Relevant bibliographies by topics / Dinitrogen

Academic literature on the topic 'Dinitrogen'

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Published: 4 June 2021
Last updated: 20 February 2023

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Journal articles on the topic "Dinitrogen"

1

KEMSLEY, JYLLIAN. "MAKING DINITROGEN." Chemical & Engineering News Archive 89, no. 41 (October 10, 2011): 10. http://dx.doi.org/10.1021/cen-v089n041.p010a.

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Wentrup, Curt, Stephan Fischer, Andre Maquestiau, and Robert Flammang. "Dinitrogen sulfide." Journal of Organic Chemistry 51, no. 10 (May 1986): 1908–10. http://dx.doi.org/10.1021/jo00360a051.

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Crossland, Justin L., and David R. Tyler. "Iron–dinitrogen coordination chemistry: Dinitrogen activation and reactivity." Coordination Chemistry Reviews 254, no. 17-18 (September 2010): 1883–94. http://dx.doi.org/10.1016/j.ccr.2010.01.005.

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Waterman, Rory, and Gregory L. Hillhouse. "Synthesis and structure of a terminal dinitrogen complex of nickel." Canadian Journal of Chemistry 83, no. 4 (April 1, 2005): 328–31. http://dx.doi.org/10.1139/v05-011.

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Reaction of petroleum ether solutions of [(dtbpe)Ni]2(η2,µ-C6H6) (1, dtbpe = 1,2-bis(di-tert-butylphosphino)ethane) with triphenylphosphine under a dinitrogen atmosphere gives the Ni(0) dinitrogen adduct (dtbpe)Ni(N2)(PPh3) (2), which can be isolated as dark red crystals in 87% yield. The X-ray crystal structure of 2 reveals pseudotetrahedral geometry about Ni and a terminal dinitrogen ligand with Ni—N(1) = 1.830(2) Å, N(1)—N(2) = 1.112(2) Å, and Ni-N(1)-N(2) = 177.5(2)°. Key words: dinitrogen, nickel, X-ray.
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Evans, William J., and David S. Lee. "Early developments in lanthanide-based dinitrogen reduction chemistry." Canadian Journal of Chemistry 83, no. 4 (April 1, 2005): 375–84. http://dx.doi.org/10.1139/v05-014.

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Although the first crystallographically characterized lanthanide dinitrogen complex was reported in 1988 with samarium, it is only in recent years that this field has expanded to include fully characterized examples for the entire series of lanthanides. The development of lanthanide dinitrogen chemistry has been aided by a series of unexpected results that present some good lessons in the development of science. This review presents a chronological account of the lanthanide dinitrogen chemistry discovered in our laboratory through the summer of 2004.Key words: lanthanides, dinitrogen, reduction, alkali metal, nitrogen fixation, diazenido.
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Hidai, Masanobu, and Yasushi Mizobe. "Chemical nitrogen fixation by using molybdenum and tungsten complexes." Pure and Applied Chemistry 73, no. 2 (January 1, 2001): 261–63. http://dx.doi.org/10.1351/pac200173020261.

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Dinitrogen complex cis-[W (N2) 2 (PMe2Ph) 4] reacts with an excess of acidic dihydrogen complexes such as trans-[RuCl (h2-H2) (dppe) 2]BF4 (dppe = 1,2-bis (diphenylphosphino) ethane) at 55 °C under 1 atm of H2 to form ammonia in moderate yield. The reaction is presumed to proceed through nucleophilic attack of the remote nitrogen of the coordinated dinitrogen on the dihydrogen ligand. The coordinated dinitrogen is also protonated by treatment with hydrosulfido-bridged dinuclear complexes such as [Cp*Ir (m-SH) 3IrCp*]Cl (Cp* = h5-C5Me5) to afford ammonia. On the other hand, the synthetic cycle for the formation of pyrrole and N-aminopyrrole from dinitrogen and 2,5-dimethoxytetrahydrofuran has been established starting from dinitrogen complexes of the type trans-[M (N2) 2 (dppe) 2 ] (M = Mo, W).
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Cheng, Qianyi, Maura C. Washington, Joseph E. Burns, Ryan C. Fortenberry, and Nathan J. DeYonker. "Spectroscopic study of magnesium dinitrogen and sodium dinitrogen cation." Monthly Notices of the Royal Astronomical Society 498, no. 4 (September 3, 2020): 5417–23. http://dx.doi.org/10.1093/mnras/staa2646.

