Journal articles on the topic 'Dust plumes'
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1
Li, Wenshuai, Wencai Wang, Yang Zhou, Yuanyuan Ma, Daizhou Zhang, and Lifang Sheng. "Occurrence and Reverse Transport of Severe Dust Storms Associated with Synoptic Weather in East Asia." Atmosphere 10, no. 1 (December 24, 2018): 4. http://dx.doi.org/10.3390/atmos10010004.
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The range and time of the environmental effects of Asian dust are closely dependent on the pathways and the speed of dust plume movement. In this study, the occurrence and movement of two dust storms in China in May 2017 were examined by using open space- and ground-based measurement data and the backward trajectories of dust plumes. Results from the European Centre for Medium-Range Weather Forecasts (ECMWF) reanalysis data showed that the dust storms were caused by the rapid coupling development of Mongolian cyclones and Asian highs. After the dust plumes arrived at the Southeastern China in the first dust event, the stable weather conditions and the Asian high slowed down the movement of the plumes, leading to the gradual diffusion of dust particles. Moreover, the Asian high in the first event and the Huabei low (a low-pressure system in North China Plain) in the second altered the movement direction of the dust plumes from southward to northward, which we denote as the “dust reverse transport (DRT)”. The DRT occurred only within the lower troposphere even though dust plumes could extended to 5–10 km in vertical direction. Statistical results of 28 spring dust events occurred in 2015–2018 showed that all these dust storms were triggered by Mongolian cyclones and/or Asian highs, and approximately 39% moved as the DRT, indicating about one third of severe spring dust storms could influence larger areas or longer time than the remained ones.
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Jones, Thomas A., and Sundar A. Christopher. "Satellite and Radar Remote Sensing of Southern Plains Grass Fires: A Case Study." Journal of Applied Meteorology and Climatology 49, no. 10 (October 1, 2010): 2133–46. http://dx.doi.org/10.1175/2010jamc2472.1.
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Abstract Many large grass fires occurred in north Texas and southern Oklahoma on 9 April 2009, destroying hundreds of homes and businesses and burning thousands of acres of grasslands, producing large smoke and debris plumes that were visible from various remote sensing platforms. At the same time, strong westerly winds were transporting large amounts of dust into the region, mixing with the smoke and debris already being generated. This research uses surface- and satellite-based remote sensing observations of this event to assess the locations of fires and the spatial distribution of smoke and dust aerosols. The authors present a unique perspective by analyzing radar observations of fire debris in conjunction with the satellite analysis of submicrometer smoke aerosol particles. Satellite data clearly show the location of the individual fires and the downwind smoke plumes as well as the large dust storm present over the region. In particular, Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol optical thickness at 0.55 μm within the dust plume was around 0.5, and it increased to greater than 1.0 when combined with smoke. Using the difference in 11- versus 12-μm brightness temperature data combined with surface observations, the large extent of the dust plume was evident through much of north-central Texas, where visibilities were low and the 11–12-μm brightness temperature difference was negative. Conversely, smoke plumes were characterized by higher reflectance at 0.6 μm (visible wavelength). Cross sections of radar data through the several smoke and debris plumes indicated the burnt debris reached up to 5 km into the atmosphere. Plume height output from modified severe storm algorithms produced similar values. Since smoke aerosols are smaller and lighter when compared with the debris, they were likely being transported even higher into the atmosphere. These results show that the combination of satellite and radar data offers a unique perspective on observing the characteristics and evolution of smoke and debris plume emanating from grass fire events.
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Southworth, B. S., S. Kempf, and J. Schmidt. "Modeling Europa's dust plumes." Geophysical Research Letters 42, no. 24 (December 28, 2015): 10,541–10,548. http://dx.doi.org/10.1002/2015gl066502.
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Popel, S. I., and A. A. Gisko. "Charged dust and shock phenomena in the Solar System." Nonlinear Processes in Geophysics 13, no. 2 (June 21, 2006): 223–29. http://dx.doi.org/10.5194/npg-13-223-2006.
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Abstract. The results on shock phenomena in dusty plasmas of the Solar System are reviewed. The problems of dust ion acoustic bow shock in interaction of the solar wind with dusty cometary coma and formation of transient atmospheres of atmosphereless cosmic bodies such as Moon, Mercury, asteroids and comets are considered. The latter assumes the evolution of meteoroid impact plumes and production of charged dust grains due to the condensation of both the plume substance and the vapor thrown from the crater and the surrounding regolith layer. Physical phenomena occurring during large meteoroid impacts can be modeled with the aid of active rocket experiments, which involve the release of some gaseous substance in near-Earth space. New vistas in investigation of shock processes in natural dusty plasmas are determined.
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Córdoba-Jabonero, C., M. Sorribas, J. L. Guerrero-Rascado, J. A. Adame, Y. Hernández, H. Lyamani, V. Cachorro, et al. "Synergetic monitoring of Saharan dust plumes and potential impact on surface: a case study of dust transport from Canary Islands to Iberian Peninsula." Atmospheric Chemistry and Physics Discussions 10, no. 11 (November 9, 2010): 27015–74. http://dx.doi.org/10.5194/acpd-10-27015-2010.
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Abstract. Synergetic use of meteorological information, remote sensing both ground-based active (lidar) and passive (sun-photometry) techniques together with backtrajectory analysis and in situ measurements is carried out for the characterization of dust intrusions. A case study of air masses advected from Saharan region to the Canary Islands and the Iberian Peninsula, relatively located close and far away from the dust sources, respectively, was monitored from 11 to 19 March 2008. The observations were performed over three Spanish geographically strategic within the dust-influenced area stations along a common dust plume pathway. A 4-day long dust event (13–16 March) over the Santa Cruz de Tenerife Observatory (SCO), and a linked short 1-day dust episode (14 March) in the Southern Iberian Peninsula over both the Atmospheric Sounding Station "El Arenosillo" (ARN) and the Granada station (GRA) were detected. Meteorological situation favoured the dust plume transport over the area under study. Backtrajectory analysis clearly showed the Saharan origin of the dust intrusion. Under the Saharan air masses influence, AERONET Aerosol Optical Depth at 500 nm (AOD500) ranged from 0.3 to 0.6 and Angstrom Exponent at 440/675 nm wavelength pair (AE440/675) was lower than 0.5, indicating a high loading and predominance of coarse particles during those dusty events. Lidar observations characterized their vertical layering structure, identifying different aerosol contributions depending on altitude. In particular, the 3-km height layer observed over ARN and GRA stations corresponds to that dust plume transported from Saharan region after crossing through Canary Islands at 3 km height as observed over SCO site as well. No significant differences were found in the lidar (extinction-to-backscatter) ratio (LR) estimation for that dust plume over all stations when a suitable aerosol scenario for lidar data retrieval is selected. Lidar-retrieved LR values of 65–70 sr were obtained during the principal dusty episodes. These similar LR values found in all the stations suggest that dust properties were kept unchanged in the course of its medium-range transport. In addition, the potential impact on surface of that Saharan dust intrusion over the Iberian Peninsula was evaluated by ground-level in situ measurements for particle deposition assessment together with backtrajectory analysis. However, no connection between those dust plumes and the particle sedimentation registered at ground level is found. Differences on particle deposition process observed in both Southern Iberian Peninsula sites are due to the particular dust transport pattern occurred in each station.
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Shin, S. K., D. Müller, K. H. Lee, D. Shin, Y. J. Kim, and Y. M. Noh. "Vertical variation of optical properties of mixed Asian dust/pollution plumes according to pathway of airmass transport over East Asia." Atmospheric Chemistry and Physics Discussions 15, no. 3 (February 6, 2015): 3381–413. http://dx.doi.org/10.5194/acpd-15-3381-2015.
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Abstract. We use five years (2009–2013) of multiwavelength Raman lidar measurements at Gwangju, Korea (35.10° N, 126.53° E) for the identification of changes of optical properties of East Asian dust in dependence of its transport path over China. Profiles of backscatter and extinction coefficients, lidar ratios, and backscatter-related Ångström exponents (wavelength pair 355/532 nm) were measured at Gwangju. Linear particle depolarization ratios were used to identify East Asian dust layers. We used backward trajectory modelling to identify the pathway and the vertical position of dust-laden air masses over China during long-range transport. Most cases of Asian dust events can be described by the emission of dust in desert areas and subsequent transport over highly polluted regions of China. The Asian dust plumes could be categorized into two classes according to the height above ground in which these plumes were transported: (I) the dust layers passed over China at high altitude levels until arrival over Gwangju, and (II) the Asian dust layers were transported near the surface and the lower troposphere over industrialized areas before they arrived over Gwangju. We find that the optical characteristics of these mixed Asian dust layers over Gwangju differ in dependence of their vertical position above ground over China and the change of height above ground during transport. The mean linear particle depolarization ratio was 0.21 ± 0.06 (at 532 nm), the mean lidar ratios were 52 ± 7 sr at 355 nm and 53 ± 8 sr at 532 nm, and the mean Ångström exponent was 0.74 ± 0.31 in case I. In contrast, plumes transported at lower altitudes (case II) showed low depolarization ratios, and higher lidar ratio and Ångström exponents. The mean linear particle depolarization ratio was 0.13 ± 0.04, the mean lidar ratios were 63 ± 9 sr at 355 nm and 62 ± 8 sr at 532 nm, respectively, and the mean Ångström exponent was 0.98 ± 0.51. These numbers show that the optical characteristics of mixed Asian plumes are more similar to optical characteristics of urban pollution. We find a decrease of the linear depolarization ratio of the mixed dust/pollution plume in dependence of transport time if the pollution layer travelled over China at low heights, i.e., below approximately 3 km above ground. In contrast we do not find such a trend if the dust plumes travelled at heights above 4 km over China. We need a longer time series of lidar measurements in order to determine the change of optical properties of dust with transport time in a quantitative way.
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Shin, S. K., D. Müller, C. Lee, K. H. Lee, D. Shin, Y. J. Kim, and Y. M. Noh. "Vertical variation of optical properties of mixed Asian dust/pollution plumes according to pathway of air mass transport over East Asia." Atmospheric Chemistry and Physics 15, no. 12 (June 17, 2015): 6707–20. http://dx.doi.org/10.5194/acp-15-6707-2015.
