Dissertations / Theses on the topic 'Laser cooling and trapping'
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Cooper, Catherine J. "Laser cooling and trapping of atoms." Thesis, University of Oxford, 1995. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.308685.
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Townsend, Christopher G. "Laser cooling and trapping of atoms." Thesis, University of Oxford, 1995. http://ora.ox.ac.uk/objects/uuid:6a3d235b-22da-412b-b34b-e064322336d5.
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A detailed experimental and theoretical investigation of a magneto-optical trap for caesium atoms is presented. Particular emphasis has been placed on achieving high spatial number densities and low temperatures. Optimizing both of these together enables efficient evaporative cooling from a conservative trap, a procedure which has recently led to the first observations of Bose-Einstein condensation in a dilute atomic vapour. The behaviour of a magneto-optical trap is nominally determined by four independent parameters: the detuning and intensity of the light field, the magnetic field gradient and the number of trapped atoms. A model is presented which incorporates previous treatments into a single description of the trap that encompasses a wide range of its behaviour. This model was tested quantitatively by measuring the temperature of the cloud and its spatial distribution as a function of the four parameters. The maximum density was found to be limited both by the reabsorption of photons scattered within the cloud and by a reduction of the confining force at small light shifts. The nonlinear variation with position of the restoring force was found to be significant in limiting the number of atoms confined to a high density. A maximum density in phase space (defined as the number of atoms in a box with sides of dimension one thermal de Broglie wavelength) of (1.5 ± 0.5) x 10-5 was observed, with a spatial density of 1.5 x 1011 atoms per cm3. Cold collision losses from a caesium magneto-optical trap have been studied with the purpose of assessing their influence on spatial densities. In contrast to previous measurements of similar quantities, these measurements did not require the use of an ultra-low (< 10-10 Torr) background vapour pressure. The dependence of the cold collision loss coefficient β on the trapping intensity was measured to permit identification of the different cold collision processes. The largest loss rates observed were those due to hyperfine structure-changing collisions, with a coefficient β = (2±1) x 10-10cm3s-1. A study is presented of a modified magneto-optical trap in which a fraction of the population is shelved into a hyperfine level that does not interact with the trapping light. In this so-called "dark" magneto-optical trap, improved densities of nearly 1012cm-3 have been previously reported for sodium. The application of the technique to caesium is not straightforward due to the larger excited state hyperfine splittings. A simple theory for caesium is presented and its main predictions verified by measurements of density, number and temperature. A density of nearly 1012cm,-3 was indeed obtained but at a temperature substantially higher than in the conventional magneto-optical trap.
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Loftus, Thomas Howard. "Laser cooling and trapping of atomic Ytterbium /." view abstract or download file of text, 2001. http://wwwlib.umi.com/cr/uoregon/fullcit?p3018379.
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Thesis (Ph. D.)--University of Oregon, 2001.Typescript. Includes vita and abstract. Includes bibliographical references (leaves 263-280). Also available for download via the World Wide Web; free to University of Oregon users.
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Kemp, Stefan Liam. "Laser cooling and optical trapping of Ytterbium." Thesis, Durham University, 2017. http://etheses.dur.ac.uk/12166/.
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This thesis presents the development of an experimental apparatus designed to investigate the ultracold collisional properties for mixtures of Cs and Yb, with a long-term view to the creation of ultracold CsYb molecules via indirect cooling methods. The unpaired electron spin that is inherent to molecules of this form gives rise to a magnetic dipole moment in addition to a ground state electric dipole moment. This enables extra control over molecular interactions and should enable the experimental simulation of spin lattice models. We focus on the implementation of a system designed to controllably laser cool and optically trap Yb. The first step in this system is the production of a magneto-optical trap (MOT) on the triplet 1S0 to 3P1 transition of Yb. With careful control over the cooling beam detunings and power, gravitational-assisted Doppler cooling allows samples of Yb to be prepared at 22 uK. This regime of enhanced Doppler cooling is investigated and proves to be a crucial step to ensuring good transfer of cold Yb to optical traps. The construction and characterisation of single and crossed beam optical dipole traps for Yb are discussed. The single beam optical trap has been used to verify a model for the optical trapping of Yb in its ground state. This trap has also been utilised as a tool for the measurement of the light shift on the 1S0 to 3P1 transition at a wavelength of 1070~nm. In the main experimental sequence, Yb atoms are loaded from the magneto-optical trap into the crossed optical dipole trap, allowing evaporative cooling ramps to quantum degeneracy to be performed. This highly-reproducible system typically forms Bose-Einstein condensates with 2 x 10^5 174Yb atoms. This thesis additionally reports on the progress made towards measurements of the interspecies scattering length for 133Cs and Yb isotopes. We present two approaches that are being developed in tandem: rethermalisation in a conservative trap, and two-photon photoassociation. Progress towards rethermalisation measurements has focussed on developing systems for the efficient transfer of Cs to an optical trap. For photoassociative measurements, a laser system has been developed and tested by producing one-photon photoassociation spectra of Cs2.
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Campbell, Corey Justin. "Trapping, laser cooling, and spectroscopy of Thorium IV." Diss., Georgia Institute of Technology, 2012. http://hdl.handle.net/1853/48973.
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Application of precision laser spectroscopy and optical clock technology to the ground and metastable, first excited state of the ²²⁹Th nucleus at < 10 eV has significant potential for use in optical frequency metrology and tests of variation of fundamental constants. This work is a report on the development of required technologies to realize such a nuclear optical clock with a single, trapped, laser cooled ²²⁹Th³⁺ ion. Creation, trapping, laser cooling, and precision spectroscopy are developed and refined first with the naturally occurring isotope, ²³²Th. These technologies are then extended to laser cooling and precision laser spectroscopy of the electronic structure of ²²⁹Th³⁺. An efficient optical excitation search protocol to directly observe this transition via the electron bridge is proposed. The extraordinarily small systematic clock shifts are estimated and the likely extraordinarily large sensitivity of the clock to variation of the fine structure constant is discussed.
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Norris, Ian. "Laser cooling and trapping of neutral calcium atoms." Thesis, University of Strathclyde, 2009. http://oleg.lib.strath.ac.uk:80/R/?func=dbin-jump-full&object_id=11540.
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Maruyama, Reina. "Optical trapping of ytterbium atoms /." Thesis, Connect to this title online; UW restricted, 2003. http://hdl.handle.net/1773/9778.
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Catala, Juan Carlos. "Laser cooling and trapping of argon metastable atomic beam." FIU Digital Commons, 1998. http://digitalcommons.fiu.edu/etd/2083.
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The high velocity of free atoms associated with the thermal motion, together with the velocity distribution of atoms has imposed the ultimate limitation on the precision of ultrahigh resolution spectroscopy. A sample consisting of low velocity atoms would provide a substantial improvement in spectroscopy resolution.
To overcome the problem of thermal motion, atomic physicists have pursued two goals; first, the reduction of the thermal motion (cooling); and second, the confinement of the atoms by means of electromagnetic fields (trapping). Cooling carried sufficiently far, eliminates the motional problems, whereas trapping allows for long observation times.
In this work the laser cooling and trapping of an argon atomic beam will be discussed. The experiments involve a time-of-flight spectroscopy on metastable argon atoms. Laser deceleration or cooling of atoms is achieved by counter propagating a photon against an atomic beam of metastable atoms. The solution to the Doppler shift problem is achieved using spatially varying magnetic field along the beam path to Zeeman shift the atomic resonance frequency so as to keep the atoms in resonance with a fixed frequency cooling laser.
