Journal articles on the topic 'Warm cloud top mixing'
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1
Small, Jennifer D., and Patrick Y. Chuang. "New Observations of Precipitation Initiation in Warm Cumulus Clouds." Journal of the Atmospheric Sciences 65, no. 9 (September 1, 2008): 2972–82. http://dx.doi.org/10.1175/2008jas2600.1.
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Abstract The mechanism responsible for formation of rain in warm clouds has been debated for over six decades. Here, the authors analyze new measurements of shallow cumulus made with a phase Doppler interferometer during the Rain in Cumulus over the Ocean (RICO) experiment. These observations show that drops sufficiently large (>55-μm diameter) to initiate precipitation (termed collision–coalescence initiators or CCIs) are found preferentially at cloud top, tend to cluster with each other, and are found in environments that are thermodynamically, dynamically, and microphysically distinct from those of smaller drops. The CCI environments exhibit cloud spectra that are shifted to larger sizes, with enhanced broadening toward larger drop sizes. Increased entrainment is also associated with CCIs, suggesting that it is an important process in CCI production. A simple model combining inhomogeneous mixing and condensation is inadequate to explain these observations. It is hypothesized that CCIs are produced in cloud-top regions where turbulence generated by entrainment mixing locally enhances collision–coalescence rates.
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Bhowmick, Taraprasad, and Michele Iovieno. "Direct Numerical Simulation of a Warm Cloud Top Model Interface: Impact of the Transient Mixing on Different Droplet Population." Fluids 4, no. 3 (August 1, 2019): 144. http://dx.doi.org/10.3390/fluids4030144.
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Turbulent mixing through atmospheric cloud and clear air interface plays an important role in the life of a cloud. Entrainment and detrainment of clear air and cloudy volume result in mixing across the interface, which broadens the cloud droplet spectrum. In this study, we simulate the transient evolution of a turbulent cloud top interface with three initial mono-disperse cloud droplet population, using a pseudo-spectral Direct Numerical Simulation (DNS) along with Lagrangian droplet equations, including collision and coalescence. Transient evolution of in-cloud turbulent kinetic energy (TKE), density of water vapour and temperature is carried out as an initial value problem exhibiting transient decay. Mixing in between the clear air and cloudy volume produced turbulent fluctuations in the density of water vapour and temperature, resulting in supersaturation fluctuations. Small scale turbulence, local supersaturation conditions and gravitational forces have different weights on the droplet population depending on their sizes. Larger droplet populations, with initial 25 and 18 μ m radii, show significant growth by droplet-droplet collision and a higher rate of gravitational sedimentation. However, the smaller droplets, with an initial 6 μ m radius, did not show any collision but a large size distribution broadening due to differential condensation/evaporation induced by the mixing, without being influenced by gravity significantly.
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Jarecka, D., H. Pawlowska, W. W. Grabowski, and A. A. Wyszogrodzki. "Modeling microphysical effects of entrainment in clouds observed during EUCAARI-IMPACT field campaign." Atmospheric Chemistry and Physics Discussions 13, no. 1 (January 15, 2013): 1489–526. http://dx.doi.org/10.5194/acpd-13-1489-2013.
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Abstract. This paper discusses aircraft observations and large-eddy simulation (LES) of the 15 May 2008, North Sea boundary-layer clouds from the EUCAARI-IMPACT field campaign. These clouds were advected from the north-east by the prevailing lower-tropspheric winds, and featured stratocumulus-over-cumulus cloud formations. Almost-solid stratocumulus deck in the upper part of the relatively deep weakly decoupled marine boundary layer overlaid a field of small cumuli with a cloud fraction of ~10%. The two cloud formations featured distinct microphysical characteristics that were in general agreement with numerous past observations of strongly-diluted shallow cumuli on the one hand and solid marine boundary-layer stratocumulus on the other. Macrophysical and microphysical cloud properties were reproduced well by the double-moment warm-rain microphysics large-eddy simulation. A novel feature of the model is its capability to locally predict homogeneity of the subgrid-scale mixing between the cloud and its cloud-free environment. In the double-moment warm-rain microphysics scheme, the homogeneity is controlled by a single parameter α, that ranges from 0 to 1 and limiting values representing the homogeneous and the extremely inhomogeneous mixing scenarios, respectively. Parameter α depends on the characteristic time scales of the droplet evaporation and of the turbulent homogenization. In the model, these scales are derived locally based on the subgrid-scale turbulent kinetic energy, spatial scale of cloudy filaments, the mean cloud droplet radius, and the humidity of the cloud-free air entrained into the cloud. Simulated mixing is on average quite inhomogeneous, with the mean parameter α around 0.7 across the entire depth of the cloud field, but with local variations across almost the entire range, especially near the base and the top of the cloud field.
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Freud, E., D. Rosenfeld, M. O. Andreae, A. A. Costa, and P. Artaxo. "Robust relations between CCN and the vertical evolution of cloud drop size distribution in deep convective clouds." Atmospheric Chemistry and Physics Discussions 5, no. 5 (October 19, 2005): 10155–95. http://dx.doi.org/10.5194/acpd-5-10155-2005.
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Abstract. In-situ measurements in convective clouds (up to the freezing level) over the Amazon basin show that smoke from deforestation fires prevents clouds from precipitating until they acquire a vertical development of at least 4 km, compared to only 1–2 km in clean clouds. The average cloud depth required for the onset of warm rain increased by ~350 m for each additional 100 cloud condensation nuclei per cm3 at a super-saturation of 0.5% (CCN0.5%). In polluted clouds, the diameter of modal liquid water content grows much slower with cloud depth (at least by a factor of ~2), due to the large number of droplets that compete for available water and to the suppressed coalescence processes. Contrary to what other studies have suggested, we did not observe this effect to reach saturation at 3000 or more accumulation mode particles per cm3. The CCN0.5% concentration was found to be a very good predictor for the cloud depth required for the onset of warm precipitation and other microphysical factors, leaving only a secondary role for the updraft velocities in determining the cloud drop size distributions. The effective radius of the cloud droplets (re) was found to be a quite robust parameter for a given environment and cloud depth, showing only a small effect of partial droplet evaporation from the cloud's mixing with its drier environment. This supports one of the basic assumptions of satellite analysis of cloud microphysical processes: the ability to look at different cloud top heights in the same region and regard their re as if they had been measured inside one well developed cloud. The dependence of re on the adiabatic fraction decreased higher in the clouds, especially for cleaner conditions, and disappeared at re≥~10 µm. We propose that droplet coalescence, which is at its peak when warm rain is formed in the cloud at re~10 µm, continues to be significant during the cloud's mixing with the entrained air, canceling out the decrease in re due to evaporation.
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Freud, E., D. Rosenfeld, M. O. Andreae, A. A. Costa, and P. Artaxo. "Robust relations between CCN and the vertical evolution of cloud drop size distribution in deep convective clouds." Atmospheric Chemistry and Physics 8, no. 6 (March 18, 2008): 1661–75. http://dx.doi.org/10.5194/acp-8-1661-2008.
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Abstract. In-situ measurements in convective clouds (up to the freezing level) over the Amazon basin show that smoke from deforestation fires prevents clouds from precipitating until they acquire a vertical development of at least 4 km, compared to only 1–2 km in clean clouds. The average cloud depth required for the onset of warm rain increased by ~350 m for each additional 100 cloud condensation nuclei per cm3 at a super-saturation of 0.5% (CCN0.5%). In polluted clouds, the diameter of modal liquid water content grows much slower with cloud depth (at least by a factor of ~2), due to the large number of droplets that compete for available water and to the suppressed coalescence processes. Contrary to what other studies have suggested, we did not observe this effect to reach saturation at 3000 or more accumulation mode particles per cm3. The CCN0.5% concentration was found to be a very good predictor for the cloud depth required for the onset of warm precipitation and other microphysical factors, leaving only a secondary role for the updraft velocities in determining the cloud drop size distributions. The effective radius of the cloud droplets (re) was found to be a quite robust parameter for a given environment and cloud depth, showing only a small effect of partial droplet evaporation from the cloud's mixing with its drier environment. This supports one of the basic assumptions of satellite analysis of cloud microphysical processes: the ability to look at different cloud top heights in the same region and regard their re as if they had been measured inside one well developed cloud. The dependence of re on the adiabatic fraction decreased higher in the clouds, especially for cleaner conditions, and disappeared at re≥~10 μm. We propose that droplet coalescence, which is at its peak when warm rain is formed in the cloud at re=~10 μm, continues to be significant during the cloud's mixing with the entrained air, cancelling out the decrease in re due to evaporation.
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Jia, Hailing, Xiaoyan Ma, Johannes Quaas, Yan Yin, and Tom Qiu. "Is positive correlation between cloud droplet effective radius and aerosol optical depth over land due to retrieval artifacts or real physical processes?" Atmospheric Chemistry and Physics 19, no. 13 (July 12, 2019): 8879–96. http://dx.doi.org/10.5194/acp-19-8879-2019.
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Abstract. The Moderate Resolution Imaging Spectroradiometer (MODIS) C6 L3, Clouds and the Earth's Radiant Energy System (CERES) Edition-4 L3 products, and the European Centre for Medium-Range Weather Forecasts (ECMWF) ERA-Interim reanalysis data are employed to systematically study aerosol–cloud correlations over three anthropogenic aerosol regions and their adjacent oceans, as well as explore the effect of retrieval artifacts and underlying physical mechanisms. This study is confined to warm phase and single-layer clouds without precipitation during the summertime (June, July, and August). Our analysis suggests that cloud effective radius (CER) is positively correlated with aerosol optical depth (AOD) over land (positive slopes), but negatively correlated with aerosol index (AI) over oceans (negative slopes) even with small ranges of liquid water path (quasi-constant). The changes in albedo at the top of the atmosphere (TOA) corresponding to aerosol-induced changes in CER also lend credence to the authenticity of this opposite aerosol–cloud correlation between land and ocean. It is noted that potential artifacts, such as the retrieval biases of both cloud (partially cloudy and 3-D-shaped clouds) and aerosol, can result in a serious overestimation of the slope of CER–AOD/AI. Our results show that collision–coalescence seems not to be the dominant cause for positive slope over land, but the increased CER caused by increased aerosol might further increase CER by initializing collision–coalescence, generating a positive feedback. By stratifying data according to the lower tropospheric stability and relative humidity near cloud top, it is found that the positive correlations more likely occur in the case of drier cloud top and stronger turbulence in clouds, while negative correlations occur in the case of moister cloud top and weaker turbulence in clouds, which implies entrainment mixing might be a possible physical interpretation for such a positive CER–AOD slope.
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Pinsky, M., A. Khain, A. Korolev, and L. Magaritz-Ronen. "Theoretical investigation of mixing in warm clouds – Part 2: Homogeneous mixing." Atmospheric Chemistry and Physics Discussions 15, no. 21 (November 4, 2015): 30269–320. http://dx.doi.org/10.5194/acpd-15-30269-2015.
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Abstract. The evolution of monodisperse and polydisperse droplet size distributions (DSDs) during homogeneous mixing is analyzed. Time-dependent universal analytical relations of supersaturation and liquid water content, which depend on a sole non-dimensional parameter, are obtained for a monodisperse DSD. The evolution of moments and moment-relation functions in the course of the homogeneous evaporation of polydisperse DSDs is analyzed using a parcel model. It is shown that the classic conceptual scheme, according to which homogeneous mixing leads to a decrease in the droplet mass under constant droplet concentration, is valid only in cases of monodisperse or initially very narrow polydisperse DSDs. In cases of wide polydisperse DSDs, mixing and successive evaporation lead to a decrease of both mass and concentration such that the characteristic droplet sizes remain nearly constant. As this feature is typically associated with inhomogeneous mixing, we conclude that in cases of an initially wide DSD at cloud top, homogeneous mixing is nearly indistinguishable from inhomogeneous mixing.