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Abstract. We use five years (2009–2013) of multiwavelength Raman lidar measurements at Gwangju, South Korea (35.10° N, 126.53° E) for the identification of changes of optical properties of East Asian dust depending on its transport path over China. Profiles of backscatter and extinction coefficients, lidar ratios, and backscatter-related Ångström exponents (wavelength pair 355/532 nm) were measured at Gwangju. Linear particle depolarization ratios were used to identify East Asian dust layers. We used backward trajectory modeling to identify the pathway and the vertical position of dust-laden air masses over China during long-range transport. Most cases of Asian dust events can be described by the emission of dust in desert areas and subsequent transport over highly polluted regions of China. The Asian dust plumes could be categorized into two classes according to the height above ground at which these plumes were transported: (case I) the dust layers passed over China at high altitude levels (> 3 km) until arrival over Gwangju, and (case II) the Asian dust layers were transported near the surface and within the lower troposphere (< 3 km) over industrialized areas before they arrived over Gwangju. We find that the optical characteristics of these mixed Asian dust layers over Gwangju differ depending on their vertical position above ground over China and the change of height above ground during transport. The mean linear particle depolarization ratio was 0.21 ± 0.06 (at 532 nm), the mean lidar ratios were 52 ± 7 sr at 355 nm and 53 ± 8 sr at 532 nm, and the mean Ångström exponent was 0.74 ± 0.31 for case I. In contrast, plumes transported at lower altitudes (case II) showed low depolarization ratios (0.13 ± 0.04 at 532 nm), and higher lidar ratio (63 ± 9 sr at 355 nm and 62 ± 8 sr at 532 nm) and Ångström exponents (0.98 ± 0.51). These numbers show that the optical characteristics of mixed Asian plumes are more similar to optical characteristics of urban pollution. We find a decrease of the linear depolarization ratio of the mixed dust/pollution plume depending on transport time if the pollution layer traveled over China at low heights, i.e., below approximately 3 km above ground. In contrast, we do not find such a trend if the dust plumes traveled at heights above 3 km over China. We need a longer time series of lidar measurements in order to determine in a quantitative way the change of optical properties of dust with transport time.
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Birmili, W., K. Schepanski, A. Ansmann, G. Spindler, I. Tegen, B. Wehner, A. Nowak, et al. "A case of extreme particulate matter concentrations over Central Europe caused by dust emitted over the southern Ukraine." Atmospheric Chemistry and Physics 8, no. 4 (February 26, 2008): 997–1016. http://dx.doi.org/10.5194/acp-8-997-2008.
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Abstract. On 24 March 2007, an extraordinary dust plume was observed in the Central European troposphere. Satellite observations revealed its origins in a dust storm in Southern Ukraine, where large amounts of soil were resuspended from dried-out farmlands at wind gusts up to 30 m s−1. Along the pathway of the plume, maximum particulate matter (PM10) mass concentrations between 200 and 1400 μg m−3 occurred in Slovakia, the Czech Republic, Poland, and Germany. Over Germany, the dust plume was characterised by a volume extinction coefficient up to 400 Mm−1 and a particle optical depth of 0.71 at wavelength 0.532 μm. In-situ size distribution measurements as well as the wavelength dependence of light extinction from lidar and Sun photometer measurements confirmed the presence of a coarse particle mode with diameters around 2–3 μm. Chemical particle analyses suggested a fraction of 75% crustal material in daily average PM10 and up to 85% in the coarser fraction PM10–2.5. Based on the particle characteristics as well as a lack of increased CO and CO2 levels, a significant impact of biomass burning was ruled out. The reasons for the high particle concentrations in the dust plume were twofold: First, dust was transported very rapidly into Central Europe in a boundary layer jet under dry conditions. Second, the dust plume was confined to a relatively stable boundary layer of 1.4–1.8 km height, and could therefore neither expand nor dilute efficiently. Our findings illustrate the capacity of combined in situ and remote sensing measurements to characterise large-scale dust plumes with a variety of aerosol parameters. Although such plumes from Southern Eurasia seem to occur rather infrequently in Central Europe, its unexpected features highlights the need to improve the description of dust emission, transport and transformation processes needs, particularly when facing the possible effects of further anthropogenic desertification and climate change.
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Kaskaoutis, D. G., A. K. Prasad, P. G. Kosmopoulos, P. R. Sinha, S. K. Kharol, P. Gupta, H. M. El-Askary, and M. Kafatos. "Synergistic Use of Remote Sensing and Modeling for Tracing Dust Storms in the Mediterranean." Advances in Meteorology 2012 (2012): 1–14. http://dx.doi.org/10.1155/2012/861026.
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This study focuses on the detection of the dust source region and monitoring of the transport of the dust plume from its primary outflow to final deposition. The application area is the Sahara desert and the eastern Mediterranean, where two dust events occurred during the period 4–6 February 2009, an unusual event for a winter period. The Aqua-MODIS and OMI observations clearly define the spatial distribution of the dust plumes, while the CALIPSO observations of total attenuated backscatter (TAB) at 532 nm, depolarization ratio (DR), and attenuated color ratio (1064/532 nm) on 5 February 2009 provide a clear view and vertical structure of the dust-laden layer. The dust source region is defined to be near the Chad-Niger-Libyan borders, using satellite observations and model (DREAM) output. This dust plume is vertically extended up to 2.5 km and is observed as a mass plume of dust from surface level to that altitude, where the vertical variation of TAB (0.002 to 0.2) and DR (0.2–0.5) implies dust-laden layer with non-spherical particles. CALIPSO profiles show that after the dust plume reached at its highest level, the dust particles start to be deposited over the Mediterranean and the initial dust plume was strongly attenuated, while features of dust were limited below about 1–1.5 km for latitudes northern of ~36° (Greek territory).
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Ben-Ami, Y., I. Koren, and O. Altaratz. "Patterns of North African dust transport over the Atlantic: winter vs. summer, based on CALIPSO first year data." Atmospheric Chemistry and Physics 9, no. 20 (October 20, 2009): 7867–75. http://dx.doi.org/10.5194/acp-9-7867-2009.
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Abstract. One of the most important factors that determine the transported dust effect on the atmosphere is its vertical distribution. In this study the vertical structure of North African dust and stratiform low clouds is analyzed over the Atlantic Ocean for the 2006–2007 boreal winter (December–February) and boreal summer of 2006 (June–August). By using the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) backscatter measurements over the dust routes, we describe the differences in dust transport between the seasons. We show a bi-modal distribution of the average dust plumes height in both seasons (it is less clear in the winter). The higher plume top height is 5.1±0.4 km, near the African coast line in the summer and 3.7±0.4 km in the winter. The lower plume merges with the marine boundary layer, in both seasons. Our study suggests that a significant part of the dust is transported near and within the marine boundary layer and interacts with low stratiform clouds.
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Shin, Sung-Kyun, Matthias Tesche, Detlef Müller, and Youngmin Noh. "Technical note: Absorption aerosol optical depth components from AERONET observations of mixed dust plumes." Atmospheric Measurement Techniques 12, no. 1 (January 30, 2019): 607–18. http://dx.doi.org/10.5194/amt-12-607-2019.
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Abstract. Absorption aerosol optical depth (AAOD) as obtained from sun–sky photometer measurements provides a measure of the light-absorbing properties of the columnar aerosol loading. However, it is not an unambiguous aerosol-type-specific parameter, particularly if several types of absorbing aerosols, for instance black carbon (BC) and mineral dust, are present in a mixed aerosol plume. The contribution of mineral dust to total aerosol light absorption is particularly important at UV wavelengths. In this study we refine a lidar-based technique applied to the separation of dust and non-dust aerosol types for the use with Aerosol Robotic Network (AERONET) direct sun and inversion products. We extend the methodology to retrieve AAOD related to non-dust aerosol (AAODnd) and BC (AAODBC). We test the method at selected AERONET sites that are frequently affected by aerosol plumes that contain a mixture of Saharan or Asian mineral dust and biomass-burning smoke or anthropogenic pollution, respectively. We find that aerosol optical depth (AOD) related to mineral dust as obtained with our methodology is frequently smaller than coarse-mode AOD. This suggests that the latter is not an ideal proxy for estimating the contribution of mineral dust to mixed dust plumes. We present the results of the AAODBC retrieval for the selected AERONET sites and compare them to coincident values provided in the Copernicus Atmosphere Monitoring System aerosol reanalysis. We find that modelled and AERONET AAODBC are most consistent for Asian sites or at Saharan sites with strong local anthropogenic sources.
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Ingersoll, A. P., and K. A. Tryka. "Triton's Plumes: The Dust Devil Hypothesis." Science 250, no. 4979 (October 19, 1990): 435–37. http://dx.doi.org/10.1126/science.250.4979.435.
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Shin, Sung-Kyun, Matthias Tesche, Youngmin Noh, and Detlef Müller. "Aerosol-type classification based on AERONET version 3 inversion products." Atmospheric Measurement Techniques 12, no. 7 (July 11, 2019): 3789–803. http://dx.doi.org/10.5194/amt-12-3789-2019.
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Abstract. This study proposes an aerosol-type classification based on the particle linear depolarization ratio (PLDR) and single-scattering albedo (SSA) provided in the AErosol RObotic NETwork (AERONET) version 3 level 2.0 inversion product. We compare our aerosol-type classification with an earlier method that uses fine-mode fraction (FMF) and SSA. Our new method allows for a refined classification of mineral dust that occurs as a mixture with other absorbing aerosols: pure dust (PD), dust-dominated mixed plume (DDM), and pollutant-dominated mixed plume (PDM). We test the aerosol classification at AERONET sites in East Asia that are frequently affected by mixtures of Asian dust and biomass-burning smoke or anthropogenic pollution. We find that East Asia is strongly affected by pollution particles with high occurrence frequencies of 50 % to 67 %. The distribution and types of pollution particles vary with location and season. The frequency of PD and dusty aerosol mixture (DDM+PDM) is slightly lower (34 % to 49 %) than pollution-dominated mixtures. Pure dust particles have been detected in only 1 % of observations. This suggests that East Asian dust plumes generally exist in a mixture with pollution aerosols rather than in pure form. In this study, we have also considered data from selected AERONET sites that are representative of anthropogenic pollution, biomass-burning smoke, and mineral dust. We find that average aerosol properties obtained for aerosol types in our PLDR–SSA-based classification agree reasonably well with those obtained at AERONET sites representative for different aerosol types.
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Denjean, C., F. Cassola, A. Mazzino, S. Triquet, S. Chevaillier, N. Grand, T. Bourrianne, et al. "Size distribution and optical properties of mineral dust aerosols transported in the western Mediterranean." Atmospheric Chemistry and Physics Discussions 15, no. 15 (August 10, 2015): 21607–69. http://dx.doi.org/10.5194/acpd-15-21607-2015.
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Abstract. This study presents in situ aircraft measurements of Saharan mineral dust transported over the western Mediterranean basin in June–July 2013 during the ChArMEx/ADRIMED (the Chemistry-Aerosol Mediterranean Experiment/Aerosol Direct Radiative Impact on the regional climate in the MEDiterranean region) airborne campaign. Dust events differing in terms of source region (Algeria, Tunisia and Morocco), time of tranport (1–5 days) and height of transport were sampled. Mineral dust were transported above the marine boundary layer, which conversely was dominated by pollution and marine aerosols. The dust vertical structure was extremely variable and characterized by either a single layer or a more complex and stratified structure with layers originating from different source regions. Mixing of mineral dust with pollution particles was observed depending on the height of transport of the dust layers. Dust layers carried higher concentration of pollution particles at intermediate altitude (1–3 km) than at elevated altitude (> 3 km), resulting in scattering Angstrom exponent up to 2.2 within the intermediate altitude. However, the optical properties of the dust plumes remained practically unchanged with respect to values previously measured over source regions, regardless of the altitude. Moderate light absorption of the dust plumes was observed with values of aerosol single scattering albedo at 530 nm ranging from 0.90 to 1.00 ± 0.04. Concurrent calculations from the aerosol chemical composition revealed a negligible contribution of pollution particles to the absorption properties of the dust plumes that was due to a low contribution of refractory black carbon in regards to the fraction of dust and sulfate particles. This suggests that, even in the presence of moderate pollution, likely a persistent feature in the Mediterranean, the optical properties of the dust plumes could be assimilated to those of native dust in radiative transfer simulations, modeling studies and satellite retrievals over the Mediterranean. Measurements also showed that the coarse mode of mineral dust was conserved even after 5 days of transport in the Mediterranean, which contrasts with the gravitational depletion of large particles observed during the transport of dust plumes over the Atlantic. Simulations with the WRF mesoscale meteorological model highlighted a strong vertical turbulence within the dust layers that could prevent deposition of large particles during their atmospheric transport. This has important implications for the dust radiative effects due to surface dimming, atmospheric heating and cloud formation. The results presented here add to the observational dataset necessary for evaluating the role of mineral dust on the regional climate and rainfall patterns in the western Mediterranean basin.
