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Journal articles on the topic 'Isobutane Oxidation'

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Author: Grafiati

Published: 10 December 2022

Last updated: 28 January 2023

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1

Mitran, Gheorghita, Ioan-Cezar Marcu, Tatiana Yuzhakova, and Ioan Sandulescu. "Selective oxidation of isobutane on V-Mo-O mixed oxide catalysts." Journal of the Serbian Chemical Society 73, no. 1 (2008): 55–64. http://dx.doi.org/10.2298/jsc0801055m.

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Four V-Mo-O mixed metal oxides were prepared, characterized and tested for the selective oxidation of isobutane in the temperature range 350-550?C, at atmospheric pressure. Isobutane was mainly oxidized to isobutene and carbon oxides. The systems with low vanadium contents showed low activities but high isobutene selectivities, while the systems with high vanadium contents showed high activities with high carbon oxides selectivities. The effects of temperature, contact time and the molar ratio iso-butane to oxygen on the conversion of isobutane and the selectivity of the oxidation were studied.

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2

Vogin, Bernard, François Baronnet, and Gérard Scacchi. "Étude chimique et cinétique de l'oxydation homogène en phase gazeuse d'alcanes légers. I. Isobutane." Canadian Journal of Chemistry 67, no. 5 (May 1, 1989): 759–72. http://dx.doi.org/10.1139/v89-115.

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A literature survey on the homogeneous gas-phase oxidation of light alkanes shows that despite a rather high number of papers there are still, even in the case of isobutane, an important number of unresolved questions, which makes the writing of a reaction scheme rather difficult. To obtain more reliable experimental data, we have studied the homogeneous gas-phase oxidation of isobutane in a conventional static system, at 310 and 340 °C and subatmospheric pressure. This investigation is chiefly aimed at identifying and measuring the major primary products of the reaction. A chain radical scheme based on the primary products and on estimation of the rate constants of the elementary steps by the methods of Thermochemical Kinetics is put forward to interpret our experimental results. Two major reaction routes appear, one corresponding to the formation of isobutene and the other to the formation of isobutene oxide. The conclusions of the present investigation and suggestions for further developments are also mentioned. Keywords: oxidation, chemical kinetics, reaction mechanism, isobutane.

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3

Guan, Jingqi, Haiyan Xu, Shubo Jing, Shujie Wu, Yuanyuan Ma, Yanqiu Shao, and Qiubin Kan. "Selective oxidation of isobutane and isobutene over vanadium phosphorus oxides." Catalysis Communications 10, no. 3 (December 2008): 276–80. http://dx.doi.org/10.1016/j.catcom.2008.09.003.

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4

Takita, Yusaku, Qing Xia, Kayo Kikutani, Kazuya Soda, Hideaki Takami, Hiroyasu Nishiguchi, and Katsutoshi Nagaoka. "Anaerobic oxidation of isobutane." Journal of Molecular Catalysis A: Chemical 248, no. 1-2 (April 2006): 61–69. http://dx.doi.org/10.1016/j.molcata.2005.12.012.

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5

Hikazudani, Susumu, Kayo Kikutani, Katsutoshi Nagaoka, Takanori Inoue, and Yusaku Takita. "Anaerobic oxidation of isobutane." Applied Catalysis A: General 345, no. 1 (July 2008): 65–72. http://dx.doi.org/10.1016/j.apcata.2008.04.022.

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6

Bergfeldt, Trevor M., William L. Waltz, Xiangrong Xu, Petr Sedlák, Uwe Dreyer, Hermann Möckel, Jochen Lilie, and John W. Stephenson. "Photobehavior of aqueous uranyl ion and photo-oxygenation of isobutane using light from the visible region." Canadian Journal of Chemistry 81, no. 3 (March 1, 2003): 219–29. http://dx.doi.org/10.1139/v03-026.

