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Journal articles on the topic 'Interfaces liquide/solide'

Author: Grafiati

Published: 25 May 2024

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1

Crumlin, Ethan J. "(Invited) Using Ambient Pressure XPS to Probe the Solid/Gas and Solid/Liquid Interface Under in Situ and Operando Conditions." ECS Meeting Abstracts MA2022-02, no. 46 (2022): 1715. http://dx.doi.org/10.1149/ma2022-02461715mtgabs.

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Interfaces play an essential role in nearly all aspects of life and are critical for electrochemistry. Prof. Robert Savinell has played a pivotal interface to me in the role of mentorship in both life and electrochemistry, and I look to honor his contributions to both through this talk. Electrochemical systems ranging from high-temperature solid oxide fuel cells (SOFC) to batteries to capacitors have a wide range of important interfaces between solids, liquids, and gases, which play a pivotal role in how energy is stored, transferred, and converted. I will share the use of ambient pressure XPS

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2

Josell, Daniel, and Frans Spaepen. "Surfaces, Interfaces, and Changing Shapes in Multilayered Films." MRS Bulletin 24, no. 2 (1999): 39–43. http://dx.doi.org/10.1557/s0883769400051538.

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It is generally recognized that the capillary forces associated with internal and external interfaces affect both the shapes of liquid-vapor surfaces and wetting of a solid by a liquid. It is less commonly understood that the same phenomenology often applies equally well to solid-solid or solid-vapor interfaces.The fundamental quantity governing capillary phenomena is the excess free energy associated with a unit area of interface. The microscopic origin of this excess free energy is often intuitively simple to understand: the atoms at a free surface have “missing bonds”; a grain boundary cont

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3

Saleman, Abdul Rafeq, Mohamad Shukri Zakaria, Ridhwan Jumaidin, Nur Hazwani Mokhtar, and Nor Aslily Sarkam. "Molecular Dynamics Study: Correlation of Heat Conduction Across S-L Interfaces Between Constant Heat Flux and Shear Applied to Liquid Systems." Journal of Mechanical Engineering 19, no. 3 (2022): 33–53. http://dx.doi.org/10.24191/jmeche.v19i3.19795.

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Heat conduction (HC) at solid-liquid (S-L) interfaces play a significant role in the performance of engineering systems. Thus, this study investigates HC at S-L interfaces and its correlation between constant heat flux (CHF) and shear applied to liquid (SAL) systems using non-equilibrium molecular dynamics simulation. The S-L interface consists of solids with the face-centred cubic (FCC) lattice of (110), (111) and (100) planes facing the liquid. The solid is modelled by Morse potential whereas the liquid is modelled by Lennard Jones potential. The interaction between solid-liquid was modelled

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4

Streubel, Robert, Xubo Liu, Xuefei Wu, and Thomas P. Russell. "Perspective: Ferromagnetic Liquids." Materials 13, no. 12 (2020): 2712. http://dx.doi.org/10.3390/ma13122712.

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Mechanical jamming of nanoparticles at liquid–liquid interfaces has evolved into a versatile approach to structure liquids with solid-state properties. Ferromagnetic liquids obtain their physical and magnetic properties, including a remanent magnetization that distinguishes them from ferrofluids, from the jamming of magnetic nanoparticles assembled at the interface between two distinct liquids to minimize surface tension. This perspective provides an overview of recent progress and discusses future directions, challenges and potential applications of jamming magnetic nanoparticles with regard

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5

Veen, J. F. van der, and H. Reichert. "Structural Ordering at the Solid–Liquid Interface." MRS Bulletin 29, no. 12 (2004): 958–62. http://dx.doi.org/10.1557/mrs2004.267.

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AbstractMany processes in nature and technology are based on the static and dynamic properties of solid–liquid interfaces. Prominent examples are crystal growth, melting, and recrystallization. These processes are strongly affected by the local structure at the solid–liquid interface. Therefore, it is mandatory to understand the change in the structure across the interface. The break of the translational symmetry at the interface induces ordering phenomena, and interactions between the liquid's molecules and the atomically corrugated solid surface may induce additional ordering effects. In the

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Titova, E. A., and D. V. Alexandrov. "The boundary integral equation for curved solid/liquid interfaces propagating into a binary liquid with convection." Journal of Physics A: Mathematical and Theoretical 55, no. 5 (2022): 055701. http://dx.doi.org/10.1088/1751-8121/ac463e.