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Denjean, C., F. Cassola, A. Mazzino, S. Triquet, S. Chevaillier, N. Grand, T. Bourrianne, et al. "Size distribution and optical properties of mineral dust aerosols transported in the western Mediterranean." Atmospheric Chemistry and Physics 16, no. 2 (February 1, 2016): 1081–104. http://dx.doi.org/10.5194/acp-16-1081-2016.
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Abstract. This study presents in situ aircraft measurements of Saharan mineral dust transported over the western Mediterranean basin in June–July 2013 during the ChArMEx/ADRIMED (the Chemistry-Aerosol Mediterranean Experiment/Aerosol Direct Radiative Impact on the regional climate in the MEDiterranean region) airborne campaign. Dust events differing in terms of source region (Algeria, Tunisia and Morocco), time of transport (1–5 days) and height of transport were sampled. Mineral dust were transported above the marine boundary layer, which conversely was dominated by pollution and marine aerosols. The dust vertical structure was extremely variable and characterized by either a single layer or a more complex and stratified structure with layers originating from different source regions. Mixing of mineral dust with pollution particles was observed depending on the height of transport of the dust layers. Dust layers carried a higher concentration of pollution particles below 3 km above sea level (a.s.l.) than above 3 km a.s.l., resulting in a scattering Ångström exponent up to 2.2 below 3 km a.s.l. However, the optical properties of the dust plumes remained practically unchanged with respect to values previously measured over source regions, regardless of the altitude. Moderate absorption of light by the dust plumes was observed with values of aerosol single scattering albedo at 530 nm ranging from 0.90 to 1.00. Concurrent calculations from the aerosol chemical composition revealed a negligible contribution of pollution particles to the absorption properties of the dust plumes that was due to a low contribution of refractory black carbon in regards to the fraction of dust and sulfate particles. This suggests that, even in the presence of moderate pollution, likely a persistent feature in the Mediterranean, the optical properties of the dust plumes could be assumed similar to those of native dust in radiative transfer simulations, modelling studies and satellite retrievals over the Mediterranean. Measurements also showed that the coarse mode of mineral dust was conserved even after 5 days of transport in the Mediterranean, which contrasts with the gravitational depletion of large particles observed during the transport of dust plumes over the Atlantic. Simulations with the WRF mesoscale meteorological model highlighted a strong vertical turbulence within the dust layers that could prevent deposition of large particles during their atmospheric transport. This has important implications for the dust radiative effects due to surface dimming, atmospheric heating and cloud formation. The results presented here add to the observational data set necessary for evaluating the role of mineral dust on the regional climate and rainfall patterns in the western Mediterranean basin and understanding their atmospheric transport at global scale.
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Córdoba-Jabonero, C., M. Sorribas, J. L. Guerrero-Rascado, J. A. Adame, Y. Hernández, H. Lyamani, V. Cachorro, et al. "Synergetic monitoring of Saharan dust plumes and potential impact on surface: a case study of dust transport from Canary Islands to Iberian Peninsula." Atmospheric Chemistry and Physics 11, no. 7 (April 1, 2011): 3067–91. http://dx.doi.org/10.5194/acp-11-3067-2011.
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Abstract. The synergetic use of meteorological information, remote sensing both ground-based active (lidar) and passive (sun-photometry) techniques together with backtrajectory analysis and in-situ measurements is devoted to the characterization of dust intrusions. A case study of air masses advected from the Saharan region to the Canary Islands and the Iberian Peninsula, located relatively close and far away from the dust sources, respectively, was considered for this purpose. The observations were performed over three Spanish geographically strategic stations within the dust-influenced area along a common dust plume pathway monitored from 11 to 19 of March 2008. A 4-day long dust event (13–16 March) over the Santa Cruz de Tenerife Observatory (SCO), and a linked short 1-day dust episode (14 March) in the Southern Iberian Peninsula over the Atmospheric Sounding Station "El Arenosillo" (ARN) and the Granada station (GRA) were detected. Meteorological conditions favoured the dust plume transport over the area under study. Backtrajectory analysis clearly revealed the Saharan region as the source of the dust intrusion. Under the Saharan air masses influence, AERONET Aerosol Optical Depth at 500 nm (AOD500) ranged from 0.3 to 0.6 and Ångström Exponent at 440/675 nm wavelength pair (AE440/675) was lower than 0.5, indicating a high loading and predominance of coarse particles during those dusty events. Lidar observations characterized their vertical layering structure, identifying different aerosol contributions depending on altitude. In particular, the 3-km height dust layer transported from the Saharan region and observed over SCO site was later on detected at ARN and GRA stations. No significant differences were found in the lidar (extinction-to-backscatter) ratio (LR) estimation for that dust plume over all stations when a suitable aerosol scenario for lidar data retrieval is selected. Lidar-retrieved LR values of 60–70 sr were obtained during the main dust episodes. These similar LR values found in all the stations suggest that dust properties were kept nearly unchanged in the course of its medium-range transport. In addition, the potential impact on surface of that Saharan dust intrusion over the Iberian Peninsula was evaluated by means of ground-level in-situ measurements for particle deposition assessment together with backtrajectory analysis. However, no connection between those dust plumes and the particle sedimentation registered at ground level is found. Differences on particle deposition processes observed in both Southern Iberian Peninsula sites are due to the particular dust transport pattern occurred over each station. Discrepancies between columnar-integrated and ground-level in-situ measurements show a clear dependence on height of the dust particle size distribution. Then, further vertical size-resolved observations are needed for evaluation of the impact on surface of the Saharan dust arrival to the Iberian Peninsula.
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Miller, Steven D., Louie D. Grasso, Qijing Bian, Sonia M. Kreidenweis, Jack F. Dostalek, Jeremy E. Solbrig, Jennifer Bukowski, et al. "<i>A Tale of Two Dust Storms</i>: analysis of a complex dust event in the Middle East." Atmospheric Measurement Techniques 12, no. 9 (September 24, 2019): 5101–18. http://dx.doi.org/10.5194/amt-12-5101-2019.
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Abstract. Lofted mineral dust over data-sparse regions presents considerable challenges to satellite-based remote sensing methods and numerical weather prediction alike. The southwest Asia domain is replete with such examples, with its diverse array of dust sources, dust mineralogy, and meteorologically driven lofting mechanisms on multiple spatial and temporal scales. A microcosm of these challenges occurred over 3–4 August 2016 when two dust plumes, one lofted within an inland dry air mass and another embedded within a moist air mass, met over the southern Arabian Peninsula. Whereas conventional infrared-based techniques readily detected the dry air mass dust plume, they experienced marked difficulties in detecting the moist air mass dust plume, becoming apparent when visible reflectance revealed the plume crossing over an adjacent dark water background. In combining information from numerical modeling, multi-satellite and multi-sensor observations of lofted dust and moisture profiles, and idealized radiative transfer simulations, we develop a better understanding of the environmental controls of this event, characterizing the sensitivity of infrared-based dust detection to column water vapor, dust vertical extent, and dust optical properties. Differences in assumptions of dust complex refractive index translate to variations in the sign and magnitude of the split-window brightness temperature difference commonly used for detecting mineral dust. A multi-sensor technique for mitigating the radiative masking effects of water vapor via modulation of the split-window dust-detection threshold, predicated on idealized simulations tied to these driving factors, is proposed and demonstrated. The new technique, indexed to an independent description of the surface-to-500 hPa atmospheric column moisture, reveals parts of the missing dust plume embedded in the moist air mass, with the best performance realized over land surfaces.
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Leaitch, W. R., A. M. Macdonald, K. G. Anlauf, P. S. K. Liu, D. Toom-Sauntry, S. M. Li, J. Liggio, et al. "Evidence for Asian dust effects from aerosol plume measurements during INTEX-B 2006 near Whistler, BC." Atmospheric Chemistry and Physics 9, no. 11 (June 3, 2009): 3523–46. http://dx.doi.org/10.5194/acp-9-3523-2009.
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Abstract. Several cases of aerosol plumes resulting from trans-Pacific transport were observed between 2 km and 5.3 km at Whistler, BC from 22 April 2006 to 15 May 2006. The fine particle (<1 μm) chemical composition of most of the plumes was dominated by sulphate that ranged from 1–5 μg m−3 as measured with a Quadrapole Aerosol Mass Spectrometer (Q-AMS). Coarse particles (>1 μm) were enhanced in all sulphate plumes. Fine particle organic mass concentrations were relatively low in most plumes and were nominally anti-correlated with the increases in the number concentrations of coarse particles. The ion chemistry of coarse particles sampled at Whistler Peak was dominated by calcium, sodium, nitrate, sulphate and formate. Scanning transmission X-ray microscopy of coarse particles sampled from the NCAR C-130 aircraft relatively close to Whistler indicated carbonate, potassium and organic functional groups, in particular the carboxyl group. Asian plumes reaching Whistler, BC during the INTEX-B study were not only significantly reduced of fine particle organic material, but organic compounds were attached to coarse particles in significant quantities. Suspension of dust with deposited organic material and scavenging of organic materials by dust near anthropogenic sources are suggested, and if any secondary organic aerosol (SOA) was formed during transport from Asian source regions across the Pacific it was principally associated with the coarse particles. An average of profiles indicates that trans-Pacific transport between 2 and 5 km during this period increased ozone by about 10 ppbv and fine particle sulphate by 0.2–0.5 μg m−3. The mean sizes of the fine particles in the sulphate plumes were larger when dust particles were present and smaller when the fine particle organic mass concentration was larger and dust was absent. The coarse particles of dust act to accumulate sulphate, nitrate and organic material in larger particles, diminishing the role of these compounds in indirect radiative forcing, but potentially enhancing their roles in direct radiative forcing.
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Zhang, Hengheng, Frank Wagner, Harald Saathoff, Heike Vogel, Gholamali Hoshyaripour, Vanessa Bachmann, Jochen Förstner, and Thomas Leisner. "Comparison of Scanning LiDAR with Other Remote Sensing Measurements and Transport Model Predictions for a Saharan Dust Case." Remote Sensing 14, no. 7 (March 31, 2022): 1693. http://dx.doi.org/10.3390/rs14071693.