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Pinsky, Mark, Alexander Khain, Alexei Korolev, and Leehi Magaritz-Ronen. "Theoretical investigation of mixing in warm clouds – Part 2: Homogeneous mixing." Atmospheric Chemistry and Physics 16, no. 14 (July 28, 2016): 9255–72. http://dx.doi.org/10.5194/acp-16-9255-2016.
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Abstract. Evolution of monodisperse and polydisperse droplet size distributions (DSD) during homogeneous mixing is analyzed. Time-dependent universal analytical expressions for supersaturation and liquid water content are derived. For an initial monodisperse DSD, these quantities are shown to depend on a sole non-dimensional parameter. The evolution of moments and moment-related functions in the course of homogeneous evaporation of polydisperse DSD is analyzed using a parcel model.It is shown that the classic conceptual scheme, according to which homogeneous mixing leads to a decrease in droplet mass at constant droplet concentration, is valid only in cases of monodisperse or initially very narrow polydisperse DSD. In cases of wide polydisperse DSD, mixing and successive evaporation lead to a decrease of both mass and concentration, so the characteristic droplet sizes remain nearly constant. As this feature is typically associated with inhomogeneous mixing, we conclude that in cases of an initially wide DSD at cloud top, homogeneous mixing is nearly indistinguishable from inhomogeneous mixing.
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Yamashita, Tatsuya, Masatsugu Odaka, Ko-ichiro Sugiyama, Kensuke Nakajima, Masaki Ishiwatari, Seiya Nishizawa, Yoshiyuki O. Takahashi, and Yoshi-Yuki Hayashi. "A Numerical Study of Convection in a Condensing CO2 Atmosphere under Early Mars-Like Conditions." Journal of the Atmospheric Sciences 73, no. 10 (October 1, 2016): 4151–69. http://dx.doi.org/10.1175/jas-d-15-0132.1.
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Abstract Cloud convection of a CO2 atmosphere where the major constituent condenses is numerically investigated under a setup idealizing a possible warm atmosphere of early Mars, utilizing a two-dimensional cloud-resolving model forced by a fixed cooling profile as a substitute for a radiative process. The authors compare two cases with different critical saturation ratios as condensation criteria and also examine sensitivity to number mixing ratio of condensed particles given externally. When supersaturation is not necessary for condensation, the entire horizontal domain above the condensation level is continuously covered by clouds irrespective of number mixing ratio of condensed particles. Horizontal-mean cloud mass density decreases exponentially with height. The circulations below and above the condensation level are dominated by dry cellular convection and buoyancy waves, respectively. When 1.35 is adopted as the critical saturation ratio, clouds appear exclusively as intense, short-lived, quasi-periodic events. Clouds start just above the condensation level and develop upward, but intense updrafts exist only around the cloud top; they do not extend to the bottom of the condensation layer. The cloud layer is rapidly warmed by latent heat during the cloud events, and then the layer is slowly cooled by the specified thermal forcing, and supersaturation gradually develops leading to the next cloud event. The periodic appearance of cloud events does not occur when number mixing ratio of condensed particles is large.
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Jarecka, D., H. Pawlowska, W. W. Grabowski, and A. A. Wyszogrodzki. "Modeling microphysical effects of entrainment in clouds observed during EUCAARI-IMPACT field campaign." Atmospheric Chemistry and Physics 13, no. 16 (August 27, 2013): 8489–503. http://dx.doi.org/10.5194/acp-13-8489-2013.
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Abstract. This paper discusses aircraft observations and large-eddy simulation (LES) modeling of 15 May 2008, North Sea boundary-layer clouds from the EUCAARI-IMPACT field campaign. These clouds are advected from the northeast by the prevailing lower-tropospheric winds and featured stratocumulus-over-cumulus cloud formations. An almost-solid stratocumulus deck in the upper part of the relatively deep, weakly decoupled marine boundary layer overlays a field of small cumuli. The two cloud formations have distinct microphysical characteristics that are in general agreement with numerous past observations of strongly diluted shallow cumuli on one hand and solid marine stratocumulus on the other. Based on the available observations, a LES model setup is developed and applied in simulations using a novel LES model. The model features a double-moment warm-rain bulk microphysics scheme combined with a sophisticated subgrid-scale scheme allowing local prediction of the homogeneity of the subgrid-scale turbulent mixing. The homogeneity depends on the characteristic time scales for the droplet evaporation and for the turbulent homogenization. In the model, these scales are derived locally based on the subgrid-scale turbulent kinetic energy, spatial scale of cloudy filaments, mean cloud droplet radius, and humidity of the cloud-free air entrained into a cloud, all predicted by the LES model. The model reproduces contrasting macrophysical and microphysical characteristics of the cumulus and stratocumulus cloud layers. Simulated subgrid-scale turbulent mixing within the cumulus layer and near the stratocumulus top is on average quite inhomogeneous, but varies significantly depending on the local conditions.
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Gettelman, A., H. Morrison, and S. J. Ghan. "A New Two-Moment Bulk Stratiform Cloud Microphysics Scheme in the Community Atmosphere Model, Version 3 (CAM3). Part II: Single-Column and Global Results." Journal of Climate 21, no. 15 (August 1, 2008): 3660–79. http://dx.doi.org/10.1175/2008jcli2116.1.
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Abstract The global performance of a new two-moment cloud microphysics scheme for a general circulation model (GCM) is presented and evaluated relative to observations. The scheme produces reasonable representations of cloud particle size and number concentration when compared to observations, and it represents expected and observed spatial variations in cloud microphysical quantities. The scheme has smaller particles and higher number concentrations over land than the standard bulk microphysics in the GCM and is able to balance the top-of-atmosphere radiation budget with 60% the liquid water of the standard scheme, in better agreement with retrieved values. The new scheme diagnostically treats both the mixing ratio and number concentration of rain and snow, and it is therefore able to differentiate the two key regimes, consisting of drizzle in shallow, warm clouds and larger rain drops in deeper cloud systems. The modeled rain and snow size distributions are consistent with observations.
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Shupe, M. D., P. O. G. Persson, I. M. Brooks, M. Tjernström, J. Sedlar, T. Mauritsen, S. Sjogren, and C. Leck. "Cloud and boundary layer interactions over the Arctic sea-ice in late summer." Atmospheric Chemistry and Physics Discussions 13, no. 5 (May 17, 2013): 13191–244. http://dx.doi.org/10.5194/acpd-13-13191-2013.
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Abstract. Observations from the Arctic Summer Cloud Ocean Study (ASCOS), in the central Arctic sea-ice pack in late summer 2008, provide a detailed view of cloud-atmosphere-surface interactions and vertical mixing processes over the sea–ice environment. Measurements from a suite of ground-based remote sensors, near surface meteorological and aerosol instruments, and profiles from radiosondes and a helicopter are combined to characterize a week-long period dominated by low-level, mixed-phase, stratocumulus clouds. Detailed case studies and statistical analyses are used to develop a conceptual model for the cloud and atmosphere structure and their interactions in this environment. Clouds were persistent during the period of study, having qualities that suggest they were sustained through a combination of advective influences and in-cloud processes, with little contribution from the surface. Radiative cooling near cloud top produced buoyancy-driven, turbulent eddies that contributed to cloud formation and created a cloud-driven mixed layer. The depth of this mixed layer was related to the amount of turbulence and condensed cloud water. Coupling of this cloud-driven mixed layer to the surface boundary layer was primarily determined by proximity. For 75% of the period of study, the primary stratocumulus cloud-driven mixed layer was decoupled from the surface and typically at a warmer potential temperature. Since the near-surface temperature was constrained by the ocean–ice mixture, warm temperatures aloft suggest that these air masses had not significantly interacted with the sea–ice surface. Instead, back trajectory analyses suggest that these warm airmasses advected into the central Arctic Basin from lower latitudes. Moisture and aerosol particles likely accompanied these airmasses, providing necessary support for cloud formation. On the occasions when cloud-surface coupling did occur, back trajectories indicated that these air masses advected at low levels, while mixing processes kept the mixed layer in equilibrium with the near-surface environment. Rather than contributing buoyancy forcing for the mixed-layer dynamics, the surface instead simply appeared to respond to the mixed-layer processes aloft. Clouds in these cases often contained slightly higher condensed water amounts, potentially due to additional moisture sources from below.
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Shupe, M. D., P. O. G. Persson, I. M. Brooks, M. Tjernström, J. Sedlar, T. Mauritsen, S. Sjogren, and C. Leck. "Cloud and boundary layer interactions over the Arctic sea ice in late summer." Atmospheric Chemistry and Physics 13, no. 18 (September 24, 2013): 9379–99. http://dx.doi.org/10.5194/acp-13-9379-2013.
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Abstract. Observations from the Arctic Summer Cloud Ocean Study (ASCOS), in the central Arctic sea-ice pack in late summer 2008, provide a detailed view of cloud–atmosphere–surface interactions and vertical mixing processes over the sea-ice environment. Measurements from a suite of ground-based remote sensors, near-surface meteorological and aerosol instruments, and profiles from radiosondes and a helicopter are combined to characterize a week-long period dominated by low-level, mixed-phase, stratocumulus clouds. Detailed case studies and statistical analyses are used to develop a conceptual model for the cloud and atmosphere structure and their interactions in this environment. Clouds were persistent during the period of study, having qualities that suggest they were sustained through a combination of advective influences and in-cloud processes, with little contribution from the surface. Radiative cooling near cloud top produced buoyancy-driven, turbulent eddies that contributed to cloud formation and created a cloud-driven mixed layer. The depth of this mixed layer was related to the amount of turbulence and condensed cloud water. Coupling of this cloud-driven mixed layer to the surface boundary layer was primarily determined by proximity. For 75% of the period of study, the primary stratocumulus cloud-driven mixed layer was decoupled from the surface and typically at a warmer potential temperature. Since the near-surface temperature was constrained by the ocean–ice mixture, warm temperatures aloft suggest that these air masses had not significantly interacted with the sea-ice surface. Instead, back-trajectory analyses suggest that these warm air masses advected into the central Arctic Basin from lower latitudes. Moisture and aerosol particles likely accompanied these air masses, providing necessary support for cloud formation. On the occasions when cloud–surface coupling did occur, back trajectories indicated that these air masses advected at low levels, while mixing processes kept the mixed layer in equilibrium with the near-surface environment. Rather than contributing buoyancy forcing for the mixed-layer dynamics, the surface instead simply appeared to respond to the mixed-layer processes aloft. Clouds in these cases often contained slightly higher condensed water amounts, potentially due to additional moisture sources from below.
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Wang, Yuqing, Haiming Xu, and Shang-Ping Xie. "Regional Model Simulations of Marine Boundary Layer Clouds over the Southeast Pacific off South America. Part II: Sensitivity Experiments*." Monthly Weather Review 132, no. 11 (November 1, 2004): 2650–68. http://dx.doi.org/10.1175/mwr2812.1.
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Abstract The sensitivity of a regional climate model to physical parameterizations and model resolution is investigated in terms of its simulation of boundary layer stratocumulus (SCu) clouds over the southeast Pacific. Specifically, the physical schemes being tested include shallow cumulus convection, subgrid vertical mixing, cloud droplet number concentration (CDNC), and drizzle. As described in Part I, the model with standard settings captures the major features of the boundary layer in the region, including a well-mixed marine boundary layer, a capping temperature inversion, SCu clouds, and the boundary layer regime transition from the well-mixed layer near the coast of South America to a decoupled cloud layer over warmer water to the west. Turning off the shallow cumulus parameterization results in a dramatic increase in the simulated SCu clouds while the boundary layer structure becomes unrealistic, losing the decoupled regime over warm water. With reduced penetrative mixing at the top of shallow cumuli, the simulated SCu clouds are somewhat increased while the boundary layer structure remained largely unchanged. Reducing the CDNC increases the size of cloud droplets and reduces the cloud albedo but has little effect on the vertical structure of the boundary layer and clouds. Allowing more drizzle decreases boundary layer clouds considerably. It is also shown that the simulated depth of the boundary layer and its decoupling is highly sensitive to the model horizontal and vertical resolutions. Insufficient horizontal or vertical resolutions produce a temperature inversion and cloud layer too close to the sea surface, a typical problem for global general circulation models. Implications of these results for global and regional modeling of boundary layer clouds and the areas that need more attention in future model development are discussed.
