Academic literature on the topic 'Hyperfine decoherence'

Using a simple model of central spin interacting with a spin bath, we study the decoherence of single electron spin states in quantum dots within one-, two- and three-dimensional nanostructure geometries. We consider a one-component hyperfine interaction term and express its strength as a smooth function of position vector. Decoherence measures are evaluated and plotted for various initial states, and we notice a decrease in decoherence time with the reduction of spin-bath dimension.

We investigate in this paper the dynamics of entanglement between a QD spin qubit and a single photon qubit inside a quantum network node, as well as its robustness against various decoherence processes. First, the entanglement dynamics is considered without decoherence. In the small detuning regime (Δ=78 μeV), there are three different conditions for maximum entanglement, which occur after 71, 93, and 116 picoseconds of interaction time. In the large detuning regime (Δ=1.5 meV), there is only one peak for maximum entanglement occurring at 625 picoseconds. Second, the entanglement dynamics is considered with decoherence by including the effects of spin-nucleus and hole-nucleus hyperfine interactions. In the small detuning regime, a decent amount of entanglement (35% entanglement) can only be obtained within 200 picoseconds of interaction. Afterward, all entanglement is lost. In the large detuning regime, a smaller amount of entanglement is realized, namely, 25%. And, it lasts only within the first 300 picoseconds.

The many-body dynamics of an electron spin−1/2 qubit coupled to a bath of nuclear spins by hyperfine interactions, as described by the central spin model in two kinds of external field, are studied in this paper. In a completely polarized bath, we use the state recurrence method to obtain the exact solution of the X X Z central spin model in a constant magnetic field and numerically analyze the influence of the disorder strength of the magnetic field on fidelity and entanglement entropy. For a constant magnetic field, the fidelity presents non-attenuating oscillations. The anisotropic parameter λ and the magnetic field strength B significantly affect the dynamic behaviour of the central spin. Unlike the periodic oscillation in the constant magnetic field, the decoherence dynamics of the central spin act like a damping oscillation in a disordered field, where the central spin undergoes a relaxation process and eventually reaches a stable state. The relaxation time of this process is affected by the disorder strength and the anisotropic parameter, where a larger anisotropic parameter or disorder strength can speed up the relaxation process. Compared with the constant magnetic field, the disordered field can regulate the decoherence over a large range, independent of the anisotropic parameter.

A viable qubit must have a long coherence time T 2 . In molecular nanomagnets, T 2 is often limited at low temperatures by the presence of dipole and hyperfine interactions, which are often mitigated through sample dilution, chemical engineering and isotope substitution in synthesis. Atomic-clock transitions offer another route to reducing decoherence from environmental fields by reducing the effective susceptibility of the working transition to field fluctuations. The Cr7Mn molecular nanomagnet, a heterometallic ring, features a clock transition at zero field. Both continuous-wave and spin-echo electron-spin resonance experiments on Cr7Mn samples, diluted via co-crystallization, show evidence of the effects of the clock transition with a maximum T 2 ∼ 390 ns at 1.8 K. We discuss improvements to the experiment that may increase T 2 further.

We have investigated with the pulsed ESR technique at X- and Q-band frequencies the coherence and relaxation of Cu spins S = 1/2 in single crystals of diamagnetically diluted mononuclear [n-Bu4N]2[Cu(opba)] (1%) in the host lattice of [n-Bu4N]2[Ni(opba)] (99%, opba = o-phenylenebis(oxamato)) and of diamagnetically diluted mononuclear [n-Bu4N]2[Cu(opbon-Pr2)] (1%) in the host lattice of [n-Bu4N]2[Ni(opbon-Pr2)] (99%, opbon-Pr2 = o-phenylenebis(N(propyl)oxamidato)). For that we have measured the electron spin dephasing time T m at different temperatures with the two-pulse primary echo and with the special Carr–Purcell–Meiboom–Gill (CPMG) multiple microwave pulse sequence. Application of the CPMG protocol has led to a substantial increase of the spin coherence lifetime in both complexes as compared to the primary echo results. It shows the efficiency of the suppression of the electron spin decoherence channel in the studied complexes arising due to spectral diffusion induced by a random modulation of the hyperfine interaction with the nuclear spins. We argue that this method can be used as a test for the relevance of the spectral diffusion for the electron spin decoherence. Our results have revealed a prominent role of the opba4– and opbon-Pr2 4– ligands for the dephasing of the Cu spins. The presence of additional 14N nuclei and protons in [Cu(opbon-Pr2)]2– as compared to [Cu(opba)]2– yields significantly shorter T m times. Such a detrimental effect of the opbon-Pr2 4− ligands has to be considered when discussing a potential application of the Cu(II)−(bis)oxamato and Cu(II)−(bis)oxamidato complexes as building blocks of more complex molecular structures in prototype spintronic devices. Furthermore, in our work we propose an improved CPMG pulse protocol that enables elimination of unwanted echoes that inevitably appear in the case of inhomogeneously broadened ESR spectra due to the selective excitation of electron spins.

