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Journal articles on the topic 'Ultracold chemistry'

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Author: Grafiati
Published: 10 December 2022
Last updated: 28 January 2023

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1

Bell, Martin T., and Timothy P. Softley. "Ultracold molecules and ultracold chemistry." Molecular Physics 107, no. 2 (January 20, 2009): 99–132. http://dx.doi.org/10.1080/00268970902724955.

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2

Hutson, J. M. "Ultracold Chemistry." Science 327, no. 5967 (February 11, 2010): 788–89. http://dx.doi.org/10.1126/science.1186703.

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3

Balakrishnan, N., and A. Dalgarno. "Chemistry at ultracold temperatures." Chemical Physics Letters 341, no. 5-6 (June 2001): 652–56. http://dx.doi.org/10.1016/s0009-2614(01)00515-2.

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4

Pérez-Ríos, Jesús, Maxence Lepers, Romain Vexiau, Nadia Bouloufa-Maafa, and Olivier Dulieu. "Progress toward ultracold chemistry: ultracold atomic and photonic collisions." Journal of Physics: Conference Series 488, no. 1 (April 10, 2014): 012031. http://dx.doi.org/10.1088/1742-6596/488/1/012031.

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5

Cornish, Simon L., and Jeremy M. Hutson. "Toward a coherent ultracold chemistry." Science 375, no. 6584 (March 4, 2022): 975–76. http://dx.doi.org/10.1126/science.abn1053.

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6

Benka, Stephen G. "Ultracold chemistry in supersonic beams." Physics Today 65, no. 12 (December 2012): 21. http://dx.doi.org/10.1063/pt.3.1811.

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7

Saßmannshausen, Heiner, Johannes Deiglmayr, and Frédéric Merkt. "Exotic Chemistry with Ultracold Rydberg Atoms." CHIMIA International Journal for Chemistry 70, no. 4 (April 27, 2016): 263–67. http://dx.doi.org/10.2533/chimia.2016.263.

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8

Richter, Florian, Daniel Becker, Cédric Bény, Torben A. Schulze, Silke Ospelkaus, and Tobias J. Osborne. "Ultracold chemistry and its reaction kinetics." New Journal of Physics 17, no. 5 (May 7, 2015): 055005. http://dx.doi.org/10.1088/1367-2630/17/5/055005.

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9

Liu, Yu, David D. Grimes, Ming-Guang Hu, and Kang-Kuen Ni. "Probing ultracold chemistry using ion spectrometry." Physical Chemistry Chemical Physics 22, no. 9 (2020): 4861–74. http://dx.doi.org/10.1039/c9cp07015j.

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10

Tennyson, Jonathan, Laura K. McKemmish, and Tom Rivlin. "Low-temperature chemistry using the R-matrix method." Faraday Discussions 195 (2016): 31–48. http://dx.doi.org/10.1039/c6fd00110f.

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Techniques for producing cold and ultracold molecules are enabling the study of chemical reactions and scattering at the quantum scattering limit, with only a few partial waves contributing to the incident channel, leading to the observation and even full control of state-to-state collisions in this regime. A new R-matrix formalism is presented for tackling problems involving low- and ultra-low energy collisions. This general formalism is particularly appropriate for slow collisions occurring on potential energy surfaces with deep wells. The many resonance states make such systems hard to treat theoretically but offer the best prospects for novel physics: resonances are already being widely used to control diatomic systems and should provide the route to steering ultracold reactions. Our R-matrix-based formalism builds on the progress made in variational calculations of molecular spectra by using these methods to provide wavefunctions for the whole system at short internuclear distances, (a regime known as the inner region). These wavefunctions are used to construct collision energy-dependent R-matrices which can then be propagated to give cross sections at each collision energy. The method is formulated for ultracold collision systems with differing numbers of atoms.
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11

Stwalley, William C. "Collisions and reactions of ultracold molecules." Canadian Journal of Chemistry 82, no. 6 (June 1, 2004): 709–12. http://dx.doi.org/10.1139/v04-035.

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It is argued that collision dynamics of atoms and molecules at ultracold temperatures (below 1 mK) are not readily predictable from knowledge of collision dynamics above 100 K. In the case of elastic collisions, it is well known that the collision cross section is constant as T → 0 K but mass and symmetry effects are dramatic. The cases of inelastic and reactive collisions are less studied, but a T–1/2 dependence of the cross section as T → 0 K is expected. It seems that extrapolations of high-temperature inelastic and reactive behavior normally greatly underestimate ultracold-temperature rates. The prospects for experimental observation of ultracold collision dynamics are rapidly improving.Key words: ultracold molecules, collisions, reactions, hydrogen, scattering length.
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12

Ivanov, Maxim V., Felix H. Bangerter, and Anna I. Krylov. "Towards a rational design of laser-coolable molecules: insights from equation-of-motion coupled-cluster calculations." Physical Chemistry Chemical Physics 21, no. 35 (2019): 19447–57. http://dx.doi.org/10.1039/c9cp03914g.