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Martucci, G., and C. D. O'Dowd. "Ground-based retrieval of continental and marine warm cloud microphysics." Atmospheric Measurement Techniques Discussions 4, no. 4 (July 29, 2011): 4825–65. http://dx.doi.org/10.5194/amtd-4-4825-2011.
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Abstract. A technique for retrieving warm cloud microphysics using synergistic ground based remote sensing instruments is presented. The SYRSOC (SYnergistic Remote Sensing Of Cloud) technique utilises a Ka-band Doppler cloud RADAR, a LIDAR-ceilometer and a multichannel microwave radiometer. SYRSOC retrieves the main microphysical parameters such as cloud droplet number concentration (CDNC), droplets effective radius (reff), cloud liquid water content (LWC), and the departure from adiabatic conditions within the cloud. Two retrievals are presented for continental and marine stratocumulus formed over the Mace Head Atmospheric Research Station. Whilst the continental case exhibited high CDCN (N = 382 cm−3; 10th-to-90th percentile [9.4–842.4] cm−3) and small mean effective radius (reff = 4.3; 10th-to-90th percentile [2.9–6.5] μm), the marine case exhibited low CDNC and large mean effective radius (N = 25 cm−3, 10th-to-90th percentile [1.5–69] cm−3; reff = 25.6 μm, 10th-to-90th percentile [11.2–42.7] μm) as expected since the continental air at this location is typically more polluted than marine air. The large reff of the marine case was determined by the contribution of drizzle drops (large radii and few occurrences) and in fact the modal radius was reffMOD = 12 μm (smaller radius and large occurrences). The mean LWC was comparable for the two cases (continental: 0.19 g m−3; marine: 0.16 g m–3) but the 10th–90th percentile range was wider in marine air (continental: 0.11–0.22 g m−3; marine: 0.01–0.38 g m−3). The calculated algorithm uncertainty for the continental and marine case for each variable was, respectively, σN=141.34 cm−3 and 11.5 cm−3, σreff=0.8 μm and 3.2 μm, σLWC = 0.03 g m−3 and 0.03 g m−3. The retrieved CDNC are compared to the cloud condensation nuclei concentrations and the best agreement is achieved for a super-saturation of 0.1 % in the continental case and between 0.1 %–0.75 % for the marine stratocumulus. The retrieved reff at the top of the clouds are compared to the MODIS satellite reff: 7 μm (MODIS) vs 6.2 μm (SYRSOC) and 16.3 μm (MODIS) vs. 17 μm (SYRSOC) for continental and marine cases, respectively. The combined analysis of the CDNC and the reff, for the marine case shows that the drizzle modifies the droplet size distribution and reff especially if compared to reffMOD. The study of the cloud subadiabaticity and the LWC shows the general sub-adiabatic character of both clouds with more pronounced departure from adiabatic conditions in the continental case due to the shallower cloud depth and more significant mixing with dry tropospheric air.
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Miltenberger, Annette K., Paul R. Field, Adrian A. Hill, Phil Rosenberg, Ben J. Shipway, Jonathan M. Wilkinson, Robert Scovell, and Alan M. Blyth. "Aerosol–cloud interactions in mixed-phase convective clouds – Part 1: Aerosol perturbations." Atmospheric Chemistry and Physics 18, no. 5 (March 5, 2018): 3119–45. http://dx.doi.org/10.5194/acp-18-3119-2018.
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Abstract. Changes induced by perturbed aerosol conditions in moderately deep mixed-phase convective clouds (cloud top height ∼ 5 km) developing along sea-breeze convergence lines are investigated with high-resolution numerical model simulations. The simulations utilise the newly developed Cloud–AeroSol Interacting Microphysics (CASIM) module for the Unified Model (UM), which allows for the representation of the two-way interaction between cloud and aerosol fields. Simulations are evaluated against observations collected during the COnvective Precipitation Experiment (COPE) field campaign over the southwestern peninsula of the UK in 2013. The simulations compare favourably with observed thermodynamic profiles, cloud base cloud droplet number concentrations (CDNC), cloud depth, and radar reflectivity statistics. Including the modification of aerosol fields by cloud microphysical processes improves the correspondence with observed CDNC values and spatial variability, but reduces the agreement with observations for average cloud size and cloud top height. Accumulated precipitation is suppressed for higher-aerosol conditions before clouds become organised along the sea-breeze convergence lines. Changes in precipitation are smaller in simulations with aerosol processing. The precipitation suppression is due to less efficient precipitation production by warm-phase microphysics, consistent with parcel model predictions. In contrast, after convective cells organise along the sea-breeze convergence zone, accumulated precipitation increases with aerosol concentrations. Condensate production increases with the aerosol concentrations due to higher vertical velocities in the convective cores and higher cloud top heights. However, for the highest-aerosol scenarios, no further increase in the condensate production occurs, as clouds grow into an upper-level stable layer. In these cases, the reduced precipitation efficiency (PE) dominates the precipitation response and no further precipitation enhancement occurs. Previous studies of deep convective clouds have related larger vertical velocities under high-aerosol conditions to enhanced latent heating from freezing. In the presented simulations changes in latent heating above the 0∘C are negligible, but latent heating from condensation increases with aerosol concentrations. It is hypothesised that this increase is related to changes in the cloud field structure reducing the mixing of environmental air into the convective core. The precipitation response of the deeper mixed-phase clouds along well-established convergence lines can be the opposite of predictions from parcel models. This occurs when clouds interact with a pre-existing thermodynamic environment and cloud field structural changes occur that are not captured by simple parcel model approaches.
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Tokinaga, Hiroki, Youichi Tanimoto, Shang-Ping Xie, Takeaki Sampe, Hiroyuki Tomita, and Hiroshi Ichikawa. "Ocean Frontal Effects on the Vertical Development of Clouds over the Western North Pacific: In Situ and Satellite Observations*." Journal of Climate 22, no. 16 (August 15, 2009): 4241–60. http://dx.doi.org/10.1175/2009jcli2763.1.
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Abstract A suite of shipboard and satellite observations are analyzed and synthesized to investigate the three-dimensional structure of clouds and influences from sea surface temperature fronts over the western North Pacific. Sharp transitions are observed across the Kuroshio Extension (KE) front in the marine atmospheric boundary layer (MABL) and its clouds. The ocean’s influence appears to extend beyond the MABL, with higher cloud tops in altitude along the KE front than the surroundings. In winter, intense turbulent heat release from the ocean takes place on the southern flank of the KE front, where the cloud top penetrates above the MABL and reaches the midtroposphere. In this band of high cloud tops, frequent lightning activity is observed. The results of this study suggest a sea level pressure mechanism for which the temperature gradient in the MABL induces strong surface wind convergence on the southern flank of the KE front, deepening the clouds there. In early summer, sea fog frequently occurs on the northern flank of the subtropical KE and subarctic fronts under southerly warm advection that suppresses surface heat flux and stabilizes the surface atmosphere. Sea fog is infrequently observed over the KE front even under southerly conditions, as the warm ocean current weakens atmospheric stratification and promotes vertical mixing. The KE front produces a narrow band of surface wind convergence, helping support a broad band of upward motion at 700 hPa that is associated with the eastward extension of the baiu rainband from Japan in June–July.
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Wang, Qian, Su-Ping Zhang, Shang-Ping Xie, Joel R. Norris, Jian-Xiang Sun, and Yu-Xi Jiang. "Observed Variations of the Atmospheric Boundary Layer and Stratocumulus over a Warm Eddy in the Kuroshio Extension." Monthly Weather Review 147, no. 5 (April 17, 2019): 1581–91. http://dx.doi.org/10.1175/mwr-d-18-0381.1.
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Abstract A research vessel sailing across a warm eddy in the Kuroshio Extension on 13 April 2016 captured an abrupt development of stratocumulus under synoptic high pressure. Shipboard observations and results from regional atmospheric model simulations indicate that increased surface heat flux over the ocean eddy lowered surface pressure and thereby accelerated southeasterly winds. The southeasterly winds transported moisture toward the low pressure and enhanced the air–sea interface heat flux, which in turn deepened the low pressure and promoted low-level convergence and rising motion over the warm eddy. The lifting condensation level lowered and the top of the marine atmospheric boundary layer (MABL) rose, thereby aiding the development of the stratocumulus. Further experiments showed that 6°C sea surface temperature anomalies associated with the 400-km-diameter warm eddy accounted for 80% of the total ascending motion and 95% of total cloud water mixing ratio in the marine atmospheric boundary layer during the development of stratocumulus. The synthesis of in situ soundings and modeling contributes to understanding of the mechanism by which the MABL and marine stratocumulus respond to ocean eddies.
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Huang, Huijun, Hongnian Liu, Jian Huang, Weikang Mao, and Xueyan Bi. "Atmospheric Boundary Layer Structure and Turbulence during Sea Fog on the Southern China Coast." Monthly Weather Review 143, no. 5 (May 1, 2015): 1907–23. http://dx.doi.org/10.1175/mwr-d-14-00207.1.
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Abstract Small-scale turbulence has an essential role in sea-fog formation and evolution, but is not completely understood. This study analyzes measurements of the small-scale turbulence, together with the boundary layer structure and the synoptic and mesoscale conditions over the life cycle of a cold advection fog event and a warm advection fog event, both off the coast of southern China. The measurement data come from two sites: one on the coast and one at sea. These findings include the following: 1) For cold advection fog, the top can extend above the inversion base, but formation of an overlaying cloud causes the fog to dissipate. 2) For warm advection fog, two layers of low cloud can merge to form deep fog, with the depth exceeding 1000 m, when strong advection of warm moist air produces active thermal-turbulence mixing above the thermal-turbulence interface. 3) Turbulence near the sea surface is mainly thermally driven for cold advection fog, but mechanically driven for warm advection fog. 4) The momentum fluxes of both fog cases are below 0.04 kg m−1 s−2. However, the sensible and latent heat flux differ between the cases: in the cold advection fog case, the sensible and latent heat fluxes are roughly upward, averaging 2.58 and 26.75 W m−2, respectively; however, in the warm advection fog case, the sensible and latent heat flux are mostly downward, averaging −6.98 and −6.22 W m−2, respectively. 5) Low-level vertical advection is important for both fogs, but has a larger influence on fog development in the warm advection fog case.
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Ricaud, Philippe, Massimo Del Guasta, Eric Bazile, Niramson Azouz, Angelo Lupi, Pierre Durand, Jean-Luc Attié, Dana Veron, Vincent Guidard, and Paolo Grigioni. "Supercooled liquid water cloud observed, analysed, and modelled at the top of the planetary boundary layer above Dome C, Antarctica." Atmospheric Chemistry and Physics 20, no. 7 (April 7, 2020): 4167–91. http://dx.doi.org/10.5194/acp-20-4167-2020.
