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Journal articles on the topic 'Versatile intermediates'

Author: Grafiati

Published: 6 September 2023

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1

Boeske, Juergen, Edgar Niecke, Edgar Ocando-Mavarez, Jean Pierre Majoral, and Guy Bertrand. "Phosphonitriles: versatile intermediates." Inorganic Chemistry 25, no. 16 (July 1986): 2695–98. http://dx.doi.org/10.1021/ic00236a008.

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2

Belletire, J. L. "Acylcyanamides: Versatile Synthetic Intermediates." Synthetic Communications 18, no. 16-17 (November 1988): 2063–71. http://dx.doi.org/10.1080/00397918808068275.

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3

R. Katritzky, Alan, Adam S. Vincek, and Peter J. Steel. "Triphenylphosphoranylidene Substituted Heterocycles as Versatile Intermediates." HETEROCYCLES 76, no. 2 (2008): 1401. http://dx.doi.org/10.3987/com-08-s(f)12.

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4

Britten, Thomas K., Paul D. Kemmitt, Nathan R. Halcovitch, and Susannah C. Coote. "1,2-Dihydropyridazines as Versatile Synthetic Intermediates." Synlett 31, no. 05 (February 13, 2020): 459–62. http://dx.doi.org/10.1055/s-0039-1690825.

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The reactivity of 1,2-dihydropyridazines under various conditions is described, leading to the formation of a variety of products, including 2-aminopyrroles, phenylenediamines, and several novel heterocyclic motifs.

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5

Bari, Ahmed. "Monosaccharidic Push-pull Butadienes: Versatile Synthetic Intermediates." Zeitschrift für Naturforschung B 69, no. 1 (January 1, 2014): 98–102. http://dx.doi.org/10.5560/znb.2014-3179.

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Monosaccharidic push-pull butadienes are interesting building blocks for the synthesis of various heterocyclic and natural products due to their biological prevalence and significant p-electron interactions between donor and acceptor groups. A series of 1,5-anhydro-3,4,6-tri-O-benzyl-2-deoxy- 2-formyl-D-arabino-hex-1-enitol (2) and 1,5-anhydro-3,4-di-O-benzyl-2-deoxy-2-formyl-L-erythrohex- 1-enitol (4) derived push-pull branched chain sugars have been synthesized by condensation with active methylene compounds using basic aluminum oxide (Al2O3) or anhydrous sodium acetate (NaOAc) at room temperature. The compounds have been fully characterized by spectroscopic techniques and elemental analyses.

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6

Attanasi, Orazio A., and Luciano Caglioti. "CONJUGATED AZOALKENES: ATTRACTIVE PRODUCTS AND VERSATILE INTERMEDIATES." Organic Preparations and Procedures International 18, no. 5 (October 1986): 299–327. http://dx.doi.org/10.1080/00304948609356836.

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7

Flashman, Emily, and Christopher J. Schofield. "The most versatile of all reactive intermediates?" Nature Chemical Biology 3, no. 2 (February 2007): 86–87. http://dx.doi.org/10.1038/nchembio0207-86.

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8

Zellner, Armin, and Manfred Schlosser. "Pentadienyltitaniums as Versatile Intermediates: Regio- and Stereoselectivities." Synlett 2001, Special Issue (2001): 1016–18. http://dx.doi.org/10.1055/s-2001-14650.

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9

Barrett, Anthony G. M., and Gregory G. Graboski. "Conjugated nitroalkenes: versatile intermediates in organic synthesis." Chemical Reviews 86, no. 5 (October 1986): 751–62. http://dx.doi.org/10.1021/cr00075a002.

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10

Michael, J. P., C. B. de Koning, D. Gravestock, G. D. Hosken, A. S. Howard, C. M. Jungmann, R. W. M. Krause, A. S. Parsons, S. C. Pelly, and T. V. Stanbury. "Enaminones: versatile intermediates for natural product synthesis." Pure and Applied Chemistry 71, no. 6 (June 30, 1999): 979–88. http://dx.doi.org/10.1351/pac199971060979.