For trapping experiments a Magnetooptical trap (MOT) will be used. The MOT is formed by three pairs of counter-propagating laser beams with mutual opposite circular polarization and a frequency tuned slightly below the center of the atomic resonance and superimposed on a magnetic quadrupole field.
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Shivitz, Robert William. "Techniques in laser cooling and trapping of atomic Ytterbium /." view abstract or download file of text, 2003. http://wwwlib.umi.com/cr/uoregon/fullcit?p3095274.
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Thesis (Ph. D.)--University of Oregon, 2003.Typescript. Includes vita and abstract. Includes bibliographical references (leaves 235-246). Also available for download via the World Wide Web; free to University of Oregon users.
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Guardado-Sanchez, Elmer. "A laser system for trapping and cooling of ⁶Li atoms." Thesis, Massachusetts Institute of Technology, 2015. http://hdl.handle.net/1721.1/100336.
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Thesis: S.B., Massachusetts Institute of Technology, Department of Physics, 2015.Cataloged from PDF version of thesis.
Includes bibliographical references (pages 59-60).
In this thesis, I designed and built a laser system for the trapping and cooling of ⁶Li atoms. The thesis starts explaining a theoretical background of the necessary laser frequencies for the realization of a Zeeman Slower and a 3D MOT. Next it describes the design of the laser system that makes use of a Raman Fiber Amplifier coupled with a Frequency Doubling Cavity and shows the finalized setup. Finally, the thesis delves into the topic of Modulation Transfer Spectroscopy which was used to lock the laser to the D₂ line transition of ⁶Li and shows the spectroscopy setup built for the laser system.
by Elmer Guardado-Sanchez.
S.B.
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Ashmore, Jonathan P., and n/a. "Laser Cooling and Trapping of Metastable Neon and Applications to Photoionization." Griffith University. School of Science, 2005. http://www4.gu.edu.au:8080/adt-root/public/adt-QGU20060202.153538.
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This thesis presents an in-depth study into the characterization and enhancement of a metastable neon laser cooled and trapped atomic beam. The apparatus consists of a standard Zeeman slowed atomic beam loaded into a magneto-optical trap and was designed for applications to electron scattering experiments and photoionization. The efficiency of the metastable neon atomic source was investigated to determine the ideal cathode type for maximum metastable production and optimal atomic beam velocity haracteristics. A series of characterization measurements were performed on the MOT, and the trap volume and population were investigated for a range of trapping and slowing laser intensities and detunings, together with the MOT and Zeeman slower magnetic fields. The volume measurements were compared to standard Doppler theory and it was found that the Doppler model inadequately explained the trap behaviour. It was found that the MOT population characteristics were governed by two processes: two-body losses that limit the trap population at high densities, and the efficiency of the atom capture process which limits the operational range of the MOT over the various parameters. The trap temperature was determined to be 1.3mK via a time-of-flight technique. This was nearly twice that predicted by Doppler theory and the lack of agreement once again suggests the inadequacies in the Doppler theory to correctly model the experiment. The application of the MOT to the photoionization cross-section measurement of the (2p53p)3D3 state of neon was investigated. The MOT decay technique was utilized to measure cross-section values of o351 = 2.9+0.2 -0.3 x 10 -18cm2 and o363 = 3.1 +0.3 -0.4 x 10-18cm2 at the wavelengths of 351nm and 363nm respectively. This is an increase in accuracy of around a factor of five from previous measurements and it was found that the results agreed well with the values predicted by current theories.
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Koo, Jenn Liam Kingston. "Laser cooling and trapping Ca⺠ions in a Penning trap." Thesis, Imperial College London, 2003. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.408719.
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Rigby, Charles Ian. "Development of a laser cooling and magneto-optical trapping experiment for Rubidium 87 atoms." Thesis, Stellenbosch : University of Stellenbosch, 2011. http://hdl.handle.net/10019.1/6492.
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Thesis (MSc)--University of Stellenbosch, 2011.ENGLISH ABSTRACT: A magneto optical trap (MOT) is capable of trapping a vapor cloud consisting of atoms cooled down to the micro Kelvin range. Three orthogonal pairs of counter-propagating laser beams of the correct circular polarisation form an optical molasses which facilitates the cooling of neutral atoms. Additionally a spatially non-uniform magnetic field produced by two current carrying coils in a Maxwell gradient configuration is used to trap the cooled atoms. In this report the effects of the trap parameters, including the laser beam intensity and frequency detuning, beam diameter and magnetic field gradient, on the number of trapped atoms are discussed. Secondly the development of an experimental setup for laser cooling and trapping of 87Rb atoms in vacuum with the aid of a MOT is presented. All trap components were implemented and characterised. The vacuum system and trapping chamber in which the cooling takes place were designed and constructed. A rubidium getter to act as a source of atoms was integrated into the vacuum system. The two external cavity diode lasers used for trapping and optical re-pumping were characterised. The optical setup required for the optical molasses was designed, constructed and characterised. Saturated absorption spectroscopy was performed to investigate the hyperfine structure of 87Rb and to frequency lock the lasers. We report on the current status of the project with regards to progress, results and future work.
AFRIKAANSE OPSOMMING: 'n Magneto-optiese val (magneto optical trap, MOT) kan 'n dampwolk van atome vang en afkoel tot in die mikro Kelvin bereik. Drie ortogonale pare laserbundels, elke paar voortplantend in teenoorgestelde rigtings, met die korrekte sirkelvormige polarisasie vorm 'n sogenaamde optiese molasse wat die afkoeling van neutrale atome moontlik maak. Bykomend word 'n ruimtelik nie-uniforme magneetveld geproduseer deur twee stroomdraende spoele in 'n Maxwell gradient-opstelling gebruik om die afgekoelde atome te vang. In hierdie verslag word die invloed van die val parameters, insluitend die laserbundel intensiteit en frekwensie afstemming, die laserbundel deursnit en magneetveld gradiënt, op die aantal atome in die val bespreek. Tweedens word die ontwikkeling van 'n eksperimentele opstelling vir laser afkoeling en vang van 87Rb atome in vakuum met die hulp van 'n MOT voorgelê. Alle komponente van die val is geïmplementeer en gekarakteriseer. Die vakuumsisteem en val-kamer waarin die afkoeling plaasvind is ontwerp en gebou. 'n Rubidium gasbinder is in die vakuumsisteem ingebou om as 'n bron van atome te dien. Die twee eksterne resonator diodelasers wat gebruik is vir die val en die optiese terugpomp is gekarakteriseer. Die optiese opstelling wat nodig is vir die optiese molasse is ontwerp, gebou en gekarakteriseer. Versadigde absorpsiespektroskopie is uitgevoer om die hiperfynstruktuur van 87Rb te ondersoek en om die lasers se frekwensies te stabiliseer. Verslag word gedoen oor die huidige stand van die projek wat betref vordering, resultate en toekomstige werk.
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Stites, Ronald William. "An Experimental Investigation of Radiation Trapping in Optical Molasses." Miami University / OhioLINK, 2005. http://rave.ohiolink.edu/etdc/view?acc_num=miami1122924988.
