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Journal articles on the topic 'Patterned polymer brushe'

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Author: Grafiati

Published: 9 March 2023

Last updated: 10 March 2023

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1

Chen, Tao, Debby P. Chang, Rainer Jordan, and Stefan Zauscher. "Colloidal lithography for fabricating patterned polymer-brush microstructures." Beilstein Journal of Nanotechnology 3 (May 15, 2012): 397–403. http://dx.doi.org/10.3762/bjnano.3.46.

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We exploit a series of robust, but simple and convenient colloidal lithography (CL) approaches, using a microsphere array as a mask or as a guiding template, and combine this with surface-initiated atom-transfer radical polymerization (SI-ATRP) to fabricate patterned polymer-brush microstructures. The advantages of the CL technique over other lithographic approaches for the fabrication of patterned polymer brushes are (i) that it can be carried out with commercially available colloidal particles at a relatively low cost, (ii) that no complex equipment is required to create the patterned templates with micro- and nanoscale features, and (iii) that polymer brush features are controlled simply by changing the size or chemical functionality of the microspheres or the substrate.

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2

Chen, Tao, Ihsan Amin, and Rainer Jordan. "Patterned polymer brushes." Chemical Society Reviews 41, no. 8 (2012): 3280. http://dx.doi.org/10.1039/c2cs15225h.

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3

Tizazu, Getachew. "Investigation of the Effect of Molecular Weight, Density, and Initiator Structure Size on the Repulsive Force between a PNIPAM Polymer Brush and Protein." Advances in Polymer Technology 2022 (October 22, 2022): 1–20. http://dx.doi.org/10.1155/2022/9741080.

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This paper focuses on the effect of degree of polymerization (N), density ( σ ), and pattern size ( x ) on the interaction force between a periodically patterned Poly(N-isopropylacrylamide) (PNIPAM) brush and protein. The hydrophobic interaction, the Van der Waals attractive force, and the steric repulsive force were expressed in terms of N , σ , and x . The osmotic constant (k1) and the entropic constant (k2) were determined from the fit of the steric repulsive force to an experimentally obtained force distance curve. The osmotic constant was 0.105, and the entropic constant was 0.255. Using these constants, the steric repulsive force was plotted as a function of the separation distance(s) between the substrate and the protein. The forces were determined at a separation distance equal to 0.3 nm, where L0 is the equilibrium thickness of the PNIPAM brush. At this separation distance, the value of the steric repulsive force was much higher than the value of the sum of the hydrophobic interaction and the Van der Waals attractive force for large degree of polymerization ( N > 100 ) and density ( σ > 0.2 chains/nm2). However, the repulsive force was comparable to the sum of the hydrophobic interaction and the Van der Waals attractive force for a small degree of polymerization ( N < 100 ) and density ( σ = 0.2 ). Furthermore, the steric repulsive force was plotted as a function of pattern size x . The plot indicated that the steric repulsive force becomes nearly zero for all degrees of polymerization and density when the value of the initiator structure size was less than 200 nm. In addition to the steric repulsive force, the lateral extension of the chains in the periodically patterned PNIPAM brush was calculated by scaling low and compared with the experimental data taken from previously published literatures. The polymer brush structure was modelled as if the immediate bare substrate is so wide that even a stretched polymer segment cannot reach to the next polymer brush structure. In such models, the value of the lateral extension was equal to the thickness of the homogenous brush. It was independent of the pattern size. However, when the polymer brush structure was modelled as if there is another polymer brush structure at a distance half of the size of the period, the lateral extension was found to be dependent on the size of the initiator structure size due to chain bridging. This was witnessed by the patterning of polymer brushes using the interferometric patterning of PNIPAM brushes and an atomic force microscopy imaging of the polymer brush structures both in air and in water. The polymer brush structure resolution in water was much lower than the resolution in air, which indicates the lateral extension of the polymer chains in water. For such kind of periodic polymer brush structures, the gap between them was calculated, and it was found dependent on the degree of polymerization, density, and initiator structure size.