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11

Joergensen, M., K. A. Lerstrup, and K. Bechgaard. "Mesoions as versatile intermediates in tetrathiafulvalene synthesis." Journal of Organic Chemistry 56, no. 19 (September 1991): 5684–88. http://dx.doi.org/10.1021/jo00019a041.

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12

Chemla, Fabrice. "α-Oxy sulfones and sulfoximines: versatile intermediates." Journal of the Chemical Society, Perkin Transactions 1, no. 3 (January 10, 2002): 275–99. http://dx.doi.org/10.1039/b009523k.

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13

Lamberth, Clemens. "Organic Isocyanates and Isothiocyanates: Versatile Intermediates in Agrochemistry." Synthesis 54, no. 05 (October 26, 2021): 1250–60. http://dx.doi.org/10.1055/a-1678-8528.

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AbstractIn recent decades, organic isocyanates and isothiocyanates have been often applied as reactive intermediates in research syntheses or manufacturing routes of many agrochemicals. These heterocumulenes allowed the installation of crucial carboxylic functions, such as carbamates, ureas, and semicarbazones, but have also been used for the construction of five- and six-membered heterocycles, such as tetrazolones, thiazoles, and uracils.1 Introduction2 Preparation of Carboxylic Acid Functions3 Preparation of Heterocyclic Rings4 Conclusion

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14

Warkentin, John. "Δ3-1,3,4-Oxadiazolines.† Versatile sources of reactive intermediates." Journal of the Chemical Society, Perkin Transactions 1, no. 14 (2000): 2161–69. http://dx.doi.org/10.1039/b000930j.

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15

Redely, D. Bhaskar, M. V. Ramana Redely, and V. Padmavathi. "Cyclohexanone Gem-Dicarboxylates - Versatile Intermediates for Fused Heterocycles." Synthetic Communications 29, no. 4 (February 1999): 667–76. http://dx.doi.org/10.1080/00397919908085815.

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16

Havel, Václav, Tereza Sadilová, and Vladimír Šindelář. "Unsubstituted Bambusurils: Post-Macrocyclization Modification of Versatile Intermediates." ACS Omega 3, no. 4 (April 27, 2018): 4657–63. http://dx.doi.org/10.1021/acsomega.8b00497.

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17

Krafft, Grant A., Ester A. Garcia, Anil Guram, Brian O'Shaughnessy, and Xialong Xu. "Simplified cytochalasins. 1. Synthesis of versatile perhydroisoindolone intermediates." Tetrahedron Letters 27, no. 24 (1986): 2691–94. http://dx.doi.org/10.1016/s0040-4039(00)84618-3.

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18

van de Wouw, Heidi L., and Rebekka S. Klausen. "BN Polystyrenes: Emerging Optical Materials and Versatile Intermediates." Journal of Organic Chemistry 84, no. 3 (January 8, 2019): 1117–25. http://dx.doi.org/10.1021/acs.joc.8b02921.

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19

Irwin, Jacob L., and Michael S. Sherburn. "Monolithiocavitands: Versatile Intermediates for New Cavitand-Based Hosts." Organic Letters 3, no. 2 (January 2001): 225–27. http://dx.doi.org/10.1021/ol006881w.

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20

Waldvogel, Siegfried R., and Sabine Möhle. "Versatile Electrochemical CH Amination via Zincke Intermediates." Angewandte Chemie International Edition 54, no. 22 (May 12, 2015): 6398–99. http://dx.doi.org/10.1002/anie.201502638.

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21

Zhang, Shu Xin. "Research on Synthesis of Benzoic Acids Intermediates." Applied Mechanics and Materials 192 (July 2012): 270–74. http://dx.doi.org/10.4028/www.scientific.net/amm.192.270.

