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Journal articles on the topic 'Formic acid decomposition'

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Author: Grafiati

Published: 10 December 2022

Last updated: 28 January 2023

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1

McBreen, P. H., S. Serghini-Monim, D. Roy, and A. Adnot. "Decomposition of formic acid on FeTi." Surface Science 195, no. 3 (January 1988): L208—L216. http://dx.doi.org/10.1016/0039-6028(88)90345-7.

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2

Gercher, Victoria A., and David F. Cox. "Formic acid decomposition on SnO2(110)." Surface Science 312, no. 1-2 (June 1994): 106–14. http://dx.doi.org/10.1016/0039-6028(94)90807-9.

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3

Li, Fumin, Qi Xue, Ge Ma, Shuni Li, Mancheng Hu, Hongchang Yao, Xin Wang, and Yu Chen. "Formic acid decomposition-inhibited intermetallic Pd3Sn2 nanonetworks for efficient formic acid electrooxidation." Journal of Power Sources 450 (February 2020): 227615. http://dx.doi.org/10.1016/j.jpowsour.2019.227615.

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4

Lee, Hyun Ju, Dong-Chang Kang, Eun-Jeong Kim, Young-Woong Suh, Dong-Pyo Kim, Haksoo Han, and Hyung-Ki Min. "Production of H2-Free Carbon Monoxide from Formic Acid Dehydration: The Catalytic Role of Acid Sites in Sulfated Zirconia." Nanomaterials 12, no. 17 (September 1, 2022): 3036. http://dx.doi.org/10.3390/nano12173036.

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The formic acid (CH2O2) decomposition over sulfated zirconia (SZ) catalysts prepared under different synthesis conditions, such as calcination temperature (500–650 °C) and sulfate loading (0–20 wt.%), was investigated. Three sulfate species (tridentate, bridging bidentate, and pyrosulfate) on the SZ catalysts were characterized by using temperature-programmed decomposition (TPDE), Fourier-transform infrared spectroscopy (FTIR), and X-ray photoelectron spectroscopy (XPS). The acidic properties of the SZ catalysts were investigated by the temperature-programmed desorption of iso-propanol (IPA-TPD) and pyridine-adsorbed infrared (Py-IR) spectroscopy and correlated with their catalytic properties in formic acid decomposition. The relative contributions of Brønsted and Lewis acid sites to the formic acid dehydration were compared, and optimal synthetic conditions, such as calcination temperature and sulfate loading, were proposed.

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5

Zhang, Yongchun, Jun Zhang, Liang Zhao, and Changdong Sheng. "Decomposition of Formic Acid in Supercritical Water†." Energy & Fuels 24, no. 1 (January 21, 2010): 95–99. http://dx.doi.org/10.1021/ef9005093.

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6

Yu, Jianli, and Phillip E. Savage. "Decomposition of Formic Acid under Hydrothermal Conditions." Industrial & Engineering Chemistry Research 37, no. 1 (January 1998): 2–10. http://dx.doi.org/10.1021/ie970182e.

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7

Kupiainen, Laura, Juha Ahola, and Juha Tanskanen. "Kinetics of glucose decomposition in formic acid." Chemical Engineering Research and Design 89, no. 12 (December 2011): 2706–13. http://dx.doi.org/10.1016/j.cherd.2011.06.005.

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8

Akiya, Naoko, and Phillip E. Savage. "Role of water in formic acid decomposition." AIChE Journal 44, no. 2 (February 1998): 405–15. http://dx.doi.org/10.1002/aic.690440217.

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9

Rieckborn, Timo Paul, Elvira Huber, Emine Karakoc, and Marc Heinrich Prosenc. "Platinum Complex Catalyzed Decomposition of Formic Acid." European Journal of Inorganic Chemistry 2010, no. 30 (September 20, 2010): 4757–61. http://dx.doi.org/10.1002/ejic.201000879.