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4

Chen, Tao, Ihsan Amin, and Rainer Jordan. "ChemInform Abstract: Patterned Polymer Brushes." ChemInform 43, no. 29 (June 21, 2012): no. http://dx.doi.org/10.1002/chin.201229275.

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5

Welch, M. Elizabeth, and Christopher K. Ober. "Responsive and patterned polymer brushes." Journal of Polymer Science Part B: Polymer Physics 51, no. 20 (August 7, 2013): 1457–72. http://dx.doi.org/10.1002/polb.23356.

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6

Ding, Zhebo, and Bruce Ganem. "Fabrication of patterned organic thin film by low-energy electron beam lithography and surface-initiated ring-opening metathesis polymerization." Canadian Journal of Chemistry 84, no. 10 (October 1, 2006): 1254–58. http://dx.doi.org/10.1139/v06-089.

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High densities of immobilized polymer brushes have been created on solid supports in a spatially addressable fashion. Octadecyltrichlorosilane was self-assembled on a silicon substrate to form an inert monolayer. The substrate was then patterned by low-energy electron beam lithography. Finally, the exposed region was back-filled with a second functionalized silane and the pattern was further amplified by surface-initiated ring-opening metathesis polymerization. The patterned substrate was imaged by scanning electron microscopy and atomic force microscopy.Key words: patterned thin film, e-beam lithography, ring-opening metathesis polymerization, polymer brushes.

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7

Chen, Chen, Chen-Gang Wang, Longqiang Xiao, and Atsushi Goto. "Photo-selective chain end transformation of polyacrylate-iodide using cysteamine and its application to facile single-step preparation of patterned polymer brushes." Chemical Communications 54, no. 97 (2018): 13738–41. http://dx.doi.org/10.1039/c8cc08157c.

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8

Zhou, Xuechang, Xuqing Liu, Zhuang Xie, and Zijian Zheng. "3D-patterned polymer brush surfaces." Nanoscale 3, no. 12 (2011): 4929. http://dx.doi.org/10.1039/c1nr11238d.

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9

Cimen, Dilek, and Tuncer Caykara. "Micro-patterned polymer brushes by a combination of photolithography and interface-mediated RAFT polymerization for DNA hybridization." Polymer Chemistry 6, no. 38 (2015): 6812–18. http://dx.doi.org/10.1039/c5py00923e.

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A novel micro-patterned poly(AHMA) brush was prepared by a combination of photolithography and interface mediated RAFT polymerization for DNA hybridization. By this method, highly resolved micro-patterned polymer brush structures down to ∼2.0 μm lines were obtained.

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10

Chen, Chen, Chen-Gang Wang, Wenxun Guan, and Atsushi Goto. "A photo-selective chain-end modification of polyacrylate-iodide and its application in patterned polymer brush synthesis." Polymer Chemistry 10, no. 43 (2019): 5913–19. http://dx.doi.org/10.1039/c9py01431d.

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11

Smenda, Joanna, Karol Wolski, Kamila Chajec, and Szczepan Zapotoczny. "Preparation of Homopolymer, Block Copolymer, and Patterned Brushes Bearing Thiophene and Acetylene Groups Using Microliter Volumes of Reaction Mixtures." Polymers 13, no. 24 (December 19, 2021): 4458. http://dx.doi.org/10.3390/polym13244458.

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The synthesis of surface-grafted polymers with variable functionality requires the careful selection of polymerization methods that also enable spatially controlled grafting, which is crucial for the fabrication of, e.g., nano (micro) sensor or nanoelectronic devices. The development of versatile, simple, economical, and eco-friendly synthetic strategies is important for scaling up the production of such polymer brushes. We have recently shown that poly (3-methylthienyl methacrylate) (PMTM) and poly (3-trimethylsilyl-2-propynyl methacrylate) (PTPM) brushes with pendant thiophene and acetylene groups, respectively, could be used for the production of ladder-like conjugated brushes that are potentially useful in the mentioned applications. However, the previously developed syntheses of such brushes required the use of high volumes of reagents, elevated temperature, or high energy UV-B light. Therefore, we present here visible light-promoted metal-free surface-initiated ATRP (metal-free SI-ATRP) that allows the economical synthesis of PMTM and PTPM brushes utilizing only microliter volumes of reaction mixtures. The versatility of this approach was shown by the formation of homopolymers but also the block copolymer conjugated brushes (PMTM and PTPM blocks in both sequences) and patterned films using TEM grids serving as photomasks. A simple reaction setup with only a monomer, solvent, commercially available organic photocatalyst, and initiator decorated substrate makes the synthesis of these complex polymer structures achievable for non-experts and ready for scaling up.