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13

Miller, Johanna L. "Ultracold chemistry: No longer a disappearing act." Physics Today 73, no. 2 (February 1, 2020): 12–14. http://dx.doi.org/10.1063/pt.3.4402.

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14

Grossman, Lisa. "Quantum weirdness sends ultracold chemistry into overdrive." New Scientist 212, no. 2839 (November 2011): 8–9. http://dx.doi.org/10.1016/s0262-4079(11)62819-4.

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15

He, Mingyuan, Chenwei Lv, Hai-Qing Lin, and Qi Zhou. "Universal relations for ultracold reactive molecules." Science Advances 6, no. 51 (December 2020): eabd4699. http://dx.doi.org/10.1126/sciadv.abd4699.

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The realization of ultracold polar molecules in laboratories has pushed physics and chemistry to new realms. In particular, these polar molecules offer scientists unprecedented opportunities to explore chemical reactions in the ultracold regime where quantum effects become profound. However, a key question about how two-body losses depend on quantum correlations in interacting many-body systems remains open so far. Here, we present a number of universal relations that directly connect two-body losses to other physical observables, including the momentum distribution and density correlation functions. These relations, which are valid for arbitrary microscopic parameters, such as the particle number, the temperature, and the interaction strength, unfold the critical role of contacts, a fundamental quantity of dilute quantum systems, in determining the reaction rate of quantum reactive molecules in a many-body environment. Our work opens the door to an unexplored area intertwining quantum chemistry; atomic, molecular, and optical physics; and condensed matter physics.
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16

Kendrick, Brian, and N. Balakrishnan. "Geometric Phase Effects in Ultracold Chemical Reactions." Atoms 7, no. 3 (July 3, 2019): 65. http://dx.doi.org/10.3390/atoms7030065.

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The role of the geometric phase effect in chemical reaction dynamics has long been a topic of active experimental and theoretical investigations. The topic has received renewed interest in recent years in cold and ultracold chemistry where it was shown to play a decisive role in state-to-state chemical dynamics. We provide a brief review of these developments focusing on recent studies of O + OH and hydrogen exchange in the H + H 2 and D + HD reactions at cold and ultracold temperatures. Non-adiabatic effects in ultracold chemical dynamics arising from the conical intersection between two electronic potential energy surfaces are also briefly discussed. By taking the hydrogen exchange reaction as an illustrative example it is shown that the inclusion of the geometric phase effect captures the essential features of non-adiabatic dynamics at collision energies below the conical intersection.
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17

Pérez-Ríos, J., M. Kim, and C. L. Hung. "Ultracold molecules strongly coupled to a nanophotonic crystal: an universal platform for ultracold chemistry experiments." Journal of Physics: Conference Series 875 (July 2017): 082006. http://dx.doi.org/10.1088/1742-6596/875/9/082006.

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18

Mani, Devendra, Ricardo Pérez de Tudela, Raffael Schwan, Nitish Pal, Saskia Körning, Harald Forbert, Britta Redlich, et al. "Acid solvation versus dissociation at “stardust conditions”: Reaction sequence matters." Science Advances 5, no. 6 (June 2019): eaav8179. http://dx.doi.org/10.1126/sciadv.aav8179.

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Chemical reactions at ultralow temperatures are of fundamental importance to primordial molecular evolution as it occurs on icy mantles of dust nanoparticles or on ultracold water clusters in dense interstellar clouds. As we show, studying reactions in a stepwise manner in ultracold helium nanodroplets by mass-selective infrared (IR) spectroscopy provides an avenue to mimic these “stardust conditions” in the laboratory. In our joint experimental/theoretical study, in which we successively add H2O molecules to HCl, we disclose a unique IR fingerprint at 1337 cm−1 that heralds hydronium (H3O+) formation and, thus, acid dissociation generating solvated protons. In stark contrast, no reaction is observed when reversing the sequence by allowing HCl to interact with preformed small embryonic ice-like clusters. Our ab initio simulations demonstrate that not only reaction stoichiometry but also the reaction sequence needs to be explicitly considered to rationalize ultracold chemistry.
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19

Wolf, Joschka, Markus Deiß, Artjom Krükow, Eberhard Tiemann, Brandon P. Ruzic, Yujun Wang, José P. D’Incao, Paul S. Julienne, and Johannes Hecker Denschlag. "State-to-state chemistry for three-body recombination in an ultracold rubidium gas." Science 358, no. 6365 (November 16, 2017): 921–24. http://dx.doi.org/10.1126/science.aan8721.