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The evolution and the properties of a Saharan dust plume were studied near the city of Karlsruhe in southwest Germany (8.4298°E, 49.0953°N) from 7 to 9 April 2018, combining a scanning LiDAR (90°, 30°), a vertically pointing LiDAR (90°), a sun photometer, and the transport model ICON-ART. Based on this Saharan dust case, we discuss the advantages of a scanning aerosol LiDAR and validate a method to determine LiDAR ratios independently. The LiDAR measurements at 355 nm showed that the dust particles had backscatter coefficients of 0.86 ± 0.14 Mm−1 sr−1, extinction coefficients of 40 ± 0.8 Mm−1, a LiDAR ratio of 46 ± 5 sr, and a linear particle depolarisation ratio of 0.27 ± 0.023. These values are in good agreement with those obtained in previous studies of Saharan dust plumes in Western Europe. Compared to the remote sensing measurements, the transport model predicted the plume arrival time, its layer height, and its structure quite well. The comparison of dust plume backscatter values from the ICON-ART model and observations for two days showed a correlation with a slope of 0.9 ± 0.1 at 355 nm. This work will be useful for future studies to characterise aerosol particles employing scanning LiDARs.
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Schrod, Jann, Daniel Weber, Jaqueline Drücke, Christos Keleshis, Michael Pikridas, Martin Ebert, Bojan Cvetković, et al. "Ice nucleating particles over the Eastern Mediterranean measured by unmanned aircraft systems." Atmospheric Chemistry and Physics 17, no. 7 (April 12, 2017): 4817–35. http://dx.doi.org/10.5194/acp-17-4817-2017.
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Abstract. During an intensive field campaign on aerosol, clouds, and ice nucleation in the Eastern Mediterranean in April 2016, we measured the abundance of ice nucleating particles (INPs) in the lower troposphere from unmanned aircraft systems (UASs). Aerosol samples were collected by miniaturized electrostatic precipitators onboard the UASs at altitudes up to 2.5 km. The number of INPs in these samples, which are active in the deposition and condensation modes at temperatures from −20 to −30 °C, were analyzed immediately after collection on site using the ice nucleus counter FRIDGE (FRankfurt Ice nucleation Deposition freezinG Experiment). During the 1-month campaign, we encountered a series of Saharan dust plumes that traveled at several kilometers' altitude. Here we present INP data from 42 individual flights, together with aerosol number concentrations, observations of lidar backscattering, dust concentrations derived by the dust transport model DREAM (Dust Regional Atmospheric Model), and results from scanning electron microscopy. The effect of the dust plumes is reflected by the coincidence of INPs with the particulate matter (PM), the lidar signal, and the predicted dust mass of the model. This suggests that mineral dust or a constituent related to dust was a major contributor to the ice nucleating properties of the aerosol. Peak concentrations of above 100 INPs std L−1 were measured at −30 °C. The INP concentration in elevated plumes was on average a factor of 10 higher than at ground level. Since desert dust is transported for long distances over wide areas of the globe predominantly at several kilometers' altitude, we conclude that INP measurements at ground level may be of limited significance for the situation at the level of cloud formation.
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Leaitch, W. R., A. M. Macdonald, K. G. Anlauf, P. S. K. Liu, D. Toom-Sauntry, S. M. Li, J. Liggio, et al. "Evidence for Asian dust effects from aerosol plume measurements during INTEX-B 2006 near Whistler, BC." Atmospheric Chemistry and Physics Discussions 8, no. 5 (October 28, 2008): 18531–89. http://dx.doi.org/10.5194/acpd-8-18531-2008.
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Abstract. Several cases of aerosol plumes resulting from trans-Pacific transport were observed between 2 km and 5.3 km at Whistler, BC from 22 April 2006 to 15 May 2006. The fine particle (<1 μm) chemical composition of most of the plumes was dominated by sulphate that ranged from 1–5 μg m−3 as measured with a Quadrapole Aerosol Mass Spectrometer (Q-AMS). Coarse particles (>1 μm) were enhanced in all sulphate plumes. Fine particle organic mass concentrations were relatively low in most plumes and anti-correlated with the increases in the coarse particles. The chemistry of coarse particles sampled at Whistler Peak was dominated by calcium, sodium, nitrate, sulphate and formate. Scanning transmission X-ray microscopy of coarse particles sampled from the NCAR C-130 aircraft relatively close to Whistler indicated carbonate, potassium and organic functional groups, in particular the carboxyl group. Asian plumes reaching Whistler, BC during the INTEX-B study were not only significantly reduced of fine particle organic material, but organic compounds were attached to coarse particles in significant quantities. Scavenging of organic aerosol precursors by dust near source regions is suggested, and any formation of secondary organic aerosol (SOA) during transport from Asian source regions across the Pacific was principally associated with the coarse particles. An average of profiles indicates that trans-Pacific transport between 2 and 5 km during this period increased ozone by about 10 ppbv and fine particle sulphate by 0.2–0.5 μg m−3. The mean sizes of the fine particles in the sulphate plumes were larger when dust particles were present and smaller when the fine particle organic mass concentration was larger and dust was absent. The coarse particles of dust act to accumulate sulphate, nitrate and organic material in larger particles, diminishing the role of these compounds in indirect radiative forcing, but potentially enhancing their roles in direct radiative forcing.
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Vandenbussche, Sophie, Sieglinde Callewaert, Kerstin Schepanski, and Martine De Mazière. "North African mineral dust sources: new insights from a combined analysis based on 3D dust aerosol distributions, surface winds and ancillary soil parameters." Atmospheric Chemistry and Physics 20, no. 23 (December 7, 2020): 15127–46. http://dx.doi.org/10.5194/acp-20-15127-2020.
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Abstract. Mineral dust aerosol is a key player in the climate system. Determining dust sources and the spatio-temporal variability of dust emission fluxes is essential for estimating the impact of dust on the atmospheric radiation budget, cloud and precipitation formation processes, the bio-productivity and, ultimately, the carbon cycle. Although much effort has been put into determining dust sources from satellite observations, geo-locating active dust sources is still challenging and uncertainties in space and time are evident. One major source of uncertainty is the lack of clear differentiation between near-source dust aerosol and transported dust aerosol. In order to reduce this uncertainty, we use 3D information on the distribution of dust aerosol suspended in the atmosphere calculated from spectral measurements obtained by the Infrared Atmospheric Sounding Interferometer (IASI) by using the Mineral Aerosols Profiling from Infrared Radiance (MAPIR) algorithm. In addition to standard dust products from satellite observations, which provide 2D information on the horizontal distribution of dust, MAPIR allows for the retrieval of additional information on the vertical distribution of dust plumes. This ultimately enables us to separate between near-source and transported dust plumes. Combined with information on near-surface wind speed and surface properties, low-altitude dust plumes can be assigned to dust emission events and low-altitude transport regimes can be excluded. Consequently, this technique will reduce the uncertainty in automatically geo-locating active dust sources. The findings of our study illustrate the spatio-temporal distribution of North African dust sources based on 9 years of data, allowing for the observation of a full seasonal cycle of dust emissions, differentiating morning and afternoon/evening emissions and providing a first glance at long-term changes. In addition, we compare the results of this new method to the results from Schepanski et al. (2012), who manually identified dust sources from Spinning Enhanced Visible and InfraRed Imager (SEVIRI) red–green–blue (RGB) images. The comparison illustrates that each method has its strengths and weaknesses that must be taken into account when using the results. This study is of particular importance for understanding future environmental changes due to a changing climate.
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Boice, Daniel C., and Raymond Goldstein. "A cometary perspective of Enceladus." Proceedings of the International Astronomical Union 5, S263 (August 2009): 151–56. http://dx.doi.org/10.1017/s1743921310001675.
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AbstractIcy plumes venting from Enceladus draw obvious comparisons to such features seen in comets. This paper outlines a consistent evolution from cometary activity to larger icy bodies in the outer solar system. The major differences are due to the systematic effects of increased gravity, including more spherical solid bodies (self-gravity), less porosity, the possible existence of liquid water due to internal sources of heat (Enceladus) versus possible cometary cyrovolcanism, internal inhomogeneities leading to jet-like features, and the possibility of a quasi-bound dusty gas atmosphere, as opposed to the extensive exospheres of comets. Similarities exist also, including gas and dust emission and the filamentary nature of jet-like features (caused by surface topography in comets), surface evolution by dust accumulation, heat and gas transport through the surface layers, among others. Initial results regarding the plume chemistry and comparisons to CAPS ion data show similarities too. Others have considered additional effects such as, charging of particles, micrometeorite impacts and complex interactions with the E-ring neutrals and plasma in great detail so these topics remain outside the scope of this paper.
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Manning, William J. "Terrorist Attacks: Do We Know How to Assess the Results?" Scientific World JOURNAL 1 (2001): 588–89. http://dx.doi.org/10.1100/tsw.2001.319.
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On September 11, 2001, terrorists destroyed the World Trade Center (WTC) in New York City. Explosions and fires resulted in the complete collapse of the two WTC towers. The collapsing towers served as enormous point sources of gaseous and particulate air pollution, seen as huge plumes of smoke and dust. The smoke contained volatile organic compounds and fine particles and aerosols. The dust fraction contained parts of ceiling tiles, carpets, concrete, adhesives, asbestos, chromium, lead, titanium, and many other elements and materials. Whether there were unusually toxic ingredients in the plumes is largely unknown.
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Dai, Guangyao, Kangwen Sun, Xiaoye Wang, Songhua Wu, Xiangying E, Qi Liu, and Bingyi Liu. "Dust transport and advection measurement with spaceborne lidars ALADIN and CALIOP and model reanalysis data." Atmospheric Chemistry and Physics 22, no. 12 (June 20, 2022): 7975–93. http://dx.doi.org/10.5194/acp-22-7975-2022.