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12

Padeste, Celestino, Harun H. Solak, Hans-Peter Brack, Michal Slaski, Selmiye Alkan Gürsel, and Günther G. Scherer. "Patterned grafting of polymer brushes onto flexible polymer substrates." Journal of Vacuum Science & Technology B: Microelectronics and Nanometer Structures 22, no. 6 (2004): 3191. http://dx.doi.org/10.1116/1.1805542.

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13

Edmondson, S., and W. T. S. Huck. "Quasi-2D Polymer Objects from Patterned, Crosslinked Polymer Brushes." Advanced Materials 16, no. 15 (August 4, 2004): 1327–31. http://dx.doi.org/10.1002/adma.200400761.

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14

Schneider, Maximilian, Zian Tang, Marcus Richter, Claudia Marschelke, Paul Förster, Erik Wegener, Ihsan Amin, et al. "Patterned Polypeptoid Brushes." Macromolecular Bioscience 16, no. 1 (November 2, 2015): 75–81. http://dx.doi.org/10.1002/mabi.201500314.

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15

Schneider, Maximilian, Zian Tang, Marcus Richter, Claudia Marschelke, Paul Förster, Erik Wegener, Ihsan Amin, et al. "Patterned Polypeptoid Brushes." Macromolecular Bioscience 16, no. 1 (January 2016): 74. http://dx.doi.org/10.1002/mabi.201670004.

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16

Kollarigowda, R. H., C. Fedele, C. Rianna, A. Calabuig, A. C. Manikas, V. Pagliarulo, P. Ferraro, S. Cavalli, and P. A. Netti. "Light-responsive polymer brushes: active topographic cues for cell culture applications." Polymer Chemistry 8, no. 21 (2017): 3271–78. http://dx.doi.org/10.1039/c7py00462a.

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17

Welch, M. Elizabeth, Youyong Xu, Hongjun Chen, Norah Smith, Michael E. Tague, Hector D. Abruna, Barbara Baird, and Christopher K. Ober. "Polymer Brushes as Functional, Patterned Surfaces for Nanobiotechnology." Journal of Photopolymer Science and Technology 25, no. 1 (2012): 53–56. http://dx.doi.org/10.2494/photopolymer.25.53.

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18

de las Heras Alarcón, Carolina, Tamer Farhan, Vicky L. Osborne, Wilhelm T. S. Huck, and Cameron Alexander. "Bioadhesion at micro-patterned stimuli-responsive polymer brushes." Journal of Materials Chemistry 15, no. 21 (2005): 2089. http://dx.doi.org/10.1039/b419142k.

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19

Kettling, Friederike, Benjamin Vonhören, Jennifer A. Krings, Susumu Saito, and Bart Jan Ravoo. "One-step synthesis of patterned polymer brushes by photocatalytic microcontact printing." Chemical Communications 51, no. 6 (2015): 1027–30. http://dx.doi.org/10.1039/c4cc08646e.

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20

Ye, Qun, Peng Xiao, Wulong Liu, Ke Chen, Tao Chen, Jianming Xue, Shiyu Du, and Qing Huang. "Exploring the potential of exfoliated ternary ultrathin Ti4AlN3 nanosheets for fabricating hybrid patterned polymer brushes." RSC Advances 5, no. 86 (2015): 70339–44. http://dx.doi.org/10.1039/c5ra09227b.

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A new type of ternary Ti₄AlN₃ nanosheets was prepared for the first time. The obtained sheets with surface groups could be further used to fabricate micro-patterns and subsequently functionalized to achieve hybrid patterned polymer brushes.