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Kangara, Jayampathi. "Design and construction of tapered amplifier systems for laser cooling and atom trapping experiments." Miami University / OhioLINK, 2012. http://rave.ohiolink.edu/etdc/view?acc_num=miami1344007693.
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Zhong, Shan. "AN IMPROVED LASER COOLING AND ATOM TRAPPING SETUP FOR OPTICAL LATTICE AND RATCHET EXPERIMENTS." Miami University / OhioLINK, 2015. http://rave.ohiolink.edu/etdc/view?acc_num=miami1438900984.
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Cook, Eryn. "Laser Cooling and Trapping of Neutral Strontium for Spectroscopic Measurements of Casimir-Polder Potentials." Thesis, University of Oregon, 2018. http://hdl.handle.net/1794/23192.
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Casimir and Casimir-Polder effects are forces between electrically neutral bodies and particles in vacuum, arising entirely from quantum fluctuations. The modification to the vacuum electromagnetic-field modes imposed by the presence of any particle or surface can result in these mechanical forces, which are often the dominant interaction at small separations. These effects play an increasingly critical role in the operation of micro- and nano-mechanical systems as well as miniaturized atomic traps for precision sensors and quantum-information devices. Despite their fundamental importance, calculations present theoretical and numeric challenges, and precise atom-surface potential measurements are lacking in many geometric and distance regimes.
The spectroscopic measurement of Casimir-Polder-induced energy level shifts in optical-lattice trapped atoms offers a new experimental method to probe atom-surface interactions. Strontium, the current front-runner among optical frequency metrology systems, has demonstrated characteristics ideal for such precision measurements. An alkaline earth atom possessing ultra-narrow intercombination transitions, strontium can be loaded into an optical lattice at the “magic” wavelength where the probe transition is unperturbed by the trap light. Translation of the lattice will permit controlled transport of tightly-confined atomic samples to well-calibrated atom- surface separations, while optical transition shifts serve as a direct probe of the Casimir-Polder potential.
We have constructed a strontium magneto-optical trap (MOT) for future Casimir-Polder experiments. This thesis will describe the strontium apparatus, initial trap performance, and some details of the proposed measurement procedure.
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Cerchiari, Giovanni [Verfasser], and Alban [Akademischer Betreuer] Kellerbauer. "Laser spectroscopy of La- and anion trapping with a view to laser cooling / Giovanni Cerchiari ; Betreuer: Alban Kellerbauer." Heidelberg : Universitätsbibliothek Heidelberg, 2018. http://d-nb.info/1177385732/34.
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Botha, G. N. "Development of an external cavity diode laser for application to spectroscopy and laser cooling and trapping of rubidium." Thesis, Stellenbosch : University of Stellenbosch, 2009. http://hdl.handle.net/10019.1/2307.
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Thesis (MSc (Physics))--University of Stellenbosch, 2009.In the presented study a diode laser was characterised and used for spec- troscopy, measuring the resonance lines of atomic rubidium. The characteristics of diode lasers and external cavity diode lasers (ECDL) for the purposes of ab- sorption spectroscopy were investigated and an experimental setup for tunable diode laser spectroscopy using an ECDL was developed. In external cavity diode lasers, the advantages of low cost, small size and e ciency of a diode laser is combined with tunability and a narrow frequency bandwidth. The ECDL was applied in experimental setups for absorption spectroscopy and saturated ab- sorption spectroscopy. Measurement of the absorption of atomic rubidium's D2 line near 780 nm is discussed. The Doppler broadened, as well as the Doppler free spectrum of the ne and hyper ne structure of the D2 line were measured and is discussed. Finer control of the ECDL's stability and frequency, using a servo circuit, were investigated and tested. An overview is given of laser cool- ing and trapping of neutral rubidium atoms, which is the main application the ECDL were developed for.
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Victory, Opeolu. "Analysis and characterisation of a closed-loop control system for laser cooling and trapping experiment." Thesis, Cape Peninsula University of Technology, 2020. http://hdl.handle.net/20.500.11838/3065.
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Thesis (MEng (Electrical Engineering))--Cape Peninsula University of Technology, 2020This research is aimed at analysing the performance of a closed-loop feedback system of an external cavity diode laser (ECDL) for a laser (Doppler) cooling and atom trapping experiment. External cavity diode lasers (ECDL) are commonly used in laser cooling exper-iments involving rubidium atoms. The laser frequency is controlled by adjusting the cavity length and the diode current. Using feedback control method, the laser is locked to an appropriate rubidium transition using a saturation absorption spectroscopy (SAS) setup together with a proportional-integral-derivative (PID) controller. At the CPUT Quantum Physics research group, we have a laser cooling and atom trapping experimental setup. This setup is a combination of multiple optical, electrical and mechanical components. We first analyse this system experimentally using test signals. By passing in basic test input signals, we were able to measure the system by identifying and extracting certain properties such as the resonant frequency, the damping constant and transient response of the system. The re-sults generated from the experimental analysis further enabled us to estimate the transfer function of the external cavity diode laser (ECDL). We then analyse the feedback setup numerically using known parameters from the experiment, and estimated parameters from the experimental analysis. We do this by first getting the mathematical model of the laser and then solving the differential equation using Euler methods in Matlab. By numerically analysing this feedback system, we are able to understand its transient behaviour. We were also able to test the system for different test scenarios e.g. tests for various controller constants, system response to different disturbance types and so on. The similarities observed between the experimental and numerical analysis pro-vide a reliable framework for future improvements when developing the feedback system. Elements such as the integrator constants, disturbance magnitudes and so on can be evaluated using the developed numerical closed-loop system.
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Hoendervanger, Lynn. "A New Metastable Helium Machine : An Investigation into the Attributes of Trapping, Cooling and Detecting Metastable Helium." Thesis, Palaiseau, Institut d'optique théorique et appliquée, 2014. http://www.theses.fr/2014IOTA0006/document.