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Abstract The boundary integral method is developed for unsteady solid/liquid interfaces propagating into undercooled binary liquids with convection. A single integrodifferential equation for the interface function is derived using the Green function technique. In the limiting cases, the obtained unsteady convective boundary integral equation transforms into a previously developed theory. This integral is simplified for the steady-state growth in arbitrary curvilinear coordinates when the solid/liquid interface is isothermal (isoconcentration). Finally, we evaluate the boundary integral for a b

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7

Briant, C. L. "Grain Boundary Chemistry and Reactions in Metals." MRS Bulletin 15, no. 10 (1990): 26–32. http://dx.doi.org/10.1557/s0883769400058632.

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An interface can be defined as a surface that serves as a common boundary between two phases. Examples include the boundaries between two solids, two immiscible liquids, a solid and a liquid, a solid and a gas, and a liquid and a gas. Interfaces have been studied for decades by scientists of many different disciplines. One reason for this interest is that the atomic structure and the chemical composition at the interface can differ from that of the bulk material on either side of it. Consequently, the properties of the interface can differ greatly from those of either bulk phase, and chemical

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8

Giunta, Giuliana, and Paola Carbone. "Cross-over in the dynamics of polymer confined between two liquids of different viscosity." Interface Focus 9, no. 3 (2019): 20180074. http://dx.doi.org/10.1098/rsfs.2018.0074.

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Using molecular dynamics simulations, we analysed the polymer dynamics of chains of different molecular weights entrapped at the interface between two immiscible liquids. We showed that on increasing the viscosity of one of the two liquids the dynamic behaviour of the chain changes from a Zimm-like dynamics typical of dilute polymer solutions to a Rouse-like dynamics where hydrodynamic interactions are screened. We observed that when the polymer is in contact with a high viscosity liquid, the number of solvent molecules close to the polymer beads is reduced and ascribed the screening effect to

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9

Howe, J. M. "Quantification of order in the liquid at a solid-liquid interface by high-resolution transmission electron microscopy (HRTEM)." Proceedings, annual meeting, Electron Microscopy Society of America 54 (August 11, 1996): 114–15. http://dx.doi.org/10.1017/s0424820100163034.

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A number of different theoretical approaches have been used to model the atomic structure and properties of solid-liquid interfaces. Most calculations indicate that ordering occurs in the first several layers of the liquid, adjacent to the crystal surface. In contrast to the numerous theoretical investigations, there have been no direct experimental observations of the atomic structure of a solid-liquid interface for comparison. Saka et al. examined solid-liquid interfaces in In and In-Sb at lattice-fringe resolution in the TEM, but their data do not reveal information about the atomic structu

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10

Pascall, Andrew J., and Todd M. Squires. "Electrokinetics at liquid/liquid interfaces." Journal of Fluid Mechanics 684 (September 28, 2011): 163–91. http://dx.doi.org/10.1017/jfm.2011.288.

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AbstractElectrokinetic effects at liquid/liquid interfaces have received considerably less attention than at solid/liquid interfaces. Because liquid/liquid interfaces are generally mobile, one might expect electrokinetic effects over a liquid/liquid interface to be faster than over an equivalent solid surface. The earliest predictions for the electrophoretic mobility of charged mercury drops – distinct approaches by Frumkin, along with Levich, and Booth – differed by $O(a/ {\lambda }_{D} )$, where $a$ is the radius of the drop and ${\lambda }_{D} $ is the Debye length. Seeking to reconcile thi

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11

Spencer Jolly, Dominic, Dominic L. R. Melvin, Isabella D. R. Stephens, et al. "Interfaces between Ceramic and Polymer Electrolytes: A Comparison of Oxide and Sulfide Solid Electrolytes for Hybrid Solid-State Batteries." Inorganics 10, no. 5 (2022): 60. http://dx.doi.org/10.3390/inorganics10050060.

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Hybrid solid-state batteries using a bilayer of ceramic and solid polymer electrolytes may offer advantages over using a single type of solid electrolyte alone. However, the impedance to Li+ transport across interfaces between different electrolytes can be high. It is important to determine the resistance to Li+ transport across these heteroionic interfaces, as well as to understand the underlying causes of these resistances; in particular, whether chemical interphase formation contributes to giving high resistances, as in the case of ceramic/liquid electrolyte interfaces. In this work, two ce

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Spencer Jolly, Dominic, Dominic L. R. Melvin, Isabella D. R. Stephens, et al. "Interfaces between Ceramic and Polymer Electrolytes: A Comparison of Oxide and Sulfide Solid Electrolytes for Hybrid Solid-State Batteries." Inorganics 10, no. 5 (2022): 60. http://dx.doi.org/10.3390/inorganics10050060.