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21

De Mets, Richard, Katharina Hennig, Lionel Bureau, and Martial Balland. "Fast and robust fabrication of reusable molds for hydrogel micro-patterning." Biomaterials Science 4, no. 11 (2016): 1630–37. http://dx.doi.org/10.1039/c6bm00364h.

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We present a method to create protein micropatterns onto polyacrylamide hydrogels, in order to control the adhesive confinement of cells in traction force microscopy experiments. The technique is based on patterned polymer brushes that serve as molds that can be re-used without repeating microfabrication steps.

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22

Cao, Qianqian. "Anisotropic electrokinetic transport in channels modified with patterned polymer brushes." Soft Matter 15, no. 20 (2019): 4132–45. http://dx.doi.org/10.1039/c9sm00385a.

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23

Choi, Jae-Hak, Dong-Ki Kim, Chan-Hee Jung, and Ramakrishnan Ganesan. "Preparation of Patterned Polymer Brushes by Radiation-Induced Grafting." Journal of the Korean Physical Society 52, no. 9(3) (March 15, 2008): 880–83. http://dx.doi.org/10.3938/jkps.52.880.

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24

Farhan, Tamer, and Wilhelm T. S. Huck. "Synthesis of patterned polymer brushes from flexible polymeric films." European Polymer Journal 40, no. 8 (August 2004): 1599–604. http://dx.doi.org/10.1016/j.eurpolymj.2004.05.001.

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25

Pernites, Roderick B., Edward L. Foster, Mary Jane L. Felipe, Michael Robinson, and Rigoberto C. Advincula. "Patterned Surfaces Combining Polymer Brushes and Conducting Polymer via Colloidal Template Electropolymerization." Advanced Materials 23, no. 10 (January 18, 2011): 1287–92. http://dx.doi.org/10.1002/adma.201004003.

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26

Ma, Wen, Md Saifur Rahaman, and Heloise Therien-Aubin. "Controlling biofouling of reverse osmosis membranes through surface modification via grafting patterned polymer brushes." Journal of Water Reuse and Desalination 5, no. 3 (March 19, 2015): 326–34. http://dx.doi.org/10.2166/wrd.2015.114.

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Thin film composite (TFC) polyamide membranes are extensively used as selective barriers in reverse osmosis processes. The major challenge faced with TFC membranes is significant fouling on the surface, which restricts the overall purification performance. To address the fouling problem, we developed novel fouling-resistant surface coatings via polyelectrolyte [poly(allylamine hydrochloride)/poly(styrene sulfonate)] layer-by-layer self-assembly, functionalized with patterned antimicrobial and antifouling/fouling-release polymer brushes. Two types of different polymer brushes, among antimicrobial poly(quaternary ammonium), antifouling poly(sulfobetaine) and fouling-release poly(dimethylsiloxane) (PDMS), were selected and grafted in a checkerboard pattern, with a square feature of 2 µm. The successful patterning and incorporation of different polymer brushes on the membrane was confirmed through X-ray photoelectron spectroscopy analysis. Grafting with sulfobetaine and PDMS significantly increased the hydrophilicity and lowered the surface energy of the membrane, respectively. The fouling-resistant property of the modified membrane was evaluated via static protein (bovine serum albumin) deposition and bacterial (Escherichia coli) cell adhesion tests. Surface modifications proved to diminish protein adhesion and exhibited 70–93% reduction in bacterial cell attachment. This observation suggests that the modified membranes have strong antifouling properties that inhibit the irreversible adhesion of organic and bio-foulants on the membrane surface.

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27

Liu, Chi-Chun, Eungnak Han, M. Serdar Onses, Christopher J. Thode, Shengxiang Ji, Padma Gopalan, and Paul F. Nealey. "Fabrication of Lithographically Defined Chemically Patterned Polymer Brushes and Mats." Macromolecules 44, no. 7 (April 12, 2011): 1876–85. http://dx.doi.org/10.1021/ma102856t.