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This article briefly describes the development of dye intermediates in China and the research and development situation on synthetic 2 - amino-5 - nitrobenzoic acids. It also tries two more new routes to practice synthesis of them, for which it focuses on speculation of the reaction mechanism of the former route and on research of process conditions of the latter, getting the optimal conditions of the synthetic 5 - nitro-isatin. 2 - Amino - 5 - nitro benzoic acid is a versatile organic intermediate, which is seldom reported both home and abroad, but research on its synthesis method and process conditions are significant to the development of China's fine intermediates industry.

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22

Roy, Tony, and Akkattu T. Biju. "Recent advances in molecular rearrangements involving aryne intermediates." Chemical Communications 54, no. 21 (2018): 2580–94. http://dx.doi.org/10.1039/c7cc09122b.

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A concise account on the recent developments in molecular rearrangements proceeding via the aryne intermediate is presented thereby shedding light on the synthetic potential of this versatile intermediate.

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23

Ducrot, Paul-Henri, Anne-Claire Hervier, and Jean-Yves Lallemand. "Stereoselective Synthesis of Versatile Intermediates for Clerodanes Total synthesis." Synthetic Communications 26, no. 23 (December 1996): 4447–57. http://dx.doi.org/10.1080/00397919608003847.

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24

Cordero, Franca M., Francesco De Sarlo, and Alberto Brandi. "5-Spirocyclopropane Isoxazolidines as Versatile Intermediates in Organic Synthesis." Monatshefte f�r Chemie / Chemical Monthly 135, no. 6 (June 1, 2004): 649–69. http://dx.doi.org/10.1007/s00706-003-0150-x.

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25

Mukaiyama, Teruaki, and Hokuto Yamabe. "Alkyl Phosphinites: Versatile Synthetic Intermediates for Dehydration Condensation Reactions." Chemistry Letters 36, no. 1 (January 2007): 2–7. http://dx.doi.org/10.1246/cl.2007.2.

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26

Schmidt, Richard R. "Functionally Substituted Vinyl Carbanions Versatile Intermediates in Heterocyclic Synthesis." Bulletin des Sociétés Chimiques Belges 92, no. 9 (September 1, 2010): 825–36. http://dx.doi.org/10.1002/bscb.19830920909.

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27

Michael, Joseph P., Charles B. De Koning, David Gravestock, Gladys D. Hosken, Arthur S. Howard, Christa M. Jungmann, Rui W. M. Krause, Andrew S. Parsons, Stephen C. Pelly, and Trevor V. Stanbury. "ChemInform Abstract: Enaminones: Versatile Intermediates for Natural Product Synthesis." ChemInform 31, no. 4 (June 11, 2010): no. http://dx.doi.org/10.1002/chin.200004280.

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28

Zellner, Armin, and Manfred Schlosser. "ChemInform Abstract: Pentadienyltitaniums as Versatile Intermediates: Regio- and Stereoselectivities." ChemInform 32, no. 40 (May 24, 2010): no. http://dx.doi.org/10.1002/chin.200140064.

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29

JOERGENSEN, M., K. A. LERSTRUP, and K. BECHGAARD. "ChemInform Abstract: Mesoions as Versatile Intermediates in Tetrathiafulvalene Synthesis." ChemInform 23, no. 6 (August 22, 2010): no. http://dx.doi.org/10.1002/chin.199206174.

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30

Chemla, Fabrice. "ChemInform Abstract: α-Oxy Sulfones and Sulfoximines: Versatile Intermediates." ChemInform 33, no. 24 (May 21, 2010): no. http://dx.doi.org/10.1002/chin.200224251.

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31

Evano, Gwilherm, Morgan Lecomte, Pierre Thilmany, and Cédric Theunissen. "Keteniminium Ions: Unique and Versatile Reactive Intermediates for Chemical Synthesis." Synthesis 49, no. 15 (July 17, 2017): 3183–214. http://dx.doi.org/10.1055/s-0036-1588452.