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10

Hafeez, Sanaa, Ilaria Barlocco, Sultan M. Al-Salem, Alberto Villa, Xiaowei Chen, Juan J. Delgado, George Manos, Nikolaos Dimitratos, and Achilleas Constantinou. "Experimental and Process Modelling Investigation of the Hydrogen Generation from Formic Acid Decomposition Using a Pd/Zn Catalyst." Applied Sciences 11, no. 18 (September 12, 2021): 8462. http://dx.doi.org/10.3390/app11188462.

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The use of hydrogen as a renewable fuel has attracted great attention in recent years. The decomposition of formic acid under mild conditions was investigated using a 2%Pd6Zn4 catalyst in a batch reactor. The results showed that the conversion of formic acid increases with reaction temperature and with the formic acid concentration. A process-simulation model was developed to predict the decomposition of formic acid using 2%Pd6Zn4 in a batch reactor. The model demonstrated very good validation with the experimental work. Further comparisons between the 2%Pd6Zn4 catalyst and a commercial Pd/C catalyst were carried out. It was found that the 2%Pd6Zn4 demonstrated significantly higher conversions when compared with the commercial catalyst.

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11

Alshammari, Hamed M., Mohammad Hayal Alotaibi, Obaid F. Aldosari, Abdulellah S. Alsolami, Nuha A. Alotaibi, Yahya A. Alzahrani, Mosaed S. Alhumaimess, Raja L. Alotaibi, and Gamal A. El-Hiti. "A Process for Hydrogen Production from the Catalytic Decomposition of Formic Acid over Iridium—Palladium Nanoparticles." Materials 14, no. 12 (June 12, 2021): 3258. http://dx.doi.org/10.3390/ma14123258.

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The present study investigates a process for the selective production of hydrogen from the catalytic decomposition of formic acid in the presence of iridium and iridium–palladium nanoparticles under various conditions. It was found that a loading of 1 wt.% of 2% palladium in the presence of 1% iridium over activated charcoal led to a 43% conversion of formic acid to hydrogen at room temperature after 4 h. Increasing the temperature to 60 °C led to further decomposition and an improvement in conversion yield to 63%. Dilution of formic acid from 0.5 to 0.2 M improved the decomposition, reaching conversion to 81%. The reported process could potentially be used in commercial applications.

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12

Chesnokov, V. V., A. S. Lisitsyn, V. I. Sobolev, E. Yu Gerasimov, I. P. Prosvirin, Yu A. Chesalov, A. S. Chichkan, and O. Yu Podyacheva. "Decomposition of Formic Acid on Pt/N-Graphene." Kinetics and Catalysis 62, no. 4 (July 2021): 518–27. http://dx.doi.org/10.1134/s0023158421040017.

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13

Sander, D., and W. Erley. "The decomposition of formic acid on Pd(100)." Journal of Vacuum Science & Technology A: Vacuum, Surfaces, and Films 8, no. 4 (July 1990): 3357–60. http://dx.doi.org/10.1116/1.576553.

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14

Thomas, Fred S., and Richard I. Masel. "Formic acid decomposition on palladium-coated Pt(110)." Surface Science 573, no. 2 (December 2004): 169–75. http://dx.doi.org/10.1016/j.susc.2004.09.047.

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15

Zhao, Yan, Li Deng, Shi-Ya Tang, Da-Ming Lai, Bing Liao, Yao Fu, and Qing-Xiang Guo. "Selective Decomposition of Formic Acid over Immobilized Catalysts." Energy & Fuels 25, no. 8 (August 18, 2011): 3693–97. http://dx.doi.org/10.1021/ef200648s.

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16

Bjerre, Anne Belinda, and Emil Soerensen. "Thermal decomposition of dilute aqueous formic acid solutions." Industrial & Engineering Chemistry Research 31, no. 6 (June 1992): 1574–77. http://dx.doi.org/10.1021/ie00006a022.

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17

Borowiak, Marek A., Michał H. Jamróz, and Ragnar Larsson. "Catalytic decomposition of formic acid on oxide catalysts." Journal of Molecular Catalysis A: Chemical 152, no. 1-2 (March 2000): 121–32. http://dx.doi.org/10.1016/s1381-1169(99)00271-x.