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ABSTRACT Despite its likely importance in astrochemistry, pure rotational spectra are not observable for gas-phase N2 since this molecule has no permanent dipole moment. Complexation of monomeric N2 with a cationic metal (MN2+) may be kinetically and thermodynamically favourable, and the detection of such MN2+ molecules could be useful tracers of N2 in order to probe its abundance and kinetics. Highly accurate quartic force field methods have been applied here to compute rotational and vibrational spectroscopic properties of the NaN2+ and MgN2+ molecules via a coupled cluster-based composite approach with additional corrections for post-CCSD(T) electron correlation and relativistic effects. The relative energies of various isomers have also been computed and show that both NaN2+ and MgN2+ have linear ground electronic states. At the highest level of theory, rotational constants (B0) of 4086.9 and 4106.0 MHz are predicted for NaN2+ and MgN2+, respectively, with dipole moments of 6.92 and 4.34 D, respectively, making them rotationally observable even at low concentrations. Post-CCSD(T) electron correlation corrections lower the N–N stretching frequency while relativistic corrections have a much smaller effect putting the fundamental frequencies at 2333.7 and 2313.6 cm−1, respective of NaN2+ and MgN2+ slightly above that in N2H+. Additive corrections do not significantly change the other two vibrational modes. An anharmonic, zero-point corrected N2 dissociation energy of 7.3 and 7.0 kcal mol−1 is, respectively, reported for NaN2+ and MgN2+ suggesting possible formation of these molecules in protoplanetary discs or planetary nebulae that are metal- and nitrogen-rich.
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Connor, Gannon P., Nicholas Lease, Andrea Casuras, Alan S. Goldman, Patrick L. Holland, and James M. Mayer. "Protonation and electrochemical reduction of rhodium– and iridium–dinitrogen complexes in organic solution." Dalton Trans. 46, no. 41 (2017): 14325–30. http://dx.doi.org/10.1039/c7dt03476h.

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Yeston, Jake. "Calcium catches dinitrogen." Science 371, no. 6534 (March 11, 2021): 1117.8–1118. http://dx.doi.org/10.1126/science.371.6534.1117-h.

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Bethany Halford. "Calcium captures dinitrogen." C&EN Global Enterprise 99, no. 9 (March 15, 2021): 4. http://dx.doi.org/10.1021/cen-09909-leadcon.

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Dissertations / Theses on the topic "Dinitrogen"

1

Stephens, R. J. "Aromatic nitrations using dinitrogen pentoxide." Thesis, University of Exeter, 1985. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.370935.

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Karriem, Fatiema. "Oxidative fixation of dinitrogen by photocatalysis." Thesis, University of Western Cape, 2000. http://etd.uwc.ac.za/index.php?module=etd&action=viewtitle&id=gen8Srv25Nme4_5777_1267648612.

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The heterogeneous photocatalytic oxidation of dinitrogen to nitrate, NO3 and/or nitrite, no2 using peroxy species of titanium (IV) in aqueous suspensions has been investigated. The photocatalysts used were titanium peroxide and Degussa p25 TiO2 pretreated with H2O2. These photocatalysts were investigated by SEM and FTIR spectroscopy.  

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Park, Rosa. "Investigating new reactions for coordinated dinitrogen." Thesis, University of British Columbia, 2008. http://hdl.handle.net/2429/2344.