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Abstract. In this paper, a long-term large-scale Saharan dust transport event which occurred between 14 and 27 June 2020 is tracked with the spaceborne lidars ALADIN (Atmospheric Laser Doppler Instrument) and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) together with ECMWF (European Centre for Medium-Range Forecasts) and HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory model) analysis. We evaluate the performance of ALADIN and CALIOP on the observations of dust optical properties and wind fields and explore the possibility of tracking the dust events and calculating the dust mass advection with the combination of satellite and model data. The dust plumes are identified with the AIRS/Aqua Dust Score Index and with the vertical feature mask product from CALIOP. The emission, dispersion, transport and deposition of the dust event are monitored using the data from AIRS/Aqua, CALIOP and HYSPLIT. With the quasi-synchronized observations by ALADIN and CALIOP, combined with the wind field and relative humidity, the dust advection values are calculated. From this study, it is found that the dust event generated on 14 and 15 June 2020 from the Sahara in North Africa dispersed and moved westward over the Atlantic Ocean, finally being deposited in the western Atlantic Ocean, the Americas and the Caribbean Sea. During the transport and deposition processes, the dust plumes are trapped in the northeasterly trade-wind zone between latitudes of 5∘ and 30∘ N and altitudes of 0 and 6 km. Aeolus provided the observations of the dynamics of this dust transport event in the Saharan Air Layer (SAL). From the measurement results on 19 June 2020, the dust plumes are captured quasi-simultaneously over the emission region (Western Sahara), the transport region (middle Atlantic) and the deposition region (western Atlantic) individually, which indicates that the dust plume area over the Atlantic on the morning of this day is quite enormous and that this dust transport event is massive and extensive. The quasi-synchronization observation results of 15, 16, 19, 24 and 27 June by ALADIN and CALIOP during the entire transport process show good agreement with the Dust Score Index data and the HYSPLIT trajectories, which indicates that the transport process of the same dust event is tracked by ALADIN and CALIOP, verifies that the dust transport spent around 2 weeks from the emission to the deposition and achieved the respective observations of this dust event's emission phase, development phase, transport phase, descent phase and deposition phase. Finally, the advection values for different dust parts and heights on 19 June and on the entire transport routine during transportation are computed. On 19 June, the mean dust advection values are about 1.91±1.21 mg m−2 s−1 over the emission region, 1.38±1.28 mg m−2 s−1 over the transport region and 0.75±0.68mgm-2s-1 over the deposition region. In the whole lifetime of the dust event, the mean dust advection values were about 1.51±1.03mgm-2s-1 on 15 June 2020, 2.19±1.72mgm-2s-1 on 16 June 2020, 1.38±1.28mgm-2s-1 on 19 June 2020, 1.60±1.08mgm-2s-1 on 24 June 2020 and 1.03±0.60mgm-2s-1 on 27 June 2020. During the dust development stage, the mean advection values gradually increased and reached their maximum on 16 June with the enhancement of the dust event. Then, the mean advection values decreased during the transport and the deposition of the dust over the Atlantic Ocean, the Americas and the Caribbean Sea.
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de Foy, B., S. P. Burton, R. A. Ferrare, C. A. Hostetler, J. W. Hair, C. Wiedinmyer, and L. T. Molina. "Aerosol plume transport and transformation in high spectral resolution lidar measurements and WRF-Flexpart simulations during the MILAGRO Field Campaign." Atmospheric Chemistry and Physics Discussions 10, no. 11 (November 19, 2010): 28471–518. http://dx.doi.org/10.5194/acpd-10-28471-2010.
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Abstract. The Mexico City Metropolitan Area (MCMA) experiences high loadings of atmospheric aerosols from anthropogenic sources, biomass burning and wind-blown dust. This paper uses a combination of measurements and numerical simulations to identify different plumes affecting the basin and to characterize transformation inside the plumes. The airborne High Spectral Resolution Lidar measures extinction coefficients and extinction to backscatter ratio at 532 nm, and backscatter coefficients and depolarization ratios at 532 and 1064 nm. These can be used to identify aerosol types. The measurement curtains are compared with particle trajectory simulations using WRF-Flexpart for different source groups. The good correspondence between measurements and simulations suggests that the aerosol transport is sufficiently well characterized by the models to estimate aerosol types and ages. Plumes in the basin undergo complex transport, and are frequently mixed together. Urban aerosols are readily identifiable by their low depolarization ratios and high lidar ratios, and dust by the opposite properties. Fresh biomass burning plumes have very low depolarization ratios which increase rapidly with age. This rapid transformation is consistent with the presence of atmospheric tar balls in the fresh plumes.
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de Foy, B., S. P. Burton, R. A. Ferrare, C. A. Hostetler, J. W. Hair, C. Wiedinmyer, and L. T. Molina. "Aerosol plume transport and transformation in high spectral resolution lidar measurements and WRF-Flexpart simulations during the MILAGRO Field Campaign." Atmospheric Chemistry and Physics 11, no. 7 (April 15, 2011): 3543–63. http://dx.doi.org/10.5194/acp-11-3543-2011.
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Abstract. The Mexico City Metropolitan Area (MCMA) experiences high loadings of atmospheric aerosols from anthropogenic sources, biomass burning and wind-blown dust. This paper uses a combination of measurements and numerical simulations to identify different plumes affecting the basin and to characterize transformation inside the plumes. The High Spectral Resolution Lidar on board the NASA LaRC B-200 King Air aircraft measured extinction coefficients and extinction to backscatter ratio at 532 nm, and backscatter coefficients and depolarization ratios at 532 and 1064 nm. These can be used to identify aerosol types. The measurement curtains are compared with particle trajectory simulations using WRF-Flexpart for different source groups. The good correspondence between measurements and simulations suggests that the aerosol transport is sufficiently well characterized by the models to estimate aerosol types and ages. Plumes in the basin undergo complex transport, and are frequently mixed together. Urban aerosols are readily identifiable by their low depolarization ratios and high lidar ratios, and dust by the opposite properties. Fresh biomass burning plumes have very low depolarization ratios which increase rapidly with age. This rapid transformation is consistent with the presence of atmospheric tar balls in the fresh plumes.
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Gutleben, Manuel, Silke Groß, Christian Heske, and Martin Wirth. "Wintertime Saharan dust transport towards the Caribbean: an airborne lidar case study during EUREC<sup>4</sup>A." Atmospheric Chemistry and Physics 22, no. 11 (June 8, 2022): 7319–30. http://dx.doi.org/10.5194/acp-22-7319-2022.
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Abstract. Wintertime Saharan dust plumes in the vicinity of Barbados are investigated by means of airborne lidar measurements. The measurements were conducted in the framework of the EUREC4A (Elucidating the Role of Cloud-Circulation Coupling in Climate) field experiment upstream the Caribbean island in January–February 2020. The combination of the water vapor differential absorption and high spectral resolution lidar techniques together with dropsonde measurements aboard the German HALO (High Altitude and Long-Range) research aircraft enable a detailed vertical and horizontal characterization of the measured dust plumes. In contrast to summertime dust transport, mineral dust aerosols were transported at lower altitudes and were always located below 3.5 km. Calculated backward trajectories affirm that the dust-laden layers have been transported in nearly constant low-level altitude over the North Atlantic Ocean. Only mixtures of dust particles with other aerosol species, i.e., biomass-burning aerosol from fires in West Africa and marine aerosol, were detected by the lidar. No pure mineral dust regimes were observed. Additionally, all the dust-laden air masses that were observed during EUREC4A came along with enhanced water vapor concentrations compared with the free atmosphere above. Such enhancements have already been observed during summertime and were found to have a great impact on radiative transfer and atmospheric stability.
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Zhou, Tian, Jianping Huang, Zhongwei Huang, Jingjing Liu, Wencai Wang, and Lei Lin. "The depolarization–attenuated backscatter relationship for dust plumes." Optics Express 21, no. 13 (June 18, 2013): 15195. http://dx.doi.org/10.1364/oe.21.015195.
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Fairlie, T. D., D. J. Jacob, J. E. Dibb, B. Alexander, M. A. Avery, A. van Donkelaar, and L. Zhang. "Impact of mineral dust on nitrate, sulfate, and ozone in transpacific Asian pollution plumes." Atmospheric Chemistry and Physics Discussions 9, no. 6 (November 17, 2009): 24477–510. http://dx.doi.org/10.5194/acpd-9-24477-2009.
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Abstract. We use a 3-d global chemical transport model (GEOS-Chem) to interpret aircraft observations of nitrate and sulfate partitioning in transpacific dust plumes during the INTEX-B campaign of April–May 2006. The model includes explicit transport of size-resolved mineral dust and its alkalinity, nitrate, and sulfate content. The observations show that particulate nitrate is primarily associated with dust, sulfate is primarily associated with ammonium, and Asian dust remains alkaline across the Pacific. This can be reproduced in the model by using a reactive uptake coefficient for HNO3 on dust (γ(HNO3)~10−3) much lower than commonly assumed in models and likely reflecting limitation of uptake by dust dissolution. The model overestimates gas-phase HNO3 by a factor of 2–3, typical of previous model studies; we show that this cannot be corrected by uptake on dust. We find that the fraction of aerosol nitrate on dust in the model increases from ~30% in fresh Asian outflow to 80–90% over the Northeast Pacific, reflecting in part the volatilization of ammonium nitrate and the resulting transfer of nitrate to the dust. Consumption of dust alkalinity by uptake of acid gases in the model is slow relative to the lifetime of dust against deposition, so that dust in general does not acidify. This argues against the hypothesis that dust iron released by acidification could become bio-available upon dust deposition. Observations in INTEX-B show no detectable ozone depletion in Asian dust plumes, consistent with the model. Uptake of HNO3 by dust, suppressing its recycling to NOx, reduces Asian pollution influence on US surface ozone in the model by 10–15% or up to 1 ppb.
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Touré, N'Datchoh Evelyne, Abdourahamane Konaré, and Siélé Silué. "Intercontinental Transport and Climatic Impact of Saharan and Sahelian Dust." Advances in Meteorology 2012 (2012): 1–14. http://dx.doi.org/10.1155/2012/157020.
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The Sahara and Sahel regions of Africa are important sources of dust particles into the atmosphere. Dust particles from these regions are transported over the Atlantic Ocean to the Eastern American Coasts. This transportation shows temporal and spatial variability and often reaches its peak during the boreal summer (June-July-August). The regional climate model (RegCM 4.0), containing a module of dust emission, transport, and deposition processes, is used in this study. Saharan and Sahelian dusts emissions, transports, and climatic impact on precipitations during the spring (March-April-May) and summer (June-July-August) were studied using this model. The results showed that the simulation were coherent with observations made by the MISR satellite and the AERONET ground stations, within the domain of Africa (Banizoumba, Cinzana, and M’Bour) and Ragged-point (Barbados Islands). The transport of dust particles was predominantly from North-East to South-West over the studied period (2005–2010). The seasonality of dust plumes’ trajectories was influenced by the altitudes reached by dusts in the troposphere. The impact of dusts on climate consisted of a cooling effect both during the boreal summer and spring over West Africa (except Southern-Guinea and Northern-Liberia), Central Africa, South-America, and Caribbean where increased precipitations were observed.
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Fairlie, T. D., D. J. Jacob, J. E. Dibb, B. Alexander, M. A. Avery, A. van Donkelaar, and L. Zhang. "Impact of mineral dust on nitrate, sulfate, and ozone in transpacific Asian pollution plumes." Atmospheric Chemistry and Physics 10, no. 8 (April 29, 2010): 3999–4012. http://dx.doi.org/10.5194/acp-10-3999-2010.
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Abstract. We use a 3-D global chemical transport model (GEOS-Chem) to interpret aircraft observations of nitrate and sulfate partitioning in transpacific dust plumes during the INTEX-B campaign of April–May 2006. The model includes explicit transport of size-resolved mineral dust and its alkalinity, nitrate, and sulfate content. The observations show that particulate nitrate is primarily associated with dust, sulfate is primarily associated with ammonium, and Asian dust remains alkaline across the Pacific. This can be reproduced in the model by using a reactive uptake coefficient for HNO3 on dust (γ(HNO3) ~10−3) much lower than commonly assumed in models and possibly reflecting limitation of uptake by dust dissolution. The model overestimates gas-phase HNO3 by a factor of 2–3, typical of previous model studies; we show that this cannot be corrected by uptake on dust. We find that the fraction of aerosol nitrate on dust in the model increases from ~30% in fresh Asian outflow to 80–90% over the Northeast Pacific, reflecting in part the volatilization of ammonium nitrate and the resulting transfer of nitrate to the dust. Consumption of dust alkalinity by uptake of acid gases in the model is slow relative to the lifetime of dust against deposition, so that dust does not acidify (at least not in the bulk). This limits the potential for dust iron released by acidification to become bio-available upon dust deposition. Observations in INTEX-B show no detectable ozone depletion in Asian dust plumes, consistent with the model. Uptake of HNO3 by dust, suppressing its recycling to NOx, reduces Asian pollution influence on US surface ozone in the model by 10–15% or up to 1 ppb.