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Hybrid solid-state batteries using a bilayer of ceramic and solid polymer electrolytes may offer advantages over using a single type of solid electrolyte alone. However, the impedance to Li+ transport across interfaces between different electrolytes can be high. It is important to determine the resistance to Li+ transport across these heteroionic interfaces, as well as to understand the underlying causes of these resistances; in particular, whether chemical interphase formation contributes to giving high resistances, as in the case of ceramic/liquid electrolyte interfaces. In this work, two ce

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13

Storaska, Garrett A., and James M. Howe. "In-Situ TEM Investigation of the Solid/Liquid Interface in Al-Si Alloys." Microscopy and Microanalysis 6, S2 (2000): 1068–69. http://dx.doi.org/10.1017/s1431927600037831.

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The solid/liquid interface is a junction between two condensed phases with completely different atomic arrangements. At the interface between the periodically ordered solid and the amorphous liquid, the atoms adopt a structure that minimizes the excess energy due to the abrupt change between the surrounding phases. Faceted and diffuse interfaces describe two extremes in morphology of a solid/liquid interface. In a faceted interface, the change from solid to liquid occurs over one atomic layer, however periodic order extends into the first few liquid layers adjacent to the crystalline solid, as

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14

Saka, H., K. Sasaki, S. Tsukimoto, and S. Arai. "In situ Observation of Solid–liquid Interfaces by Transmission Electron Microscopy." Journal of Materials Research 20, no. 7 (2005): 1629–40. http://dx.doi.org/10.1557/jmr.2005.0212.

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Recent progress in in situ observation of solid–liquid interfaces by means of transmission electron microscopy, carried out by the Nagoya group, was reviewed. The results obtained on pure materials are discussed based on Jackson's theory. The structure of the solid–liquid interfaces of eutectic alloys was also observed. The in situ observation technique of solid–liquid interface is applied to industrially important reactions which include liquid phases.

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15

Kurihara, Kazue. "Surface forces measurement for materials science." Pure and Applied Chemistry 91, no. 4 (2019): 707–16. http://dx.doi.org/10.1515/pac-2019-0101.

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Abstract This article reviews the surface forces measurement as a novel tool for materials science. The history of the measurement is briefly described in the Introduction. The general overview covers specific features of the surface forces measurement as a tool for studying the solid-liquid interface, confined liquids and soft matter. This measurement is a powerful way for understanding interaction forces, and for characterizing (sometime unknown) phenomena at solid-liquid interfaces and soft complex matters. The surface force apparatus (SFA) we developed for opaque samples can study not only

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16

You, Hoydoo, and Zoltán Nagy. "Applications of Synchrotron Surface X-Ray Scattering Studies of Electrochemical Interfaces." MRS Bulletin 24, no. 1 (1999): 36–40. http://dx.doi.org/10.1557/s088376940005171x.

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Aqueous-solution/solid interfaces are ubiquitous in modern manufacturing environments as well as in our living environment, and studies of such interfaces are an active area of science and engineering research. An important area is the study of liquid/solid interfaces under active electrochemical control, which has many immediate technological implications, for example, corrosion/passivation of metals and energy storage in batteries and ultracapacitors. The central phenomenon of electrochemistry is the charge transfer at the interface, and the region of interest is usually wider than a single

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17

Alexandrova, Lidia A., Ljudmil S. Grigorov, Nikolay A. Grozev, and Stoyan I. Karakashev. "Investigation of Interfacial Free Energy of Three-Phase Contact on a Glass Sphere in Case of Cationic-Anionic Surfactant Aqueous Mixtures." Coatings 10, no. 6 (2020): 573. http://dx.doi.org/10.3390/coatings10060573.

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The wetting of adsorbed surfactants solids is important for various technological applications in particular for the process of foam flotation. The present work aims at calculating the surface tensions of the three phase interfaces at different surfactant concentrations using the Girifalco and Good method. For this purpose, the surface tension and contact angle vs. surfactant concentration of the test substances amines and sulfonates and their mixture were measured for liquid–air interface. Calculated surface tension of solid–air interface vs. concentration for C10 amine and mixed systems are

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18

Fan, Feng Ru. "(Invited) novel Charged Interfaces for Catalysis and Energy Conversion." ECS Meeting Abstracts MA2023-01, no. 34 (2023): 1885. http://dx.doi.org/10.1149/ma2023-01341885mtgabs.