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The chemistry of the tantalum dinitrogen complex ([NPN]Ta)₂‚‚(μ-H)₂‚‚(μ-η¹:η²-N₂‚‚)Ta-[NPN], 1, (where [NPN] represents the acyclic tridentate ligand [(PhNSiMe₂‚‚CH₂‚‚)₂‚‚-PPh]²‚‚-), with primary alkenes, group IV and V metallocene complexes, and GaCp* is explored. The reaction of 1 with 1-pentene and 1-hexene occurs via olefin-insertion into the metal-hydride bond to give two new complexes, ([NPN]Ta(CH₂)₄CH₃)₂‚‚(μ-η¹:η¹-N₂‚‚), 10, and ([NPN]Ta(CH₂‚‚)₅CH₃)₂‚‚(μ-η¹:η¹-N₂‚‚), 11, which were characterized using NMR spectroscopy. The solid-state structure of 11 was established and revealed that N₂ has been transformed into a bridging end-on mode. In contrast to its G symmetry in solution, the solid-state structure of 11 is C, symmetric; a VT-NMR study was performed and showed that 11 exists as an equilibrium between two isomers in solution: a C, symmetric isomer 11A,which is the predominant isomer at room temperature, and a C, symmetric isomer 11B,which is the minor isomer. The reactivity of 1 with group IV and V metallocenes was investigated. The reaction of 1 with Cp₂‚‚Hf(PMe₃)(η²-Me₃SiCCSiMe₃) produces [N(μ-P=N)N]Ta(μ-H)₂(μ-N(Hf-Cp₂‚‚))Ta[NPN], 14, in which N₂ is cleaved and new Hf-N and P=N bonds have formed. The reaction of 1 with group V metallocene hydrides Cp₂‚‚MH₃ (M Nb, Ta) was also attempted however these complexes do not react with 1. The reaction of 1 with GaCp* produces a new complex, [NPN]Ta(μ-N(GaCp*))Ta(=NPμ)[NPIA,-N], 18, which was characterized using NMR spectroscopy. Complex 18 decomposes over several days in solution, and one product of decomposition that was isolated was [(PhNH)(NPμ-N)Ta]₂‚‚, 19. The solid-state structure of 19 showed that the [NPN] ligand was cleaved at the N-Si bond, similar to that observed for the reaction of 1 with 9-BBN and HB(C₆H₅)₂‚‚. A mechanism for the formation of complexes 18 and 19 is proposed.
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Dormer, Jonathan Charles. "Nitrations and oxidations with dinitrogen pentoxide." Thesis, University of Exeter, 1994. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.385700.

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Chan, Sam Yun Fu. "Extended-chain complexes of dinitrogen-based ligands." Thesis, University of Reading, 2004. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.408160.

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Sanderson, A. J. "Nitration with dinitrogen pentoxide in nitric acid." Thesis, University of Exeter, 1988. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.232979.

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Bultitude, John. "Vanadium complexes in relation to dinitrogen fixation." Thesis, University of Surrey, 1987. http://epubs.surrey.ac.uk/847178/.

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The aim of this work was to investigate the chemistry of vanadium in relation to dinitrogen fixation and consequently the literature concerning vanadium systems which reduce dinitrogen in protic media and the coordination compounds of vanadium(II) and vanadium(III) has been surveyed. In view of the importance of tertiary phosphines in the stabilisation of dinitrogen complexes of second and third row transition metals, methyldiphenylphosphine complexes of vanadium(III), (VCl3(PPh2Me)2) and (VCl3(MeCN) (PPh2Me)2) have been prepared and their electronic spectra and magnetic moments measured. The structures, determined by single crystal X-ray diffraction methods, are trigonal bipyramidal, (VCl3(PPh2Me)2), and octahedral, (VCl3(MeCN) (PPH2Me)2), with the phosphines occupying axial positions in both complexes. Attempts to reduce these complexes did not give any products reactive towards dinitrogen. Hydrated vanadium(II) salts (V(H2O)6)SO4, trans-(V(H2O)4Cl2), and (V(H2O)6)Br2 , were prepared by electrolytic reduction of the corresponding vanadyl solutions for use in the preparation of more reactive vanadium(II) complexes. (V(MeOH)6)Br2 was prepared from the hydrate and used to prepare (VBr2(thf)2) which was used in turn to prepare (VBr2(dppe)2). The diffuse reflectance spectra and magnetic moments of these complexes are consistent with octahedral stereochemistries throughout. The tetrahydrofuran complex is thought to be a bromide-bridged polymer and the phosphine complex is thought to be trans-(VBr2(dppe)2).
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Smith, Steven Escar. "Satellite measurements of dinitrogen pentoxide in the stratosphere." Thesis, University of Oxford, 1996. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.337541.

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Doyle, Laurence. "Dinitrogen activation and reduction with iron phosphine complexes." Thesis, Imperial College London, 2015. http://hdl.handle.net/10044/1/51149.

