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Journal articles on the topic 'Multicatalyse'

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1

Poe, Sarah L., Muris Kobašlija, and D. Tyler McQuade. "Microcapsule Enabled Multicatalyst System." Journal of the American Chemical Society 128, no. 49 (December 2006): 15586–87. http://dx.doi.org/10.1021/ja066476l.

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2

Hofmann, Christine, Sören M. M. Schuler, Raffael C. Wende, and Peter R. Schreiner. "En route to multicatalysis: kinetic resolution of trans-cycloalkane-1,2-diols via oxidative esterification." Chem. Commun. 50, no. 10 (2014): 1221–23. http://dx.doi.org/10.1039/c3cc48584f.

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We demonstrate the application of a multicatalyst to the oxidation of a broad variety of aldehydes and subsequent enantioselective esterification of the incipient acids with (±)-trans-cycloalkane-1,2-diols.
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3

Mata, José A., F. Ekkehardt Hahn, and Eduardo Peris. "Heterometallic complexes, tandem catalysis and catalytic cooperativity." Chem. Sci. 5, no. 5 (2014): 1723–32. http://dx.doi.org/10.1039/c3sc53126k.

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4

Ma, Jin-Tao, and Ying Cheng. "Construction of enantiopure imine bridged benzo[c]azepinones by a silver(i) and chiral N-heterocyclic carbene multicatalytic reaction sequence of N′-(2-alkynylbenzylidene)hydrazides and cyclopropanecarbaldehydes." Organic Chemistry Frontiers 7, no. 21 (2020): 3459–67. http://dx.doi.org/10.1039/d0qo00877j.

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5

Jürjens, Gerrit, Andreas Kirschning, and David A. Candito. "Lessons from the Synthetic Chemist Nature." Natural Product Reports 32, no. 5 (2015): 723–37. http://dx.doi.org/10.1039/c4np00160e.

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Nature's strategy of performing ideal multistep (bio)synthesis are based on multicatalysis, domino reactions, iteration and compartmentation. These are discussed and compared with chemical synthesis in this conceptual review.
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6

Tang, Xinxin, Lan Gan, Xin Zhang, and Zheng Huang. "n-Alkanes to n-alcohols: Formal primary C─H bond hydroxymethylation via quadruple relay catalysis." Science Advances 6, no. 47 (November 2020): eabc6688. http://dx.doi.org/10.1126/sciadv.abc6688.

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Nature is able to synergistically combine multiple enzymes to conduct well-ordered biosynthetic transformations. Mimicking nature’s multicatalysis in vitro may give rise to new chemical transformations via interplay of numerous molecular catalysts in one pot. The direct and selective conversion of abundant n-alkanes to valuable n-alcohols is a reaction with enormous potential applicability but has remained an unreached goal. Here, we show that a quadruple relay catalysis system involving three discrete transition metal catalysts enables selective synthesis of n-alcohols via n-alkane primary C─H bond hydroxymethylation. This one-pot multicatalysis system is composed of Ir-catalyzed alkane dehydrogenation, Rh-catalyzed olefin isomerization and hydroformylation, and Ru-catalyzed aldehyde hydrogenation. This system is further applied to synthesis of α,ω-diols from simple α-olefins through terminal-selective hydroxymethylation of silyl alkanes.
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7

Pellissier, Hélène. "Recent developments in enantioselective multicatalysed tandem reactions." Tetrahedron 69, no. 35 (September 2013): 7171–210. http://dx.doi.org/10.1016/j.tet.2013.06.020.

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8

Martínez, Sebastián, Lukas Veth, Bruno Lainer, and Paweł Dydio. "Challenges and Opportunities in Multicatalysis." ACS Catalysis 11, no. 7 (March 15, 2021): 3891–915. http://dx.doi.org/10.1021/acscatal.0c05725.

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9

Tsoung, Jennifer, Jane Panteleev, Matthias Tesch, and Mark Lautens. "Multicomponent-Multicatalyst Reactions (MC)2R: Efficient Dibenzazepine Synthesis." Organic Letters 16, no. 1 (December 13, 2013): 110–13. http://dx.doi.org/10.1021/ol4030925.

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10

Marafi, A., F. Maruyama, A. Stanislaus, and E. Kam. "Multicatalyst System Testing Methodology for Upgrading Residual Oils." Industrial & Engineering Chemistry Research 47, no. 3 (February 2008): 724–41. http://dx.doi.org/10.1021/ie071103u.