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28

Enright, Timothy P., Daniel Hagaman, Maryana Kokoruz, Natalia Coleman, and Alexander Sidorenko. "Gradient and patterned polymer brushes by photoinitiated “grafting through” approach." Journal of Polymer Science Part B: Polymer Physics 48, no. 14 (March 15, 2010): 1616–22. http://dx.doi.org/10.1002/polb.21962.

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29

Clarkson, Christopher G., Alexander Johnson, Graham J. Leggett, and Mark Geoghegan. "Slow polymer diffusion on brush-patterned surfaces in aqueous solution." Nanoscale 11, no. 13 (2019): 6052–61. http://dx.doi.org/10.1039/c9nr00341j.

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30

Cho, Ha, Ayoung Choe, Woon Park, Hyunhyub Ko, and Myunghwan Byun. "Lithography-Free Route to Hierarchical Structuring of High-χ Block Copolymers on a Gradient Patterned Surface." Materials 13, no. 2 (January 9, 2020): 304. http://dx.doi.org/10.3390/ma13020304.

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A chemically defined patterned surface was created via a combined process of controlled evaporative self-assembly of concentric polymer stripes and the selective surface modification of polymer brush. The former process involved physical adsorption of poly (methyl methacrylate) (PMMA) segments into silicon oxide surface, thus forming ultrathin PMMA stripes, whereas the latter process was based on the brush treatment of silicon native oxide surface using a hydroxyl-terminated polystyrene (PS-OH). The resulting alternating PMMA- and PS-rich stripes provided energetically favorable regions for self-assembly of high χ polystyrene-block-polydimethylsiloxane (PS-b-PDMS) in a simple and facile manner, dispensing the need for conventional lithography techniques. Subsequently, deep reactive ion etching and oxygen plasma treatment enabled the transition of the PDMS blocks into oxidized groove-shaped nanostructures.

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31

Gao, Tingting, Xiaolong Wang, Bo Yu, Qiangbing Wei, Yanqiu Xia, and Feng Zhou. "Noncovalent Microcontact Printing for Grafting Patterned Polymer Brushes on Graphene Films." Langmuir 29, no. 4 (January 15, 2013): 1054–60. http://dx.doi.org/10.1021/la304385r.

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32

Wang, Chen-Gang, Hui Wen Yong, and Atsushi Goto. "Effective Synthesis of Patterned Polymer Brushes with Tailored Multiple Graft Densities." ACS Applied Materials & Interfaces 11, no. 15 (April 2, 2019): 14478–84. http://dx.doi.org/10.1021/acsami.9b03570.

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33

Becer, C. Remzi, Claudia Haensch, Stephanie Hoeppener, and Ulrich S Schubert. "Patterned Polymer Brushes Grafted from Bromine-Functionalized, Chemically Active Surface Templates." Small 3, no. 2 (February 5, 2007): 220–25. http://dx.doi.org/10.1002/smll.200600234.

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34

Sato, Tomoya, Gary J. Dunderdale, Chihiro Urata, and Atsushi Hozumi. "Spatially-Regulated Deposition of Quantum Dots on the Patterned Polymer Brush." Journal of Nanoscience and Nanotechnology 20, no. 8 (August 1, 2020): 5201–10. http://dx.doi.org/10.1166/jnn.2020.18523.

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We have demonstrated direct patterning of surface initiator layer (SIL) for Atom Transfer Radical Polymerization (ATRP) using a sol–gel based “ink” containing (p-chloromethyl)phenyltrimethoxysilane and tetraethoxysilane for an inkjet printer. Mechanically/chemically robust and smooth micropatterns of SIL several tens of micrometer in width and 15 nm thickness were directly printed on silicon substrates under mild conditions (open to the atmosphere, at ~28 °C under >60% relative humidity). Subsequent surface-initiated ATRP of glycidyl methacrylate (GMA) under the air atmosphere gave area-selective/stepwise growth of homogeneous polyGMA brushes (pGMA) from the micropatterns of SIL. This area-selective growth of pGMA was also confirmed by a fluorescence microscopy. Because of chemical reactivity of epoxy groups on the grafted pGMA surfaces toward amino-functionalized nanomaterials, CdS/ZnS-alloyed quantum dots were spatially deposited only on the pGMA-covered regions with a complete area-selectivity.