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The photochemical and photophysical behavior of the aqueous uranyl ion [UO2(H2O)5]2+ has been studied under the influence of visible light and with added perchloric acid over the range of 0.014 M. In the presence of 2-methylpropane (isobutane), photo-oxygenation of isobutane occurs to yield, as the major product, 2-methyl-2-propanol (tert-butyl alcohol) along with lesser amounts of 2-methyl-2-propene (isobutene) and other C1C8 products. The quantum yield for formation of tert-butyl alcohol is independent of light intensity at the irradiation wavelength of 415 nm and of uranyl concentration, but it increases from 0.016 ± 0.001 at 0.01 M HClO4 (pH 2) to 0.13 ± 0.01 at 4 M HClO4. The emission spectrum from the electronically excited uranyl ion and the associated quantum yields have been measured in the presence and absence of isobutane, as a function of added perchloric acid. While in both cases the shape of the spectrum remains invariant, the quantum yields increase with increasing perchloric acid concentration. The strong dependence on added perchloric acid is interpreted within the context of the presence and interconversion of two electronically excited species, an acid form, *[UO2(H2O)5]2+, and a base form, *[UO2(H2O)n(OH)]+. It is proposed that both forms react with isobutane to give a tert-butyl radical, and that oxidation of coordinated aqua ligands occur, the latter generating a hydroxyl radical whose reaction with isobutane rapidly leads also to a tert-butyl radical. The reaction of this alkyl radical with ground-state [UO2(H2O)5]2+ then gives rise to the stable tert-butyl alcohol product and reduced forms of uranyl ion. Based upon the values of the quantum yields and of excited-state lifetime measurements reported in the literature, a comprehensive mechanism has been developed in a quantitative manner to provide calculated values of the rate constants for the individual mechanistic steps. The calculated rate constants provide a basis to calculate the values of quantum yields for emission and chemical reaction, as well as for lifetimes, that agree very satisfactorily with the experimental values over a 400-fold concentration change in added perchloric acid.Key words: photo-oxidation, photo-oxygenation, uranyl ion, isobutane, tert-butyl alcohol, lifetime, quantum yield, acidbase dissociation.

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7

Vogin, B., F. Baronnet, and G. Scacchi. "Étude chimique et cinétique de l'oxydation homogène en phase gazeuse d'alcanes légers. II. Propane et mécanisme généralisé." Canadian Journal of Chemistry 69, no. 1 (January 1, 1991): 43–61. http://dx.doi.org/10.1139/v91-008.

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An experimental study of the homogeneous gas phase oxidation of propane at 350 °C and subatmospheric pressure has been performed in order to identify and to measure the major primary products of the reaction. The experimental results have been interpreted by a chain radical mechanism, deduced from these results and from estimates of the rate constants for the elementary steps obtained by the methods of Thermochemical Kinetics. The proposed elementary steps are discussed and compared with the experimental observations. The results that we have obtained and their interpretation are compared with a similar detailed investigation performed on the oxidation of isobutane. As in the case of isobutane, two parallel reaction pathways appear, a dominant one leading to the conjugated alkene (propylene) and another one leading to the epoxide of this olefin (here propylene oxide). The oxidation of isobutane and that of propane appear to be quite similar, which corroborates the results that we have obtained. Key words: oxidation, kinetics, reaction mechanism, propane, thermochemical kinetics.

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8

SATO, Minoru, Hiroaki SHIGEOKA, and Yoshio NISHIMOTO. "Catalytic Oxidation of Flammable Refrigerant Isobutane." Proceedings of the JSME annual meeting 2004.5 (2004): 193–94. http://dx.doi.org/10.1299/jsmemecjo.2004.5.0_193.

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9

SATO, Minoru, Hiroaki SHIGEOKA, and Yoshio NISHIMOTO. "Catalytic Oxidation of Hydrocarbon Refrigerant Isobutane." Transactions of the Japan Society of Mechanical Engineers Series B 72, no. 724 (2006): 2992–98. http://dx.doi.org/10.1299/kikaib.72.2992.

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10

Zhang, Li, Sébastien Paul, Franck Dumeignil, and Benjamin Katryniok. "Selective Oxidation of Isobutane to Methacrylic Acid and Methacrolein: A Critical Review." Catalysts 11, no. 7 (June 25, 2021): 769. http://dx.doi.org/10.3390/catal11070769.