Abstract The fidelity of the gate operation and the coherence time of neutral atoms trapped in an optical dipole trap are figures of merit for the applications. The motion of the trapped atom is one of the key factors which influence the gate fidelity and coherence time. However, it has been considered as a classical oscillator in analysis of the coherence time. Here we treat the motion as a quantum oscillator, and the population on the vibrational states of the atom are taken into account in analyzing the gate fidelity and decoherence. We show that the fidelity of a coherent rotation gate between two hyperfine states is dramatically limited by the population distribution on the vibrational states. We also find that the description of the decoherence caused by the previously regarded inhomogeneous dephasing due to the thermal motion of the atom is actually homogeneous in a quantum view. The phase between the two hyperfine states is still preserved on different vibrational states, and the observed interference fringe will recover naturally if the differential frequency shift is stable and the vibrational states do not change. The decoherence due to the fluctuations of the trap laser intensity is also discussed. Both the gate fidelity and coherence time can be dramatically enhanced by cooling the atom into vibrational ground states and/or by using a blue-detuned trap. More importantly, we propose a ``magic'' trapping condition by preparing the atom into specific vibrational states.

[Mathematical symbols can be only approximated here. For the correct display see the Abstract in the PDF files linked below] This work has demonstrated that hyperfine decoherence times sufficiently long for QIP and quantum optics applications are achievable in rare earth ion centres. Prior to this work there were several QIP proposals using rare earth hyperfine states for long term coherent storage of optical interactions [1, 2, 3]. The very long T_1 (~weeks [4]) observed for rare-earth hyperfine transitions appears promising but hyperfine T_2s were only a few ms, comparable to rare earth optical transitions and therefore the usefulness of such proposals was doubtful. ¶ This work demonstrated an increase in hyperfine T_2 by a factor of 7 × 10^4 compared to the previously reported hyperfine T_2 for Pr^[3+]:Y_2SiO_5 through the application of static and dynamic magnetic field techniques. This increase in T_2 makes previous QIP proposals useful and provides the first solid state optically active Lamda system with very long hyperfine T_2 for quantum optics applications. ¶ The first technique employed the conventional wisdom of applying a small static magnetic field to minimise the superhyperfine interaction [5, 6, 7], as studied in chapter 4. This resulted in hyperfine transition T_2 an order of magnitude larger than the T_2 of optical transitions, ranging fro 5 to 10 ms. The increase in T_2 was not sufficient and consequently other approaches were required. ¶ Development of the critical point technique during this work was crucial to achieving further gains in T_2. The critical point technique is the application of a static magnetic field such that the Zeeman shift of the hyperfine transition of interest has no first order component, thereby nulling decohering magnetic interactions to first order. This technique also represents a global minimum for back action of the Y spin bath due to a change in the Pr spin state, allowing the assumption that the Pr ion is surrounded by a thermal bath. The critical point technique resulted in a dramatic increase of the hyperfine transition T_2 from ~10 ms to 860 ms. ¶ Satisfied that the optimal static magnetic field configuration for increasing T_2 had been achieved, dynamic magnetic field techniques, driving either the system of interest or spin bath were investigated. These techniques are broadly classed as Dynamic Decoherence Control (DDC) in the QIP community. The first DDC technique investigated was driving the Pr ion using a CPMG or Bang Bang decoupling pulse sequence. This significantly extended T_2 from 0.86 s to 70 s. This decoupling strategy has been extensively discussed for correcting phase errors in quantum computers [8, 9, 10, 11, 12, 13, 14, 15], with this work being the first application to solid state systems. ¶ Magic Angle Line Narrowing was used to investigate driving the spin bath to increase T_2. This experiment resulted in T_2 increasing from 0.84 s to 1.12 s. Both dynamic techniques introduce a periodic condition on when QIP operation can be performed without the qubits participating in the operation accumulating phase errors relative to the qubits not involved in the operation. ¶ Without using the critical point technique Dynamic Decoherence Control techniques such as the Bang Bang decoupling sequence and MALN are not useful due to the sensitivity of the Pr ion to magnetic field fluctuations. Critical point and DDC techniques are mutually beneficial since the critical point is most effective at removing high frequency perturbations while DDC techniques remove the low frequency perturbations. A further benefit of using the critical point technique is it allows changing the coupling to the spin bath without changing the spin bath dynamics. This was useful for discerning whether the limits are inherent to the DDC technique or are due to experimental limitations. ¶ Solid state systems exhibiting long T_2 are typically very specialised systems, such as 29Si dopants in an isotopically pure 28Si and therefore spin free host lattice [16]. These systems rely on on the purity of their environment to achieve long T_2. Despite possessing a long T_2, the spin system remain inherently sensitive to magnetic field fluctuations. In contrast, this work has demonstrated that decoherence times, sufficiently long to rival any solid state system [16], are achievable when the spin of interest is surrounded by a concentrated spin bath. Using the critical point technique results in a hyperfine state that is inherently insensitive to small magnetic field perturbations and therefore more robust for QIP applications.