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18

Parandaman, Arathala, Josue E. Perez, and Amitabha Sinha. "Atmospheric Decomposition of Trifluoromethanol Catalyzed by Formic Acid." Journal of Physical Chemistry A 122, no. 49 (November 14, 2018): 9553–62. http://dx.doi.org/10.1021/acs.jpca.8b09316.

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19

Iglesia, Enrique. "Unimolecular and bimolecular formic acid decomposition on copper." Journal of Physical Chemistry 90, no. 21 (October 1986): 5272–74. http://dx.doi.org/10.1021/j100412a074.

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20

SOLYMOSI, F. "Decomposition of formic acid on supported Rh catalysts." Journal of Catalysis 91, no. 2 (February 1985): 327–37. http://dx.doi.org/10.1016/0021-9517(85)90346-x.

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21

Kisfaludi, G., K. Matusek, Z. Schay, L. Guczi, and A. Lovas. "Decomposition of formic acid on Fe80B20 metallic glasses." Materials Science and Engineering 99, no. 1-2 (March 1988): 547–49. http://dx.doi.org/10.1016/0025-5416(88)90395-3.

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22

Machado, Gladson de Souza, Eduardo Monteiro Martins, Leonardo Baptista, and Glauco Favilla Bauerfeldt. "Theoretical investigation of the formic acid decomposition kinetics." International Journal of Chemical Kinetics 52, no. 3 (December 22, 2019): 188–96. http://dx.doi.org/10.1002/kin.21341.

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23

Raeva, V. M., and O. V. Gromova. "Separation of water – formic acid – acetic acid mixtures in the presence of sulfolane." Fine Chemical Technologies 14, no. 4 (September 15, 2019): 24–32. http://dx.doi.org/10.32362/2410-6593-2019-14-4-24-32.

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In this paper, extractive distillation flowsheets for water–formic acid–acetic acid mixtures were designed. Flowsheets not involving preliminary dehydration were considered, and the relative volatilities of the components in the presence of sulfolane were analyzed. The result of extractive distillation depends on the amount of sulfolane. The structure of the flowsheet is determined by the results of the basic ternary mixture extractive distillation. In three-column flowsheets (schemes I, II), water is isolated in the distillate of the extractive distillation column. In the second column, distillation of the formic acid–acetic acid–sulfolane mixture is carried out, yielding formic acid (90 wt %) and acetic acid (80 wt %). The recycled flow is returned to the first column. Dilution of the formic acid–acetic acid–sulfolane mixture with sulfolane (second column of flowsheet II) allows for acids of higher quality (main substance content equal to or more than 98.5 wt %) to be obtained. Flowsheet III includes four columns and two recycling stages. First, the water–formic acid mixture is isolated in the distillate of the extractive distillation column. Then, water and formic acid are separated in a two-column complex by extractive distillation, also with sulfolane. We were carrying out calculations for column working pressure 101.32 and 13.33 kPa. To prevent thermal decomposition of sulfolane, working pressure for regeneration columns was always 13.33 kPa. The extractive distillation column of the basic three-component mixture is the main factor contributing to the total energy consumption for separation (in all schemes).

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24

Wolf, Mark E., Justin M. Turney, and Henry F. Schaefer. "High level ab initio investigation of the catalytic effect of water on formic acid decomposition and isomerization." Physical Chemistry Chemical Physics 22, no. 44 (2020): 25638–51. http://dx.doi.org/10.1039/d0cp03796f.

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25

Pechenkin, Alexey, Sukhe Badmaev, Vladimir Belyaev, and Vladimir Sobyanin. "Production of Hydrogen-Rich Gas by Formic Acid Decomposition over CuO-CeO2/γ-Al2O3 Catalyst." Energies 12, no. 18 (September 19, 2019): 3577. http://dx.doi.org/10.3390/en12183577.