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Abstract. A comprehensive analysis of the water budget over the Dome C (Concordia, Antarctica) station has been performed during the austral summer 2018–2019 as part of the Year of Polar Prediction (YOPP) international campaign. Thin (∼100 m deep) supercooled liquid water (SLW) clouds have been detected and analysed using remotely sensed observations at the station (tropospheric depolarization lidar, the H2O Antarctica Microwave Stratospheric and Tropospheric Radiometer (HAMSTRAD), net surface radiation from the Baseline Surface Radiation Network (BSRN)), radiosondes, and satellite observations (CALIOP, Cloud-Aerosol LIdar with Orthogonal Polarization/CALIPSO, Cloud Aerosol Lidar and Infrared Pathfinder Satellite Observations) combined with a specific configuration of the numerical weather prediction model: ARPEGE-SH (Action de Recherche Petite Echelle Grande Echelle – Southern Hemisphere). The analysis shows that SLW clouds were present from November to March, with the greatest frequency occurring in December and January when ∼50 % of the days in summer time exhibited SLW clouds for at least 1 h. Two case studies are used to illustrate this phenomenon. On 24 December 2018, the atmospheric planetary boundary layer (PBL) evolved following a typical diurnal variation, which is to say with a warm and dry mixing layer at local noon thicker than the cold and dry stable layer at local midnight. Our study showed that the SLW clouds were observed at Dome C within the entrainment and the capping inversion zones at the top of the PBL. ARPEGE-SH was not able to correctly estimate the ratio between liquid and solid water inside the clouds with the liquid water path (LWP) strongly underestimated by a factor of 1000 compared to observations. The lack of simulated SLW in the model impacted the net surface radiation that was 20–30 W m−2 higher in the BSRN observations than in the ARPEGE-SH calculations, mainly attributable to the BSRN longwave downward surface radiation being 50 W m−2 greater than that of ARPEGE-SH. The second case study took place on 20 December 2018, when a warm and wet episode impacted the PBL with no clear diurnal cycle of the PBL top. SLW cloud appearance within the entrainment and capping inversion zones coincided with the warm and wet event. The amount of liquid water measured by HAMSTRAD was ∼20 times greater in this perturbed PBL than in the typical PBL. Since ARPEGE-SH was not able to accurately reproduce these SLW clouds, the discrepancy between the observed and calculated net surface radiation was even greater than in the typical PBL case, reaching +50 W m−2, mainly attributable to the downwelling longwave surface radiation from BSRN being 100 W m−2 greater than that of ARPEGE-SH. The model was then run with a new partition function favouring liquid water for temperatures below −20 down to −40 ∘C. In this test mode, ARPEGE-SH has been able to generate SLW clouds with modelled LWP and net surface radiation consistent with observations during the typical case, whereas, during the perturbed case, the modelled LWP was 10 times less than the observations and the modelled net surface radiation remained lower than the observations by ∼50 W m−2. Accurately modelling the presence of SLW clouds appears crucial to correctly simulate the surface energy budget over the Antarctic Plateau.
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You, Cheng, Michael Tjernström, and Abhay Devasthale. "Warm and moist air intrusions into the winter Arctic: a Lagrangian view on the near-surface energy budgets." Atmospheric Chemistry and Physics 22, no. 12 (June 21, 2022): 8037–57. http://dx.doi.org/10.5194/acp-22-8037-2022.
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Abstract. In this study, warm and moist air intrusions (WaMAIs) over the Arctic Ocean sectors of Barents Sea, Kara Sea, Laptev Sea, East Siberian Sea, Chukchi Sea, and Beaufort Sea in 40 recent winters (from 1979 to 2018) are identified from the ERA5 reanalysis using both Eulerian and Lagrangian views. The analysis shows that WaMAIs, fueled by Arctic blocking, cause a relative surface warming and hence a sea-ice reduction by exerting positive anomalies of net thermal irradiances and turbulent fluxes on the surface. Over Arctic Ocean sectors with land-locked sea ice in winter, such as Laptev Sea, East Siberian Sea, Chukchi Sea, and Beaufort Sea, the total surface energy-budget is dominated by net thermal irradiance. From a Lagrangian perspective, total water path (TWP) increases linearly with the downstream distance from the sea-ice edge over the completely ice-covered sectors, inducing almost linearly increasing net thermal irradiance and total surface energy-budget. However, over the Barents Sea, with an open ocean to the south, total net surface energy-budget is dominated by the surface turbulent flux. With the energy in the warm-and-moist air continuously transported to the surface, net surface turbulent flux gradually decreases with distance, especially within the first 2∘ north of the ice edge, inducing a decreasing but still positive total surface energy-budget. The boundary-layer energy-budget patterns over the Barents Sea can be categorized into three classes: radiation-dominated, turbulence-dominated, and turbulence-dominated with cold dome, comprising about 52 %, 40 %, and 8 % of all WaMAIs, respectively. Statistically, turbulence-dominated cases with or without cold dome occur along with 1 order of magnitude larger large-scale subsidence than the radiation-dominated cases. For the turbulence-dominated category, larger turbulent fluxes are exerted to the surface, probably because of stronger wind shear. In radiation-dominated WaMAIs, stratocumulus develops more strongly and triggers intensive cloud-top radiative cooling and related buoyant mixing that extends from cloud top to the surface, inducing a thicker well-mixed layer under the cloud. With the existence of cold dome, fewer liquid water clouds were formed, and less or even negative turbulent fluxes could reach the surface.
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MacDonald, Alexander B., Ali Hossein Mardi, Hossein Dadashazar, Mojtaba Azadi Aghdam, Ewan Crosbie, Haflidi H. Jonsson, Richard C. Flagan, John H. Seinfeld, and Armin Sorooshian. "On the relationship between cloud water composition and cloud droplet number concentration." Atmospheric Chemistry and Physics 20, no. 13 (July 2, 2020): 7645–65. http://dx.doi.org/10.5194/acp-20-7645-2020.
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Abstract. Aerosol–cloud interactions are the largest source of uncertainty in quantifying anthropogenic radiative forcing. The large uncertainty is, in part, due to the difficulty of predicting cloud microphysical parameters, such as the cloud droplet number concentration (Nd). Even though rigorous first-principle approaches exist to calculate Nd, the cloud and aerosol research community also relies on empirical approaches such as relating Nd to aerosol mass concentration. Here we analyze relationships between Nd and cloud water chemical composition, in addition to the effect of environmental factors on the degree of the relationships. Warm, marine, stratocumulus clouds off the California coast were sampled throughout four summer campaigns between 2011 and 2016. A total of 385 cloud water samples were collected and analyzed for 80 chemical species. Single- and multispecies log–log linear regressions were performed to predict Nd using chemical composition. Single-species regressions reveal that the species that best predicts Nd is total sulfate (Radj2=0.40). Multispecies regressions reveal that adding more species does not necessarily produce a better model, as six or more species yield regressions that are statistically insignificant. A commonality among the multispecies regressions that produce the highest correlation with Nd was that most included sulfate (either total or non-sea-salt), an ocean emissions tracer (such as sodium), and an organic tracer (such as oxalate). Binning the data according to turbulence, smoke influence, and in-cloud height allowed for examination of the effect of these environmental factors on the composition–Nd correlation. Accounting for turbulence, quantified as the standard deviation of vertical wind speed, showed that the correlation between Nd with both total sulfate and sodium increased at higher turbulence conditions, consistent with turbulence promoting the mixing between ocean surface and cloud base. Considering the influence of smoke significantly improved the correlation with Nd for two biomass burning tracer species in the study region, specifically oxalate and iron. When binning by in-cloud height, non-sea-salt sulfate and sodium correlated best with Nd at cloud top, whereas iron and oxalate correlated best with Nd at cloud base.
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Grabowski, Wojciech W., and Hugh Morrison. "Indirect Impact of Atmospheric Aerosols in Idealized Simulations of Convective–Radiative Quasi Equilibrium. Part II: Double-Moment Microphysics." Journal of Climate 24, no. 7 (April 1, 2011): 1897–912. http://dx.doi.org/10.1175/2010jcli3647.1.
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Abstract This paper extends the previous cloud-resolving modeling study concerning the impact of cloud microphysics on convective–radiative quasi equilibrium (CRQE) over a surface with fixed characteristics and prescribed solar input, both mimicking the mean conditions on earth. The current study applies sophisticated double-moment warm-rain and ice microphysics schemes, which allow for a significantly more realistic representation of the impact of aerosols on precipitation processes and on the coupling between clouds and radiative transfer. Two contrasting cloud condensation nuclei (CCN) characteristics are assumed, representing pristine and polluted conditions, as well as contrasting representations of the effects of entrainment and mixing on the mean cloud droplet size. In addition, four sets of sensitivity simulations are also performed with changes that provide a reference for the main simulation set. As in the previous study, the CRQE mimics the estimates of globally and annually averaged water and energy fluxes across the earth’s atmosphere. There are some differences from the previous study, however, consistent with the slightly lower water vapor content in the troposphere and significantly reduced lower-tropospheric cloud fraction in current simulations. There is also a significant reduction of the difference between the pristine and polluted cases, from ∼20 to ∼4 W m−2 at the surface from ∼20 to ∼9 W m−2 at the top of the atmosphere (TOA). The difference between the homogeneous and extremely inhomogeneous mixing scenarios, ∼20 W m−2 in the previous study, is reduced to a mere 2 (1) W m−2 at the surface (TOA). An unexpected difference between the previous and current simulations is the lower Bowen ratio of the surface heat flux, the partitioning of the total flux into sensible and latent components. It is shown that most of the change comes from the difference in the representation of rain evaporation in the subcloud layer in the single- and double-moment microphysics schemes. The difference affects the mean air temperature and humidity near the surface, and thus the Bowen ratio. The differences between the various simulations are discussed, contrasting the process-level approach with the impact of cloud microphysics on the quasi-equilibrium state with a more appropriate system dynamics approach. The key distinction is that the latter includes the interactions among all the processes in the modeled system.
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Morrison, H., and W. W. Grabowski. "Cloud-system resolving model simulations of aerosol indirect effects on tropical deep convection and its thermodynamic environment." Atmospheric Chemistry and Physics Discussions 11, no. 5 (May 23, 2011): 15573–629. http://dx.doi.org/10.5194/acpd-11-15573-2011.
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Abstract. This paper presents results from 240-member ensemble simulations of aerosol indirect effects on tropical deep convection and its thermodynamic environment. Simulations using a two-dimensional cloud system-resolving model are run with pristine, polluted, or highly polluted aerosol conditions and large-scale forcing from a 6-day period of active monsoon conditions during the 2006 Tropical Warm Pool – International Cloud Experiment (TWP-ICE). Domain-mean surface precipitation is insensitive to aerosols primarily because the large-scale forcing is prescribed and dominates the water and static energy budgets. The spread of the top-of-atmosphere (TOA) shortwave and longwave radiative fluxes among different ensemble members for the same aerosol loading is surprisingly large, exceeding 25 W m−2 even when averaged over the 6-day period. This variability is caused by random fluctuations in the strength and timing of individual deep convective events. The ensemble approach demonstrates a small weakening of convection averaged over the 6-day period in the polluted simulations compared to pristine. Despite this weakening, the cloud top heights and anvil ice mixing ratios are higher in polluted conditions. This occurs because of the larger concentrations of cloud droplets that freeze, leading directly to higher ice particle concentrations, smaller ice particle sizes, and smaller fall velocities compared to simulations with pristine aerosols. Weaker convection in polluted conditions is a direct result of the changes in anvil ice characteristics and subsequent upper-tropospheric radiative heating and weaker tropospheric destabilization. Such a conclusion offers a different interpretation of recent satellite observations of tropical deep convection in pristine and polluted environments compared to the hypothesis of aerosol-induced convective invigoration. Sensitivity tests using the ensemble approach with modified microphysical parameters or domain configuration (horizontal gridlength, domain size) produce results that are similar to baseline, although there are quantitative differences in estimates of aerosol impacts on TOA radiative fluxes.
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Morrison, H., and W. W. Grabowski. "Cloud-system resolving model simulations of aerosol indirect effects on tropical deep convection and its thermodynamic environment." Atmospheric Chemistry and Physics 11, no. 20 (October 24, 2011): 10503–23. http://dx.doi.org/10.5194/acp-11-10503-2011.