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Selective oxidation of isobutane to methacrolein (MAC) and methacrylic acid (MAA) has received great interest both in the chemical industry and in academic research. The advantages of this reaction originate not only from the low cost of the starting material and reduced process complexity, but also from limiting the use of toxic reactants and the production of wastes. Successive studies and reports have shown that heteropolycompounds (HPCs) with Keggin structure (under the form of partially neutralized acids with increased stability) can selectively convert isobutane to MAA and MAC due to their strong and tunable acidity and redox properties. This review hence aims to discuss the Keggin-type HPCs that have been used in recent years to catalyze the oxidation of isobutane to MAA and MAC, and to review alternative metal oxides with proper redox properties for the same reaction. In addition, the influence of the main reaction conditions will be discussed.

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11

SATO, Minoru, Hiroaki SHIGEOKA, and Yoshio NISHIMOTO. "Catalytic Oxidation of Hydrocarbon System Refrigerant Isobutane." Proceedings of the Symposium on Environmental Engineering 2004.14 (2004): 235–37. http://dx.doi.org/10.1299/jsmeenv.2004.14.235.

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12

Guan, Jingqi, Cheng Xu, Zhuqian Wang, Ying Yang, Bo Liu, Fanpeng Shang, Yanqiu Shao, and Qiubin Kan. "Selective Oxidation of Isobutane and Isobutene to Methacrolein over Te–Mo Mixed Oxide Catalysts." Catalysis Letters 124, no. 3-4 (April 30, 2008): 428–33. http://dx.doi.org/10.1007/s10562-008-9496-3.

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13

Liu, Yanchun, Jingfang He, Wenling Chu, and Weishen Yang. "Polyoxometalate catalysts with co-substituted VO2+ and transition metals and their catalytic performance for the oxidation of isobutane." Catalysis Science & Technology 8, no. 22 (2018): 5774–81. http://dx.doi.org/10.1039/c8cy01101j.

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14

SATO, Minoru, and Yoshio NISHIMOTO. "224 Catalytic Oxidation System of Hydrocarbon Refrigerant Isobutane." Proceedings of the Symposium on Environmental Engineering 2006.16 (2006): 217–20. http://dx.doi.org/10.1299/jsmeenv.2006.16.217.

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15

Jalowiecki-Duhamel, L., A. Monnier, Y. Barbaux, and G. Hecquet. "Oxidation of isobutane on a heteropolycompound hydrogen reservoir." Catalysis Today 32, no. 1-4 (December 1996): 237–41. http://dx.doi.org/10.1016/s0920-5861(96)00180-0.

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16

Paul, Johan S., Marijke H. Groothaert, Christine E. A. Kirschhock, Oleg I. Lebedev, Pierre A. Jacobs, and Wilhelm F. Maier. "Novel MoVSbO -type catalysts for selective isobutane oxidation." Catalysis Today 91-92 (July 2004): 265–69. http://dx.doi.org/10.1016/j.cattod.2004.03.041.

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17

Guan, Jingqi, Zhuqian Wang, Chen Xu, Ying Yang, Bo Liu, Xiaofang Yu, and Qiubin Kan. "Partial Oxidation of Isobutane over Vanadium Phosphorus Oxides." Catalysis Letters 128, no. 3-4 (November 11, 2008): 356–62. http://dx.doi.org/10.1007/s10562-008-9753-5.

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18

SATO, Minoru, Hiroaki SHIGEOKA, and Yoshio NISHIMOTO. "3802 Catalytic Oxidation of Flammable Refrigerant Isobutane (2nd Report)." Proceedings of the JSME annual meeting 2005.5 (2005): 465–66. http://dx.doi.org/10.1299/jsmemecjo.2005.5.0_465.

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19

Nenoff, Tina M., Margaret C. Showalter, and Kenneth A. Salaz. "Supported metalloporphyrins catalyze the oxidation of isobutane by dioxygen." Journal of Molecular Catalysis A: Chemical 121, no. 2-3 (July 1997): 123–29. http://dx.doi.org/10.1016/s1381-1169(96)00458-x.

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20

Deng, Qian, Shaoliang Jiang, Tiejun Cai, Zhenshan Peng, and Zhengjun Fang. "Selective oxidation of isobutane over HxFe0.12Mo11VPAs0.3Oy heteropoly compound catalyst." Journal of Molecular Catalysis A: Chemical 229, no. 1-2 (March 2005): 165–70. http://dx.doi.org/10.1016/j.molcata.2004.11.013.