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The conversion of dinitrogen to ammonia is a fundamental process for sustaining life on our planet. Ammonia provides a source of fixed nitrogen for nitrification and assimilation into plants, and is the ultimate source of almost all nitrogenated compounds. Synthetic ammonia is produced on a colossal scale by the Haber Bosch process, with an annual ammonia output exceeding 130 million tonnes. However, the intensive operating conditions of this process require a staggering energy cost; hence, the development of a lower energy solution is recognised as one of the major challenges of modern chemistry. This dissertation explores the chemistry of homogeneous systems based on iron diphosphine complexes that are able to transform coordinated dinitrogen into ammonia. A greater understanding of these systems may provide insight into the iron-based catalysts utilised in both biological nitrogen fixation and the industrial Haber Bosch process. Ultimately, this could lead to a more sustainable process for meeting the global requirement for fixed nitrogen. Chapter 1 provides a general introduction into dinitrogen fixation chemistry, with a particular focus on homogeneous systems involving iron. Chapter 2 describes a convenient synthetic protocol to 1,2-bis(dialkylphosphino)ethanes. These are among the most versatile ligands used in inorganic chemistry, although issues with prior syntheses, often involving extremely hazardous phosphine precursors, has limited their accessibility. Chapter 3 is an exploration of a seminal work on dinitrogen fixation involving iron complexes, which facilitate the conversion of coordinated dinitrogen to ammonia in what is known as the Leigh cycle. Mechanistic understanding of the key ammonia producing step has provided the focus of considerable interest and speculation for over a decade. Chapter 4 provides insight into the dinitrogen and dihydrogen affinity of an iron(I) complex. Chapter 5 details the experimental procedures performed in this work.
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Curley, John Joseph. "Dinitrogen fixation chemistry of a molybdenum trisanilide system." Thesis, Massachusetts Institute of Technology, 2009. http://hdl.handle.net/1721.1/49549.

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Thesis (Ph. D.)--Massachusetts Institute of Technology, Dept. of Chemistry, 2009.
This electronic version was submitted by the student author. The certified thesis is available in the Institute Archives and Special Collections.
Vita.
Includes bibliographical references.
Dinitrogen cleavage by Mo(N[t-Bu]Ar)3 (Ar = 3,5-C6H3Me2) proceeds through the intermediate ([mu]-N2)[Mo(N[t-Bu]Ar)3]2 before forming N=Mo(N[t-Bu]Ar)3 as the product. Both the intermediate bridging N2 complex and the nitride product have been structurally characterized by single-crystal X-ray diffraction. The spectroscopic and structural features of this bridging N2 complex are discussed in comparison to its one- and two-electron oxidized congeners, [([mu]-N2)[Mo(N[t-Bu]Ar)3]2]n+, n = 1, 2. This series of three complexes share a common chromophore, the nature of which was identified with the aid of time-dependent density functional theory. A photochemical reaction of ([mu]-N2)[Mo(N[t-Bu]Ar)3]2 that forms both Mo(N[t-Bu]Ar)3 and N=Mo(N[t-Bu]Ar)3 is described. The dynamics of this photochemical reaction are explored by ultrafast transient absorbance spectroscopy. A synthetic scheme for nitrogen fixation in the form of organic nitriles is initiated from the product of dinitrogen cleavage, N=Mo(N[t-Bu]Ar)3. This synthetic scheme is a closed cycle that returns the molybdenum nitride starting material at the conclusion of the cycle. To achieve this synthetic goal, new methods were developed to form C-N bonds between organic electrophiles and the weakly nucleophilic terminal nitride. In a key reaction, Mo(IV) ketimide complexes, R'O(R)CNMo (N[t-Bu]Ar)3, were shown to react with either SnCl2 or ZnCl2 to afford the corresponding nitrile, RCN, and a ClMo(N[t-Bu]Ar)3 in essentially quantitative yields.
(cont.) The chloromolybdenum complex may be reductively recycled to yield Mo(N[t-Bu]Ar)3 for subsequent dinitrogen cleavage. A series of cationic diazoalkane complexes [4-RC6H4C(H)NNMo(N[t-Bu]Ar)3][AlCl4], R = NMe2, Me, H, Br, CN, have been prepared by treatment of the N2-derived diazenido complex Me3SiNNMo(N[t-Bu]Ar)3 with 4-RC6H4CHO and 2 equiv AlCl3. The physical properties of these complexes were determined by the use of X-ray crystallography, cyclic voltammetry, infrared, Raman, UV-vis, and 15N NMR spectroscopies. Electrochemical reduction of these cationic diazoalkane complexes forms the C-C bonded dimer, [mu]-(4-RC6H4C(H)NN)2[Mo(N[t-Bu]Ar)3]2, in a reaction that is proposed to proceed through the neutral, odd-electron complex 4-RC6H4C(H)NNMo(N[t-Bu]Ar)3. The structure of this odd-electron compound is described with the aid of density functional theory. The central C-C bond in [mu]-(4-RC6H4C(H)NN)2[Mo(N[t-Bu]Ar)3]2 is redox non-innocent, and oxidation of these compounds returns the cationic diazoalkane complex from which they were prepared.
by John Joseph Curley.
Ph.D.
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Books on the topic "Dinitrogen"