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Yang, W., A. Marshak, T. Várnai, O. V. Kalashnikova, and A. B. Kostinski. "CALIPSO observations of transatlantic dust: vertical stratification and effect of clouds." Atmospheric Chemistry and Physics Discussions 12, no. 5 (May 10, 2012): 12051–80. http://dx.doi.org/10.5194/acpd-12-12051-2012.
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Abstract. We use CALIOP nighttime measurements of lidar backscatter, color and depolarization ratios during the summer of 2007 to study transatlantic dust properties downwind of Saharan sources, and to examine the interaction of clouds and dust. Our analysis suggests that (1) while lidar backscatter doesn't change much with altitude in the Saharan Air Layer (SAL), depolarization and color ratios both increase with altitude in the SAL; (2) lidar backscatter and color ratio increase as dust is transported westward in the SAL; (3) the vertical lapse rate of dust depolarization ratio, introduced here, increases within SAL as plumes move westward; (4) nearby clouds barely affect the backscatter and color ratio of dust volumes within SAL but not so below SAL. Moreover, the presence of nearby clouds tends to decrease the depolarization of dust volumes within SAL. Finally, (5) the odds of CALIOP finding dust below SAL next to clouds are about 2/3 of those far away from clouds. This feature, together with an apparent increase in depolarization ratio near clouds, indicates that particles in some dusty volumes lose asphericity in the humid air near clouds, and cannot be identified by CALIPSO as dust.
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Vaughan, M., C. Trepte, C. Hostetler, and D. Winker. "Airborne dust distributions over the Tibetan Plateau and surrounding areas derived from the first year of CALIPSO lidar observations." Atmospheric Chemistry and Physics Discussions 8, no. 2 (March 25, 2008): 5957–77. http://dx.doi.org/10.5194/acpd-8-5957-2008.
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Abstract. Airborne dust is a major environmental hazard in Asia. Using an analysis of the first full year of CALIPSO lidar measurements, this paper derives unprecedented, altitude-resolved seasonal distributions of desert dust transported over the Tibetan Plateau (TP) and the surrounding areas. The CALIPSO lidar observations include numerous large dust plumes over the northern slope and eastern part of the TP, with the largest number of dust events occurring in the spring of 2007, and some layers being lofted to altitudes of 10 km and higher. Generation of the Tibetan airborne dusts appears to be largely associated with source regions to the north and on the eastern part of the plateau. Examination of the CALIPSO time history reveals an "airborne dust corridor" due to the eastward transport of dusts originating primarily in these source areas. This corridor extends from west to east and shows a seasonality largely modulated by the TP through its dynamical and thermal forcing on the atmospheric flows. On the southern side, desert dust particles originate predominately in North India and Pakistan. The dust transport occurs primarily in dry seasons around the TP western and southern slopes and dust particles become mixed with local polluted aerosols. No significant amount of dust appears to be transported over the Himalayas. Extensive forward trajectory simulations are also conducted to confirm the dust transport pattern from the nearby sources observed by the CALIPSO lidar.
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Liu, Z., D. Liu, J. Huang, M. Vaughan, I. Uno, N. Sugimoto, C. Kittaka, et al. "Airborne dust distributions over the Tibetan Plateau and surrounding areas derived from the first year of CALIPSO lidar observations." Atmospheric Chemistry and Physics 8, no. 16 (August 29, 2008): 5045–60. http://dx.doi.org/10.5194/acp-8-5045-2008.
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Abstract. Using an analysis of the first full year of CALIPSO lidar measurements, this paper derives unprecedented, altitude-resolved seasonal distributions of desert dust transported over the Tibetan Plateau (TP) and the surrounding areas. The CALIPSO lidar observations include numerous large dust plumes over the northern slope and eastern part of the TP, with the largest number of dust events occurring in the spring of 2007, and some layers being lofted to altitudes of 11–12 km. Generation of the Tibetan airborne dusts appears to be largely associated with source regions to the north and on the eastern part of the plateau. Examination of the CALIPSO time history reveals an "airborne dust corridor" due to the eastward transport of dusts originating primarily in these source areas. This corridor extends from west to east and shows a seasonality largely modulated by the TP through its dynamical and thermal forcing on the atmospheric flows. On the southern side, desert dust particles originate predominately in Northwest India and Pakistan. The dust transport occurs primarily in dry seasons around the TP western and southern slopes and dust particles become mixed with local polluted aerosols. No significant amount of dust appears to be transported over the Himalayas. Extensive forward trajectory simulations are also conducted to confirm the dust transport pattern from the nearby sources observed by the CALIPSO lidar. Comparisons with the OMI and MODIS measurements show the unique capability of the CALIPSO lidar to provide unambiguous, altitude-resolved dust measurements.
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Raga, Graciela B., Luis A. Ladino, Darrel Baumgardner, Carolina Ramirez-Romero, Fernanda Córdoba, Harry Alvarez-Ospina, Daniel Rosas, et al. "ADABBOY: African Dust And Biomass Burning Over Yucatan." Bulletin of the American Meteorological Society 102, no. 8 (August 2021): E1543—E1556. http://dx.doi.org/10.1175/bams-d-20-0172.1.
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AbstractBiomass burning (BB) emissions and African dust (AD) are often associated with poor regional air quality, particularly in the tropics. The Yucatan Peninsula is a fairly pristine site due to predominant trade winds, but occasionally BB and AD plumes severely degrade its air quality. The African Dust And Biomass Burning Over Yucatan (ADABBOY) project (January 2017–August 2018) was conducted in the Yucatan Peninsula to characterize physical and biological properties of particulate pollution at remote seaside and urban sites. The 18-month-long project quantified the large interannual variability in frequency and spatial extent of BB and AD plumes. Remote and urban sites experienced air quality degradation under the influence of these plumes, with up to 200% and 300% increases in coarse particle mass under BB and AD influence, respectively. ADABBOY is the first project to systematically characterize elemental composition of airborne particles as a function of these sources and identify bioaerosol over Yucatan. Bacteria, actinobacteria (both continental and marine), and fungi propagules vary seasonally and interannually and revealed the presence of very different species and genera associated with different sources. A novel contribution of ADABBOY was the determination of the ice-nucleating abilities of particles emitted by different sources within an undersampled region of the world. BB particles were found to be inefficient ice-nucleating particles at temperatures warmer than −20°C, whereas both AD and background marine aerosol activated ice-nucleating particles below −10°C.
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Liu, Chuan, Zhenping Yin, Yun He, and Longlong Wang. "Climatology of Dust Aerosols over the Jianghan Plain Revealed with Space-Borne Instruments and MERRA-2 Reanalysis Data during 2006–2021." Remote Sensing 14, no. 17 (September 5, 2022): 4414. http://dx.doi.org/10.3390/rs14174414.
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In recent years, climate change and the intervention of anthropogenic activities have altered the seasonal features of Asian dust storms. This may also cause seasonal variations (including dust occurrence frequency and optical/microphysical properties) in dust aerosols transported to downstream regions. The Jianghan Plain is dramatically influenced by multiple dust sources due to its geographical location in central China. In this study, we focused on the climatology of dust aerosols over the Jianghan Plain based on the 15-year (2006–2021) continuous space-borne observations of the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) as well as Modern-Era Retrospective Analysis for Research and Applications version 2 (MERRA-2) reanalysis data. A typical dust event that intrudes the Jianghan Plain was studied in detail. According to the statistical results, dust aerosols frequently intrude into the Jianghan Plain in spring and winter, with occurrence frequencies (under cloud free condition hereafter) exceeding 0.70 and higher altitudes of 4–6 km. The dust occurrence frequency declined to approximately 0.40 in autumn and nearly zero in summer, while the dust plumes were generally located at lower altitudes of 1–3 km. The dust plumes observed in the Jianghan Plain were simultaneously linked to the Taklimakan Desert and Gobi Desert in spring and mainly originated from the Taklimakan Desert in winter and autumn. The dust particles were mainly distributed below 4-km altitude, with the largest dust extinction coefficients and dust mass concentrations in spring. In all seasons, the particle depolarization ratios are 0.1–0.2 below 4-km altitude, suggesting a possible mix with local anthropogenic aerosols. The mean dust column mass concentrations in spring showed an evident declining trend from 210 µg m−2 in 2006 to 100 µg m−2 in 2021 in the Jianghan Plain, attributed to the reduced dust activity in the source regions of Asian dust.
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Johnson, M. S., N. Meskhidze, V. P. Kiliyanpilakkil, and S. Gassó. "Understanding the transport of Patagonian dust and its influence on marine biological activity in the South Atlantic Ocean." Atmospheric Chemistry and Physics Discussions 10, no. 11 (November 10, 2010): 27283–320. http://dx.doi.org/10.5194/acpd-10-27283-2010.
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Abstract. The supply of bioavailable iron to the high-nitrate low-chlorophyll (HNLC) waters of the Southern Ocean through atmospheric pathways could stimulate phytoplankton blooms and have major implications for the global carbon cycle. In this study, model results and remotely-sensed data are analyzed to examine the horizontal and vertical transport pathways of Patagonian dust and quantify the effect of iron-laden mineral dust deposition on marine biological productivity in the surface waters of the South Atlantic Ocean (SAO). Model simulations for the atmospheric transport and deposition of mineral dust and bioavailable iron are carried out for two large dust outbreaks originated at the source regions of Northern Patagonia during the austral summer of 2009. Model-simulated horizontal and vertical transport pathways of Patagonian dust plumes are in reasonable agreement with remotely-sensed data. Simulations indicate that the synoptic meteorological patterns of high and low pressure systems are largely accountable for dust transport trajectories over the SAO. According to model results and retrievals from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO), synoptic flows caused by opposing pressure systems (a high pressure system located to the east or north-east of a low pressure system) elevate the South American dust plumes well above the marine boundary layer. Under such conditions, the bulk concentration of mineral dust can quickly be transported around the low pressure system in a clockwise manner, follow the southeasterly advection pathway, and reach the HNLC waters of the SAO and Antarctica in ~3–4 days after emission from the source regions of Northern Patagonia. Two different mechanisms for dust-iron mobilization into a bioavailable form are considered in this study. A global 3-D chemical transport model (GEOS-Chem), implemented with an iron dissolution scheme, is employed to estimate the atmospheric fluxes of soluble iron, while a dust/biota assessment tool (Boyd et al., 2010) is applied to evaluate the amount of bioavailable iron formed through the slow and sustained leaching of dust in the ocean mixed layer. The effect of iron-laden mineral dust supply on surface ocean biomass is investigated by comparing predicted surface chlorophyll-a concentration ([Chl-a]) to remotely-sensed data. As the dust transport episodes examined here represent large summertime outflows of mineral dust from South American continental sources, this study suggests that (1) atmospheric fluxes of mineral dust from Patagonia are not likely to be the major source of bioavailable iron to ocean regions characterized by high primary productivity; (2) even if Patagonian dust plumes may not cause visible algae blooms, they could still influence background [Chl-a] in the South Atlantic sector of the Southern Ocean.