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Experimental investigation of chemical reactions with full quantum state resolution for all reactants and products has been a long-term challenge. Here we prepare an ultracold few-body quantum state of reactants and demonstrate state-to-state chemistry for the recombination of three spin-polarized ultracold rubidium (Rb) atoms to form a weakly bound Rb2 molecule. The measured product distribution covers about 90% of the final products, and we are able to discriminate between product states with a level splitting as small as 20 megahertz multiplied by Planck’s constant. Furthermore, we formulate propensity rules for the distribution of products, and we develop a theoretical model that predicts many of our experimental observations. The scheme can readily be adapted to other species and opens a door to detailed investigations of inelastic or reactive processes.
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20

Hazra, Jisha, Brian K. Kendrick, and Naduvalath Balakrishnan. "Importance of Geometric Phase Effects in Ultracold Chemistry." Journal of Physical Chemistry A 119, no. 50 (September 9, 2015): 12291–303. http://dx.doi.org/10.1021/acs.jpca.5b06410.

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21

Quéméner, Goulven, and Paul S. Julienne. "Ultracold Molecules under Control!" Chemical Reviews 112, no. 9 (August 24, 2012): 4949–5011. http://dx.doi.org/10.1021/cr300092g.

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22

Zappa, Fabio, Stephan Denifl, Ingo Mähr, Arntraud Bacher, Olof Echt, Tilmann D. Märk, and Paul Scheier. "Ultracold Water Cluster Anions." Journal of the American Chemical Society 130, no. 16 (April 2008): 5573–78. http://dx.doi.org/10.1021/ja075421w.

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23

He, Xiaodong, Kunpeng Wang, Jun Zhuang, Peng Xu, Xiang Gao, Ruijun Guo, Cheng Sheng, et al. "Coherently forming a single molecule in an optical trap." Science 370, no. 6514 (September 24, 2020): 331–35. http://dx.doi.org/10.1126/science.aba7468.

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Ultracold single molecules have wide-ranging potential applications, such as ultracold chemistry, precision measurements, quantum simulation, and quantum computation. However, given the difficulty of achieving full control of a complex atom-molecule system, the coherent formation of single molecules remains a challenge. Here, we report an alternative route to coherently bind two atoms into a weakly bound molecule at megahertz levels by coupling atomic spins to their two-body relative motion in a strongly focused laser with inherent polarization gradients. The coherent nature is demonstrated by long-lived atom-molecule Rabi oscillations. We further manipulate the motional levels of the molecules and measure the binding energy precisely. This work opens the door to full control of all degrees of freedom in atom-molecule systems.
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24

Isaev, Timur A., and Robert Berger. "Towards Ultracold Chiral Molecules." CHIMIA International Journal for Chemistry 72, no. 6 (June 27, 2018): 375–78. http://dx.doi.org/10.2533/chimia.2018.375.

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25

Mitra, Debayan, Nathaniel B. Vilas, Christian Hallas, Loïc Anderegg, Benjamin L. Augenbraun, Louis Baum, Calder Miller, Shivam Raval, and John M. Doyle. "Direct laser cooling of a symmetric top molecule." Science 369, no. 6509 (September 10, 2020): 1366–69. http://dx.doi.org/10.1126/science.abc5357.

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Ultracold polyatomic molecules have potentially wide-ranging applications in quantum simulation and computation, particle physics, and quantum chemistry. For atoms and small molecules, direct laser cooling has proven to be a powerful tool for quantum science in the ultracold regime. However, the feasibility of laser-cooling larger, nonlinear polyatomic molecules has remained unknown because of their complex structure. We laser-cooled the symmetric top molecule calcium monomethoxide (CaOCH3), reducing the temperature of ~104 molecules from 22 ± 1 millikelvin to 1.8 ± 0.7 millikelvin in one dimension and state-selectively cooling two nuclear spin isomers. These results demonstrate that the use of proper ro-vibronic transitions enables laser cooling of nonlinear molecules, thereby opening a path to efficient cooling of chiral molecules and, eventually, optical tweezer arrays of complex polyatomic species.
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26

Booth, D., S. T. Rittenhouse, J. Yang, H. R. Sadeghpour, and J. P. Shaffer. "Production of trilobite Rydberg molecule dimers with kilo-Debye permanent electric dipole moments." Science 348, no. 6230 (April 2, 2015): 99–102. http://dx.doi.org/10.1126/science.1260722.