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Cette thèse décrit le travail accompli au cours des trois dernières années sur la nouvelle expérience d’Hélium métastable de l'Institut d'Optique à Palaiseau.Le premier chapitre décrit une étude visant à améliorer à la fois l'efficacité et la précision du système de détection par galettes à micro-canaux (MCP). Nous avons fait des mesures avec des galettes recouvertes d'une couche d'or sur la face avant, obtenant un accroissement de l'efficacité de détection mais également une réduction de la précision. L'ajout d'une tension intermédiaires entre les deux galettes empilées a au contraire améliorer à la fois l'efficacité et la précision des MCP, en l’absence d’une couche d’or.Le deuxième chapitre est consacré à la construction de l'appareil expérimental pour le refroidissement et le piégeage d’atomes. L’excitation de l'état fondamental de l’Hélium à l'état métastable est décrite, ainsi que la collimation et le refroidissement ultérieur par Zeeman lent du faisceau atomique chaud résultant. Le faisceau ralenti est alors capturé dans un piège magnéto-optique (PMO), dans lequel nous avons capturé 8x108 atomes.Dans le troisième chapitre une étude originale du refroidissement Doppler tridimensionnel dans un PMO et une mélasse désaccordée vers le rouge de la transition atomique est discutée. L’atome d’Hélium métastable est unique et ses propriétés ont permis une telle étude. En effet, les faibles densités atomiques impliquent qu’il n'y a pas de diffusion multiple de photons d’une part, et la faible masse et la faible largeur de la transition 23S1 -> 23P2 rend inefficace les processus de refroidissement sous la limite Doppler. Ces conditions nous ont permis d’observer pour la première fois à trois dimensions un gaz refroidit dans le régime Doppler.Le quatrième chapitre présente une étude sur les collisions dans un piège magnéto-optique d’Hélium métastable. Les collisions Penning induites par la lumière, en particulier à des intensités élevées et à des fréquences proches de la fréquence de transition, sont responsables de pertes élevées d’atomes piégés. Nous mesurons le coefficient de taux associé à ces pertes, Ksp = 2,8 ± 0,4 x 10-7cm3/ sThis thesis describes the work done over the past three and a half years on the new metastable helium experiment at the Institut d'Optique in Palaiseau. In the first chapter it describes a study to improve both the efficiency and the accuracy of the Microchannel Plate (MCP) detection system. We have experimented with adding a gold layer on the top of the input plate, something that we have found increases the efficiency but also decreases the accuracy. The addition of a voltage between the two stacked plates has been shown to both raise the efficiency and improve the accuracy in non-coated MCPs.The second chapter is devoted to the construction of the experimental apparatus. Here the excitation of ground state helium to its metastable state is described, as well as the subsequent collimation and cooling by Zeeman slower of the resulting hot atomic beam. The slowed beam is then captured in a Magneto-Optical Trap, in which we have captured 8x108 atoms.In the third chapter an original study on three-dimensional Doppler cooling in a red-detuned molasses and in the Magneto-Optical trap is presented. The metastable helium system is unique as there is no multiple scattering of photons and there are no sub-Doppler effects. This allows for a never before seen experimental realisation of pure Doppler cooling theory. The fourth chapter describes a study on collisions in a magneto-optical trap of metastable helium. Light-induced Penning collisions are responsible for high trap losses at high intensities and at frequencies close to the transition frequency. We measure the constant rate coefficient to Ksp = 2.8 ± 0.4 x 10-7cm3/s
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Anđelković, Zoran [Verfasser]. "Setup of a Penning trap for precision laser spectroscopy at HITRAP : trapping, cooling and electronic detection of externally produced ions / Zoran Andelkovic." Mainz : Universitätsbibliothek Mainz, 2012. http://d-nb.info/1023187825/34.
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Kalita, Mukut R. "Search for a Permanent Electric Dipole Moment of 225Ra." UKnowledge, 2015. http://uknowledge.uky.edu/physastron_etds/34.
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The observation of a permanent electric dipole moment (EDM) in a non-degenerate system would indicate the violation of discrete symmetries of Time reversal (T) or combined application of Charge (C) and Parity (P) symmetry violation through the CPT theorem. The diamagnetic 225Ra atom with nuclear spin I=1/2 is a favorable candidate for an EDM search. Experimental sensitivity to its EDM is enhanced due to its high atomic mass and the increased Schiff moment of its octupole deformed nucleus. An experimental setup is developed where laser cooled neutral radium atoms are collected in a magneto-optical trap (MOT). The collected atoms are transported 1 meter with a far off-resonant optical dipole trap (ODT) and then the atoms are transferred to a second standing-wave ODT in an experimental chamber. The atoms are then optically polarized and allowed to Larmor precess in parallel and antiparallel electric and magnetic fields. The difference between the Larmor precession frequency for parallel and antiparallel fields is experimentally determined to measure the EDM. This thesis is about the first measurement of the EDM of the 225Ra atom where an upper limit of |d(225Ra)|<5.0*10-22 e cm (95\% confidence) is reached.
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Steer, Edward. "Development and characterisation of a cold molecule source and ion trap for studying cold ion-molecule chemistry." Thesis, University of Oxford, 2016. https://ora.ox.ac.uk/objects/uuid:13c3a622-ba78-4a53-902c-666ec461f708.
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A novel apparatus, combining buffer-gas cooling, electrostatic velocity selection and ion trapping, has been constructed and characterised. This apparatus is designed to investigate cold ion-molecule chemistry in the laboratory, at a variable translational and internal (rotational) temperature. This improves on previous experiments with translationally cold but rotationally hot molecule sources. The ability to vary the rotational temperature of cold molecules will allow for the experimental investigation of post-Langevin capture theories.
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Muniz, Sérgio Ricardo. "Estudo de Blindagem Óptica em Colisões Frias." Universidade de São Paulo, 1998. http://www.teses.usp.br/teses/disponiveis/76/76131/tde-06052005-162937/.
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Neste trabalho, mostramos que é possível suprimir a maioria dos processos inelásticos que podem causar perdas de átomos em armadilhas magneto-ópticas. Nossos resultados revelam que o processo de blindagem óptica (demonstrado pelo nosso grupo, pela primeira vez para o processo de ionização fotoassociativa Phys. Rev. Lett. 73, 1911 (1994)) é bem mais geral do que se supunha. Permitindo, inclusive, a supressão de colisões entre átomos no estado fundamental. E provavelmente qualquer outro processo inelástico que ocorra a curtas distâncias internucleares. Para se chegar a esses resultados, foi necessário desenvolver uma nova técnica de aprisionamento, que permite o estudo de colisões frias, mesmo em armadilhas cujo potencial de confinamento é pequeno. Graças a essa técnica foi possível, pela primeira vez, observar perdas causadas por mudança de estrutura hiperfina, numa armadilha de átomos de sódio operando na linha D1 (carregada a partir de uma célula de vapor). Essa técnica ainda nos permitiu medir a taxa de colisões frias () no trap da linha D1, um dado que até então não existia na literatura. Para verificar a confiabilidade dos resultados obtidos por essa técnica, realizamos também medidas de na linha D2 e comparamos esses resultados com outros existentes na literatura (obtidos por uma técnica diferente). A boa concordância entre esses resultados nos deixa confiantes em dizer que essa técnica, além de ser muito interessante, no estudo de armadilhas rasas (seja isso devido à intensidade dos lasers de aprisionamento, seja devido a natureza própria da armadilha), é também bastante confiávelIn this work, we showed that is possible to suppress most of the inelastic processes that may cause losses of atoms in a magneto-optical trap. Our results reveal that the process of optical shielding (demonstrated by our group, for the first time to photoassociative ionization - Phys. Rev. Lett. 73, 1911 (1994)) is much more general than it was supposed. Even allowing the suppression of ground state collisions and probably any other inelastic process that happens at short internuclear distances. To achieve those results, it was necessary to develop a new trapping technique, which allows the study of cold collisions, even in traps whose confinement potential is small. Thanks to that technique it was possible, for the first time, to observe losses caused by hyperfine changing collisions, in a trap of sodium atoms operating in the D1 line (loaded from a vapor cell). That technique has still allowed us to measure the rate of cold collisions () for the D1 line trap, a result which, until now, did not exist in the literature. To verify the reliability of the results obtained by that technique, we also accomplished measures of in the D2 line and compared those results with other existent ones in the literature (obtained by a different technique). The good agreement among those results, made us confident in saying that this technique, besides being very interesting in the study of shallow traps (due to the intensity of the trapping lasers, or due to the own nature of the trap), it is also quite reliable.
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Tuboy, Aparecida Marika. "Preparação de laser de diodo e sua utilização em aprisionamento e estudo de átomos frios." Universidade de São Paulo, 1996. http://www.teses.usp.br/teses/disponiveis/76/76132/tde-17042009-125921/.