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Charged interfaces are ubiquitous in many research fields such as electrochemistry, catalysis, and energy chemistry, and are key places where physical and chemical processes occur. The charged interface structure can also be affected by external fields such as light, electricity, and force, and becomes the key to regulating chemical reactions. It is of great significance for the development of surface and interface science, electrochemistry, catalysis and energy science to deeply understand the physical and chemical reaction process and mechanism of various charged interface systems, and to cl

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19

Howe, James M., and Hiroyasu Saka. "In Situ Transmission Electron Microscopy Studies of the Solid–Liquid Interface." MRS Bulletin 29, no. 12 (2004): 951–57. http://dx.doi.org/10.1557/mrs2004.266.

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AbstractIn situtransmission electron microscopy (TEM) studies allow one to determine the structure, chemistry, and kinetic behavior of solid–liquid (S–L) interfaces with subnanometer spatial resolution. This article illustrates some important contributions ofin situTEM to our understanding of S–L interfaces in Al-Si alloys and liquid In particles in Al and Fe matrices.Four main areas are discussed:ordering in the liquid at a S–L interface, compositional changes across the interface, the kinetics and mechanisms of interface migration, and the contact angles and equilibrium melting temperature o

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20

Spaepen, Frans. "Structure of Liquids and Solid-Liquid Interfaces." Bulletin de la Classe des sciences 14, no. 1 (2003): 195–96. http://dx.doi.org/10.3406/barb.2003.28361.

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21

Paris, Oskar, Barbara Aichmayer, and Peter Fratzl. "Small-angle scattering from spherical particles on randomly oriented interfaces." International Journal of Materials Research 97, no. 3 (2006): 290–94. http://dx.doi.org/10.1515/ijmr-2006-0046.

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Abstract Small-angle scattering (SAS) has long been used to study nucleation and growth of particles in solid or liquid matrices. In some special cases, nucleation of particles occurs on interfaces, e. g., grain boundaries in crystalline solids or membranes in a solvent. Clearly, the position of the particles is constrained in this case to a narrow region close to the interface, which leads to correlations between the particles. In the present paper, we derive simple expressions for the analysis of SAS data from particles located on planar interfaces, and compare the analytical approximations

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22

Negahdar, Leila, Christopher M. A. Parlett, Mark A. Isaacs, Andrew M. Beale, Karen Wilson, and Adam F. Lee. "Shining light on the solid–liquid interface: in situ/operando monitoring of surface catalysis." Catalysis Science & Technology 10, no. 16 (2020): 5362–85. http://dx.doi.org/10.1039/d0cy00555j.

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Many industrially important chemical transformations occur at the interface between a solid catalyst and liquid reactants. In situ and operando spectroscopies offer unique insight into the reactivity of such catalytically active solid–liquid interfaces.

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23

CHAUDHURI, ABHISHEK, DEBASISH CHAUDHURI, and SURAJIT SENGUPTA. "INDUCED INTERFACES AT NANOSCALES: STRUCTURE AND DYNAMICS." International Journal of Nanoscience 04, no. 05n06 (2005): 995–99. http://dx.doi.org/10.1142/s0219581x05003966.

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We show how interfaces may be induced in materials using external fields. The structure and the dynamics of these interfaces may then be manipulated externally to achieve desired properties. We discuss three types of such interfaces: an Ising interface in a nonuniform magnetic field, a solid–liquid interface and an interface between a solid and a smectic like phase. In all of these cases we explicitly show how small size, leading to atomic-scale discreteness and stiff constraints produce interesting effects which may have applications in the fabrication of nanostructured materials.

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Nemoshkalenko, V. V., O. P. Fedorov, E. I. Zhivolub, E. I. Bersudsky, and G. P. Chemerinsky. "«Morphos» Experiment Experimental study of solid-liquid interface in transparent substances." Kosmìčna nauka ì tehnologìâ 6, no. 4 (2000): 135–36. http://dx.doi.org/10.15407/knit2000.04.151.

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25

Zhao, Yu Hong, Wei Jin Liu, Hua Hou, and Yu Hui Zhao. "Impact on Solidification Dendrite Growth by Interfacial Atomic Motion Time with Phase Field Method." Materials Science Forum 749 (March 2013): 660–67. http://dx.doi.org/10.4028/www.scientific.net/msf.749.660.