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Permanent electric dipole moments are important for understanding symmetry breaking in molecular physics, control of chemical reactions, and realization of strongly correlated many-body quantum systems. However, large molecular permanent electric dipole moments are challenging to realize experimentally. We report the observation of ultralong-range Rydberg molecules with bond lengths of ~100 nanometers and kilo-Debye permanent electric dipole moments that form when an ultracold ground-state cesium (Cs) atom becomes bound within the electronic cloud of an extended Cs electronic orbit. The electronic character of this hybrid class of “trilobite” molecules is dominated by degenerate Rydberg manifolds, making them difficult to produce by conventional photoassociation. We used detailed coupled-channel calculations to reproduce their properties quantitatively. Our findings may lead to progress in ultracold chemistry and strongly correlated many-body physics.
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27

Xie, Rui-Hua, and Paul Brumer. "Quantum Reflection of Ultracold Atoms in Magnetic Traps." Zeitschrift für Naturforschung A 54, no. 3-4 (April 1, 1999): 167–70. http://dx.doi.org/10.1515/zna-1999-3-401.

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Ultracold neutral atoms can be trapped in spatially inhomogeneous magnetic fields. In this paper, we present a theoretical model and demonstrate by using Landau-Zener tool that if the magnetic resonant transition region is very narrow, "potential barriers" appear and quantum reflection of such ultracold atoms can be observed in this region.
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28

Dulieu, Olivier, and Pierre Pillet. "Playing With a Pair of Ultracold Atoms and Lasers: Towards a Novel Ultracold Photochemistry?" Israel Journal of Chemistry 44, no. 1-3 (October 2004): 253–62. http://dx.doi.org/10.1560/rhhr-c4m6-pffn-8a8j.

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29

Vogel, Manuel. "Molecules in electromagnetic fields: from ultracold physics to controlled chemistry." Contemporary Physics 61, no. 4 (October 1, 2020): 307–8. http://dx.doi.org/10.1080/00107514.2021.1890826.

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30

Balakrishnan, N. "Perspective: Ultracold molecules and the dawn of cold controlled chemistry." Journal of Chemical Physics 145, no. 15 (October 21, 2016): 150901. http://dx.doi.org/10.1063/1.4964096.

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31

Rvachov, Timur M., Hyungmok Son, Juliana J. Park, Pascal M. Notz, Tout T. Wang, Martin W. Zwierlein, Wolfgang Ketterle, and Alan O. Jamison. "Photoassociation of ultracold NaLi." Physical Chemistry Chemical Physics 20, no. 7 (2018): 4746–51. http://dx.doi.org/10.1039/c7cp08480c.

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32

Liu, Yu, Ming-Guang Hu, Matthew A. Nichols, Dongzheng Yang, Daiqian Xie, Hua Guo, and Kang-Kuen Ni. "Precision test of statistical dynamics with state-to-state ultracold chemistry." Nature 593, no. 7859 (May 19, 2021): 379–84. http://dx.doi.org/10.1038/s41586-021-03459-6.

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33

Ivanov, Maxim V., Felix H. Bangerter, Paweł Wójcik, and Anna I. Krylov. "Toward Ultracold Organic Chemistry: Prospects of Laser Cooling Large Organic Molecules." Journal of Physical Chemistry Letters 11, no. 16 (July 27, 2020): 6670–76. http://dx.doi.org/10.1021/acs.jpclett.0c01960.

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34

Ospelkaus, S., K. K. Ni, M. H. G. de Miranda, B. Neyenhuis, D. Wang, S. Kotochigova, P. S. Julienne, D. S. Jin, and J. Ye. "Ultracold polar molecules near quantum degeneracy." Faraday Discussions 142 (2009): 351. http://dx.doi.org/10.1039/b821298h.

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35

Herschbach, Dudley. "Molecular collisions, from warm to ultracold." Faraday Discussions 142 (2009): 9. http://dx.doi.org/10.1039/b910118g.

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36

Hutson, Jeremy M., and Pavel Soldán. "Molecule formation in ultracold atomic gases." International Reviews in Physical Chemistry 25, no. 4 (October 2006): 497–526. http://dx.doi.org/10.1080/01442350600921772.

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37

Hutson, Jeremy M., and Pavel Soldán. "Molecular collisions in ultracold atomic gases." International Reviews in Physical Chemistry 26, no. 1 (January 2007): 1–28. http://dx.doi.org/10.1080/01442350601084562.