1

Nishibayashi, Yoshiaki, ed. Transition Metal-Dinitrogen Complexes. Weinheim, Germany: Wiley-VCH Verlag GmbH & Co. KGaA, 2019. http://dx.doi.org/10.1002/9783527344260.

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Hauck, R. D., and R. W. Weaver, eds. Field Measurement of Dinitrogen Fixation and Denitrification. Madison, WI, USA: Soil Science Society of America, 1986. http://dx.doi.org/10.2136/sssaspecpub18.

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Reinsvold, R. J. Use of biological dinitrogen-fixers for amelioration of minesoils. S.l: s.n, 1985.

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Wang, Haichao. The Chemistry of Nitrate Radical (NO3) and Dinitrogen Pentoxide (N2O5) in Beijing. Singapore: Springer Singapore, 2021. http://dx.doi.org/10.1007/978-981-15-8795-5.

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Jensen, E. S. Use of 15N Enriched Plant Material for labelling of soil nitrogen in legume dinitrogen fixaton experiments. Roskilde: Riso Library, 1989.

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Nishibayashi, Yoshiaki. Transition Metal-Dinitrogen Complexes: Preparation and Reactivity. Wiley & Sons, Incorporated, John, 2019.

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Nishibayashi, Yoshiaki. Transition Metal-Dinitrogen Complexes: Preparation and Reactivity. Wiley & Sons, Incorporated, John, 2019.

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Nishibayashi, Yoshiaki. Transition Metal-Dinitrogen Complexes: Preparation and Reactivity. Wiley & Sons, Incorporated, John, 2019.

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Hauck, Roland D., and R. W. Weaver. Field Measurement of Dinitrogen Fixation and Denitrification. Wiley & Sons, Limited, John, 2015.

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Nishibayashi, Yoshiaki. Transition Metal-Dinitrogen Complexes: Preparation and Reactivity. Wiley & Sons, Limited, John, 2019.

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Book chapters on the topic "Dinitrogen"

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Cleaves, Henderson James. "Dinitrogen." In Encyclopedia of Astrobiology, 653–54. Berlin, Heidelberg: Springer Berlin Heidelberg, 2015. http://dx.doi.org/10.1007/978-3-662-44185-5_438.

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Cleaves, Henderson James. "Dinitrogen." In Encyclopedia of Astrobiology, 437–38. Berlin, Heidelberg: Springer Berlin Heidelberg, 2011. http://dx.doi.org/10.1007/978-3-642-11274-4_438.

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Cleaves, Henderson James. "Dinitrogen." In Encyclopedia of Astrobiology, 1–2. Berlin, Heidelberg: Springer Berlin Heidelberg, 2014. http://dx.doi.org/10.1007/978-3-642-27833-4_438-4.

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Cleaves, Henderson James. "Dinitrogen." In Encyclopedia of Astrobiology, 1–2. Berlin, Heidelberg: Springer Berlin Heidelberg, 2022. http://dx.doi.org/10.1007/978-3-642-27833-4_438-5.

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Haubold, Reinhard, Claudia Heinrich-Sterzel, Peter Merlet, Ulrike Ohms-Bredeman, Carol Strametz, and Astrid Wietelmann. "Dinitrogen Compounds." In N Nitrogen, 1–86. Berlin, Heidelberg: Springer Berlin Heidelberg, 1993. http://dx.doi.org/10.1007/978-3-662-06336-1_1.