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11

Zhou, Jian. "Recent Advances in Multicatalyst Promoted Asymmetric Tandem Reactions." Chemistry - An Asian Journal 5, no. 3 (March 1, 2010): 422–34. http://dx.doi.org/10.1002/asia.200900458.

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12

Poe, Sarah L., Muris Kobašlija, and D. Tyler McQuade. "Mechanism and Application of a Microcapsule Enabled Multicatalyst Reaction." Journal of the American Chemical Society 129, no. 29 (July 2007): 9216–21. http://dx.doi.org/10.1021/ja071706x.

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13

Sancheti, Shashank P., Urvashi, Mosami P. Shah, and Nitin T. Patil. "Ternary Catalysis: A Stepping Stone toward Multicatalysis." ACS Catalysis 10, no. 5 (January 8, 2020): 3462–89. http://dx.doi.org/10.1021/acscatal.9b04000.

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14

Pellissier, Hélène. "Recent Developments in Enantioselective Multicatalyzed Tandem Reactions." Advanced Synthesis & Catalysis 362, no. 12 (May 15, 2020): 2289–325. http://dx.doi.org/10.1002/adsc.202000210.

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15

Ambrosini, Lisa M., and Tristan H. Lambert. "Multicatalysis: Advancing Synthetic Efficiency and Inspiring Discovery." ChemCatChem 2, no. 11 (September 17, 2010): 1373–80. http://dx.doi.org/10.1002/cctc.200900323.

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16

Tsoung, Jennifer, Jane Panteleev, Matthias Tesch, and Mark Lautens. "ChemInform Abstract: Multicomponent-Multicatalyst Reactions (MC)2R: Efficient Dibenzazepine Synthesis." ChemInform 45, no. 23 (May 22, 2014): no. http://dx.doi.org/10.1002/chin.201423059.

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17

Zhou, Jian. "ChemInform Abstract: Recent Advances in Multicatalyst Promoted Asymmetric Tandem Reactions." ChemInform 41, no. 23 (June 8, 2010): no. http://dx.doi.org/10.1002/chin.201023205.

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18

Zhang, Lei, Lorenzo Sonaglia, Jason Stacey, and Mark Lautens. "Multicomponent Multicatalyst Reactions (MC)2R: One-Pot Synthesis of 3,4-Dihydroquinolinones." Organic Letters 15, no. 9 (April 19, 2013): 2128–31. http://dx.doi.org/10.1021/ol4006008.

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19

Jindal, Garima, and Raghavan B. Sunoj. "Mechanistic Insights on Cooperative Asymmetric Multicatalysis Using Chiral Counterions." Journal of Organic Chemistry 79, no. 16 (July 29, 2014): 7600–7606. http://dx.doi.org/10.1021/jo501322v.

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20

Kim, Mahn-Joo, Min Young Choi, Min Young Han, Yoon Kyung Choi, Jae Kwan Lee, and Jaiwook Park. "Asymmetric Transformations of Acyloxyphenyl Ketones by Enzyme−Metal Multicatalysis." Journal of Organic Chemistry 67, no. 26 (December 2002): 9481–83. http://dx.doi.org/10.1021/jo026122m.

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21

Pellissier, Helene. "ChemInform Abstract: Recent Developments in Enantioselective Multicatalyzed Tandem Reactions." ChemInform 44, no. 43 (October 7, 2013): no. http://dx.doi.org/10.1002/chin.201343223.

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22

Ambrosini, Lisa M., and Tristan H. Lambert. "ChemInform Abstract: Multicatalysis: Advancing Synthetic Efficiency and Inspiring Discovery." ChemInform 42, no. 9 (February 3, 2011): no. http://dx.doi.org/10.1002/chin.201109248.

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23

Hrdina, Radim, Christian E. Müller, Raffael C. Wende, Lukas Wanka, and Peter R. Schreiner. "Enantiomerically enriched trans-diols from alkenes in one pot: a multicatalyst approach." Chemical Communications 48, no. 19 (2012): 2498. http://dx.doi.org/10.1039/c2cc17435a.