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35

Zhang, Ren, Bongjoon Lee, Christopher M. Stafford, Jack F. Douglas, Andrey V. Dobrynin, Michael R. Bockstaller, and Alamgir Karim. "Entropy-driven segregation of polymer-grafted nanoparticles under confinement." Proceedings of the National Academy of Sciences 114, no. 10 (February 22, 2017): 2462–67. http://dx.doi.org/10.1073/pnas.1613828114.

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The modification of nanoparticles with polymer ligands has emerged as a versatile approach to control the interactions and organization of nanoparticles in polymer nanocomposite materials. Besides their technological significance, polymer-grafted nanoparticle (PGNP) dispersions have attracted interest as model systems to understand the role of entropy as a driving force for microstructure formation. For instance, densely and sparsely grafted nanoparticles show distinct dispersion and assembly behaviors within polymer matrices due to the entropy variation associated with conformational changes in brush and matrix chains. Here we demonstrate how this entropy change can be harnessed to drive PGNPs into spatially organized domain structures on submicrometer scale within topographically patterned thin films. This selective segregation of PGNPs is induced by the conformational entropy penalty arising from local perturbations of grafted and matrix chains under confinement. The efficiency of this particle segregation process within patterned mesa−trench films can be tuned by changing the relative entropic confinement effects on grafted and matrix chains. The versatility of topographic patterning, combined with the compatibility with a wide range of nanoparticle and polymeric materials, renders SCPINS (soft-confinement pattern-induced nanoparticle segregation) an attractive method for fabricating nanostructured hybrid films with potential applications in nanomaterial-based technologies.

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36

Xiao, Peng, Jincui Gu, Jing Chen, Jiawei Zhang, Rubo Xing, Yanchun Han, Jun Fu, Wenqin Wang, and Tao Chen. "Micro-contact printing of graphene oxide nanosheets for fabricating patterned polymer brushes." Chemical Communications 50, no. 54 (2014): 7103. http://dx.doi.org/10.1039/c4cc01467g.

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37

Léonforte, F., and M. Müller. "Morphology Modulation of Multicomponent Polymer Brushes in Selective Solvent by Patterned Surfaces." Macromolecules 48, no. 1 (December 30, 2014): 213–28. http://dx.doi.org/10.1021/ma502256p.

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38

Wang, Yu-Hsuan, Miao-Ken Hung, Chun-Hao Lin, Hsiao-Chien Lin, and Jyh-Tsung Lee. "Patterned nitroxide polymer brushes for thin-film cathodes in organic radical batteries." Chem. Commun. 47, no. 4 (2011): 1249–51. http://dx.doi.org/10.1039/c0cc02442b.

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39

Yu, Kai, Yang Cong, Jun Fu, Rubo Xing, Nana Zhao, and Yanchun Han. "Patterned self-adaptive polymer brushes by “grafting to” approach and microcontact printing." Surface Science 572, no. 2-3 (November 2004): 490–96. http://dx.doi.org/10.1016/j.susc.2004.09.037.

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40

Panzarasa, Guido, Guido Soliveri, Silvia Ardizzone, and Katia Sparnacci. "Photocatalytic Lithography: An Innovative Approach to Obtain Patterned pH-responsive Polymer Brushes." Materials Today: Proceedings 2, no. 8 (2015): 4183–89. http://dx.doi.org/10.1016/j.matpr.2015.09.001.

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41

Koo, Hyung-Jun, Kristopher V. Waynant, Chunjie Zhang, and Paul V. Braun. "Polymer Brushes Patterned with Micrometer-Scale Chemical Gradients Using Laminar Co-Flow." ACS Applied Materials & Interfaces 6, no. 16 (July 9, 2014): 14320–26. http://dx.doi.org/10.1021/am503609x.