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Keteniminium ions have been demonstrated to be remarkably useful and versatile reactive intermediates in chemical synthesis. These unique heterocumulenes are pivotal electrophilic species involved in a number of efficient and selective transformations. More recently, even more reactive ‘activated’ keteniminium ions bearing an additional electron-withdrawing group on the nitrogen atom have been extensively investigated. The chemistry of these unique reactive intermediates, including representative methods for their in situ generation, will be overviewed in this review article.1 Introduction2 The Chemistry of Keteniminium Ions3 The Chemistry of Activated Keteniminium Ions4 Keteniminium Ions: Pivotal Intermediates for the Synthesis of Natural and/or Biologically Relevant Molecules5 Conclusions and Perspectives

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32

Tian, Feitao, Guobing Yan, and Jian Yu. "Recent advances in the synthesis and applications of α-(trifluoromethyl)styrenes in organic synthesis." Chemical Communications 55, no. 90 (2019): 13486–505. http://dx.doi.org/10.1039/c9cc06465f.

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33

Iwanejko, Jakub, and Elżbieta Wojaczyńska. "Cyclic imines – preparation and application in synthesis." Organic & Biomolecular Chemistry 16, no. 40 (2018): 7296–314. http://dx.doi.org/10.1039/c8ob01874j.

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34

Dong, Kuiyong, Mengting Liu, and Xinfang Xu. "Recent Advances in Catalytic Alkyne Transformation via Copper Carbene Intermediates." Molecules 27, no. 10 (May 11, 2022): 3088. http://dx.doi.org/10.3390/molecules27103088.

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As one of the abundant and inexpensive metals on the earth, copper has demonstrated broad applications in synthetic chemistry and catalysis. Among these copper-catalyzed advances, copper carbenes are versatile and reactive intermediates that can mediate a variety of transformations, which have attracted much attention in the past decades. The present review summarizes two different reaction models that take place between a copper carbene intermediate and alkyne species, including the cross-coupling reaction of copper carbene intermediate with terminal alkyne, and the addition of copper carbene intermediate onto the C–C triple bond. This article will cover the profile from 2010 to 2021 by placing emphasis on the detailed catalytic models and highlighting the synthetic applications offered by these practical and mild methods.

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35

Liew, Sean K., Aleksandra Holownia, Diego B. Diaz, Philip A. Cistrone, Philip E. Dawson, and Andrei K. Yudin. "Borylated oximes: versatile building blocks for organic synthesis." Chem. Commun. 53, no. 81 (2017): 11237–40. http://dx.doi.org/10.1039/c7cc06579e.

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36

Berger, Olivier, and Jean-Luc Montchamp. "General synthesis of P-stereogenic compounds: the menthyl phosphinate approach." Organic & Biomolecular Chemistry 14, no. 31 (2016): 7552–62. http://dx.doi.org/10.1039/c6ob01413e.

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37

Bayer, Patrick, Josef Schachtner, Michal Májek, and Axel Jacobi von Wangelin. "Visible light-mediated photo-oxygenation of arylcyclohexenes." Organic Chemistry Frontiers 6, no. 16 (2019): 2877–83. http://dx.doi.org/10.1039/c9qo00493a.

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38

Santamaría, Javier, and Enrique Aguilar. "Beyond Fischer and Schrock carbenes: non-heteroatom-stabilized group 6 metal carbene complexes – a general overview." Organic Chemistry Frontiers 3, no. 11 (2016): 1561–88. http://dx.doi.org/10.1039/c6qo00206d.

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39

Hearne, Zoë, and Chao-Jun Li. "Palladium-catalysed atom-economical synthesis of conjugated dienals from terminal acetylenes and acrolein." Chemical Communications 53, no. 45 (2017): 6136–39. http://dx.doi.org/10.1039/c7cc02767b.

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40

Iftikhar, Ramsha, Aqsa Mazhar, Muhammad Saqlain Iqbal, Faiza Zahid Khan, Syed Hassan Askary, and Hifza Sibtain. "Ring forming transformations of ynamides via cycloaddition." RSC Advances 13, no. 16 (2023): 10715–56. http://dx.doi.org/10.1039/d3ra00139c.