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21

Shah, U., S. M. Mahajani, M. M. Sharma, and T. Sridhar. "Effect of supercritical conditions on the oxidation of isobutane." Chemical Engineering Science 55, no. 1 (January 2000): 25–35. http://dx.doi.org/10.1016/s0009-2509(99)00185-2.

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22

Erol, Zuhal, Saliha Cetinyokus Kilicarslan, and Meltem Dogan. "Investigation of Isobutane Dehydrogenation on CrOx/MCM-41 Catalyst." Macedonian Journal of Chemistry and Chemical Engineering 39, no. 1 (May 30, 2020): 109. http://dx.doi.org/10.20450/mjcce.2020.1842.

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The syntheses of MCM-41 (Mobil Composition of Matter No. 41) supported chromium oxide cat-alysts at different chromium concentrations (4–10 % by mass) were carried out hydrothermally. The aim of this study was to determine the effect of chromium concentration in the catalyst structure on the chro-mate types and chromium oxidation states, as well as the activity of the catalyst in the isobutane dehydro-genation reaction. Inactive α-Cr2O3 crystals for isobutane dehydrogenation were shown to increase in the catalyst structure as the chromium loading increased. The highest amount of Cr6+ on the catalyst surface was detected in the catalyst (H4-MCM-41) with 4 % chromium by mass. Catalytic tests (T = 600 °C, P = atmospheric pressure, WHSV = 26 h–1) were performed under fixed bed reactor conditions. The high-est isobutane conversion (~60 %) and selectivity (~80 %) were observed on the H4-MCM-41 catalyst, which had the highest amount of Cr6+ and monochromate structures. Catalyst deactivation was not due to coke deposition but, rather, was caused by the formation of inactive α-Cr2O3 crystal structures.

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23

Guan, Jingqi, Ke Song, Haiyan Xu, Zhuqian Wang, Yuanyuan Ma, Fanpeng Shang, and Qiubin Kan. "Oxidation of isobutane and isobutene to methacrolein over hydrothermally synthesized Mo–V–Te–O mixed oxide catalysts." Catalysis Communications 10, no. 5 (January 2009): 528–32. http://dx.doi.org/10.1016/j.catcom.2008.10.025.

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24

Zhang, Li, Jérémie Zaffran, Franck Dumeignil, Sébastien Paul, Axel Löfberg, and Benjamin Katryniok. "Catalytic selective oxidation of isobutane in a decoupled redox-process." Applied Catalysis A: General 643 (August 2022): 118798. http://dx.doi.org/10.1016/j.apcata.2022.118798.

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25

SATO, Minoru, Hiroaki SHIGEOKA, and Yoshio NISHIMOTO. "227 Catalytic Oxidation of Hydrocarbon System Refrigerant Isobutane (2nd Report)." Proceedings of the Symposium on Environmental Engineering 2005.15 (2005): 200–202. http://dx.doi.org/10.1299/jsmeenv.2005.15.200.

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26

SATO, Minoru, Hiroaki SHIGEOKA, and Yoshio NISHIMOTO. "3801 Development of the Isobutane Treatment System with Catalytic Oxidation." Proceedings of the JSME annual meeting 2005.5 (2005): 463–64. http://dx.doi.org/10.1299/jsmemecjo.2005.5.0_463.

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27

Paul, Sébastien, Véronique Le Courtois, and Dominique Vanhove. "Kinetic Investigation of Isobutane Selective Oxidation over a Heteropolyanion Catalyst." Industrial & Engineering Chemistry Research 36, no. 8 (August 1997): 3391–99. http://dx.doi.org/10.1021/ie960683k.

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28

Mizuno, Noritaka, and Hidenori Yahiro. "Oxidation of Isobutane Catalyzed by Partially Salified Cesium Molybdovanadophosphoric Acids." Journal of Physical Chemistry B 102, no. 2 (January 1998): 437–43. http://dx.doi.org/10.1021/jp972677n.