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Johnson, M. S., N. Meskhidze, V. P. Kiliyanpilakkil, and S. Gassó. "Understanding the transport of Patagonian dust and its influence on marine biological activity in the South Atlantic Ocean." Atmospheric Chemistry and Physics 11, no. 6 (March 17, 2011): 2487–502. http://dx.doi.org/10.5194/acp-11-2487-2011.
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Abstract. The supply of bioavailable iron to the high-nitrate low-chlorophyll (HNLC) waters of the Southern Ocean through atmospheric pathways could stimulate phytoplankton blooms and have major implications for the global carbon cycle. In this study, model results and remotely-sensed data are analyzed to examine the horizontal and vertical transport pathways of Patagonian dust and quantify the effect of iron-laden mineral dust deposition on marine biological productivity in the surface waters of the South Atlantic Ocean (SAO). Model simulations for the atmospheric transport and deposition of mineral dust and bioavailable iron are carried out for two large dust outbreaks originated at the source regions of northern Patagonia during the austral summer of 2009. Model-simulated horizontal and vertical transport pathways of Patagonian dust plumes are in reasonable agreement with remotely-sensed data. Simulations indicate that the synoptic meteorological patterns of high and low pressure systems are largely accountable for dust transport trajectories over the SAO. According to model results and retrievals from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO), synoptic flows caused by opposing pressure systems (a high pressure system located to the east or north-east of a low pressure system) elevate the South American dust plumes well above the marine boundary layer. Under such conditions, the bulk concentration of mineral dust can quickly be transported around the low pressure system in a clockwise manner, follow the southeasterly advection pathway, and reach the HNLC waters of the SAO and Antarctica in ~3–4 days after emission from the source regions of northern Patagonia. Two different mechanisms for dust-iron mobilization into a bioavailable form are considered in this study. A global 3-D chemical transport model (GEOS-Chem), implemented with an iron dissolution scheme, is employed to estimate the atmospheric fluxes of soluble iron, while a dust/biota assessment tool (Boyd et al., 2010) is applied to evaluate the amount of bioavailable iron formed through the slow and sustained leaching of dust in the ocean mixed layer. The effect of iron-laden mineral dust supply on surface ocean biomass is investigated by comparing predicted surface chlorophyll-a concentration ([Chl-a]) to remotely-sensed data. As the dust transport episodes examined here represent large summertime outflows of mineral dust from South American continental sources, this study suggests that (1) atmospheric fluxes of mineral dust from Patagonia are not likely to be the major source of bioavailable iron to ocean regions characterized by high primary productivity; (2) even if Patagonian dust plumes may not cause visible algae blooms, they could still influence background [Chl-a] in the South Atlantic sector of the Southern Ocean.
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Smith, David J., Hilkka J. Timonen, Daniel A. Jaffe, Dale W. Griffin, Michele N. Birmele, Kevin D. Perry, Peter D. Ward, and Michael S. Roberts. "Intercontinental Dispersal of Bacteria and Archaea by Transpacific Winds." Applied and Environmental Microbiology 79, no. 4 (December 7, 2012): 1134–39. http://dx.doi.org/10.1128/aem.03029-12.
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ABSTRACTMicroorganisms are abundant in the upper atmosphere, particularly downwind of arid regions, where winds can mobilize large amounts of topsoil and dust. However, the challenge of collecting samples from the upper atmosphere and reliance upon culture-based characterization methods have prevented a comprehensive understanding of globally dispersed airborne microbes. In spring 2011 at the Mt. Bachelor Observatory in North America (2.8 km above sea level), we captured enough microbial biomass in two transpacific air plumes to permit a microarray analysis using 16S rRNA genes. Thousands of distinct bacterial taxa spanning a wide range of phyla and surface environments were detected before, during, and after each Asian long-range transport event. Interestingly, the transpacific plumes delivered higher concentrations of taxa already in the background air (particularlyProteobacteria,Actinobacteria, andFirmicutes). While some bacterial families and a few marine archaea appeared for the first and only time during the plumes, the microbial community compositions were similar, despite the unique transport histories of the air masses. It seems plausible, when coupled with atmospheric modeling and chemical analysis, that microbial biogeography can be used to pinpoint the source of intercontinental dust plumes. Given the degree of richness measured in our study, the overall contribution of Asian aerosols to microbial species in North American air warrants additional investigation.
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Vernon, Charles J., Ryan Bolt, Timothy Canty, and Ralph A. Kahn. "The impact of MISR-derived injection height initialization on wildfire and volcanic plume dispersion in the HYSPLIT model." Atmospheric Measurement Techniques 11, no. 11 (November 21, 2018): 6289–307. http://dx.doi.org/10.5194/amt-11-6289-2018.
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Abstract. The dispersion of particles from wildfires, volcanic eruptions, dust storms, and other aerosol sources can affect many environmental factors downwind, including air quality. Aerosol injection height is one source attribute that mediates downwind dispersion, as wind speed and direction can vary dramatically with elevation. Using plume heights derived from space-based, multi-angle imaging, we examine the impact of initializing plumes in the NOAA Air Resources Laboratory's Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model with satellite-measured vs. nominal (model-calculated or VAAC-reported) injection height on the simulated dispersion of six large aerosol plumes. When there are significant differences in nominal vs. satellite-derived particle injection heights, especially if both heights are in the free troposphere or if one injection height is within the planetary boundary layer (PBL) and the other is above the PBL, differences in simulation results can arise. In the cases studied with significant nominal vs. satellite-derived injection height differences, the HYSPLIT model can represent plume evolution better, relative to independent satellite observations, if the injection height in the model is constrained by hyper-stereo satellite retrievals.
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Kaskaoutis, Francis, Rashki, Chaboureau, and Dumka. "Atmospheric Dynamics from Synoptic to Local Scale During an Intense Frontal Dust Storm over the Sistan Basin in Winter 2019." Geosciences 9, no. 10 (October 22, 2019): 453. http://dx.doi.org/10.3390/geosciences9100453.
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The Sistan Basin has been recognized as one of the most active dust sources and windiest desert environments in the world. Although the dust activity in Sistan maximizes during the summer, rare but intense dust storms may also occur in the winter. This study aims to elucidate the atmospheric dynamics related to dust emission and transport, dust-plume characteristics, and impacts on aerosol properties and air quality during an intense dust storm over Sistan in February 2019. The dust storm was initiated by strong northerly winds (~20 ms−1) associated with the intrusion of a cold front from high latitudes. The upper-level potential vorticity (PV)-trough evolved into a cut-off low in the mid and upper troposphere and initiated unstable weather over Afghanistan and northern Pakistan. At the surface, density currents emanating from deep convective clouds and further strengthened by downslope winds from the mountains, caused massive soil erosion. The passage of the cold front reduced the temperature by ~10 °C and increased the atmospheric pressure by ~10 hPa, while the visibility was limited to less than 200 m. The rough topography played a major role in modulating the atmospheric dynamics, wind field, dust emissions, and transport pathways. Meso-NH model simulates large amounts of columnar mass dust loading (> 20 g m−2) over Sistan, while the intense dust plume was mainly traveling below 2 km and increased the particulate matter (PM10) concentrations up to 1800 µg m−3 at Zabol. The dust storm was initially moving in an arc-shaped pathway over the Sistan Basin and then it spread away. Plumes of dust covered a large area in southwest Asia, reaching the northern Arabian Sea, and the Thar desert one to two days later, while they strongly affected the aerosol properties at Karachi, Pakistan, by increasing the aerosol optical depth (AOD > 1.2) and the coarse-mode fraction at ~0.7.
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Wagner, Robert, Michael Jähn, and Kerstin Schepanski. "Wildfires as a source of airborne mineral dust – revisiting a conceptual model using large-eddy simulation (LES)." Atmospheric Chemistry and Physics 18, no. 16 (August 20, 2018): 11863–84. http://dx.doi.org/10.5194/acp-18-11863-2018.
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Abstract. Airborne mineral dust is a key player in the Earth system and shows manifold impacts on atmospheric properties such as the radiation budget and cloud microphysics. Investigations of smoke plumes originating from wildfires found significant fractions of mineral dust within these plumes – most likely raised by strong, turbulent fire-related winds. This study presents and revisits a conceptual model describing the emission of mineral dust particles during wildfires. This is achieved by means of high-resolution large-eddy simulation (LES), conducted with the All Scale Atmospheric Model (ASAM). The impact of (a) different fire properties representing idealized grassland and shrubland fires, (b) different ambient wind conditions modulated by the fire's energy flux, and (c) the wind's capability to mobilize mineral dust particles was investigated. Results from this study illustrate that the energy release of the fire leads to a significant increase in near-surface wind speed, which consequently enhances the dust uplift potential. This is in particular the case within the fire area where vegetation can be assumed to be widely removed and uncovered soil is prone to wind erosion. The dust uplift potential is very sensitive to fire properties, such as fire size, shape, and intensity, but also depends on the ambient wind velocity. Although measurements already showed the importance of wildfires for dust emissions, pyro-convection is so far neglected as a dust emission process in atmosphere–aerosol models. The results presented in this study can be seen as the first step towards a systematic parameterization representing the connection between typical fire properties and related dust emissions.
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Moseley, Eric R., Jonathan Squire, and Philip F. Hopkins. "Non-linear evolution of instabilities between dust and sound waves." Monthly Notices of the Royal Astronomical Society 489, no. 1 (August 12, 2019): 325–38. http://dx.doi.org/10.1093/mnras/stz2128.
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ABSTRACT We study the non-linear evolution of the acoustic ‘resonant drag instability’ (RDI) using numerical simulations. The acoustic RDI is excited in a dust–gas mixture when dust grains stream through gas, interacting with sound waves to cause a linear instability. We study this process in a periodic box by accelerating neutral dust with an external driving force. The instability grows as predicted by linear theory, eventually breaking into turbulence and saturating. As in linear theory, the non-linear behaviour is characterized by three regimes – high, intermediate, and low wavenumbers – the boundary between which is determined by the dust–gas coupling strength and the dust-to-gas mass ratio. The high and intermediate wavenumber regimes behave similarly to one another, with large dust-to-gas ratio fluctuations while the gas remains largely incompressible. The saturated state is highly anisotropic: dust is concentrated in filaments, jets, or plumes along the direction of acceleration, with turbulent vortex-like structures rapidly forming and dissipating in the perpendicular directions. The low-wavenumber regime exhibits large fluctuations in gas and dust density, but the dust and gas remain more strongly coupled in coherent ‘fronts’ perpendicular to the acceleration. These behaviours are qualitatively different from those of dust ‘passively’ driven by external hydrodynamic turbulence, with no back-reaction force from dust on to gas. The virulent nature of these instabilities has interesting implications for dust-driven winds in a variety of astrophysical systems, including around cool stars, in dusty torii around active-galactic-nuclei, and in and around giant molecular clouds.