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The Phase Field model of solidification processes was carried out coupled with temperature field model. The influence of interface atomic time on dendrite growth morphology in undercooled melt was simulated with pure nickel. The experimental results show that when the interface atomic motion time parameter is minor, the liquid-solid interfaces were unstable, disturbance can be amplified easily so the complicated side branches will grow, and the disturbance speed up the dendrite growth. With the increase of , the liquid-solid interfaces become more stable and finally the smooth dendrite morphol

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Chuiko, Myroslava, Lidiia Vytvytska, and Nataliia Pindus. "Method and device for the control of surface properties of porous solids at the boundary of their contact with liquids and gases." Ukrainian Metrological Journal, no. 2 (July 2, 2021): 55–59. http://dx.doi.org/10.24027/2306-7039.2.2021.236089.

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The article indicates the relevance of the problem of controlling the surface properties of solids, analyzes the features of interaction between porous solids in direct contact with liquids. The process of adhesive interaction of the system “liquid – porous solid” at the interface of these phases is analyzed and the dependence of the degree of wetting by a liquid of the surface of a solid on the structure of the porous body and the surface properties of the liquid is established. The dependence of the contact angle hysteresis of the solid with liquid on the porosity and roughness of the

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Lee, Joon-Hyung, Jeong-Joo Kim, Haifeng Wang, and Sang-Hee Cho. "Observation of Intergranular Films in BaB2O4-added BaTiO3 Ceramics." Journal of Materials Research 15, no. 7 (2000): 1600–1604. http://dx.doi.org/10.1557/jmr.2000.0229.

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Distribution characteristics of boundary phase in BaB2O4 added BaTiO3 ceramics were investigated with a focus on the curvature difference of solid–liquid interfaces at two-grain and triple junctions. High-resolution transmission electron microscopy revealed that the triple junction of solid grains showed the positive curvature of solid–liquid interface and consisted of the mixture of liquid phase and crystallized BaB2O4 phase. On the other hand, flat amorphous thin film of 2.5-nm thickness was observed at the two-grain junction. This kind of boundary phase distribution characteristic was expla

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28

Aharon, Hannah, Omer Shavit, Matan Galanty, and Adi Salomon. "Second Harmonic Generation for Moisture Monitoring in Dimethoxyethane at a Gold-Solvent Interface Using Plasmonic Structures." Nanomaterials 9, no. 12 (2019): 1788. http://dx.doi.org/10.3390/nano9121788.

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Second harmonic generation (SHG) is forbidden from most bulk metals because metals are characterized by centrosymmetric symmetry. Adsorption or desorption of molecules at the metal interface can break the symmetry and lead to SHG responses. Yet, the response is relatively low, and minute changes occurring at the interface, especially at solid/liquid interfaces, like in battery electrodes are difficult to assess. Herein, we use a plasmonic structure milled in a gold electrode to increase the overall SHG signal from the interface and gain information about small changes occurring at the interfac

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Wang, Xiaoyu, Cynthia J. Jameson, and Sohail Murad. "Interfacial Thermal Conductivity and Its Anisotropy." Processes 8, no. 1 (2019): 27. http://dx.doi.org/10.3390/pr8010027.

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There is a significant effort in miniaturizing nanodevices, such as semi-conductors, currently underway. However, a major challenge that is a significant bottleneck is dissipating heat generated in these energy-intensive nanodevices. In addition to being a serious operational concern (high temperatures can interfere with their efficient operation), it is a serious safety concern, as has been documented in recent reports of explosions resulting from many such overheated devices. A significant barrier to heat dissipation is the interfacial films present in these nanodevices. These interfacial fi

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Heinze, M. T., J. C. Zill, J. Matysik, W. D. Einicke, R. Gläser, and A. Stark. "Solid–ionic liquid interfaces: pore filling revisited." Phys. Chem. Chem. Phys. 16, no. 44 (2014): 24359–72. http://dx.doi.org/10.1039/c4cp02749c.

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Spencer, B. J., S. H. Davis, G. B. McFadden, and P. W. Voorhees. "Effects of Elastic Stress on the Stability of a Solid-Liquid Interface." Applied Mechanics Reviews 43, no. 5S (1990): S54—S55. http://dx.doi.org/10.1115/1.3120850.

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The effects of elastic stress on the stability of solid-liquid interfaces under a variety of conditions are discussed. In the cases discussed, the nonuniform composition field in the solid, which accompanies either the melting process or the development of a perturbation on the solid-liquid interface during solidification, generates nonhydrostatic stresses in the solid. Such compositionally generated elastic stresses have been shown experimentally to induce a solidifying solid-liquid interface to become unstable. We are in the process of analyzing the effects of these stresses on the condition

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Zhuang, Tieshuan, Jun Wu, Tao Zhang, and Xiangwei Dong. "A weakly compressible smoothed particle hydrodynamics framework for melting multiphase flow." AIP Advances 12, no. 2 (2022): 025329. http://dx.doi.org/10.1063/5.0057583.