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Formic acid decomposition to H2-rich gas was investigated over a CuO-CeO2/γ-Al2O3 catalyst. The catalyst was characterized by XRD, HR TEM and EDX methods. A 100% conversion of formic acid was observed over the copper-ceria catalyst under ambient pressure, at 200–300 °C, N2:HCOOH = 75:25 vol.% and flow rate 3500–35,000 h−1 with H2 yield of 98%, wherein outlet CO concentration is below the equilibrium data (<0.5 vol.%). The copper-ceria catalyst proved to be promising for multifuel processor application, and the H2 generation from dimethoxymethane, methanol, dimethyl ether and formic acid on the same catalyst for fuel cell supply.

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26

Che Abdul Rahim, Azzah Nazihah, Shotaro Yamada, Haruki Bonkohara, Sergio Mestre, Tsuyoshi Imai, Yung-Tse Hung, and Izumi Kumakiri. "Influence of Salts on the Photocatalytic Degradation of Formic Acid in Wastewater." International Journal of Environmental Research and Public Health 19, no. 23 (November 26, 2022): 15736. http://dx.doi.org/10.3390/ijerph192315736.

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Conventional wastewater treatment technologies have difficulties in feasibly removing persistent organics. The photocatalytic oxidation of these contaminants offers an economical and environmentally friendly solution. In this study, TiO2 membranes and Ag/TiO2 membranes were prepared and used for the decomposition of dissolved formic acid in wastewater. The photochemical deposition of silver on a TiO2 membrane improved the decomposition rate. The rate doubled by depositing ca. 2.5 mg of Ag per 1 g of TiO2. The influence of salinity on formic acid decomposition was studied. The presence of inorganic salts reduced the treatment performance of the TiO2 membranes to half. Ag/TiO2 membranes had a larger reduction of ca. 40%. The performance was recovered by washing the membranes with water. The anion adsorption on the membrane surface likely caused the performance reduction.

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27

Sims, Jeffrey J., Cherif Aghiles Ould Hamou, Romain Réocreux, Carine Michel, and Javier B. Giorgi. "Adsorption and Decomposition of Formic Acid on Cobalt(0001)." Journal of Physical Chemistry C 122, no. 35 (August 14, 2018): 20279–88. http://dx.doi.org/10.1021/acs.jpcc.8b04751.

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28

Chen, Benjamin W. J., and Manos Mavrikakis. "Formic Acid: A Hydrogen-Bonding Cocatalyst for Formate Decomposition." ACS Catalysis 10, no. 19 (August 26, 2020): 10812–25. http://dx.doi.org/10.1021/acscatal.0c02902.

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29

Ida, Tomonori, Manami Nishida, and Yuta Hori. "Revisiting Formic Acid Decomposition by a Graph-Theoretical Approach." Journal of Physical Chemistry A 123, no. 44 (October 18, 2019): 9579–86. http://dx.doi.org/10.1021/acs.jpca.9b05994.

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30

Haq, S., J. G. Love, H. E. Sanders, and D. A. King. "Adsorption and decomposition of formic acid on Ni{110}." Surface Science 325, no. 3 (March 1995): 230–42. http://dx.doi.org/10.1016/0039-6028(94)00694-6.

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31

Gao, Yuan, Joshi Kuncheria, Richard J. Puddephatt, and Glenn P. A. Yap. "An efficient binuclear catalyst for decomposition of formic acid." Chemical Communications, no. 21 (1998): 2365–66. http://dx.doi.org/10.1039/a805789c.

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32

Popova, G. Ya, I. I. Zakharov, and T. V. Andrushkevich. "Mechanism of formic acid decomposition on P−Mo heteropolyacid." Reaction Kinetics and Catalysis Letters 66, no. 2 (March 1999): 251–56. http://dx.doi.org/10.1007/bf02475798.

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33

Wang, Xian, Qinglei Meng, Liqin Gao, Zhao Jin, Junjie Ge, Changpeng Liu, and Wei Xing. "Recent progress in hydrogen production from formic acid decomposition." International Journal of Hydrogen Energy 43, no. 14 (April 2018): 7055–71. http://dx.doi.org/10.1016/j.ijhydene.2018.02.146.