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38

Li, Yuqing, Xiaofeng Wang, Jizhou Wu, Guosheng Feng, Wenliang Liu, Vladimir B. Sovkov, Jie Ma, Bimalendu Deb, Liantuan Xiao, and Suotang Jia. "The effects of Feshbach resonance on spectral shifts in photoassociation of Cs atoms." Physical Chemistry Chemical Physics 23, no. 1 (2021): 641–46. http://dx.doi.org/10.1039/d0cp04840b.

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39

Hannaford, P., and R. J. McLean. "Atomic absorption with ultracold atoms." Spectrochimica Acta Part B: Atomic Spectroscopy 54, no. 14 (December 1999): 2183–94. http://dx.doi.org/10.1016/s0584-8547(99)00146-9.

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40

Kendrick, Brian K., Hui Li, Ming Li, Svetlana Kotochigova, James F. E. Croft, and Naduvalath Balakrishnan. "Non-adiabatic quantum interference in the ultracold Li + LiNa → Li2 + Na reaction." Physical Chemistry Chemical Physics 23, no. 9 (2021): 5096–112. http://dx.doi.org/10.1039/d0cp05499b.

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41

Dawid, Anna, and Michał Tomza. "Magnetic properties and quench dynamics of two interacting ultracold molecules in a trap." Physical Chemistry Chemical Physics 22, no. 48 (2020): 28140–53. http://dx.doi.org/10.1039/d0cp05542e.

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42

Wang, Xiaofeng, Wenliang Liu, Yuqing Li, Jizhou Wu, Vladimir B. Sovkov, Jie Ma, Sofiia Onishchenko, et al. "Hyperfine structure of the NaCs b3Π2 state near the dissociation limit 3S1/2 + 6P3/2 observed with ultracold atomic photoassociation." Physical Chemistry Chemical Physics 22, no. 7 (2020): 3809–16. http://dx.doi.org/10.1039/c9cp05870b.

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43

Gasenzer, T. "Ultracold gases far from equilibrium." European Physical Journal Special Topics 168, no. 1 (February 2009): 89–148. http://dx.doi.org/10.1140/epjst/e2009-00960-5.

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44

Cassidy, David. "An introduction to cold and ultracold chemistry: atoms, molecules, ions and Rydbergs." Contemporary Physics 61, no. 4 (October 1, 2020): 309–10. http://dx.doi.org/10.1080/00107514.2021.1890828.

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45

Balakrishnan, N., and A. Dalgarno. "Erratum to: `Chemistry at ultracold temperatures' [Chem. Phys. Lett. 341 (2001) 652]." Chemical Physics Letters 351, no. 1-2 (January 2002): 159–60. http://dx.doi.org/10.1016/s0009-2614(01)01363-x.

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46

Dulitz, Katrin, and Leon Karpa. "Focus on the cold and ultracold chemistry of atoms, ions and molecules." New Journal of Physics 24, no. 12 (December 1, 2022): 120401. http://dx.doi.org/10.1088/1367-2630/aca929.

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47

Gong, Ting, Zhonghua Ji, Jiaqi Du, Yanting Zhao, Liantuan Xiao, and Suotang Jia. "Microwave-assisted coherent control of ultracold polar molecules in a ladder-type configuration of rotational states." Physical Chemistry Chemical Physics 23, no. 7 (2021): 4271–76. http://dx.doi.org/10.1039/d1cp00202c.

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48

Morita, Masato, and Naduvalath Balakrishnan. "Stereodynamics of ultracold rotationally inelastic collisions." Journal of Chemical Physics 153, no. 18 (November 14, 2020): 184307. http://dx.doi.org/10.1063/5.0030808.

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49

Botsi, Sofia, Anbang Yang, Mark M. Lam, Sambit B. Pal, Sunil Kumar, Markus Debatin, and Kai Dieckmann. "Empirical LiK excited state potentials: connecting short range and near dissociation expansions." Physical Chemistry Chemical Physics 24, no. 6 (2022): 3933–40. http://dx.doi.org/10.1039/d1cp04707h.

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High-resolution excited state spectroscopy of ultracold LiK molecules. The fully empirical curve obtained serves as a starting point for the identification of a spectroscopic pathway to the absolute dipolar ground state.
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50

Ji, Zhonghua, Ting Gong, Yonglin He, Jeremy M. Hutson, Yanting Zhao, Liantuan Xiao, and Suotang Jia. "Microwave coherent control of ultracold ground-state molecules formed by short-range photoassociation." Physical Chemistry Chemical Physics 22, no. 23 (2020): 13002–7. http://dx.doi.org/10.1039/d0cp01191f.

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We report the observation of microwave coherent control of rotational states of ultracold 85Rb133Cs molecules formed in their vibronic ground state by short-range photoassociation.
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