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In this study, the transient process of solid–liquid phase change is modeled and simulated by the multiphase smoothed particle hydrodynamics (SPH) method. First, to simulate the interfacial behaviors of melt liquids, the multiphase SPH model is established for immiscible viscous fluids with a large density ratio, where the environmental liquid surrounding the solid phase is considered, and the surface tension of the melt liquid can be accurately modeled by the continuum surface force method. Based on the multiphase model, the thermal dynamics model is incorporated to describe the heat conducti

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Favaro, Marco, Fatwa Abdi, Ethan Crumlin, Zhi Liu, Roel van de Krol, and David Starr. "Interface Science Using Ambient Pressure Hard X-ray Photoelectron Spectroscopy." Surfaces 2, no. 1 (2019): 78–99. http://dx.doi.org/10.3390/surfaces2010008.

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The development of novel in situ/operando spectroscopic tools has provided the opportunity for a molecular level understanding of solid/liquid interfaces. Ambient pressure photoelectron spectroscopy using hard X-rays is an excellent interface characterization tool, due to its ability to interrogate simultaneously the chemical composition and built-in electrical potentials, in situ. In this work, we briefly describe the “dip and pull” method, which is currently used as a way to investigate in situ solid/liquid interfaces. By simulating photoelectron intensities from a functionalized TiO2 surfac

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McFadden, G. B., S. R. Coriell, L. N. Brush, and K. A. Jackson. "Interface Instabilities During Laser Melting of Thin Films." Applied Mechanics Reviews 43, no. 5S (1990): S70—S75. http://dx.doi.org/10.1115/1.3120854.

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Thin silicon films on a cooled substrate are often found to develop two-phase lamellar structures upon radiative heating. Jackson and Kurtz developed a two-dimensional model for the process in which the heated film consists of alternating parallel bands of liquid and solid phases separated by straight solid-liquid interfaces. To understand the cellular or dendritic structures that sometimes are observed in these interfaces, they also performed a linearized morphological stability analysis and obtained the conditions for the growth or decay of infinitesimal perturbations to the interface. In th

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Yu, C. J., G. Evmenenko, A. G. Richter, A. Datta, J. Kmetko, and P. Dutta. "Order in molecular liquids near solid–liquid interfaces." Applied Surface Science 182, no. 3-4 (2001): 231–35. http://dx.doi.org/10.1016/s0169-4332(01)00410-x.

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Magalhães e Silva, Diogo, Tânia Ribeiro, Luís C. Branco, Rogério Colaço, Amélia Gonçalves da Silva, and Benilde Saramago. "Hydrophobic ionic liquids at liquid and solid interfaces." Tribology International 129 (January 2019): 459–67. http://dx.doi.org/10.1016/j.triboint.2018.08.018.

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Divya, Velpula, and M. V. Sangaranarayanan. "Electrodeposition of Polymer Nanostructures using Three Diffuse Double Layers: Polymerization beyond the Liquid/Liquid Interfaces." Electrochemical Energy Technology 4, no. 1 (2018): 6–20. http://dx.doi.org/10.1515/eetech-2018-0002.

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Abstract Nanostructured conducting polymers have received immense attention during the past few decades on account of their phenomenal usefulness in diverse contexts, while the interface between two immiscible liquids is of great interest in chemical and biological applications. Here we propose a novel Electrode(solid)/Electrolyte(aqueous)/Electrolyte(organic) Interfacial assembly for the synthesis of polymeric nanostructures using a novel concept of three diffuse double layers. There exist remarkable differences between the morphologies of the polymers synthesized using the conventional elect

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Zachman, Michael J., Emily Asenath-Smith, Lara A. Estroff, and Lena F. Kourkoutis. "Site-Specific Preparation of Intact Solid–Liquid Interfaces by Label-Free In Situ Localization and Cryo-Focused Ion Beam Lift-Out." Microscopy and Microanalysis 22, no. 6 (2016): 1338–49. http://dx.doi.org/10.1017/s1431927616011892.

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AbstractScanning transmission electron microscopy (STEM) allows atomic scale characterization of solid–solid interfaces, but has seen limited applications to solid–liquid interfaces due to the volatility of liquids in the microscope vacuum. Although cryo-electron microscopy is routinely used to characterize hydrated samples stabilized by rapid freezing, sample thinning is required to access the internal interfaces of thicker specimens. Here, we adapt cryo-focused ion beam (FIB) “lift-out,” a technique recently developed for biological specimens, to prepare intact internal solid–liquid interfac

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Rettenmayr, Markus, Oleg Kashin, and Stephanie Lippmann. "Simulation of Liquid Film Migration during Melting." Materials Science Forum 790-791 (May 2014): 127–32. http://dx.doi.org/10.4028/www.scientific.net/msf.790-791.127.