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34

Malinowski, Marek, Krystyna Malinowska, and Leon Wiesław Zatorski. "The catalytic decomposition of formic acid into carbon monoxide." Bulletin des Sociétés Chimiques Belges 92, no. 3 (September 1, 2010): 225–27. http://dx.doi.org/10.1002/bscb.19830920304.

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35

Halasi, Gyula, Tamás Bánsági, Erika Varga, and Frigyes Solymosi. "Photocatalytic Decomposition of Formic Acid on Mo2C-Containing Catalyst." Catalysis Letters 145, no. 3 (February 14, 2015): 875–80. http://dx.doi.org/10.1007/s10562-015-1494-7.

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36

He, Nan, and Zhen Hua Li. "Palladium-atom catalyzed formic acid decomposition and the switch of reaction mechanism with temperature." Physical Chemistry Chemical Physics 18, no. 15 (2016): 10005–17. http://dx.doi.org/10.1039/c6cp00186f.

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37

Lee, Jin-Yeon, Da-Hee Kwak, Young-Woo Lee, Seul Lee, and Kyung-Won Park. "Synthesis of cubic PtPd alloy nanoparticles as anode electrocatalysts for methanol and formic acid oxidation reactions." Physical Chemistry Chemical Physics 17, no. 14 (2015): 8642–48. http://dx.doi.org/10.1039/c5cp00892a.

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38

Li, Si-jia, Yun Ping, Jun-Min Yan, Hong-Li Wang, Ming Wu, and Qing Jiang. "Facile synthesis of AgAuPd/graphene with high performance for hydrogen generation from formic acid." Journal of Materials Chemistry A 3, no. 28 (2015): 14535–38. http://dx.doi.org/10.1039/c5ta03111g.

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39

Wang, Ying-Ying. "Theoretical study of the oxidation of formic acid on a PtPd(111) surface." Progress in Reaction Kinetics and Mechanism 44, no. 1 (February 2019): 67–73. http://dx.doi.org/10.1177/1468678319830512.

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By performing density functional theory calculations, the adsorption configurations of formic acid and possible reaction pathway for HCOOH oxidation on PtPd(111) surface are located. Results show that CO2 is preferentially formed as the main product of the catalytic oxidation of formic acid. The formation of CO on the pure Pd surface could not possibly occur during formic acid decomposition on the PtPd(111) surface owing to the high reaction barrier. Therefore, no poisoning of catalyst would occur on the PtPd(111) surface. Our results indicate that the significantly increased catalytic activity of bimetallic PtPd catalyst towards HCOOH oxidation should be attributed to the reduction in poisoning by CO.

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40

Kosider, Axel, Dominik Blaumeiser, Simon Schötz, Patrick Preuster, Andreas Bösmann, Peter Wasserscheid, Jörg Libuda, and Tanja Bauer. "Enhancing the feasibility of Pd/C-catalyzed formic acid decomposition for hydrogen generation – catalyst pretreatment, deactivation, and regeneration." Catalysis Science & Technology 11, no. 12 (2021): 4259–71. http://dx.doi.org/10.1039/d1cy00300c.

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41

Bulushev, Dmitri A. "Progress in Catalytic Hydrogen Production from Formic Acid over Supported Metal Complexes." Energies 14, no. 5 (March 1, 2021): 1334. http://dx.doi.org/10.3390/en14051334.

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Formic acid is a liquid organic hydrogen carrier giving hydrogen on demand using catalysts. Metal complexes are known to be used as efficient catalysts for the hydrogen production from formic acid decomposition. Their performance could be better than those of supported catalysts with metal nanoparticles. However, difficulties to separate metal complexes from the reaction mixture limit their industrial applications. This problem can be resolved by supporting metal complexes on the surface of different supports, which may additionally provide some surface sites for the formic acid activation. The review analyzes the literature on the application of supported metal complexes in the hydrogen production from formic acid. It shows that the catalytic activity of some stable Ru and Ir supported metal complexes may exceed the activity of homogeneous metal complexes used for deposition. Non-noble metal-based complexes containing Fe demonstrated sufficiently high performance in the reaction; however, they can be poisoned by water present in formic acid. The proposed review could be useful for development of novel catalysts for the hydrogen production.