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Abstract. This paper presents results from 240-member ensemble simulations of aerosol indirect effects on tropical deep convection and its thermodynamic environment. Simulations using a two-dimensional cloud-system resolving model are run with pristine, polluted, or highly polluted aerosol conditions and large-scale forcing from a 6-day period of active monsoon conditions during the 2006 Tropical Warm Pool – International Cloud Experiment (TWP-ICE). Domain-mean surface precipitation is insensitive to aerosols primarily because the large-scale forcing is prescribed and dominates the water and static energy budgets. The spread of the top-of-atmosphere (TOA) shortwave and longwave radiative fluxes among different ensemble members for the same aerosol loading is surprisingly large, exceeding 25 W m−2 even when averaged over the 6-day period. This variability is caused by random fluctuations in the strength and timing of individual deep convective events. The ensemble approach demonstrates a small weakening of convection averaged over the 6-day period in the polluted simulations compared to pristine. Despite this weakening, the cloud top heights and anvil ice mixing ratios are higher in polluted conditions. This occurs because of the larger concentrations of cloud droplets that freeze, leading directly to higher ice particle concentrations, smaller ice particle sizes, and smaller fall velocities compared to simulations with pristine aerosols. Weaker convection in polluted conditions is a direct result of the changes in anvil ice characteristics and subsequent upper-tropospheric radiative heating and weaker tropospheric destabilization. Such a conclusion offers a different interpretation of recent satellite observations of tropical deep convection in pristine and polluted environments compared to the hypothesis of aerosol-induced convective invigoration. Sensitivity tests using the ensemble approach with modified microphysical parameters or domain configuration (horizontal gridlength, domain size) produce results that are similar to baseline, although there are quantitative differences in estimates of aerosol impacts on TOA radiative fluxes.
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Lee, Eunjeong, Jung-Hoon Kim, Ki-Young Heo, and Yang-Ki Cho. "Advection Fog over the Eastern Yellow Sea: WRF Simulation and Its Verification by Satellite and In Situ Observations." Remote Sensing 13, no. 8 (April 12, 2021): 1480. http://dx.doi.org/10.3390/rs13081480.
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An observed sea fog event over the Eastern Yellow Sea on 15–16 April 2012 was reproduced in the Weather Research and Forecasting (WRF) simulation with high-resolution to investigate the roles of physical processes and synoptic-scale flows on advection fog with phase transition. First, it was verified by a satellite-based fog detection algorithm and in situ observation data. In the simulation, longwave (infrared) radiative cooling (LRC) with a downward turbulent sensible heat flux (SHF), due to the turbulence after sunset, triggered cloud formation over the surface when warm-moist air advection occurred. At night, warm air advection with continuous cooling due to longwave radiation and SHF near the surface modulated the change of the SHF from downward to upward, resulting in a drastic increase in the turbulent latent heat flux (LHF) that provided sufficient moisture at the lower atmosphere (self-moistening). This condition represents a transition from cold-sea fog to warm-sea fog. Enhanced turbulent mixing driven by a buoyancy force increased the depth of the sea fog and the marine atmospheric boundary layer (MABL) height, even at nighttime. In addition, cold air advection with a prevailing northerly wind at the top of the MABL led to a drastic increase in turbulent mixing and the MABL height and rapid growth of the height of sea fog. After sunrise, shortwave radiative warming in the fog layers offsetting the LRC near the surface weakened thermal instability, which contributed to the reduction in the MABL height, even during the daytime. In addition, dry advection of the northerly wind induced dissipation of the fog via evaporation. An additional sensitivity test of sea surface salinity showed weaker and shallower sea fog than the control due to the decrease in both the LHF and local self-moistening. Detailed findings from the simulated fog event can help to provide better guidance for fog detection using remote sensing.
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Gupta, Siddhant, Greg M. McFarquhar, Joseph R. O'Brien, David J. Delene, Michael R. Poellot, Amie Dobracki, James R. Podolske, et al. "Impact of the variability in vertical separation between biomass burning aerosols and marine stratocumulus on cloud microphysical properties over the Southeast Atlantic." Atmospheric Chemistry and Physics 21, no. 6 (March 25, 2021): 4615–35. http://dx.doi.org/10.5194/acp-21-4615-2021.
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Abstract. Marine stratocumulus cloud properties over the Southeast Atlantic Ocean are impacted by contact between above-cloud biomass burning aerosols and cloud tops. Different vertical separations (0 to 2000 m) between the aerosol layer and cloud tops were observed on six research flights in September 2016 during the NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign. There were 30 contact profiles, where an aerosol layer with aerosol concentration (Na) > 500 cm−3 was within 100 m of cloud tops, and 41 separated profiles, where the aerosol layer with Na > 500 cm−3 was located more than 100 m above cloud tops. For contact profiles, the average cloud droplet concentration (Nc) in the cloud layer was up to 68 cm−3 higher, the effective radius (Re) up to 1.3 µm lower, and the liquid water content (LWC) within 0.01 g m−3 compared to separated profiles. Free-tropospheric humidity was higher in the presence of biomass burning aerosols, and contact profiles had a smaller decrease in humidity (and positive buoyancy) across cloud tops with higher median above-cloud Na (895 cm−3) compared to separated profiles (30 cm−3). Due to droplet evaporation from entrainment mixing of warm, dry free-tropospheric air into the clouds, the median Nc and LWC for contact profiles decreased with height by 21 and 9 % in the top 20 % of the cloud layer. The impact of droplet evaporation was stronger during separated profiles as a greater decrease in humidity (and negative buoyancy) across cloud tops led to greater decreases in median Nc (30 %) and LWC (16 %) near cloud tops. Below-cloud Na was sampled during 61 profiles, and most contact profiles (20 out of 28) were within high-Na (> 350 cm−3) boundary layers, while most separated profiles (22 out of 33) were within low-Na (< 350 cm−3) boundary layers. Although the differences in below-cloud Na were statistically insignificant, contact profiles within low-Na boundary layers had up to 34.9 cm−3 higher Nc compared to separated profiles. This is consistent with a weaker impact of droplet evaporation in the presence of biomass burning aerosols within 100 m above cloud tops. For contact profiles within high-Na boundary layers, the presence of biomass burning aerosols led to higher below-cloud Na (up to 70.5 cm−3) and additional droplet nucleation above the cloud base along with weaker droplet evaporation. Consequently, the contact profiles in high-Na boundary layers had up to 88.4 cm−3 higher Nc compared to separated profiles. These results motivate investigations of aerosol–cloud–precipitation interactions over the Southeast Atlantic since the changes in Nc and Re induced by the presence of above-cloud biomass burning aerosols are likely to impact precipitation rates, liquid water path, and cloud fraction, and modulate closed-to-open-cell transitions.
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Dayan, Chen, Erick Fredj, Pawel K. Misztal, Maor Gabay, Alex B. Guenther, and Eran Tas. "Emission of biogenic volatile organic compounds from warm and oligotrophic seawater in the Eastern Mediterranean." Atmospheric Chemistry and Physics 20, no. 21 (November 4, 2020): 12741–59. http://dx.doi.org/10.5194/acp-20-12741-2020.
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Abstract. Biogenic volatile organic compounds (BVOCs) from terrestrial vegetation and marine organisms contribute to photochemical pollution and affect the radiation budget, cloud properties and precipitation via secondary organic aerosol formation. Their emission from both marine and terrestrial ecosystems is substantially affected by climate change in ways that are currently not well characterized. The Eastern Mediterranean Sea was identified as a climate change “hot spot”, making it a natural laboratory for investigating the impact of climate change on BVOC emissions from both terrestrial and marine vegetation. We quantified the mixing ratios of a suite of volatile organic compounds (VOCs), including isoprene, dimethyl sulfide (DMS), acetone, acetaldehyde and monoterpenes, at a mixed vegetation site ∼4 km from the southeastern tip of the Levantine Basin, where the sea surface temperature (SST) maximizes and ultra-oligotrophic conditions prevail. The measurements were performed between July and October 2015 using a proton transfer reaction time-of-flight mass spectrometer (PTR-ToF-MS). The analyses were supported by the Model of Emissions of Gases and Aerosols from Nature (MEGAN v2.1). For isoprene and DMS mixing ratios, we identified a dominant contribution from the seawater. Our analyses further suggest a major contribution, at least for monoterpenes, from the seawater. Our results indicate that the Levantine Basin greatly contributes to isoprene emissions, corresponding with mixing ratios of up to ∼9 ppbv several kilometers inland from the sea shore. This highlights the need to update air quality and climate models to account for the impact of SST on marine isoprene emission. The DMS mixing ratios were 1 to 2 orders of magnitude lower than those measured in 1995 in the same area, suggesting a dramatic decrease in emissions due to changes in the species composition induced by the rise in SST.
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Liu, W. Timothy, Xiaosu Xie, and Pearn P. Niiler. "Ocean–Atmosphere Interaction over Agulhas Extension Meanders." Journal of Climate 20, no. 23 (December 1, 2007): 5784–97. http://dx.doi.org/10.1175/2007jcli1732.1.
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Abstract Many years of high-resolution measurements by a number of space-based sensors and from Lagrangian drifters became available recently and are used to examine the persistent atmospheric imprints of the semipermanent meanders of the Agulhas Extension Current (AEC), where strong surface current and temperature gradients are found. The sea surface temperature (SST) measured by the Advanced Microwave Scanning Radiometer-Earth Observing System (AMSR-E) and the chlorophyll concentration measured by the Sea-viewing Wide Field-of-view Sensor (SeaWiFS) support the identification of the meanders and related ocean circulation by the drifters. The collocation of high and low magnitudes of equivalent neutral wind (ENW) measured by Quick Scatterometer (QuikSCAT), which is uniquely related to surface stress by definition, illustrates not only the stability dependence of turbulent mixing but also the unique stress measuring capability of the scatterometer. The observed rotation of ENW in opposition to the rotation of the surface current clearly demonstrates that the scatterometer measures stress rather than winds. The clear differences between the distributions of wind and stress and the possible inadequacy of turbulent parameterization affirm the need of surface stress vector measurements, which were not available before the scatterometers. The opposite sign of the stress vorticity to current vorticity implies that the atmosphere spins down the current rotation through momentum transport. Coincident high SST and ENW over the southern extension of the meander enhance evaporation and latent heat flux, which cools the ocean. The atmosphere is found to provide negative feedback to ocean current and temperature gradients. Distribution of ENW convergence implies ascending motion on the downwind side of local SST maxima and descending air on the upwind side and acceleration of surface wind stress over warm water (deceleration over cool water); the convection may escalate the contrast of ENW over warm and cool water set up by the dependence of turbulent mixing on stability; this relation exerts a positive feedback to the ENW–SST relation. The temperature sounding measured by the Atmospheric Infrared Sounder (AIRS) is consistent with the spatial coherence between the cloud-top temperature provided by the International Satellite Cloud Climatology Project (ISCCP) and SST. Thus ocean mesoscale SST anomalies associated with the persistent meanders may have a long-term effect well above the midlatitude atmospheric boundary layer, an observation not addressed in the past.
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Paulik, L. C., and T. Birner. "Quantifying the deep convective temperature signal within the tropical tropopause layer (TTL)." Atmospheric Chemistry and Physics 12, no. 24 (December 21, 2012): 12183–95. http://dx.doi.org/10.5194/acp-12-12183-2012.