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24

Shugrue, Christopher R., Bianca R. Sculimbrene, Elizabeth R. Jarvo, Brandon Q. Mercado, and Scott J. Miller. "Outer-Sphere Control for Divergent Multicatalysis with Common Catalytic Moieties." Journal of Organic Chemistry 84, no. 3 (January 4, 2019): 1664–72. http://dx.doi.org/10.1021/acs.joc.8b03068.

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25

Richmond, Edward, Ismat Ullah Khan, and Joseph Moran. "Enantioselective and Regiodivergent Functionalization ofN-Allylcarbamates by Mechanistically Divergent Multicatalysis." Chemistry - A European Journal 22, no. 35 (July 27, 2016): 12274–77. http://dx.doi.org/10.1002/chem.201602792.

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26

Juraidan, Mohammed, Mahmoud Al-Shamali, Hasan Qabazard, and Ezra K. T. Kam. "A Refined Hydroprocessing Multicatalyst Deactivation and Reactor Performance ModelPilot-Plant Accelerated Test Applications." Energy & Fuels 20, no. 4 (July 2006): 1354–64. http://dx.doi.org/10.1021/ef0504265.

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27

Kam, E. K. T., M. Al-Shamali, M. Juraidan, and H. Qabazard. "A Hydroprocessing Multicatalyst Deactivation and Reactor Performance Model−Pilot-Plant Life Test Applications." Energy & Fuels 19, no. 3 (May 2005): 753–64. http://dx.doi.org/10.1021/ef049843s.

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28

Zhang, Lei, Lorenzo Sonaglia, Jason Stacey, and Mark Lautens. "ChemInform Abstract: Multicomponent Multicatalyst Reactions (MC)2R: One-Pot Synthesis of 3,4-Dihydroquinolinones." ChemInform 44, no. 35 (August 8, 2013): no. http://dx.doi.org/10.1002/chin.201335149.

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29

Gaur, Akshay, Shivam Dubey, Zainab Mufarreh Elqahtani, Samia ben Ahmed, Mohammed Sultan Abdulghaffar Al-Buriahi, Rahul Vaish, and Vishal Singh Chauhan. "Effect of Poling on Multicatalytic Performance of 0.5Ba(Zr0.2Ti0.8)O3-0.5(Ba0.7Sr0.3)TiO3 Ferroelectric Ceramic for Dye Degradation." Materials 15, no. 22 (November 18, 2022): 8217. http://dx.doi.org/10.3390/ma15228217.

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Ferroelectric materials with a spontaneous polarization are proven to be potential multicatalysts in water remediation applications. The composition of 0.5Ba(Zr0.2Ti0.8)O3-0.5(Ba0.7Sr0.3)TiO3 (BST-BZT) was examined for photocatalysis, piezocatalysis, and piezo-photocatalysis processes by degrading an azo dye named methylene blue (MB). Generally, dis-aligned dipoles restrict the catalytic activities due to which the BST-BZT powder sample was poled by the corona poling technique. Coupled piezocatalysis and photocatalysis process, i.e., the piezo-photocatalysis process has shown maximum dye degradation. There was a significant improvement in degradation efficiency by using a poled BST-BZT sample compared to the unpoled sample in all processes, thus the results suggest an extensive scope of poled ferroelectric ceramic powder in the catalysis field.
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30

Collina, G., A. Pelliconi, P. Sgarzi, F. Sartori, and G. Baruzzi. "Highly flexible heterophasic copolymers through the novel multicatalysts reactor granule technology." Polymer Bulletin 39, no. 2 (August 1997): 241–47. http://dx.doi.org/10.1007/s002890050144.

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31

Júnior, Aldo Araújo da Trindade, Yan Ferraz Ximenes Ladeira, Alexandre da Silva França, Rodrigo Octavio Mendonça Alves de Souza, Adolfo Henrique Moraes, Robert Wojcieszak, Ivaldo Itabaiana Jr., and Amanda Silva de Miranda. "Multicatalytic Hybrid Materials for Biocatalytic and Chemoenzymatic Cascades—Strategies for Multicatalyst (Enzyme) Co-Immobilization." Catalysts 11, no. 8 (July 31, 2021): 936. http://dx.doi.org/10.3390/catal11080936.