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Este trabalho relata o desenvolvimento de todo o aparato experimental para a realização de aprisionamento de césio através de uma armadilha magneto-óptica. As fontes de luz neste processo foram os lasers de diodo e todo seu sistema para operação, estabilização e redução da largura de linha foi construído. As medidas das constantes de mola e amortecimento foram realizadas como função dos parâmetros característicos das armadilhas de césio e de sódio. Também realizamos outros experimentos com átomos aprisionados de sódio na presença de duas freqüências, linha D1 e D2. A primeira medida constitui na obtenção da taxa de colisões entre átomos aprisionados na linha D1 e depois foi realizado observações de uma nova estrutura operando neste regime.This thesis describes the development of a complete experimental setup for trapping cesium by a magneto-optical trap (MOT). In this work we have employed diode lasers as light sources and built the entire system for their operation, stabilization and linewidth reduction. We have measured the MOT spring and damping constants as functions of the characteristic parameters of the cesium and sodium traps. We have also carried out two other experiments on trapped sodium atoms operating in the simultaneous presence of the D1 and D2 line frequencies. The first experiment has established the collision rate of trapped atoms in the D1 line MOT and the second has allowed us to observe a new structure operating in this two-frequency regime.
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Kamsap, Marius Romuald. "Horloge micro-onde à ions : analyse et transport d'un nuage d'ions dans un piège à plusieurs zones." Thesis, Aix-Marseille, 2015. http://www.theses.fr/2015AIXM4781/document.
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Cette thèse a été effectuée dans le cadre d'un projet qui vise à explorer les facteurs limitants des performances d'une horloge à ions dans le domaine des fréquences micro-onde. Ce travail repose sur l'observation et la manipulation d'un grand nuage d'ions dans des potentiels de géométries différentes. Le but est l'analyse et le transport d'un grand nuage pouvant dépasser 10^6 ions dans un piège radio-fréquence linéaire à plusieurs zones. Notre groupe à construit un piège à trois zones destiné au piégeage d'ions calcium: deux parties quadrupolaires et une partie octupolaire montées en ligne. Les ions sont créés dans la première partie quadrupolaire et refroidis par laser le long de l'axe du piège. Nous avons d'abord étudié la création d'un grand nuage. La limite actuelle des paramètres du système permet de confiner et détecter des nuages de taille maximale 1,2.10^5 ions. Ensuite, grâce à un protocole de transport rapide et optimisé, ces ions sont transportés dans le deuxième et troisième piège avec une efficacité pouvant atteindre 100%. Les résultats en fonction de la durée de transport montrent une asymétrie entre les deux sens de transport que nous exploitons pour ajouter des ions dans le deuxième piège sans perte du nuage initialement présent. Cette technique d'accumulation a permis de piégér 2,5.10^5 ions dans le deuxième et troisième piège. Ce nombre semble limité par les refroidissement. Enfin, dans l'octupole, les observations montrent que, contrairement aux structures creuses attendues par les modèles, les ions froids s'organisent dans trois minima locaux de potentiels. La cause de cette différence est un petit défaut dans la symétrie octupolaire des barreauxThis thesis is part of a project aiming to explore the performance limiting factors of a microwave ion clock. This work is based on the observation and manipulation of a large ion cloud in potentials with different geometries. The purpose is to analyze and transport a large cloud of more than 10^6 ions in a linear radio-frequency trap with several zones. Our group has build a three-zone trap for calcium ion trapping: two quadrupole parts and an octupole part mounted inline. Ions are created in the first quadrupole part and cooled by lasers along the trap symmetry axis. We study the creation of a large ion cloud. The current trapping and cooling parameters limit the maximum size of the cloud to 1,2.10^5 ions. with a rapid and optimized transport protocol, these ions are transfered in the second part of the trap and then in the octupole trap with an efficiency of up to 100%. The result as function of the transport duration shows an asymmetry between the two transport directions. We exploit this feature to add ions in the second or third trap without loss of the already trapped ions. This accumulation technique has allowed to trap 2,5.10^5 ions in the second and third trap. The cooling laser power seems to be the major limiting factor of this number. Finally the observation of the ions in the octupole shows that the cold ions are localised in three different potential wells. This is in contradiction with the hollow structure predicted by the analytical fluid model and molecular dynamics simulations. The cause of this difference is a tiny defect in the octupole symmetry of the RF-electrodes which leads to local minima in the multipole potential
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Gingell, Alexander David. "Applications of Coulomb crystals in cold chemistry." Thesis, University of Oxford, 2010. http://ora.ox.ac.uk/objects/uuid:3b93832d-b9eb-49e1-b4a4-1bb43d7c9c00.
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This thesis describes the study of a range of ion-molecule reactions at very low collision energies using a newly developed experimental technique which involves the reaction of velocity-selected beams of translationally cold neutral molecules with very low kinetic energy ion ensembles. These studies have been enabled by the construction of a new apparatus for trapping and laser-cooling gas phase atomic ions (40Ca⁺). The laser-cooling process results in the formation of ordered, low kinetic energy, lattice-like ion structures, also known as "Coulomb crystals". The properties of single and multicomponent Coulomb crystals (which may also involve molecular ions), and their manipulation via modulation of the applied fields, are explored experimentally and with the use of molecular dynamics simulations. Variations in the laser-cooling parameters are shown to result in different steady-state populations of the electronic states of 40Ca⁺ involved with the laser cooling cycle, and these are modelled within an appropriate theoretical framework. The imaging of 40Ca⁺ fluorescence as a function of time allows the study of various ion-molecule reactions at collision energies around 300 K, with single ion sensitivity. These reaction studies are extended to low-temperature (collision energies close to 1 K), by combination of the ion trap apparatus with a bent quadrupole guide velocity-selector. Ion-molecule collision energies are shown to be variable over a short range through a change in the quadrupole guide voltage, or the ion trapping parameters; the effect of these modulations on the rate constant is explored for Ca⁺ + CH₃F. Bimolecular rate constants for the reactions of 40Ca⁺ with CH₃F, CH₂F₂ and CH₃Cl have been determined for a range of 40Ca⁺ state populations, allowing resolution of the global rate contributions from the ground and combined excited states. These results are analysed in the context of capture theories and ab initio electronic structure calculations. In each case, suppression of the ground state rate constant is explained by the presence of either a submerged or real barrier on the ground state potential surface. Rates of reaction from the combined excited states are generally found to be in line with capture theories, and in some cases variation is found between the high and low collision energy regimes. Molecular product ions generated in these experiments have been shown to be sympathetically-cooled into the crystal structure, and subsequently identified through resonance-excitation mass spectrometry. Molecular ions were also produced by multiphoton laser ionisation of a thermal background gas of OCS molecules. An ion-molecule reaction involving a molecular ion, that of charge transfer between OCS⁺ and ND₃, has been studied at a collision energy near 1 K for the first time using sympathetically-cooled OCS⁺ and velocity-selected ND₃. These experiments illustrate the generality of the techniques described herein, and should lead to many possibilities for future studies.
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Oldham, James Martin. "Combination of a cold ion and cold molecular source." Thesis, University of Oxford, 2014. http://ora.ox.ac.uk/objects/uuid:ef33adcb-609a-4329-b4d8-aca8a1c48661.