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42

Yang, Sung Yun, Dul-Yi Kim, Sang-Mi Jeong, and Ji-Woong Park. "Stimuli-Responsive Hybrid Coatings of Polyelectrolyte Multilayers and Nano-Patterned Polymer Brushes." Macromolecular Rapid Communications 29, no. 9 (May 2, 2008): 729–36. http://dx.doi.org/10.1002/marc.200800017.

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43

Thode, Christopher J., Peter L. Cook, Yaming Jiang, M. Serdar Onses, Shengxiang Ji, Franz J. Himpsel, and Paul F. Nealey. "In situmetallization of patterned polymer brushes created by molecular transfer print and fill." Nanotechnology 24, no. 15 (March 22, 2013): 155602. http://dx.doi.org/10.1088/0957-4484/24/15/155602.

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44

Mathieu, Mareike, Alexander Friebe, Steffen Franzka, Mathias Ulbricht, and Nils Hartmann. "Surface-Initiated Polymerization on Laser-Patterned Templates: Morphological Scaling of Nanoconfined Polymer Brushes." Langmuir 25, no. 20 (October 20, 2009): 12393–98. http://dx.doi.org/10.1021/la901718k.

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45

Liu, Yong, Viktor Klep, and Igor Luzinov. "To Patterned Binary Polymer Brushes via Capillary Force Lithography and Surface-Initiated Polymerization." Journal of the American Chemical Society 128, no. 25 (June 2006): 8106–7. http://dx.doi.org/10.1021/ja061646f.

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46

Jia, Xinyan, Xuesong Jiang, Rui Liu, and Jie Yin. "Facile Approach to Patterned Binary Polymer Brush through Photolithography and Surface-Initiated Photopolymerization." ACS Applied Materials & Interfaces 2, no. 4 (April 2, 2010): 1200–1205. http://dx.doi.org/10.1021/am100035d.

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47

Dong, Rong, Sitaraman Krishnan, Barbara A. Baird, Manfred Lindau, and Christopher K. Ober. "Patterned Biofunctional Poly(acrylic acid) Brushes on Silicon Surfaces." Biomacromolecules 8, no. 10 (October 2007): 3082–92. http://dx.doi.org/10.1021/bm700493v.

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48

Laktionov, Mikhail Y., Ekaterina B. Zhulina, Ralf P. Richter, and Oleg V. Borisov. "Polymer Brush in a Nanopore: Effects of Solvent Strength and Macromolecular Architecture Studied by Self-Consistent Field and Scaling Theory." Polymers 13, no. 22 (November 14, 2021): 3929. http://dx.doi.org/10.3390/polym13223929.

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To study conformational transition occuring upon inferior solvent strength in a brush formed by linear or dendritically branched macromolecules tethered to the inner surface of cylindrical or planar (slit-like) pore, a self-consistent field analytical approach is employed. Variations in the internal brush structure as a function of variable solvent strength and pore radius, and the onset of formation of a hollow channel in the pore center are analysed. The predictions of analytical theory are supported and complemented by numerical modelling by a self-consistent field Scheutjens–Fleer method. Scaling arguments are used to study microphase segregation under poor solvent conditions leading to formation of a laterally and longitudinally patterned structure in planar and cylindrical pores, respectively, and the effects of confinement on "octopus-like" clusters in the pores of different geometries.

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49

Foster, Edward L., Maria Celeste R. Tria, Roderick B. Pernites, Steven J. Addison, and Rigoberto C. Advincula. "Patterned polymer brushes via electrodeposited ATRP, ROMP, and RAFT initiators on colloidal template arrays." Soft Matter 8, no. 2 (2012): 353–59. http://dx.doi.org/10.1039/c1sm06406a.

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Chen, Tao, Debby P. Chang, and Stefan Zauscher. "Polymer brushes: Fabrication of Patterned Polymer Brushes on Chemically Active Surfaces by in situ Hydrogen-Bond-Mediated Attachment of an Initiator (Small 14/2010)." Small 6, no. 14 (July 9, 2010): n/a. http://dx.doi.org/10.1002/smll.201090044.

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