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Abstract. Dynamics on a vast range of spatial and temporal scales, from individual convective plumes to planetary-scale circulations, play a role in driving the temperature variability in the tropical tropopause layer (TTL). Here, we aim to better quantify the deep convective temperature signal within the TTL using multiple datasets. First, we investigate the link between ozone and temperature in the TTL using the Southern Hemisphere Additional Ozonesondes (SHADOZ) dataset. Low ozone concentrations in the TTL are indicative of deep convective transport from the boundary layer. We confirm the usefulness of ozone as an indicator of deep convection by identifying a typical temperature signal associated with reduced ozone events: an anomalously warm mid to upper troposphere and an anomalously cold upper TTL. We quantify these temperature signals using two diagnostics: (1) the "ozone minimum" diagnostic, which has been used in previous studies and identifies the upper tropospheric minimum ozone concentration as a proxy for the level of main convective outflow; and (2) the "ozone mixing height", which we introduce in order to identify the maximum altitude in a vertical ozone profile up to which reduced ozone concentrations, typical of transport from the boundary layer are observed. Results indicate that the ozone mixing height diagnostic better separates profiles with convective influence than the ozone minimum diagnostic. Next, we collocate deep convective clouds identified by CloudSat 2B-CLDCLASS with temperature profiles based on Constellation Observing System for Meteorology, Ionosphere, and Climate (COSMIC) Global Position System (GPS) radio occultations. We find a robust large-scale deep convective TTL temperature signal, that is persistent in time. However, it is only the convective events that penetrate into the upper half of the TTL that have a significant impact on TTL temperature. A distinct seasonal difference in the spatial scale and the persistence of the temperature signal is identified. Deep-convective cloud top heights are on average found to be well described by the level of neutral buoyancy.
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Komaromi, William A. "An Investigation of Composite Dropsonde Profiles for Developing and Nondeveloping Tropical Waves during the 2010 PREDICT Field Campaign." Journal of the Atmospheric Sciences 70, no. 2 (February 1, 2013): 542–58. http://dx.doi.org/10.1175/jas-d-12-052.1.
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Abstract Composite dropsonde profiles are analyzed for developing and nondeveloping tropical waves in an attempt to improve the understanding of tropical cyclogenesis. These tropical waves were sampled by 25 reconnaissance missions during the 2010 Pre-Depression Investigation of Cloud-Systems in the Tropics (PREDICT) field campaign. Comparisons are made between mean profiles of temperature, mixing ratio, relative humidity, radial and tangential winds, relative vorticity, and virtual convective available potential energy (CAPE) for genesis and nongenesis cases. Genesis soundings are further analyzed in temporal progression to investigate whether significant changes in the thermodynamic or wind fields occur during the transition from tropical wave to tropical cyclone. Significant results include the development of positive temperature anomalies from 500 to 200 hPa 2 days prior to genesis in developing waves. This is not observed in the nongenesis mean. Progressive mesoscale moistening of the column is observed within 150 km of the center of circulation prior to genesis. The genesis composite is found to be significantly moister than the nongenesis composite at the middle levels, while comparatively drier at low levels, suggesting that dry air is more detrimental to genesis when located at the middle levels. Time-varying tangential wind profiles reveal an initial delay in intensification, followed by an increase in organization 24 h pregenesis. The vertical evolution of relative vorticity, in addition to a warm-over-cold thermal structure, is more consistent with a top-down than a bottom-up genesis mechanism. Last, CAPE values are much greater for nongenesis than genesis profiles, indicating that greater instability does not necessarily favor genesis.
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Jeong, Gill-Ran. "Weather Effects of Aerosols in the Global Forecast Model." Atmosphere 11, no. 8 (August 12, 2020): 850. http://dx.doi.org/10.3390/atmos11080850.
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The weather effects of aerosol types were investigated using well-posed aerosol climatology through the aerosol sensitivity test of thermodynamic and hydrometeor fields, and the weather forecast performances in July of 2017. The largest aerosol direct radiative forcing (ADRF) in July was due to dust aerosols at the surface and atmosphere, and sulfate at the top of the atmosphere (TOA), respectively. The ADRF of total aerosols had unilateral tendencies in thermodynamic and hydrometeor fields. The contribution of individual aerosols was linearly additive to those of total aerosols in the heat fluxes, heating rates, humidity, and convective precipitation. However, no such linearity existed in temperature, geopotential height, cloud liquid or ice contents, and large-scale precipitation. Dust was the most influential forcing agent in July among five aerosol types due to the largest light-absorption capacity. Such unilateral tendencies of total aerosols and a part of the linearity of individual aerosols were exerted on the weather systems. The verification of medium-range forecasts showed that aerosols alleviated the overestimation of surface shortwave (SW) downward fluxes, the negative biases of temperature and geopotential heights at TOA and surface, and the underestimation in light and moderate precipitation. In contrast, they enhanced warm biases at the mid-atmosphere and underestimation in heavy precipitations, particularly negative biases in the intertropical convergence zone (ITCZ). Weather forecast scores including current aerosol information were improved in geopotential height (GPH) of the northern hemisphere (NH); however, they got worse in the temperature and the upper atmosphere GPH of the southern hemisphere (SH), which was mostly due to black carbon (BC) aerosols in the tropical regions. The missing mechanisms such as aerosol–cloud interactions, better aerosol spectral optical properties including mixing states and aging, and the near-real-time (NRT) based aerosol loading data are worthwhile to be tried in the near future for fixing the intrinsic underestimation of precipitation in ITCZ and surface radiative fluxes in the desert and biomass burning area.
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Sokol, Adam B., and Dennis L. Hartmann. "Radiative Cooling, Latent Heating, and Cloud Ice in the Tropical Upper Troposphere." Journal of Climate 35, no. 5 (March 1, 2022): 1643–54. http://dx.doi.org/10.1175/jcli-d-21-0444.1.
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Abstract The radiative cooling rate in the tropical upper troposphere is expected to increase as climate warms. Since the tropics are approximately in radiative–convective equilibrium (RCE), this implies an increase in the convective heating rate, which is the sum of the latent heating rate and the eddy heat flux convergence. We examine the impact of these changes on the vertical profile of cloud ice amount in cloud-resolving simulations of RCE. Three simulations are conducted: a control run, a warming run, and an experimental run in which there is no warming but a temperature forcing is imposed to mimic the warming-induced increase in radiative cooling. Surface warming causes a reduction in cloud fraction at all upper-tropospheric temperature levels but an increase in the ice mixing ratio within deep convective cores. The experimental run has more cloud ice than the warming run at fixed temperature despite the fact that their latent heating rates are equal, which suggests that the efficiency of latent heating by cloud ice increases with warming. An analytic expression relating the ice-related latent heating rate to a number of other factors is derived and used to understand the model results. This reveals that the increase in latent heating efficiency is driven mostly by 1) the migration of isotherms to lower pressure and 2) a slight warming of the top of the convective layer. These physically robust changes act to reduce the residence time of ice at any particular temperature level, which tempers the response of the mean cloud ice profile to warming. Significance Statement Here we examine how the amount of condensed ice in part of the atmosphere—the tropical upper troposphere (UT)—responds to global warming. In the UT, the energy released during ice formation is balanced by the emission of radiation to space. This emission will strengthen with warming, suggesting that there will also be more ice. Using a model of the tropical atmosphere, we find that the increase in ice amount is mitigated by a reduction in the amount of time ice spends in the UT. This could have important implications for the cloud response to global warming, and future work should focus on how these changes are manifested across the distribution of convective cloud types.
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Fierro, Alexandre O., Lance M. Leslie, Edward R. Mansell, and Jerry M. Straka. "Numerical Simulations of the Microphysics and Electrification of the Weakly Electrified 9 February 1993 TOGA COARE Squall Line: Comparisons with Observations." Monthly Weather Review 136, no. 1 (January 1, 2008): 364–79. http://dx.doi.org/10.1175/2007mwr2156.1.
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Abstract A cloud scale model with a 12-class bulk microphysics scheme, including 10 ice phases and a 3D lightning parameterization, was used to investigate the electrical properties of a well-documented tropical squall line from the Tropical Ocean Global Atmosphere Coupled Ocean–Atmosphere Response Experiment (TOGA COARE). Consistent with observations, the simulated maximum updraft speeds across the squall line seldom exceeded 10 m s−1, which was expected given the relatively shallow 30-dBZ echo tops that rarely extended above the top of the mixed-phase layer (−20°C isotherm). Enhanced warm rain processes caused most of the liquid water to precipitate near the gust front at lower levels (below 4 km AGL), which accounted for the small amounts of graupel and cloud water content present in the mixed-phase region and, consequently, for generally weak charging and electrification. Most of the charge present in the squall line was generated within a few storm cells just behind the leading edge of the gust front that had sufficiently strong updraft speeds near the melting level to produce moderate values of graupel mixing ratio (>0.5 g kg−1). In contrast, the trailing stratiform region at the back of the line, which was mainly composed of ice crystals and snow particles, contained only weak net charge densities (<0.03 nC m−3). The spatial collocation of regions characterized by charge densities exceeding 0.01 nC m−3 and noninductive (NI) charging rates greater than 0.1 pC m−3 s−1 in this stratiform region suggests that NI charging is a plausible source for the majority of this charge, which was confined to discrete regions having small amounts of graupel (approximately 0.1–0.3 g kg−1) and cloud water content (CWC; ∼0.1 g m−3). The simulated weak updraft speeds and shallow echo tops resulted in a system exhibiting little overall total lightning activity. Although the 5-min average intracloud (IC) flash rate rarely exceeded 10 flashes per minute and only 3 negative cloud-to-ground (−CG) lightning flashes were produced during the entire 4 h and 30 min of simulation, this still was more electrical activity than observed. This tendency for the model to generate more lightning flashes than observed remained when the inductive charging mechanism was turned off, which reduced the total amount of simulated flashes by about 43%. The three CG flashes and the great majority of the IC flashes occurred within the strongest cells located in the mature zone, which exhibited a normal tripole charge structure.
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Brâncuş, Mihaela, David M. Schultz, Bogdan Antonescu, Christopher Dearden, and Sabina Ştefan. "Origin of Strong Winds in an Explosive Mediterranean Extratropical Cyclone." Monthly Weather Review 147, no. 10 (September 27, 2019): 3649–71. http://dx.doi.org/10.1175/mwr-d-19-0009.1.
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Abstract During 2–3 December 2012, the Black Sea and east coast of Romania were affected by a rapidly deepening Mediterranean cyclone. The cyclone developed a bent-back front along which short-lived (2–4 h) strong winds up to 38 m s−1 were recorded equatorward of the cyclone center. A mesoscale model simulation was used to analyze the evolution of the wind field, to investigate the physical processes that were responsible for the strong winds and their acceleration, and to investigate the relative importance of the stability of the boundary layer to those strong winds. The origin of the air in the wind maximum equatorward of the cyclone center was twofold. The first was associated with a sting jet, a descending airstream from the midlevels of the cloud head and the lower part of the cyclonic branch of the warm conveyor belt. The sting jet started to descend west of the cyclone center, ending at the frontolytic tip of the bent-back front. The second was a low-level airstream associated with the cold conveyor belt that originated northeast of the cyclone center and traveled below 900 hPa along the cold side of the bent-back front, ending behind the cold front. Both airstreams were accelerated by the along-flow pressure gradient force, with the largest accelerations acting on the sting-jet air before entering into the near-surface strong-wind area. The sensible heat fluxes destabilized the boundary layer to near-neutral conditions south of the cyclone center, facilitating downward mixing and allowing the descending air to reach the surface. Mesoscale instabilities appeared to be unimportant in the sting-jet formation.
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Barreto, África, Emilio Cuevas, Rosa D. García, Judit Carrillo, Joseph M. Prospero, Luka Ilić, Sara Basart, et al. "Long-term characterisation of the vertical structure of the Saharan Air Layer over the Canary Islands using lidar and radiosonde profiles: implications for radiative and cloud processes over the subtropical Atlantic Ocean." Atmospheric Chemistry and Physics 22, no. 2 (January 18, 2022): 739–63. http://dx.doi.org/10.5194/acp-22-739-2022.