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42

LUO, QIQUAN, MATTHIAS BELLER, and HAIJUN JIAO. "FORMIC ACID DEHYDROGENATION ON SURFACES — A REVIEW OF COMPUTATIONAL ASPECT." Journal of Theoretical and Computational Chemistry 12, no. 07 (November 2013): 1330001. http://dx.doi.org/10.1142/s0219633613300012.

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In this review, we have mainly shown the recent computational studies on formic acid adsorption and selective dissociation to produce hydrogen ( HCOOH → CO 2 + H 2) on several metal ( Pt , Pd , Ni , Cu , Rh and Au ) and metal oxide ( TiO 2, MgO , ZnO and NiO ) surfaces, and both thermal decomposition and electro-catalytic oxidation have been discussed. The decomposition mechanisms of formic acid have been studied by using different computational models and methods, not only interesting and exciting but also different and controversial results have been reported. It is noted that the model systems used in these studies are too simple and idealized, and they cannot represent the real catalysts or the catalytic systems, and more sophisticated computational methodologies and real model systems under the consideration of the working conditions are therefore needed.

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43

Chauvier, Clément, Anis Tlili, Christophe Das Neves Gomes, Pierre Thuéry, and Thibault Cantat. "Metal-free dehydrogenation of formic acid to H2 and CO2 using boron-based catalysts." Chemical Science 6, no. 5 (2015): 2938–42. http://dx.doi.org/10.1039/c5sc00394f.

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44

Hattori, Masashi, Hisahiro Einaga, Takeshi Daio, and Masaharu Tsuji. "Efficient hydrogen production from formic acid using TiO2-supported AgPd@Pd nanocatalysts." Journal of Materials Chemistry A 3, no. 8 (2015): 4453–61. http://dx.doi.org/10.1039/c4ta06988a.

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45

Tsuji, Masaharu, Daisuke Shimamoto, Keiko Uto, Masashi Hattori, and Hiroki Ago. "Enhancement of catalytic activity of AgPd@Pd/TiO2 nanoparticles under UV and visible photoirradiation." Journal of Materials Chemistry A 4, no. 38 (2016): 14649–56. http://dx.doi.org/10.1039/c6ta05699g.

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46

Liu, Xin, Timo Jacob, and Wang Gao. "Progress of fundamental mechanism of formic acid decomposition and electrooxidation." Journal of Energy Chemistry 70 (July 2022): 292–309. http://dx.doi.org/10.1016/j.jechem.2022.02.017.

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47

Wang, Baoshan, Hua Hou, and Yueshu Gu. "New Mechanism for the Catalyzed Thermal Decomposition of Formic Acid†." Journal of Physical Chemistry A 104, no. 45 (November 2000): 10526–28. http://dx.doi.org/10.1021/jp001173d.

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48

Lu, Guo-Qiang, Alechia Crown, and Andrzej Wieckowski. "Formic Acid Decomposition on Polycrystalline Platinum and Palladized Platinum Electrodes." Journal of Physical Chemistry B 103, no. 44 (November 1999): 9700–9711. http://dx.doi.org/10.1021/jp992297x.

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49

Sun, Y. ‐K, and W. H. Weinberg. "Catalytic decomposition of formic acid on Ru(001): Transient measurements." Journal of Chemical Physics 94, no. 6 (March 15, 1991): 4587–99. http://dx.doi.org/10.1063/1.460587.

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50

Yoo, Jong Suk, Frank Abild-Pedersen, Jens K. Nørskov, and Felix Studt. "Theoretical Analysis of Transition-Metal Catalysts for Formic Acid Decomposition." ACS Catalysis 4, no. 4 (March 24, 2014): 1226–33. http://dx.doi.org/10.1021/cs400664z.

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