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29

SATO, Minoru, and Yoshio NISHIMOTO. "5413 Catalytic Oxidation System of Hydrocarbon Refrigerant Isobutane (2nd Report)." Proceedings of the JSME annual meeting 2006.5 (2006): 557–58. http://dx.doi.org/10.1299/jsmemecjo.2006.5.0_557.

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30

Fan, Li, Yuri Nakayama, and Kaoru Fujimoto. "Air oxidation of supercritical phase isobutane to tert-butyl alcohol." Chemical Communications, no. 13 (1997): 1179–80. http://dx.doi.org/10.1039/a702308a.

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31

Venegas, Juan M., Joseph T. Grant, William P. McDermott, Samuel P. Burt, Jack Micka, Carlos A. Carrero, and Ive Hermans. "Selective Oxidation ofn-Butane and Isobutane Catalyzed by Boron Nitride." ChemCatChem 9, no. 12 (March 24, 2017): 2118–27. http://dx.doi.org/10.1002/cctc.201601686.

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32

Paul, Sébastien, Wei Chu, Manzoor Sultan, and Elisabeth Bordes-Richard. "Keggin-type H4PVMo11O40-based catalysts for the isobutane selective oxidation." Science China Chemistry 53, no. 9 (September 2010): 2039–46. http://dx.doi.org/10.1007/s11426-010-4073-1.

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33

Mizuno, Noritaka, Masaki Tateishi, and Masakazu Iwamoto. "Oxidation of Isobutane Catalyzed by CsxH3−xPMo12O40-Based Heteropoly Compounds." Journal of Catalysis 163, no. 1 (September 1996): 87–94. http://dx.doi.org/10.1006/jcat.1996.0307.

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34

Weber, D., P. Weidler, and B. Kraushaar-Czarnetzki. "Partial Oxidation of Isobutane and Isobutene to Methacrolein Over a Novel Mo–V–Nb(–Te) Mixed Oxide Catalyst." Topics in Catalysis 60, no. 17-18 (June 1, 2017): 1401–7. http://dx.doi.org/10.1007/s11244-017-0830-0.

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35

Jing, Fangli, Benjamin Katryniok, Franck Dumeignil, Elisabeth Bordes-Richard, and Sébastien Paul. "Catalytic selective oxidation of isobutane over Csx(NH4)3−xHPMo11VO40mixed salts." Catalysis Science & Technology 4, no. 9 (June 2, 2014): 2938. http://dx.doi.org/10.1039/c4cy00518j.

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36

Basevich, V. Ya, A. A. Belyaev, S. N. Medvedev, V. S. Posvyanskii, and S. M. Frolov. "Detailed kinetic mechanism of the multistage oxidation and combustion of isobutane." Russian Journal of Physical Chemistry B 9, no. 2 (March 2015): 268–74. http://dx.doi.org/10.1134/s1990793115020177.

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37

Suresh, A. K. "Isobutane oxidation in the liquid and supercritical phases: comparison of features." Journal of Supercritical Fluids 12, no. 2 (April 1998): 165–76. http://dx.doi.org/10.1016/s0896-8446(97)00048-x.

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38

Jia, M. J., R. X. Valenzuela, P. Amorós, D. Beltrán-Porter, J. El-Haskouri, M. D. Marcos, and V. Cortés Corberán. "Direct oxidation of isobutane to methacrolein over V-MCM-41 catalysts." Catalysis Today 91-92 (July 2004): 43–47. http://dx.doi.org/10.1016/j.cattod.2004.03.007.

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39

Paul, J. "Combinatorial discovery of new catalysts for the selective oxidation of isobutane." Applied Catalysis A: General 265, no. 2 (July 8, 2004): 185–93. http://dx.doi.org/10.1016/j.apcata.2004.01.023.

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40

Hu, Jing, Zhifang Li, Xiaoyuan Yang, Wenli Ding, and Jingqi Guan. "Effect of Different Silicate Supports on the Catalytic Performance of MoVTeO Mixed Oxides in Partial Oxidation of Isobutane." International Journal of Chemical Reactor Engineering 12, no. 1 (January 1, 2014): 623–28. http://dx.doi.org/10.1515/ijcre-2013-0153.

