic states are the keys to understanding the atomic-scale images. The case of spin-polarized STM and the chemical identification of surface atoms are also discussed in terms of tip electronic structure. The chapter concludes with discussions of experimental verifications of the reciprocity principle: at atomic resolution, the role of tip electronic states and the sample electronic states are interchangeable.
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Chen, C. Julian. « Tunneling Phenomenon ». Dans Introduction to Scanning Tunneling Microscopy, 45–76. Oxford University Press, 2021. http://dx.doi.org/10.1093/oso/9780198856559.003.0002.

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This chapter presents basic experimental methods and the basic theory of tunneling. The classical metal-insulator-metal tunneling junction experiment of Giaever, designed to verify the Bardeen-Cooper-Schrieffer theory of superconductivity, is the motivation for Bardeen to invent his perturbation theory of tunneling. That Bardeen theory then became the starting point of the most useful models of STM. Section 2.2 presents the Bardeen tunneling theory from time-dependent perturbation theory of quantum mechanics, starting from a one-dimensional case, then proceeds to three-dimensional version with wave-function corrections. The Bardeen theory in second-quantization format, the transfer-Hamiltonian formalism, is also presented. As extensions of the original Bardeen theory, the theories and experiments of inelastic tunneling and spin-polarized tunneling are discussed in depth.
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Actes de conférences sur le sujet "Spin polarized STM/STS"

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Nussinov, Z. « Noise Spectroscopy of a Single Spin with Spin Polarized STM ». Dans SCANNING TUNNELING MICROSCOPY/SPECTROSCOPY AND RELATED TECHNIQUES : 12th International Conference STM'03. AIP, 2003. http://dx.doi.org/10.1063/1.1639759.

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Yamada, T. K. « Data Evaluation for Spin-Polarized Scanning Tunneling Spectroscopy Measurements ». Dans SCANNING TUNNELING MICROSCOPY/SPECTROSCOPY AND RELATED TECHNIQUES : 12th International Conference STM'03. AIP, 2003. http://dx.doi.org/10.1063/1.1639758.

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Diekhöner, L. « Spin Polarized Surface States of Cobalt Nanoislands on Cu(111) ». Dans SCANNING TUNNELING MICROSCOPY/SPECTROSCOPY AND RELATED TECHNIQUES : 12th International Conference STM'03. AIP, 2003. http://dx.doi.org/10.1063/1.1639677.

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Ceballos, S. F. « Fabrication of Magnetic Probes for Spin-Polarized STM Studies of the Fe3O4 (001) and (111) Surfaces ». Dans SCANNING TUNNELING MICROSCOPY/SPECTROSCOPY AND RELATED TECHNIQUES : 12th International Conference STM'03. AIP, 2003. http://dx.doi.org/10.1063/1.1639710.

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Yamada, T. « Photoemission and STM, STS study of Cs/p-GaAs(110) ». Dans The fourteenth international spin physics symposium, SPIN2000. AIP, 2001. http://dx.doi.org/10.1063/1.1384223.

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Matsuda, T., A. Tonomura, T. K. Yamada, D. Okuyama, N. Mizuno, A. L. Vazquez de Parga, H. van Kempen et T. Mizoguchi. « Characterization of Fe/W spin-polarized tips by means of holographic TEM and spin-polarized-STS of optically pumped p-GaAs ». Dans INTERMAG Asia 2005 : Digest of the IEEE International Magnetics Conference. IEEE, 2005. http://dx.doi.org/10.1109/intmag.2005.1463525.

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Sueoka, K., A. Subagyo et K. Mukasa. « Spin Polarized Electron Injection through Tunneling Junctions and Its Application for SP-STM ». Dans 2002 International Conference on Solid State Devices and Materials. The Japan Society of Applied Physics, 2002. http://dx.doi.org/10.7567/ssdm.2002.d-6-1.

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