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Abstract. Every year, large-scale African dust outbreaks frequently pass over the Canary Islands (Spain). Here we describe the seasonal evolution of atmospheric aerosol extinction and meteorological vertical profiles on Tenerife over the period 2007–2018 using long-term micropulse lidar (MPL-3) and radiosonde observations. These measurements are used to categorise the different patterns of dust transport over the subtropical North Atlantic and, for the first time, to robustly describe the dust vertical distribution in the Saharan Air Layer (SAL) over this region. Three atmospheric scenarios dominate the aerosol climatology: dust-free (clean) conditions, the Saharan summer scenario (summer-SAL) and the Saharan winter scenario (winter-SAL). A relatively well-mixed marine boundary layer (MBL) was observed in the case of clean (dust-free) conditions; it was associated with rather constant lidar extinction coefficients (α) below 0.036 km−1 with minimum α (< 0.022 km−1) in the free troposphere (FT). The summer-SAL has been characterised as a dust-laden layer strongly affecting both the MBL (Δα = +48 % relative to clean conditions) and the FT. The summer-SAL appears as a well-stratified layer, relatively dry at lower levels (Δr∼-44 % at the SAL’s base, where r is the water vapour mixing ratio) but more humid at higher levels compared with clean FT conditions (Δr∼+332 % at 5.3 km), with a peak of α> 0.066 km−1 at ∼ 2.5 km. Desert dust is present up to ∼ 6.0 km, the SAL top based on the altitude of SAL's temperature inversion. In the winter-SAL scenario, the dust layer is confined to lower levels below 2 km altitude. This layer is characterised by a dry anomaly at lower levels (Δr∼ −38 % in comparison to the clean scenario) and a dust peak at ∼ 1.3 km height. Clean FT conditions were found above 2.3 km. Our results reveal the important role that both dust and water vapour play in the radiative balance within the summer-SAL and winter-SAL. The dominant dust-induced shortwave (SW) radiative warming in summer (heating rates up to +0.7 K d−1) is found slightly below the dust maximum. However, the dominant contribution of water vapour was observed as a net SW warming observed within the SAL (from 2.1 to 5.7 km) and as a strong cold anomaly near the SAL's top (−0.6 K d−1). The higher water vapour content found to be carried on the summer-SAL, despite being very low, represents a high relative variation in comparison to the very dry clean free troposphere in the subtropics. This relevant aspect should be properly taken into account in atmospheric modelling processes. In the case of the winter-SAL, we observed a dust-induced radiative effect dominated by SW heating (maximum heating of +0.7 K d−1 at 1.5 km, near the dust peak); both dust and atmospheric water vapour impact heating in the atmospheric column. This is the case of the SW heating within the SAL (maximum near the r peak), the dry anomaly at lower levels (Δr∼ −38 % at 1 km) and the thermal cooling (∼ 0.3 K d−1) from the temperature inversion upwards. Finally, we hypothesise that the SAL can impact heterogeneous ice nucleation processes through the frequent occurrence of mid-level clouds observed near the SAL top at relatively warm temperatures. A dust event that affected Tenerife on August 2015 is simulated using the regional DREAM model to assess the role of dust and water vapour carried within SAL in the ice nucleation processes. The modelling results reproduce the arrival of the dust plume and its extension over the island and confirm the observed relationship between the summer-SAL conditions and the formation of mid- and high-level clouds.
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STEVENS, B. "Cloud-top entrainment instability?" Journal of Fluid Mechanics 660 (September 16, 2010): 1–4. http://dx.doi.org/10.1017/s0022112010003575.
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Mixing processes at cloud boundaries are thought to play a critical role in determining cloud lifetime, spatial extent and cloud microphysical structure. High-fidelity direct numerical simulations by Mellado (J. Fluid Mech., 2010, this issue, vol. 660, pp. 5–36) show, for the first time, the character and potency of a curious instability that may arise as a result of molecular mixing processes at cloud boundaries, an instability which until now has been thought by many to control the distribution of climatologically important cloud regimes.
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Morrison, Hugh, and Wojciech W. Grabowski. "Modeling Supersaturation and Subgrid-Scale Mixing with Two-Moment Bulk Warm Microphysics." Journal of the Atmospheric Sciences 65, no. 3 (March 1, 2008): 792–812. http://dx.doi.org/10.1175/2007jas2374.1.
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Abstract This paper describes further developments of a two-moment warm rain bulk microphysics scheme suitable for addressing the indirect impact of atmospheric aerosols on ice-free clouds in large-eddy simulation (LES) models. The emphasis is on the prediction of supersaturation, activation of cloud droplets, and the representation of microphysical transformations during parameterized turbulent mixing. A comprehensive approach is proposed that is capable of simulating droplet activation at the cloud base, in the cloud interior due to increasing updraft strength, and at the lateral edges due to entrainment. Such an approach requires high spatial resolution to capture maximum supersaturation at cloud base as well as to resolve entraining eddies that lead to additional activation above the cloud base. This approach can be used as a benchmark for developing and testing schemes suitable for lower spatial resolutions. A novel approach for predicting the supersaturation field is proposed, with an emphasis on its application in an Eulerian framework. This approach produces consistency among the thermodynamic variables and mitigates the problem of spurious cloud-edge supersaturation noted in the past. A new subgrid scheme is also developed to treat microphysical transformations during turbulent entrainment and mixing. This scheme is designed to be as flexible as possible, allowing for the entire range of mixing scenarios from homogeneous to extremely inhomogeneous. The above developments are applied in 2D simulations of moist convection for an idealized rising thermal, assuming either pristine or polluted aerosol conditions. The mixing scenario has a substantial impact on the cloud microphysical and optical properties. As expected, extremely inhomogeneous mixing results in substantially smaller mean droplet number concentration, larger effective radius, and smaller cloud optical depth compared to the run with homogeneous mixing. The subgrid mixing of cloud condensation nuclei (CCN) and formation of CCN from evaporated droplets during extremely inhomogeneous mixing are relatively less important for this case.
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MELLADO, JUAN PEDRO. "The evaporatively driven cloud-top mixing layer." Journal of Fluid Mechanics 660 (July 27, 2010): 5–36. http://dx.doi.org/10.1017/s0022112010002831.
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Direct numerical simulations of the turbulent temporally evolving cloud-top mixing layer are used to investigate the role of evaporative cooling by isobaric mixing locally at the stratocumulus top. It is shown that the system develops a horizontal layered structure whose evolution is determined by molecular transport. A relatively thin inversion with a constant thickness h = κ/we is formed on top and travels upwards at a mean velocity we ≃ 0.1(κ |bs|χc2)1/3, where κ is the mixture-fraction diffusivity, bs < 0 is the buoyancy anomaly at saturation conditions χs and χc is the cross-over mixture fraction defining the interval of buoyancy reversing mixtures. A turbulent convection layer develops below and continuously broadens into the cloud (the lower saturated fluid). This turbulent layer approaches a self-preserving state that is characterized by the convection scales constructed from a constant reference buoyancy flux Bs = |bs|we/χs. Right underneath the inversion base, a transition or buffer zone is defined based on a strong local conversion of vertical to horizontal motion that leads to a cellular pattern and sheet-like plumes, as observed in cloud measurements and reported in other free-convection problems. The fluctuating saturation surface (instantaneous cloud top) is contained inside this intermediate region. Results show that the inversion is not broken due to the turbulent convection generated by the evaporative cooling, and the upward mean entrainment velocity we is negligibly small compared to the convection velocity scale w* of the turbulent layer and the corresponding growth rate into the cloud.
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Mellado, Juan Pedro, Bjorn Stevens, Heiko Schmidt, and Norbert Peters. "Buoyancy reversal in cloud-top mixing layers." Quarterly Journal of the Royal Meteorological Society 135, no. 641 (April 2009): 963–78. http://dx.doi.org/10.1002/qj.417.
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Huang, Yi, Steven Siems, Michael Manton, Alain Protat, Leon Majewski, and Hanh Nguyen. "Evaluating Himawari-8 Cloud Products Using Shipborne and CALIPSO Observations: Cloud-Top Height and Cloud-Top Temperature." Journal of Atmospheric and Oceanic Technology 36, no. 12 (December 2019): 2327–47. http://dx.doi.org/10.1175/jtech-d-18-0231.1.
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AbstractCloud-top height (CTH) and cloud-top temperature (CTT) retrieved from the Himawari-8 observations are evaluated using the active shipborne radar–lidar observations derived from the 31-day Clouds, Aerosols, Precipitation Radiation and Atmospheric Composition over the Southern Ocean (CAPRICORN) experiment in 2016 and 1-yr observations from the spaceborne Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) cloud product over a large sector of the Southern Ocean. The results show that the Himawari-8 CTH (CTT) retrievals agree reasonably well with both the shipborne estimates, with a correlation coefficient of 0.837 (0.820), a mean bias error of 0.226 km (−2.526°C), and an RMSE of 1.684 km (10.069°C). In the comparison with CALIOP, the corresponding quantities are found to be 0.786 (0.480), −0.570 km (1.343°C), and 2.297 km (25.176°C). The Himawari-8 CTH (CTT) generally falls between the physical CTHs observed by CALIOP and the shipborne radar–lidar estimates. However, major systematic biases are also identified. These errors include (i) a low (warm) bias in CTH (CTT) for warm liquid cloud type, (ii) a cold bias in CTT for supercooled liquid water cloud type, (iii) a lack of CTH at ~3 km that does not have a corresponding gap in CTT, (iv) a tendency of misclassifying some low-/mid-top clouds as cirrus and overlap cloud types, and (v) a saturation of CTH (CTT) around 10 km (−40°C), particularly for cirrus and overlap cloud types. Various challenges that underpin these biases are also explored, including the potential of parallax bias, low-level inversion, and cloud heterogeneity.
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Ruiz-Donoso, Elena, André Ehrlich, Michael Schäfer, Evelyn Jäkel, Vera Schemann, Susanne Crewell, Mario Mech, et al. "Small-scale structure of thermodynamic phase in Arctic mixed-phase clouds observed by airborne remote sensing during a cold air outbreak and a warm air advection event." Atmospheric Chemistry and Physics 20, no. 9 (May 12, 2020): 5487–511. http://dx.doi.org/10.5194/acp-20-5487-2020.
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Abstract. The combination of downward-looking airborne lidar, radar, microwave, and imaging spectrometer measurements was exploited to characterize the vertical and small-scale (down to 10 m) horizontal distribution of the thermodynamic phase of low-level Arctic mixed-layer clouds. Two cloud cases observed in a cold air outbreak and a warm air advection event observed during the Arctic CLoud Observations Using airborne measurements during polar Day (ACLOUD) campaign were investigated. Both cloud cases exhibited the typical vertical mixed-phase structure with mostly liquid water droplets at cloud top and ice crystals in lower layers. The horizontal, small-scale distribution of the thermodynamic phase as observed during the cold air outbreak is dominated by the liquid water close to the cloud top and shows no indication of ice in lower cloud layers. Contrastingly, the cloud top variability in the case observed during a warm air advection showed some ice in areas of low reflectivity or cloud holes. Radiative transfer simulations considering homogeneous mixtures of liquid water droplets and ice crystals were able to reproduce the horizontal variability in this warm air advection. Large eddy simulations (LESs) were performed to reconstruct the observed cloud properties, which were used subsequently as input for radiative transfer simulations. The LESs of the cloud case observed during the cold air outbreak, with mostly liquid water at cloud top, realistically reproduced the observations. For the warm air advection case, the simulated ice water content (IWC) was systematically lower than the measured IWC. Nevertheless, the LESs revealed the presence of ice particles close to the cloud top and confirmed the observed horizontal variability in the cloud field. It is concluded that the cloud top small-scale horizontal variability is directly linked to changes in the vertical distribution of the cloud thermodynamic phase. Passive satellite-borne imaging spectrometer observations with pixel sizes larger than 100 m miss the small-scale cloud top structures.