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This thesis describes the combination of two sources of cold atomic or molecular species which can be used to study a wide range of ion-molecule reactions. The challenges in forming these species and in determining the fate of reactive events are explored throughout. Reactions occur in a volume within a radio-frequency ion trap, in which ions have previously been cooled to sub-Kelvin temperatures. Ions are laser-cooled, with migration of ions slowed sufficiently to form a quasi-crystalline spheroidal structure, deemed a Coulomb crystal. Fluorescence emitted as a consequence of laser-cooling is detected; the subsequent fluorescence profiles are used to determine the number of ions in the crystal and, in combination with complementary simulations, the temperature of these ions. Motion imparted by trapping fields can be substantial and simulations are required to accurately determine collision energies. A beam of decelerated molecules is aimed at this stationary ion target. An ammonia seeded molecular beam enters a Stark decelerator, based on the original design of Meijer and co-workers. The decelerator uses time-varying electric fields to remove kinetic energy from the molecules, which exit at speeds down to 35 m/s. A fast-opening shutter and focussing elements are subsequently used to maximise the decelerated flux in the reaction volume while minimising undecelerated molecule transmission. Substantial fluxes of decelerated ammonia are obtained with narrow velocity distributions to provide a suitable source of reactant molecules. Combination of these two techniques permits studies of reactions between atomic ions and decelerated molecules that can be entirely state-specific. Changes in the Coulomb crystal fluorescence profile denote changes in the ion identities, the rate of these changes can be used to obtain rate constants. Determination of rate constants is even possible despite the fact that neither reactant nor product ions are directly observed. This work has studied reactions between sympathetically cooled Xe+ ions and guided ND3 and has obtained data consistent with prior studies. Determination of reactive events is complicated if ion identities can change without affecting the fluorescence profile, or if multiple reaction channels are possible. A range of spectroscopic techniques are discussed and considered in regards to determining rate constants and product identities. Pulsed axial excitation of trapped ions can follow rapid changes in average ion weights and subtle changes for small crystals. Time-of-flight mass spectrometry is also demonstrated using the trapping electrodes and is suitable for discrimination of ions formed within the trap.
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Martin, Jocelyn L. "Magnetic trapping and cooling in caesium." Thesis, University of Oxford, 1997. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.361996.
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Joffe, Michael Arnold. "Trapping and cooling atoms at high densities." Thesis, Massachusetts Institute of Technology, 1993. http://hdl.handle.net/1721.1/12229.
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Chen, Ruiping. "Laser cooling of atoms for ultracold cooling." Thesis, Queen's University Belfast, 2008. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.479242.
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Van, Dongen Janelle. "Simultaneous cooling and trapping of 6Li and 85/87Rb." Thesis, University of British Columbia, 2007. http://hdl.handle.net/2429/351.
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This thesis provides a summary of the laser system constructed in the Quantum Degenerate Gases Laboratory for laser cooling and trapping of 85/87Rband 6Li as well as of experiments that have been pursued in our lab to date. The first chapter provides an overview of the experimental focus of the QDG lab. The second and third chapters provide the fundamental theory behind laser cooling and trapping. The fourth chapter provides details of the laser system. The fifth chapter describes an experiment performed on the subject of dual-injection, performed in collaboration with Dr. James Booth of the British Columbia Institute of Technology (BCIT) involving the dual-injection of a single slave amplifier. The last chapter describes the progress made on the experimental setup needed for the study of Feshbach resonances between 85/87Rb and 6Li and the photoassociative formation of molecules.
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Hillenbrand, Gerd. "Laser cooling of atoms." Thesis, University of Oxford, 1994. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.259952.
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Steane, A. M. "Laser cooling of atoms." Thesis, University of Oxford, 1991. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.315817.
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Rayner, Anton. "Laser cooling of solids /." St. Lucia, Qld, 2002. http://www.library.uq.edu.au/pdfserve.php?image=thesisabs/absthe16448.pdf.
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Zhelyazkova, Valentina. "Laser cooling of CaF molecules." Thesis, Imperial College London, 2014. http://hdl.handle.net/10044/1/24740.
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Cold and ultracold molecules are highly desirable for a diverse range of applications in physics and chemistry such as precision measurements, tests of fundamental physics, quantum simulation and information processing, quantum chemistry, and the physics of strongly correlated quantum matter. Laser cooling is usually infeasible in molecules because their rotational and vibrational transitions make is difficult to come up with a closed scattering cycle. Recently, a narrow range of diatomic molecules, one of which is CaF, has been shown to possess a convenient electronic structure and a highly-diagonal Franck-Condon matrix and thus be amenable to laser cooling. This thesis describes experiments on laser cooling of CaF radicals produced in a supersonic source. We first investigate the increased fluorescence when multi-frequency resonant light excites the molecules from the four hyperfine levels of the ground X²Σ+(N = 1, v = 0) state to the first excited A²π½(J' = 1=2; v' = 0) state. The number of photons scattered per molecule increases significantly from one or two in the single frequency case to more than 50 before the molecules get pumped into the X²Σ+(N = 1; v = 1) state. We demonstrate laser cooling and slowing of CaF using counter-propagating laser light which causes the molecules to scatter more than a thousand photons on the X (N = 1, v = 0, 1) <->A (J' = 1=2; v' = 0) transition. The effect of the laser cooling is to slow a group of molecules from 600 ms-1 to about 580 ms-1 and to narrow their velocity distribution from an initial temperature of 3 K down to 300 mK. In addition, chirping the frequency of the cooling light to keep it on resonance with the decelerating molecules doubles the deceleration and further compresses the velocity distribution. The effect of the laser cooling is limited by the optical pumping of molecules in the X (N = 1, v = 2) state.
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Matsushima, Aki. "Transverse laser cooling of SrF." Thesis, Imperial College London, 2014. http://hdl.handle.net/10044/1/17839.
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This thesis discusses an experiment, which has demonstrated transverse laser cooling of a pulsed supersonic beam of strontium monofluoride (SrF) molecules. Producing ultracold molecules is important because they could advance many fields including many-body physics, quantum chemistry and precision measurements to explore fundamental forces in nature. Direct laser cooling of molecules is a new and promising way to produce molecules with temperatures in the sub-millikelvin range. In the experiment, SrF molecules produced from a pulsed supersonic source were cooled in the transverse direction using light from just two lasers. The molecular beam brightness was increased by about 20%. I discuss the detailed experimental setup, laser system and data analysis. I also present several theoretical models, which give insight into the cooling experiment. Finally, I discuss improvements to this experiment, which should enable higher yields of ultracold molecules to be produced.
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Cerrillo, Moreno Javier. "Laser cooling of quantum systems." Thesis, Imperial College London, 2013. http://hdl.handle.net/10044/1/12788.
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In this thesis novel methods for the laser cooling of quantum systems are presented. The use of quantum interference allows for the tailored cancelation of heating processes, so that an approximation to a cooling operator is possible that does not rely on the rotating wave approximation. This makes these schemes considerably faster and more efficient than existing ground state cooling methods, and allow for a significant relaxation of current experimental constraints. Several approaches are investigated in different systems. On the one hand, a special laser configuration, applicable to trapped ions, atoms or cantilevers, generates a double dark state that eliminates both the blue sideband and the carrier transition. As a consequence, vanishing phonon occupation up to first order in the perturbative expansion is achieved. Underlying this scheme is a combined action of two cooling schemes which makes the proposal very stable under parameter fluctuations. Its suitability as a cooling scheme for several ions in a trap or for a cloud of atoms in a dipole trap is shown. On the other hand, a pulsed cooling scheme for optomechanical systems is presented. It can be implemented for both strongly and weakly coupled optomechanical systems in both weakly and highly dissipative cavities. Its underlying mechanism is based on interferometric control of optomechanical interactions, and its efficiency is demonstrated with pulse sequences that are obtained by using methods from optimal control. Finally, it is shown how this pulsed method can be combined with continuous measurement to drive mechanical oscillators to highly squeezed steady states. Its mechanism relies on the modification of the dissipation and measurement terms, which drive the system towards a specific quadrature eigenstate. The scheme is robust to measurement inefficiencies and works also with highly dissipative cavities, which makes it accessible to implementation with state of the art technology.