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During recent decades, the use of enzymes or chemoenzymatic cascades for organic chemistry has gained much importance in fundamental and industrial research. Moreover, several enzymatic and chemoenzymatic reactions have also served in green and sustainable manufacturing processes especially in fine chemicals, pharmaceutical, and flavor/fragrance industries. Unfortunately, only a few processes have been applied at industrial scale because of the low stabilities of enzymes along with the problematic processes of their recovery and reuse. Immobilization and co-immobilization offer an ideal solution to these problems. This review gives an overview of all the pathways for enzyme immobilization and their use in integrated enzymatic and chemoenzymatic processes in cascade or in a one-pot concomitant execution. We place emphasis on the factors that must be considered to understand the process of immobilization. A better understanding of this fundamental process is an essential tool not only in the choice of the best route of immobilization but also in the understanding of their catalytic activity.
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32

Müller, Christian E., Radim Hrdina, Raffael C. Wende, and Peter R. Schreiner. "A Multicatalyst System for the One‐Pot Desymmetrization/Oxidation of meso ‐1,2‐Alkane Diols." Chemistry – A European Journal 17, no. 23 (April 27, 2011): 6309–14. http://dx.doi.org/10.1002/chem.201100498.

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33

Hrdina, Radim, Christian E. Mueller, Raffael C. Wende, Lukas Wanka, and Peter R. Schreiner. "ChemInform Abstract: Enantiomerically Enriched trans-Diols from Alkenes in One Pot: A Multicatalyst Approach." ChemInform 43, no. 27 (June 11, 2012): no. http://dx.doi.org/10.1002/chin.201227023.

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34

Xiao, Pin, Haiyan Yuan, Jianquan Liu, Yiying Zheng, Xihe Bi, and Jingping Zhang. "Radical Mechanism of Isocyanide-Alkyne Cycloaddition by Multicatalysis of Ag2CO3, Solvent, and Substrate." ACS Catalysis 5, no. 10 (September 22, 2015): 6177–84. http://dx.doi.org/10.1021/acscatal.5b01703.

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35

Georgi, Anett, Miriam Velasco Polo, Klara Crincoli, Katrin Mackenzie, and Frank-Dieter Kopinke. "Accelerated Catalytic Fenton Reaction with Traces of Iron: An Fe–Pd-Multicatalysis Approach." Environmental Science & Technology 50, no. 11 (May 26, 2016): 5882–91. http://dx.doi.org/10.1021/acs.est.6b01049.

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36

Jeong, Youngmin, Jonghyun Park, and Myungwan Han. "Design and Control of a Fixed-Bed Recycle Reactor with Multicatalyst Layers: Methanation of Carbon Dioxide." Industrial & Engineering Chemistry Research 60, no. 12 (March 19, 2021): 4650–67. http://dx.doi.org/10.1021/acs.iecr.0c05784.

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37

Alachraf, M. Wasim, Raffael C. Wende, Sören M. M. Schuler, Peter R. Schreiner, and Wolfgang Schrader. "Functionality, Effectiveness, and Mechanistic Evaluation of a Multicatalyst-Promoted Reaction Sequence by Electrospray Ionization Mass Spectrometry." Chemistry - A European Journal 21, no. 45 (September 25, 2015): 16203–8. http://dx.doi.org/10.1002/chem.201502640.

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38

Du, Jiang, Xiaohua Zhang, and Charles C. Han. "Fluctuation-assisted crystallization of an iPP/PEOc polymer alloy prepared on a single multicatalyst reactor granule." Journal of Polymer Science Part B: Polymer Physics 47, no. 2 (January 15, 2009): 166–72. http://dx.doi.org/10.1002/polb.21627.

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39

Youn, So Won, Hyoung Sub Song, and Jong Hyub Park. "Asymmetric Domino Multicatalysis for the Synthesis of 3-Substituted Phthalides: Cinchonine/NHC Cooperative System." Organic Letters 16, no. 3 (January 24, 2014): 1028–31. http://dx.doi.org/10.1021/ol5000617.

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40

Pan, Zhentao, Xuancheng Yang, Bo Chen, Shuaijun Shi, Tong Liu, Xuqiong Xiao, Linlin Shen, Li Lou, and Yongmin Ma. "Employing Visible-Light Photoredox Catalysis in Multicomponent–Multicatalyst Reactions: One-Pot Synthesis of Spiroquinazolin-2-(thi)ones." Journal of Organic Chemistry 87, no. 5 (February 11, 2022): 3596–604. http://dx.doi.org/10.1021/acs.joc.1c03151.