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Malinowski, S. P., H. Gerber, I. Jen-La Plante, M. K. Kopec, W. Kumala, K. Nurowska, P. Y. Chuang, D. Khelif, and K. E. Haman. "Physics of Stratocumulus Top (POST): turbulent mixing across capping inversion." Atmospheric Chemistry and Physics Discussions 13, no. 6 (June 11, 2013): 15233–69. http://dx.doi.org/10.5194/acpd-13-15233-2013.
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Abstract. High spatial resolution measurements of temperature and liquid water content, accompanied by moderate resolution measurements of humidity and turbulence, collected during the Physics of Stratocumulus Top experiment are analyzed. Two thermodynamically, meteorologically and even optically different cases are investigated. An algorithmic division of the cloud top region into layers is proposed. Analysis of dynamic stability across these layers leads to the conclusion that the inversion capping the cloud and the cloud top region are turbulent due to the wind shear, which is strong enough to compensate for high static stability of the inversion. The thickness of this mixing layer adapts to wind and temperature jumps such that the gradient Richardson number stays close to its critical value. Turbulent mixing governs transport across the inversion, but the consequences of this mixing depend on the thermodynamic properties of cloud top and free troposphere. The effects of buoyancy-sorting of the mixed parcels in the cloud top region are different in conditions that permit or prevent cloud top entrainment instability. Removal of negatively buoyant air from the cloud top is observed in the first case, while buildup of the diluted cloud top layer is observed in the second one.
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Malinowski, S. P., H. Gerber, I. Jen-La Plante, M. K. Kopec, W. Kumala, K. Nurowska, P. Y. Chuang, D. Khelif, and K. E. Haman. "Physics of Stratocumulus Top (POST): turbulent mixing across capping inversion." Atmospheric Chemistry and Physics 13, no. 24 (December 17, 2013): 12171–86. http://dx.doi.org/10.5194/acp-13-12171-2013.
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Abstract. High spatial resolution measurements of temperature and liquid water content, accompanied by moderate-resolution measurements of humidity and turbulence, collected during the Physics of Stratocumulus Top experiment are analyzed. Two thermodynamically, meteorologically and even optically different cases are investigated. An algorithmic division of the cloud-top region into layers is proposed. Analysis of dynamic stability across these layers leads to the conclusion that the inversion capping the cloud and the cloud-top region is turbulent due to the wind shear, which is strong enough to overcome the high static stability of the inversion. The thickness of this mixing layer adapts to wind and temperature jumps such that the gradient Richardson number stays close to its critical value. Turbulent mixing governs transport across the inversion, but the consequences of this mixing depend on the thermodynamic properties of cloud top and free troposphere. The effects of buoyancy sorting of the mixed parcels in the cloud-top region are different in conditions that permit or prevent cloud-top entrainment instability. Removal of negatively buoyant air from the cloud top is observed in the first case, while buildup of the diluted cloud-top layer is observed in the second one.
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Liu, Qiong, Hailin Wang, Xiaoqin Lu, Bingke Zhao, Yonghang Chen, Wenze Jiang, and Haijiang Zhou. "Tropical Cyclone Temperature Profiles and Cloud Macro-/Micro-Physical Properties Based on AIRS Data." Atmosphere 11, no. 11 (November 2, 2020): 1181. http://dx.doi.org/10.3390/atmos11111181.
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We used the observations from Atmospheric Infrared Sounder (AIRS) onboard Aqua over the northwest Pacific Ocean from 2006–2015 to study the relationships between (i) tropical cyclone (TC) temperature structure and intensity and (ii) cloud macro-/micro-physical properties and TC intensity. TC intensity had a positive correlation with warm-core strength (correlation coefficient of 0.8556). The warm-core strength increased gradually from 1 K for tropical depression (TD) to >15 K for super typhoon (Super TY). The vertical areas affected by the warm core expanded as TC intensity increased. The positive correlation between TC intensity and warm-core height was slightly weaker. The warm-core heights for TD, tropical storm (TS), and severe tropical storm (STS) were concentrated between 300 and 500 hPa, while those for typhoon (TY), severe typhoon (STY), and Super TY varied from 200 to 350 hPa. Analyses of the cloud macro-/micro-physical properties showed that the top of TC cloud systems mainly consisted of ice clouds. For TCs of all intensities, areas near the TC center showed lower cloud-top pressures and lower cloud-top temperatures, more cloud fractions, and larger ice-cloud effective diameters. With the increase in TC intensity, the levels of ice clouds around the TC center became higher and the spiral cloud-rain bands became larger. When a TC developed into a TY, STY, or Super TY, the convection in the clouds was stronger, releasing more heat, thus forming a much warmer warm core.
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Burnet, Frédéric, and Jean-Louis Brenguier. "Observational Study of the Entrainment-Mixing Process in Warm Convective Clouds." Journal of the Atmospheric Sciences 64, no. 6 (June 2007): 1995–2011. http://dx.doi.org/10.1175/jas3928.1.
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Thermodynamical and microphysical measurements collected in convective clouds are examined within the frame of the homogeneous/inhomogeneous mixing concept, to determine how entrainment-mixing processes affect cloud droplets, their number concentration, and their mean size. The three selected case studies—one stratocumulus layer and two cumulus clouds—exhibit very different values of the cloud updraft intensity, of the adiabatic droplet mean volume diameter, and of the saturation deficit in the environment, all three parameters that are expected to govern the microphysical response to entrainmentmixing. The results confirm that the observed microphysical features are sensitive to the droplet response time to evaporation and to the turbulent homogenization time scale, as suggested by the inhomogeneous mixing concept. They also reveal that an instrumental artifact due to the heterogeneous spatial droplet distribution may be partly responsible for the observed heterogeneous mixing features. The challenge remains, however, to understand why spatially homogeneous cloud volumes larger than the instrument resolution scale (10 m) are so rarely observed. The analysis of the buoyancy of the cloud and clear air mixtures suggests that dynamical sorting could also be efficient for the selection, among all possible mixing scenarios, of those that minimize the local buoyancy production.
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Ding, Yuhao, Qi Liu, and Ping Lao. "Characteristics of Oceanic Warm Cloud Layers within Multilevel Cloud Systems Derived by Satellite Measurements." Atmosphere 10, no. 8 (August 14, 2019): 465. http://dx.doi.org/10.3390/atmos10080465.
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Low-level warm clouds are a major component in multilayered cloud systems and they are generally hidden from the top-down view of satellites with passive measurements. This study conducts an investigation on oceanic warm clouds embedded in multilayered structures by using spaceborne radar data with fine vertical resolution. The occurrences of warm cloud overlapping and the geometric features of several kinds of warm cloud layers are examined. It is found that there are three main types of cloud systems that involve warm cloud layers, including warm single layer clouds, cold-warm double layer clouds, and warm-warm double layer clouds. The two types of double layer clouds account for 23% and in the double layer occurrences warm-warm double layer subsets contribute about 13%. The global distribution patterns of these three types differ from each other. Single-layer warm clouds and the lower warm clouds in the cold-warm double layer system they have nearly identical geometric parameters, while the upper and lower layer warm clouds in the warm-warm double layer system are distinct from the previous two forms of warm cloud layers. In contrast to the independence of the two cloud layers in cold-warm double layer system, the two kinds of warm cloud layers in the warm-warm double layer system may be coupled. The distance between the two layers in the warm-warm double layer system is weakly dependent on cloud thickness. Given the upper and lower cloud layer with moderate thickness of around 1 km, the cloudless gap reaches its maximum when exceeding 600 m. The cloudless gap decreases in thickness as the two cloud layers become even thinner or thicker.
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Lee, S. S., L. J. Donner, and V. T. J. Phillips. "Sensitivity of aerosol and cloud effects on radiation to cloud types: comparison between deep convective clouds and warm stratiform clouds over one-day period." Atmospheric Chemistry and Physics 9, no. 7 (April 8, 2009): 2555–75. http://dx.doi.org/10.5194/acp-9-2555-2009.
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Abstract. Cloud and aerosol effects on radiation in two contrasting cloud types, a deep mesoscale convective system (MCS) and warm stratocumulus clouds, are simulated and compared. At the top of the atmosphere, 45–81% of shortwave cloud forcing (SCF) is offset by longwave cloud forcing (LCF) in the MCS, whereas warm stratiform clouds show the offset of less than ~20%. 28% of increased negative SCF is offset by increased LCF with increasing aerosols in the MCS at the top of the atmosphere. However, the stratiform clouds show the offset of just around 2–5%. Ice clouds as well as liquid clouds play an important role in the larger offset in the MCS. Lower cloud-top height and cloud depth, characterizing cloud types, lead to the smaller offset of SCF by LCF and the offset of increased negative SCF by increased LCF at high aerosol in stratocumulus clouds than in the MCS. Supplementary simulations show that this dependence of modulation of LCF on cloud depth and cloud-top height is also simulated among different types of convective clouds.
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Heus, Thijs, Gertjan van Dijk, Harm J. J. Jonker, and Harry E. A. Van den Akker. "Mixing in Shallow Cumulus Clouds Studied by Lagrangian Particle Tracking." Journal of the Atmospheric Sciences 65, no. 8 (August 1, 2008): 2581–97. http://dx.doi.org/10.1175/2008jas2572.1.
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Abstract Mixing between shallow cumulus clouds and their environment is studied using large-eddy simulations. The origin of in-cloud air is studied by two distinct methods: 1) by analyzing conserved variable mixing diagrams (Paluch diagrams) and 2) by tracing back cloud-air parcels represented by massless Lagrangian particles that follow the flow. The obtained Paluch diagrams are found to be similar to many results in the literature, but the source of entrained air found by particle tracking deviates from the source inferred from the Paluch analysis. Whereas the classical Paluch analysis seems to provide some evidence for cloud-top mixing, particle tracking shows that virtually all mixing occurs laterally. Particle trajectories averaged over the entire cloud ensemble also clearly indicate the absence of significant cloud-top mixing in shallow cumulus clouds.
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Song, Hwan-Jin, Byunghwan Lim, and Sangwon Joo. "Evaluation of Rainfall Forecasts with Heavy Rain Types in the High-Resolution Unified Model over South Korea." Weather and Forecasting 34, no. 5 (September 9, 2019): 1277–93. http://dx.doi.org/10.1175/waf-d-18-0140.1.
Full textAbstract:
Abstract Heavy rainfall events account for most socioeconomic damages caused by natural disasters in South Korea. However, the microphysical understanding of heavy rain is still lacking, leading to uncertainties in quantitative rainfall prediction. This study is aimed at evaluating rainfall forecasts in the Local Data Assimilation and Prediction System (LDAPS), a high-resolution configuration of the Unified Model over the Korean Peninsula. The rainfall of LDAPS forecasts was evaluated with observations based on two types of heavy rain events classified from K-means clustering for the relationship between surface rainfall intensity and cloud-top height. LDAPS forecasts were characterized by more heavy rain cases with high cloud-top heights (cold-type heavy rain) in contrast to observations showing frequent moderate-intensity rain systems with relatively lower cloud-top heights (warm-type heavy rain) over South Korea. The observed cold-type and warm-type events accounted for 32.7% and 67.3% of total rainfall, whereas LDAPS forecasts accounted for 65.3% and 34.7%, respectively. This indicates severe overestimation and underestimation of total rainfall for the cold-type and warm-type forecast events, respectively. The overestimation of cold-type heavy rainfall was mainly due to its frequent occurrence, whereas the underestimation of warm-type heavy rainfall was affected by both its low occurrence and weak intensity. The rainfall forecast skill for the warm-type events was much lower than for the cold-type events, due to the lower rainfall intensity and smaller rain area of the warm-type. Therefore, cloud parameterizations for warm-type heavy rain should be improved to enhance rainfall forecasts over the Korean Peninsula.