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Abstract A series of 5% MoV0.3Te0.25 supported on different silicates (i.e. SiO2, HMS, MCM-41, and MCM-48) have been prepared, characterized, and tested as catalysts in the partial oxidation of isobutane to methacrolein. Characterization results showed that the supports almost kept intact structures after supporting 5 wt.% MoV0.3Te0.25 and the supported catalysts had large specific surface areas. Catalytic tests showed that the specific surface area played a key role in the catalytic activity for the supported catalysts.

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41

Guan, Jingqi, Ke Song, Haiyan Xu, Yuanyuan Ma, Xiaofang Yu, Yanqiu Shao, and Qiubin Kan. "Effect of calcination conditions on the catalytic behavior of Te-Mo mixed oxide catalysts in oxidation of isobutane and isobutene." Reaction Kinetics and Catalysis Letters 95, no. 2 (December 2008): 321–28. http://dx.doi.org/10.1007/s11144-008-5348-9.

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42

de Leitenburg, Carla, Alessandro Trovarelli, Jordi Llorca, Fabrizio Cavani, and Gianluca Bini. "The effect of doping CeO2 with zirconium in the oxidation of isobutane." Applied Catalysis A: General 139, no. 1-2 (June 1996): 161–73. http://dx.doi.org/10.1016/0926-860x(95)00334-7.

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43

Guan, Jingqi, Haiyan Xu, Ke Song, Bo Liu, Fanpeng Shang, Xiaofang Yu, and Qiubin Kan. "Selective Oxidation and Oxidative Dehydrogenation of Isobutane over Hydrothermally Synthesized Mo–V–O Mixed Oxide Catalysts." Catalysis Letters 126, no. 3-4 (September 3, 2008): 293–300. http://dx.doi.org/10.1007/s10562-008-9613-3.

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44

Yinga, Fang, Shuiju Wang, Chak-Tong Au, and Suk-Yin Lai. "Effect of the oxidation state of gold on the complete oxidation of isobutane on Au/CeO2 catalysts." Gold Bulletin 43, no. 4 (December 2010): 241–51. http://dx.doi.org/10.1007/bf03214994.

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45

King, Clinton R., Ashley Holdaway, George Durrant, Josh Wheeler, Lorna Suaava, Michael M. Konnick, Roy A. Periana, and Daniel H. Ess. "Supermetal: SbF5-mediated methane oxidation occurs by C–H activation and isobutane oxidation occurs by hydride transfer." Dalton Transactions 48, no. 45 (2019): 17029–36. http://dx.doi.org/10.1039/c9dt03564h.

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46

Zhang, Li, Franck Dumeignil, Sébastien Paul, and Benjamin Katryniok. "Supported Rb- or Cs-containing HPA catalysts for the selective oxidation of isobutane." Applied Catalysis A: General 628 (November 2021): 118400. http://dx.doi.org/10.1016/j.apcata.2021.118400.

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47

Raybold, Troy M., and Marylin C. Huff. "Oxidation of isobutane over supported noble metal catalysts in a palladium membrane reactor." Catalysis Today 56, no. 1-3 (February 2000): 35–44. http://dx.doi.org/10.1016/s0920-5861(99)00260-6.

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48

Fan, Li, Takashi Watanabe, and Kaoru Fujimoto. "Reaction phase effect on tertiary butyl alcohol synthesis by air oxidation of isobutane." Applied Catalysis A: General 158, no. 1-2 (September 1997): L41—L46. http://dx.doi.org/10.1016/s0926-860x(97)00178-6.

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49

Liu, Haichao, Eric M. Gaigneaux, Hideo Imoto, Takafumi Shido, and Yasuhiro Iwasawa. "Novel Re–Sb–O catalysts for the selective oxidation of isobutane and isobutylene." Applied Catalysis A: General 202, no. 2 (August 2000): 251–64. http://dx.doi.org/10.1016/s0926-860x(00)00539-1.

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50

Paul, Johan S., Rob Janssens, Joeri F. M. Denayer, Gino V. Baron, and Pierre A. Jacobs. "Optimization of MoVSb Oxide Catalyst for Partial Oxidation of Isobutane by Combinatorial Approaches." Journal of Combinatorial Chemistry 7, no. 3 (May 2005): 407–13. http://dx.doi.org/10.1021/cc0500046.

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