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Melting of a single-phase polycrystalline material is known to start by the formation of liquid films at the surface and at grain boundaries. The internal liquid films are not necessarily quiescent, but can migrate to avoid/reduce supersaturation in the solid phase. The migration is discussed in the literature to be governed by coherency strains of the solid/liquid interface, by concentration gradients in the liquid or by concentration gradients in the solid phase. A phase transformation model for diffusional phase transformations considering interface thermodynamics (possible deviations from

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Welland, M. E., S. O'Shea, A. W. McKinnon, and T. M. H. Wong. "Applications of AFM and STM: Solvation forces in liquids and inelastic photon excitation." Proceedings, annual meeting, Electron Microscopy Society of America 50, no. 2 (1992): 1156–57. http://dx.doi.org/10.1017/s0424820100130419.

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We describe here non-standard applications of scanned probe microscopy; one application making use of the force sensitivity of the AFM to measure solvation forces at the liquid-solid interface and the other application based on the STM where the tunnelling current is used to excite photon emission from a surface.An interesting aspect of the solid-liquid interface is the molecular order induced in the liquid by the solid surface. This order can give rise to observable changes in the short range forces acting between two solids in a liquid medium; so called “solvation” or “structural” forces. As

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Agathopoulos, Simeon, D. U. Tulyaganov, and José Maria F. Ferreira. "Stages of Reactive Wetting." Key Engineering Materials 280-283 (February 2007): 1801–4. http://dx.doi.org/10.4028/www.scientific.net/kem.280-283.1801.

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A universal model for describing the wetting kinetics at solid/liquid interfaces, where interfacial chemical reaction occurs, is proposed, whereby four distinct stages separated from each other by transition points are anticipated. The stages are described by means of comparing the dimensions of the base of the liquid sessile drop with the evolution of the reaction product forming on the solid/liquid interface, over time.

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Lojkowski, Witold, Akira Otsuki, and Andrzej Morawski. "High-pressure effect on grain boundary wetting in aluminium bicrystals." International Journal of Materials Research 96, no. 10 (2005): 1211–12. http://dx.doi.org/10.1515/ijmr-2005-0208.

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Abstract The effect of pressure and misorientation on grain boundary wetting in aluminium bicrystals has been investigated. The grain boundaries were of [100] symmetrical tilt type. The wetting liquid was an Sn– Zn alloy. It is shown that the wetting angle is a function of misorientation but not of pressure. The reasons of the above results are discussed, assuming a linear dependence between the interface energy and pressure. It is shown that the difference of energy of the liquid/solid and solid/solid interface as well as the misorientation dependence of energy is simply proportional to the f

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Kawano, Satoyuki, Hiroyuki Hashimoto, Akio Ihara, and Keiji Shin. "Sequential Production of mm-Sized Spherical Shells in Liquid-Liquid Gas Systems." Journal of Fluids Engineering 118, no. 3 (1996): 614–18. http://dx.doi.org/10.1115/1.2817804.

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A new device has been developed for sequential production of mm-sized solid spherical shells using liquid-liquid gas systems. This device comprises a cylindrical vessel, for containing two kinds of immiscible liquids, and a gas injection orifice, set at the center of the vessel’s bottom. Solid spherical shells are successfully and sequentially produced by solidifying rising liquid spherical shells, formed sequentially at the horizontal interface between two immiscible liquids.

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Quan, Jiliang, Guanzhen Ke, Yali Zhang, Jian Liu, and Jinqiang Huang. "Study on Growth Interface of Large Nd:YAG Crystals." Crystals 13, no. 6 (2023): 970. http://dx.doi.org/10.3390/cryst13060970.

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A study was performed on the growth interface of a large-diameter 1 at% neodymium-doped yttrium aluminum garnet (Nd:YAG) single crystal grown using the Czochralski method. Red parallel light and an orthogonal polarizing system were used to observe the distribution of the central and lateral cores of the crystal at different growth interfaces. The solid–liquid interface of large-diameter Nd:YAG crystal growth was mainly determined via the interaction between natural and forced convection. The shape of the solid–liquid interface was mainly controlled via maintaining the crystal rotation rate and

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Weinhardt, L., M. Blum, O. Fuchs, et al. "RIXS investigations of liquids, solutions, and liquid/solid interfaces." Journal of Electron Spectroscopy and Related Phenomena 188 (June 2013): 111–20. http://dx.doi.org/10.1016/j.elspec.2012.10.006.