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41

Lied, Fabian, Helena Brodnik Žugelj, Steffen Kress, Bogdan Štefane, Frank Glorius, and Mark Lautens. "Employing Pd-Catalyzed C–H Arylation in Multicomponent-Multicatalyst Reactions (MC)2R: One-Pot Synthesis of Dihydrobenzoquinolines." ACS Catalysis 7, no. 2 (January 20, 2017): 1378–82. http://dx.doi.org/10.1021/acscatal.6b03209.

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42

Galli, P., G. Collina, P. Sgarzi, G. Baruzzi, and E. Marchetti. "Combining Ziegler-Natta and mettalocene catalysis: New heterophasic propylene copolymers from the novel multicatalyst reactor granule technology." Journal of Applied Polymer Science 66, no. 9 (November 28, 1997): 1831–37. http://dx.doi.org/10.1002/(sici)1097-4628(19971128)66:9<1831::aid-app22>3.0.co;2-w.

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43

Lorion, Mélanie M., Nikolaos Kaplaneris, Jongwoo Son, Rositha Kuniyil, and Lutz Ackermann. "Late‐Stage Peptide Diversification through Cobalt‐Catalyzed C−H Activation: Sequential Multicatalysis for Stapled Peptides." Angewandte Chemie 131, no. 6 (January 9, 2019): 1698–702. http://dx.doi.org/10.1002/ange.201811668.

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44

Ramachary, Dhevalapally B., Rumpa Mondal, and Chintalapudi Venkaiah. "Rapid Synthesis of Functionalized Indenes, Triazoles, and Glucocorticoid Receptor Modulators by Sequential Multicatalysis Cascade Reactions." European Journal of Organic Chemistry 2010, no. 17 (May 3, 2010): 3205–10. http://dx.doi.org/10.1002/ejoc.201000220.

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45

Lorion, Mélanie M., Nikolaos Kaplaneris, Jongwoo Son, Rositha Kuniyil, and Lutz Ackermann. "Late‐Stage Peptide Diversification through Cobalt‐Catalyzed C−H Activation: Sequential Multicatalysis for Stapled Peptides." Angewandte Chemie International Edition 58, no. 6 (January 9, 2019): 1684–88. http://dx.doi.org/10.1002/anie.201811668.

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46

Breder, Alexander, and Christian Depken. "Light‐Driven Single‐Electron Transfer Processes as an Enabling Principle in Sulfur and Selenium Multicatalysis." Angewandte Chemie International Edition 58, no. 48 (November 25, 2019): 17130–47. http://dx.doi.org/10.1002/anie.201812486.

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47

Du, Jiang, Hui Niu, Jin-Yong Dong, Xia Dong, Dujin Wang, Aihua He, and Charles C. Han. "Nascent Phase Separation and Crystallization Kinetics of an iPP/PEOc Polymer Alloy Prepared on a Single Multicatalyst Reactor Granule." Macromolecules 41, no. 4 (February 2008): 1421–29. http://dx.doi.org/10.1021/ma7021869.

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48

Jin, Zhichao, Jianfeng Xu, Song Yang, Bao-An Song, and Yonggui Robin Chi. "Enantioselective Sulfonation of Enones with Sulfonyl Imines by Cooperative N-Heterocyclic-Carbene/Thiourea/Tertiary-Amine Multicatalysis." Angewandte Chemie 125, no. 47 (October 2, 2013): 12580–84. http://dx.doi.org/10.1002/ange.201305023.

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49

Hofmann, Christine, Soeren M. M. Schuler, Raffael C. Wende, and Peter R. Schreiner. "ChemInform Abstract: En route to Multicatalysis: Kinetic Resolution of trans-Cycloalkane-1,2-diols via Oxidative Esterification." ChemInform 45, no. 22 (May 15, 2014): no. http://dx.doi.org/10.1002/chin.201422067.

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50

Youn, So Won, Hyoung Sub Song, and Jong Hyub Park. "ChemInform Abstract: Asymmetric Domino Multicatalysis for the Synthesis of 3-Substituted Phthalides: Cinchonine/NHC Cooperative System." ChemInform 45, no. 29 (July 3, 2014): no. http://dx.doi.org/10.1002/chin.201429125.

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