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41

Turrini, Nikolaus G., Răzvan C. Cioc, Daan J. H. van der Niet, Eelco Ruijter, Romano V. A. Orru, Mélanie Hall, and Kurt Faber. "Biocatalytic access to nonracemic γ-oxo esters via stereoselective reduction using ene-reductases." Green Chemistry 19, no. 2 (2017): 511–18. http://dx.doi.org/10.1039/c6gc02493a.

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42

Prasad, Sure Siva, Dirgha Raj Joshi, Jeong Hwa Lee, and Ikyon Kim. "One-pot access to 2-amino-3-arylbenzofurans: direct entry to polyheterocyclic chemical space." Organic & Biomolecular Chemistry 18, no. 40 (2020): 8119–40. http://dx.doi.org/10.1039/d0ob01715a.

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43

Lynch, Dylan M., and Eoin M. Scanlan. "Thiyl Radicals: Versatile Reactive Intermediates for Cyclization of Unsaturated Substrates." Molecules 25, no. 13 (July 7, 2020): 3094. http://dx.doi.org/10.3390/molecules25133094.

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Sulfur centered radicals are widely employed in chemical synthesis, in particular for alkene and alkyne hydrothiolation towards thioether bioconjugates. The steadfast radical chain process that enables efficient hydrothiolation has been explored in the context of cascade reactions to furnish complex molecular architectures. The use of thiyl radicals offers a much cheaper and less toxic alternative to the archetypal organotin-based radical methods. This review outlines the development of thiyl radicals as reactive intermediates for initiating carbocyclization cascades. Key developments in cascade cyclization methodology are presented and applications for natural product synthesis are discussed. The review provides a chronological account of the field, beginning in the early seventies up to very recent examples; a span of almost 50 years.

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44

X. Xiang, Alan, Ricardo Lira, Konstantinos A. Agrios, Thomas Doundoulakis, Klaus B. Simonsen, and Stephen E. Webber. "An Efficient Synthesis of (±)-Myxopyronin B via Versatile Pyridone Intermediates." HETEROCYCLES 68, no. 6 (2006): 1099. http://dx.doi.org/10.3987/com-06-10733.

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45

Barcelo, Gérard, Jean-Pierre Senet, and Gérard Sennyey. "1,2,2,2-Tetrachloroethyl Carbamates: Versatile Intermediates for the Synthesis ofN-Nitrosoureas." Synthesis 1987, no. 11 (1987): 1027–29. http://dx.doi.org/10.1055/s-1987-28160.

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46

Dondoni, Alessandro, and Alberto Marra. "Thiazolylketoses: a new class of versatile intermediates for glycoside synthesis." Chemical Communications, no. 21 (1999): 2133–45. http://dx.doi.org/10.1039/a903758f.

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47

Maduli, Elvis J. M., Steven J. Edeson, Stephen Swanson, Panayiotis A. Procopiou, and Joseph P. A. Harrity. "2-Iodoisatogens: Versatile Intermediates for the Synthesis of Nitrogen Heterocycles." Organic Letters 17, no. 2 (December 23, 2014): 390–92. http://dx.doi.org/10.1021/ol503487f.

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48

Kataja, Antti O., and Géraldine Masson. "Imine and iminium precursors as versatile intermediates in enantioselective organocatalysis." Tetrahedron 70, no. 46 (November 2014): 8783–815. http://dx.doi.org/10.1016/j.tet.2014.06.101.

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49

Wu, Chien-Hsin, Li-Yun Chen, Ru-Jong Jeng, and Shenghong A. Dai. "100% Atom-Economy Efficiency of Recycling Polycarbonate into Versatile Intermediates." ACS Sustainable Chemistry & Engineering 6, no. 7 (May 28, 2018): 8964–75. http://dx.doi.org/10.1021/acssuschemeng.8b01326.

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50

Martin, Stephen F., and Michael P. Dwyer. "Iodocyclopropanes as versatile intermediates for the synthesis of substituted cyclopropanes." Tetrahedron Letters 39, no. 12 (March 1998): 1521–24. http://dx.doi.org/10.1016/s0040-4039(98)00072-0.

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