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van de Watering, Fenna F., and Wojciech I. Dzik. "Dinitrogen Reduction." In Non-Noble Metal Catalysis, 549–81. Weinheim, Germany: Wiley-VCH Verlag GmbH & Co. KGaA, 2018. http://dx.doi.org/10.1002/9783527699087.ch20.

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Weaver, R. W., and Seth K. A. Danso. "Dinitrogen Fixation." In SSSA Book Series, 1019–45. Madison, WI, USA: Soil Science Society of America, 2018. http://dx.doi.org/10.2136/sssabookser5.2.c43.

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Layzell, David B., and Angela H. M. Moloney. "Dinitrogen Fixation." In Physiology and Determination of Crop Yield, 311–35. Madison, WI, USA: American Society of Agronomy, Crop Science Society of America, Soil Science Society of America, 2015. http://dx.doi.org/10.2134/1994.physiologyanddetermination.c21.

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Beattie, I. R. "Dinitrogen Trioxide." In Progress in Inorganic Chemistry, 1–26. Hoboken, NJ, USA: John Wiley & Sons, Inc., 2007. http://dx.doi.org/10.1002/9780470166062.ch1.

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Vogt, J. "832 N4O Dinitrogen monoxide - dinitrogen (1/1)." In Asymmetric Top Molecules. Part 3, 481. Berlin, Heidelberg: Springer Berlin Heidelberg, 2011. http://dx.doi.org/10.1007/978-3-642-14145-4_254.

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Conference papers on the topic "Dinitrogen"

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Julie Larsen, John Classen, and Sarah Liehr. "Dinitrogen Gas Collection Method for Lagoon Waste Treatment Systems." In 2003, Las Vegas, NV July 27-30, 2003. St. Joseph, MI: American Society of Agricultural and Biological Engineers, 2003. http://dx.doi.org/10.13031/2013.14962.

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Baranov, Yu I., E. L. Baranova, and F. V. Kashin. "Ecological monitoring of methane, carbon oxides, and dinitrogen monoxide in air by Fourier-transform spectroscopy." In Sixth International Symposium on Atmospheric and Ocean Optics, edited by Gennadii G. Matvienko and Vladimir P. Lukin. SPIE, 1999. http://dx.doi.org/10.1117/12.370534.

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Tsuji, Takafumi, Yuuki Morimoto, Daisuke Funaki, Naoki Osawa, and Yoshio Yoshioka. "Decrease in dinitrogen monoxide (N2O) generation of air-fed ozone generator using Atmospheric Pressure Townsend Discharge." In 2014 IEEE 41st International Conference on Plasma Sciences (ICOPS) held with 2014 IEEE International Conference on High-Power Particle Beams (BEAMS). IEEE, 2014. http://dx.doi.org/10.1109/plasma.2014.7012617.

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Reports on the topic "Dinitrogen"

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Schrock, Richard. The Catalytic Reduction of Dinitrogen Under Mild Conditions. Office of Scientific and Technical Information (OSTI), May 2019. http://dx.doi.org/10.2172/1512074.

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Torrey, J. Structure and function of Frankia vesicles in dinitrogen fixing actinorhizal plants. Office of Scientific and Technical Information (OSTI), January 1990. http://dx.doi.org/10.2172/7192111.

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Sita, Lawrence. Investigation of Energy-Efficient Dinitrogen Activation and N-atom Transfer Processes. Office of Scientific and Technical Information (OSTI), August 2014. http://dx.doi.org/10.2172/1149037.

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Sherrill, William M., and Eric C. Johnson. A New Method for the Production of Tetranitroglycoluril From Imidazo-[4,5-d]-Imidazoles With the Loss of Dinitrogen Oxide. Fort Belvoir, VA: Defense Technical Information Center, February 2014. http://dx.doi.org/10.21236/ada598881.

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National Institute for Petroleum and Energy Research quarterly technical report, July 1--September 30, 1992. [Dinitrogen compound 1,10-phenanthroline]. Office of Scientific and Technical Information (OSTI), January 1993. http://dx.doi.org/10.2172/6733754.

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