This thesis describes theoretical and experimental work whose main aim is the development of techniques for using trapped ⁴³Ca⁺ ions for quantum information processing. I present a rate equations model of ⁴³Ca⁺, and compare it with experimental data. The model is then used to investigate and optimise an electron-shelving readout method from a ground-level hyperfine qubit. The process is robust against common experimental imperfections. A shelving fidelity of up to 99.97% is theoretically possible, taking 100 μs. The laser pulse sequence can be greatly simplified for only a small reduction in the fidelity. The simplified method is tested experimentally with fidelities up to 99.8%. The shelving procedure could be applied to other commonly-used species of ion qubit. An entangling two-qubit quantum controlled-phase gate was attempted between a ⁴⁰Ca⁺ and a ⁴³Ca⁺ ion. The experiment did not succeed due to frequent decrystallisation of the ion pair, and strong motional decoherence. The source of the problems was never identified despite significant experimental effort, and the decision was made to suspend the experiments and continue them in an improved ion trap which is under construction. A sequence of pi-pulses, inspired by the Hahn spin-echo, was derived that is capable of greatly reducing dephasing of any qubit. If the qubit precession frequency varies with time as an nth-order polynomial, an (n+1) pulse sequence is theoretically capable of perfectly cancelling the resulting phase error. The sequence is used on a 43Ca+ magnetic-field-sensitive hyperfine qubit, with 20 pulses increasing the coherence time by a factor of 75 compared to an experiment without any spin-echo. In our ambient noise environment the well-known Carr-Purcell-Meiboom-Gill dynamic-decoupling method was found to be comparably effective.

This work has demonstrated that hyperfine decoherence times sufficiently long for QIP and quantum optics applications are achievable in rare earth ion centres. Prior to this work there were several QIP proposals using rare earth hyperfine states for long term coherent storage of optical interactions. The very long T_1 (~weeks ) observed for rare-earth hyperfine transitions appears promising but hyperfine T_2s were only a few ms, comparable to rare earth optical transitions and therefore the usefulness of such proposals was doubtful. ¶ This work demonstrated an increase in hyperfine T_2 by a factor of 7 × 10^4 compared to the previously reported hyperfine T_2 for Pr^[3+]:Y_2SiO_5 through the application of static and dynamic magnetic field techniques. This increase in T_2 makes previous QIP proposals useful and provides the first solid state optically active Lamda system with very long hyperfine T_2 for quantum optics applications. ¶ ...

The discussion of the electron spin decoherence and relaxation phenomena via the hyperfine interaction with host lattice spins is presented here. The spin relaxation processes processes limit the conservation time of spin states as well as the response time of the spin system to external perturbations. The central spin model, where the spin of charge carrier interacts with the bath of nuclear spins, is formulated. We also present different methods to calculate the spin dynamics within this model. Simple but physically transparent semiclassical treatment where the nuclear spins are considered as largely static classical magnetic moments is followed by more advanced quantum mechanical approach where the feedback of electron spin dynamics on the nuclei is taken into account. The chapter concludes with an overview of experimental data and its comparison with model calculations.

In recent years, the physics community has experienced a revival of interest in spin effects in solid state systems. On one hand, solid state systems, particularly semicon- ductors and semiconductor nanosystems, allow one to perform benchtop studies of quantum and relativistic phenomena. On the other hand, interest is supported by the prospects of realizing spin-based electronics where the electron or nuclear spins can play a role of quantum or classical information carriers. This book aims at rather detailed presentation of multifaceted physics of interacting electron and nuclear spins in semiconductors and, particularly, in semiconductor-based low-dimensional structures. The hyperfine interaction of the charge carrier and nuclear spins increases in nanosystems compared with bulk materials due to localization of electrons and holes and results in the spin exchange between these two systems. It gives rise to beautiful and complex physics occurring in the manybody and nonlinear system of electrons and nuclei in semiconductor nanosystems. As a result, an understanding of the intertwined spin systems of electrons and nuclei is crucial for in-depth studying and control of spin phenomena in semiconductors. The book addresses a number of the most prominent effects taking place in semiconductor nanosystems including hyperfine interaction, nuclear magnetic resonance, dynamical nuclear polarization, spin-Faraday and -Kerr effects, processes of electron spin decoherence and relaxation, effects of electron spin precession mode-locking and frequency focusing, as well as fluctuations of electron and nuclear spins.