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Nisantzi, A., R. E. Mamouri, A. Ansmann, and D. Hadjimitsis. "Injection of mineral dust into the free troposphere during fire events observed with polarization lidar at Limassol, Cyprus." Atmospheric Chemistry and Physics Discussions 14, no. 11 (June 27, 2014): 17299–329. http://dx.doi.org/10.5194/acpd-14-17299-2014.
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Abstract. Four-year observations (2010–2014) with EARLINET polarization lidar and AERONET sun/sky photometer at Limassol (34.7° N, 33° E), Cyprus, were used to study the soil dust content in lofted fire smoke plumes advected from Turkey. This first systematic attempt to characterize less than 3 days old smoke plumes in terms of particle depolarization contributes to the more general effort to properly describe the life cycle of free-tropospheric smoke–dust mixtures from the emission event to phases of long-range transport (>4 days after emission). We found significant differences in the particle depolarization ratio (PDR) with values from 9–18% in lofted aerosol layers when Turkish fires contributed to the aerosol burden and of 3–13% when Turkish fires were absent. High Ångström exponents of 1.4–2.2 during all these events with lofted smoke layers, occuring between 1 and 3 km height, suggest the absence of a pronounced particle coarse mode. When plotted vs. the travel time (spatial distance between Limassol and last fire area), PDR decreased strongly from initial values around 16–18% (one day travel) to 4–8% after 4 days of travel caused by deposition processes. This behavior was found to be in close agreement with the literature. Computation of particle extinction coefficient and mass concentrations, separately for fine-mode dust, coarse-mode dust, and non-dust aerosol components show extinction-related dust fractions of the order of 10% (for PDR = 4%, travel times >4 days) and 50% (PDR = 15%, one day travel time) and mass-related dust fractions of 25% (PDR = 4%) to 80% (PDR = 15%). Biomass burning should be considered as another source of free tropospheric soil dust.
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Rizza, Umberto, Vagner Anabor, Cristina Mangia, Mario Marcello Miglietta, Gervasio Annes Degrazia, and Giorgio Passerini. "WRF-CHEM SIMULATION OF A SAHARAN DUST OUTBREAK OVER THE MEDITERRANEAN REGIONS." Ciência e Natura 38 (July 20, 2016): 330. http://dx.doi.org/10.5902/2179460x20249.
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A fully coupled meteorology-chemistry-aerosol model (WRF-Chem) is applied to simulate the Saharan dust outbreak over the Mediterranean regions. Two dust emission schemes, namely, those of Jones et al., (2010), and Shao (2001) are evaluated using the the GOCART aerosol model. To investigate the performance of each dust emission scheme, a case study was carried out for a Mediterranean dust event that took place between 21 and 23 May 2014. Considering the time average Aerosol Optical Depth, simulation results reproduced satisfactorily the outbreak and transport pattern of dust plumes. However, the estimated dust emission amounts in each scheme differ greatly due to the presence of several tuning parameters, that must be adjusted considering satellite and ground based experimental data.
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Lu, Xiaoman, Xiaoyang Zhang, Fangjun Li, Mark A. Cochrane, and Pubu Ciren. "Detection of Fire Smoke Plumes Based on Aerosol Scattering Using VIIRS Data over Global Fire-Prone Regions." Remote Sensing 13, no. 2 (January 8, 2021): 196. http://dx.doi.org/10.3390/rs13020196.
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Smoke from fires significantly influences climate, weather, and human health. Fire smoke is traditionally detected using an aerosol index calculated from spectral contrast changes. However, such methods usually miss thin smoke plumes. It also remains challenging to accurately separate smoke plumes from dust, clouds, and bright surfaces. To improve smoke plume detections, this paper presents a new scattering-based smoke detection algorithm (SSDA) depending mainly on visible and infrared imaging radiometer suite (VIIRS) blue and green bands. The SSDA is established based on the theory of Mie scattering that occurs when the diameter of an atmospheric particulate is similar to the wavelength of the scattered light. Thus, smoke commonly causes Mie scattering in VIIRS blue and green bands because of the close correspondence between smoke particulate diameters and the blue/green band wavelengths. For developing the SSDA, training samples were selected from global fire-prone regions in North America, South America, Africa, Indonesia, Siberia, and Australia. The SSDA performance was evaluated against the VIIRS aerosol detection product and smoke detections from the ultraviolet aerosol index using manually labeled fire smoke plumes as a benchmark. Results show that the SSDA smoke detections are superior to existing products due chiefly to the improved ability of the algorithm to detect thin smoke and separate fire smoke from other surface types. Moreover, the SSDA smoke distribution pattern exhibits a high spatial correlation with the global fire density map, suggesting that SSDA is capable of detecting smoke plumes of fires in near real-time across the globe.
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Lu, Xiaoman, Xiaoyang Zhang, Fangjun Li, Mark A. Cochrane, and Pubu Ciren. "Detection of Fire Smoke Plumes Based on Aerosol Scattering Using VIIRS Data over Global Fire-Prone Regions." Remote Sensing 13, no. 2 (January 8, 2021): 196. http://dx.doi.org/10.3390/rs13020196.
Full textAbstract:
Smoke from fires significantly influences climate, weather, and human health. Fire smoke is traditionally detected using an aerosol index calculated from spectral contrast changes. However, such methods usually miss thin smoke plumes. It also remains challenging to accurately separate smoke plumes from dust, clouds, and bright surfaces. To improve smoke plume detections, this paper presents a new scattering-based smoke detection algorithm (SSDA) depending mainly on visible and infrared imaging radiometer suite (VIIRS) blue and green bands. The SSDA is established based on the theory of Mie scattering that occurs when the diameter of an atmospheric particulate is similar to the wavelength of the scattered light. Thus, smoke commonly causes Mie scattering in VIIRS blue and green bands because of the close correspondence between smoke particulate diameters and the blue/green band wavelengths. For developing the SSDA, training samples were selected from global fire-prone regions in North America, South America, Africa, Indonesia, Siberia, and Australia. The SSDA performance was evaluated against the VIIRS aerosol detection product and smoke detections from the ultraviolet aerosol index using manually labeled fire smoke plumes as a benchmark. Results show that the SSDA smoke detections are superior to existing products due chiefly to the improved ability of the algorithm to detect thin smoke and separate fire smoke from other surface types. Moreover, the SSDA smoke distribution pattern exhibits a high spatial correlation with the global fire density map, suggesting that SSDA is capable of detecting smoke plumes of fires in near real-time across the globe.
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Sekiyama, T. T., T. Y. Tanaka, and T. Miyoshi. "A simulation study of the ensemble-based data assimilation of satellite-borne lidar aerosol observations." Geoscientific Model Development Discussions 5, no. 3 (July 23, 2012): 1877–947. http://dx.doi.org/10.5194/gmdd-5-1877-2012.
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Abstract. A four-dimensional ensemble-based data assimilation system was assessed by observing system simulation experiments (OSSEs), in which the CALIPSO satellite was emulated via simulated satellite-borne lidar aerosol observations. Its performance over athree-month period was validated according to the Method for Object-based Diagnostic Evaluation (MODE), using aerosol optical thickness (AOT) distributions in East Asia as the objects of analysis. Consequently, this data assimilation system demonstrated the ability to produce better analyses of sulfate and dust aerosols in comparison to a free-running simulation model. For example, the mean centroid distance (from the truth) over a three-month collection period of aerosol plumes was improved from 2.15 grids (&approx; 600 km) to 1.45 grids (&approx; 400 km) for sulfate aerosols and from 2.59 grids (&approx; 750 km) to 1.14 grids (&approx; 330 km) for dust aerosols; the mean area ratio (to the truth) over a three-month collection period of aerosol plumes was improved from 0.49 to 0.76 for sulfate aerosols and from 0.51 to 0.72 for dust aerosols. The satellite-borne lidar data assimilation successfully improved the aerosol plume analysis and the dust emission estimation in the OSSEs. These results present great possibilities for the beneficial use of lidar data, whose distribution is vertically/temporally dense but horizontally sparse, when coupled with a four-dimensional data assimilation system. In addition, sensitivity tests were conducted, and their results indicated that the degree of freedom to control the aerosol variables was probably limited in the data assimilation because the meteorological field in the system was constrained to weather reanalysis using Newtonian relaxation. Further improvements to the aerosol analysis can be performed through the simultaneous assimilation of aerosol observations with meteorological observations. The OSSE results strongly suggest that the use of real CALIPSO data will have a beneficial effect on obtaining more accurate sulfate and dust aerosol analyses. Furthermore, the use of the same OSSE technique will allow us to perform a prior assessment of the next-generation lidar satellite EarthCARE, which will be launched in 2015.
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Marinou, Eleni, Vassilis Amiridis, Ioannis Binietoglou, Athanasios Tsikerdekis, Stavros Solomos, Emannouil Proestakis, Dimitra Konsta, et al. "Three-dimensional evolution of Saharan dust transport towards Europe based on a 9-year EARLINET-optimized CALIPSO dataset." Atmospheric Chemistry and Physics 17, no. 9 (May 12, 2017): 5893–919. http://dx.doi.org/10.5194/acp-17-5893-2017.
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Abstract. In this study we use a new dust product developed using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) observations and EARLINET (European Aerosol Research Lidar Network) measurements and methods to provide a 3-D multiyear analysis on the evolution of Saharan dust over North Africa and Europe. The product uses a CALIPSO L2 backscatter product corrected with a depolarization-based method to separate pure dust in external aerosol mixtures and a Saharan dust lidar ratio (LR) based on long-term EARLINET measurements to calculate the dust extinction profiles. The methodology is applied on a 9-year CALIPSO dataset (2007–2015) and the results are analyzed here to reveal for the first time the 3-D dust evolution and the seasonal patterns of dust over its transportation paths from the Sahara towards the Mediterranean and Continental Europe. During spring, the spatial distribution of dust shows a uniform pattern over the Sahara desert. The dust transport over the Mediterranean Sea results in mean dust optical depth (DOD) values up to 0.1. During summer, the dust activity is mostly shifted to the western part of the desert where mean DOD near the source is up to 0.6. Elevated dust plumes with mean extinction values between 10 and 75 Mm−1 are observed throughout the year at various heights between 2 and 6 km, extending up to latitudes of 40° N. Dust advection is identified even at latitudes of about 60° N, but this is due to rare events of episodic nature. Dust plumes of high DOD are also observed above the Balkans during the winter period and above northwest Europe during autumn at heights between 2 and 4 km, reaching mean extinction values up to 50 Mm−1. The dataset is considered unique with respect to its potential applications, including the evaluation of dust transport models and the estimation of cloud condensation nuclei (CCN) and ice nuclei (IN) concentration profiles. Finally, the product can be used to study dust dynamics during transportation, since it is capable of revealing even fine dynamical features such as the particle uplifting and deposition on European mountainous ridges such as the Alps and Carpathian Mountains.