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Rupper, Greg. "Theory of Semiconductor Laser Cooling." Diss., The University of Arizona, 2010. http://hdl.handle.net/10150/194520.
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Recently laser cooling of semiconductors has received renewed attention, with the hope that a semiconductor cooler might be able to achieve cryogenic temperatures. In order to study semiconductor laser cooling at cryogenic temperatures, it is crucial that the theory include both the effects of excitons and the electron-hole plasma. In this dissertation, I present a theoreticalanalysis of laser cooling of bulk GaAs based on a microscopic many-particle theory of absorptionand luminescence of a partially ionized electron-hole plasma.This theory has been analyzed from a temperature 10K to 500K. It is shown that at high temperatures (above 300K), cooling can be modeled using older models with a few parameter changes. Below 200K, band filling effects dominate over Auger recombination. Below 30K excitonic effects are essential for laser cooling. In all cases, excitonic effects make cooling easier then predicted by a free carrier model.The initial cooling model is based on the assumption of a homogeneous undoped semiconductor. This model has been systematically modified to include effects that are present in real laser cooling experiments. The following modifications have been performed. 1) Propagation and polariton effects have been included. 2) The effect of p-doping has been included. (n-doping can be modeled in a similar fashion.) 3) In experiments, a passivation layer is required to minimize non-radiative recombination. The passivation results in a npn heterostructure. The effect of the npn heterostructure on cooling has been analyzed. 4) The effect of a Gaussian pump beam was analyzed and 5) Some of the parameters in the cooling model have a large uncertainty. The effect of modifying these parameters has been analyzed.Most of the extensions to the original theory have only had a modest effect on the overall results. However we find that the current passivation technique may not be sufficient to allow cooling. The passivation technique currently used appears to be very good at low densities, but loses some of it's effectiveness at the moderately high densities required for laser cooling. We suggest one possible solution that might enable laser cooling. If the sample can be properly passivated, then we expect laser cooling to be possible.
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Kahra, Steffen. "Trapping and cooling of single molecular ions for time resolved experiments." Diss., lmu, 2011. http://nbn-resolving.de/urn:nbn:de:bvb:19-128803.
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Stoll, Michael. "Buffer gas cooling and magnetic trapping of CrH and MnH molecules." Berlin mbv, 2008. http://d-nb.info/992996392/04.
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Clark, Joanne Louise. "Laser cooling in the condensed phase." Thesis, Imperial College London, 1997. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.266518.
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Ryjkov, Vladimir Leonidovich. "Laser cooling and sympathetic cooling in a linear quadrupole rf trap." Texas A&M University, 2003. http://hdl.handle.net/1969.1/1637.
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An investigation of the sympathetic cooling
method for the studies of large ultra-cold molecular ions in a quadrupole ion trap has been conducted.Molecular dynamics simulations are performed to study the rf heating mechanisms in the ion trap. The dependence of
rf heating rates on the ion temperature, trapping parameters,
and the number of ions is obtained. New rf heating mechanism
affecting ultra-cold ion clouds exposed to laser radiation is described.The saturation spectroscopy setup of the hyperfine spectra
of the molecular iodine has been built to provide an accurate frequency reference for the laser wavelength. This reference is used to obtain the fluorescence lineshapes of
the laser cooled Mg$^+$ ions under different trapping conditions.The ion temperatures are deduced from the measurements, and
the influence of the rf heating rates on the fluorescence lineshapes
is also discussed. Cooling of the heavy ($m=720$a.u.) fullerene ions to under 10K by the means of the sympathetic cooling by the Mg$^+$ ions($m=24$a.u.) is demonstrated. The single-photon imaging system has been developed and used to obtain the images of the Mg$^+$ ion crystal structures at mK temperatures.
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Ganic, Djenan, and dga@rovsing dk. "Far-field and near-field optical trapping." Swinburne University of Technology. Centre for Micro-Photonics, 2005. http://adt.lib.swin.edu.au./public/adt-VSWT20051130.135436.
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Optical trapping techniques have become an important and irreplaceable tool in many research disciplines for reaching non-invasively into the microscopic world and to manipulate, cut, assemble and transform micro-objects with nanometer precision and sub-micrometer resolution. Further advances in optical trapping techniques promise to bridge the gap and bring together the macroscopic world and experimental techniques and applications of Microsystems in areas of physics, chemistry and biology.
In order to understand the optical trapping process and to improve and tailor experimental techniques and applications in a variety of scientific disciplines, an accurate knowledge of trapping forces exerted on particles and their dependency on environmental and morphological factors is of crucial importance. Furthermore, the recent trend in novel laser trapping experiments sees the use of complex laser beams in trapping arrangements for achieving more controllable laser trapping techniques. Focusing of such beams with a high numerical aperture (NA) objective required for efficient trapping leads to a complicated amplitude, phase and polarisation distributions of an electromagnetic field in the focal region. Current optical trapping models based on ray optics theory and the Gaussian beam approximation are inadequate to deal with such a focal complexity.
Novel applications of the laser trapping such as the particle-trapped scanning near field optical microscopy (SNOM) and optical-trap nanometry techniques are currently investigated largely in the experimental sense or with approximated theoretical models. These applications are implemented using the efficient laser trapping with high NA and evanescent wave illumination of the sample for high resolution sensing. The proper study of these novel laser trapping applications and the potential benefits of implementation of these applications with complex laser beams requires an exact physical model for the laser trapping process and a nanometric sensing model for detection of evanescent wave scattering.
This thesis is concerned with comprehensive and rigorous modelling and characterisation of the trapping process of spherical dielectric particles implemented using far-field and near-field optical trapping modalities. Two types of incident illuminations are considered, the plane wave illumination and the doughnut beam illumination of various topological charges. The doughnut beams represent one class of complex laser beams. However, our optical trapping model presented in this thesis is in no way restricted to this type of incident illumination, but is equally applicable to other types of complex laser beam illuminations. Furthermore, the thesis is concerned
with development of a physical model for nanometric sensing, which is of great importance for optical trapping systems that utilise evanescent field illumination for achieving high resolution position monitoring and imaging.
The nanometric sensing model, describing the conversion of evanescent photons into propagating photons, is realised using an analytical approach to evanescent wave scattering by a microscopic particle. The effects of an interface at which the evanescent wave is generated are included by considering the scattered
field reflection from the interface. Collection and imaging of the resultant scattered field by a high numerical aperture objective is described using vectorial diffraction theory. Using our sensing model, we have investigated the dependence of the scattering on the particle size and refractive index, the effects of the interface on the scattering cross-section, morphology dependent resonance effects associated with the scattering process, and the effects of the incident angle of a laser beam undergoing total internal reflection to generate an evanescent field. Furthermore, we have studied the detectability of the scattered signal using a wide area detector and a pinhole detector. A good agreement between our experimental measurements of the focal intensity distribution in the back focal region of the collecting objective and the theoretical predictions confirm the validity of our approach.