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Yan, Shuo, Ali Merati, Chae-Ho Yim, Elena Baranova, Arnaud Weck, and Yaser Abu-Lebdeh. "Understanding the Role of Liquid Electrolytes in Performance Improvement of Solid-State Lithium Metal Batteries." ECS Meeting Abstracts MA2022-01, no. 4 (2022): 551. http://dx.doi.org/10.1149/ma2022-014551mtgabs.

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Abstract Garnet-type Li7La3Zr2O12 (LLZO) Solid-State Electrolytes (SSEs) enable Solid-State Lithium Metal Batteries (SSLMBs) with high power density due to their superior ionic conductivity over 1 mS cm-1 at room temperature and good chemical stability against Lithium (Li) metal. A major cause of failure in SSLMBs is the large interfacial resistance between LLZO and electrodes. The high resistance at the interfaces is normally associated with insufficient solid-solid surface contact. It is a common practice to introduce a Liquid Electrolyte (LE) in SSLMBs either in combination with SSEs to for

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Sun, Zhouting, Mingyi Liu, Yong Zhu, et al. "Issues Concerning Interfaces with Inorganic Solid Electrolytes in All-Solid-State Lithium Metal Batteries." Sustainability 14, no. 15 (2022): 9090. http://dx.doi.org/10.3390/su14159090.

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All-solid-state batteries have attracted wide attention for high-performance and safe batteries. The combination of solid electrolytes and lithium metal anodes makes high-energy batteries practical for next-generation high-performance devices. However, when a solid electrolyte replaces the liquid electrolyte, many different interface/interphase issues have arisen from the contact with electrodes. Poor wettability and unstable chemical/electrochemical reaction at the interfaces with lithium metal anodes will lead to poor lithium diffusion kinetics and combustion of fresh lithium and active mate

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Nishi, Naoya, Naohiro Yoshida, Yishan Zhou, Yuko Yokoyama, and Tetsuo Sakka. "Electroless Deposition of Base Metals at the Liquid/Liquid Interface of Ionic Liquids." ECS Meeting Abstracts MA2023-02, no. 56 (2023): 2714. http://dx.doi.org/10.1149/ma2023-02562714mtgabs.

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Metal nanostructures can be formed at the electrochemical liquid/liquid interface, so-called ITIES. Our group has presented a method to form metal nanostructures at the liquid/liquid interface between ionic liquid (IL) and water (W) [1-10]. This IL/W method utilizes the spatial selectivity of the reaction site only at the liquid/liquid interface, which is achieved by the separation of metal precursor ions dissolved in the W phase and reducing agent in the IL phase. The metal reduction reaction is regarded as the electron transfer across the IL/W interface, which enables us to analyze the react

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Cucinotta, Clotilde S. "(Invited) Towards a Realistic Modelling of Solid-Liquid Interfaces." ECS Meeting Abstracts MA2023-01, no. 30 (2023): 1806. http://dx.doi.org/10.1149/ma2023-01301806mtgabs.

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In this talk I will introduce some issues connected with the simulation of electrified interfaces at the nanoscale focusing on simulating the effect of an applied potential to an electrode, using realistic models for the charged electrode electrolyte interface. I will present some recent progress in the simulation of the double layer of fundamental solid liquid interfaces of interest for corrosion and water splitting, and its response to changes of potential applied to the cell [1]; this is obtained applying a general ab initio electrode-charging approach we developed. [1] R. Khatib, A. Kumar,

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Zhang, Han Long, Yan Feng Han, Jun Wang, Yong Bing Dai, and Bao De Sun. "Grain Refinement Mechanism of Al-5Ti-1B Master Alloy by Ab Initio Calculations." Materials Science Forum 794-796 (June 2014): 746–51. http://dx.doi.org/10.4028/www.scientific.net/msf.794-796.746.

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To exactly understand the grain refining mechanism of α-Al by the Al-5Ti-1B master alloy, the structural properties of α-Al/solid-TiB2(S/S) and liquid-Al/solid-TiB2(L/S) interfaces were studied using the first-principles method. Different ordered structures were formed on the interfaces with different terminations of TiB2(0001) surface, which determines the nucleant potency of TiB2. The heterogeneous nucleation of α-Al on the B-terminated surface is frustrated by an AlB2-like structure formed at the interface. In contrast, a five-layer quasi-solid region with stacking sequence of fcc-Al (111)

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