The optical trapping model is implemented using a rigorous vectorial diffraction theory for characterisation of the electromagnetic field distribution in the focal region of a high NA objective. It is an exact model capable of considering arbitrary amplitude, phase and polarisation of the incident laser beam as well as apodisation functions of the focusing objective. The interaction of a particle with the complex focused field is described by an extension of the classical plane wave Lorentz-Mie theory with the expansion of the incident field requiring numerical integration of finite surface integrals only. The net force exerted on the particle is then determined using the Maxwell stress tensor approach. Using the optical trapping model one can
consider the laser trapping process in the far-field of the focusing objective, also known as the far-field trapping, and the laser trapping achieved by focused evanescent field, i.e. near-field optical trapping.
Investigations of far-field laser trapping show that spherical aberration plays a significant role in the trapping process if a refractive index mismatch exists between the objective immersion and particle suspension media. An optical trap efficiency is severely degraded under the presence of spherical aberration. However, our study shows that the spherical aberration effect can be successfully dealt with using our optical trapping model. Theoretical investigations of the trapping process achieved using an obstructed laser beam indicate that the transverse trapping efficiency decreases rapidly with increasing size of the obstruction, unlike the trend predicted using a ray optics model. These theoretical investigations are in a good agreement with our experimentally observed results.
Far-field optical trapping with complex doughnut laser beams leads to reduced lifting force for small dielectric particles, compared with plane wave illumination, while for large particles it is relatively unchanged. A slight advantage of using a doughnut laser beam over plane wave illumination for far-field trapping of large dielectric particles manifests in a higher forward axial trapping efficiency, which increases for increasing doughnut beam topological charge. It is indicated that the maximal transverse trapping efficiency decreases for reducing particle size and that the rate of decrease is higher for doughnut beam illumination, compared with plane wave illumination, which has been confirmed by experimental measurements.
A near-field trapping modality is investigated by considering a central obstruction placed before the focusing objective so that the obstruction size corresponds to the minimum convergence angle larger than the critical angle. This implies that the portion of the incident wave that is passed through the high numerical aperture objective satisfies the total internal reflection condition at the surface of the coverslip, so that only a focused evanescent field is present in the particle suspension medium. Interaction of this focused near-field with a dielectric micro-particle is described and investigated using our optical trapping model with a central obstruction. Our investigation shows that the maximal backward axial trapping efficiency or the lifting
force is comparable to that achieved by the far-field trapping under similar conditions for either plane wave illumination or complex doughnut beam illumination. The dependence of the maximal axial trapping efficiency on the particle size is nearly linear for near-field trapping with focused evanescent wave illumination in the Mie size regime, unlike that achieved using the far-field trapping technique.
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Ganic, Djenan. "Far-field and near-field optical trapping." Australasian Digital Thesis Program, 2005. http://adt.lib.swin.edu.au/public/adt-VSWT20051130.135436.
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Thesis (PhD) - Swinburne University of Technology, Faculty of Engineering and Industrial Sciences, Centre for Micro-Photonics, 2005.A thesis submitted for the degree of Doctor of Philosophy, Centre for Micro-Photonics, Faculty of Engineering and Industrial Sciences, 2005. Typescript. Includes bibliographical references (p. 164-177). Also available on cd-rom.
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Raymond, Ooi Chong Heng. "Quantum optics of laser cooling of molecules." [S.l. : s.n.], 2003. http://deposit.ddb.de/cgi-bin/dokserv?idn=968928978.
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Holland, Darren. "Progress towards laser cooling of BH molecules." Thesis, Imperial College London, 2016. http://hdl.handle.net/10044/1/45433.
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This thesis investigates the suitability of BH molecules for laser cooling and describes progress towards the laser cooling of this molecule. We produce a molecular beam of BH and measure the branching ratios for the excited electronic state, A^{1}\Pi(v_{0}=0), to decay to the various vibrational states of the ground electronic state, X^{1}\Sigma. We verify that the branching ratio for the spin-forbidden transition to an intermediate triplet state is inconsequentially small. We measure the frequency of the lowest rotational transition of the X state, and the hyper fine structure in the relevant levels of both the X and A states, and determine the nuclear electric quadrupole and magnetic dipole coupling constants. We use a semiclassical model of the molecule-light interaction to investigate the expected cycling behaviour on the main cooling transition using light with modulated polarisation. The results of the model are compared with the effect of modulating the polarisation experimentally using an electro-optic modulator. In order to repump the population that leaks into the first vibrationally excited state, we have designed, built and tested a suitable repump laser and have demonstrated that we can drive the repump transition. We have also designed a Zeeman slower for slowing molecules to low velocity so that they can be trapped. Our results show that a relatively simple laser cooling scheme can be used to cool, slow and trap BH molecules.
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Schnitzler, Harald. "Development of an experiment for trapping, cooling, and spectroscopy of molecular hydrogen ions." [S.l. : s.n.], 2001. http://www.bsz-bw.de/cgi-bin/xvms.cgi?SWB9424100.
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Levonian, David (David S. ). "A Cavity-stabilized diode laser for dipole trapping of ytterbium." Thesis, Massachusetts Institute of Technology, 2015. http://hdl.handle.net/1721.1/105998.
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Thesis: M. Eng., Massachusetts Institute of Technology, Department of Electrical Engineering and Computer Science, 2015.This electronic version was submitted by the student author. The certified thesis is available in the Institute Archives and Special Collections.
Cataloged from student-submitted PDF version of thesis.
Includes bibliographical references (pages 99-103).
Bad-cavity lasers using a gain medium with a narrower linewidth than the laser cavity have the potential to achieve very narrow linewidths and extremely long coherence times. Such lasers could serve as active frequency standards or enable very-long-baseline interferometric telescopes at optical frequencies. The 6s6p³P₀ to 6s²¹S₀ ground state transition in ¹⁷¹Yb is a promising candidate for the gain medium of a bad-cavity laser due to its 44 mHz linewidth. For ytterbium to be used efficiently as a gain medium, its inhomogeneous broadening must be suppressed to a level lower than the linewidth of its gain transition. In this thesis, I design, implement, and characterize an optical lattice trap for ytterbium atoms. The trap consists of a diode laser which is frequency stabilized to an adjustable-length cavity where the ytterbium atoms are trapped. The length of this cavity is then locked by comparison of the laser frequency to a stable reference cavity. The resulting standing wave has high enough intensity that the recoil energy of the gain transition is smaller than the energy spacing between motional modes of the trapped atoms. This situation is known as the Lamb-Dicke regime and means that there is an absence of recoil broadening. The large spacing between motional modes of the trap also enables sideband resolved cooling of the atoms, which allows cooling to temperatures of 3 [mu]K, near the ground state of the trapping potential. Additionally, if the wavelength of the optical lattice is chosen to be at the magic wavelength for ytterbium, where the relative AC Stark shift for the two levels of the gain transition is zero to first order, there is no broadening due to varying intensity in the trap. Since the Doppler effect, recoil broadening and the AC Stark shift are the main sources of inhomogeneous broadening, this trapping scheme is expected to suppress inhomogeneous broadening to a level of 1 Hz.
by David Levonian.
M. Eng.