Relevant bibliographies by topics / Carotenoids, Ultrafast

Academic literature on the topic 'Carotenoids, Ultrafast'

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Published: 10 March 2023

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Journal articles on the topic "Carotenoids, Ultrafast"

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Son, Minjung, Alberta Pinnola, Roberto Bassi, and Gabriela S. Schlau-Cohen. "Ultrabroadband two-dimensional electronic spectroscopy reveals energy flow pathways in LHCII across the visible spectrum." EPJ Web of Conferences 205 (2019): 09034. http://dx.doi.org/10.1051/epjconf/201920509034.

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We utilise ultrabroadband two-dimensional electronic spectroscopy to map out pathways of energy flow in LHCII across the entire visible region. In addition to the well-established, low-lying chlorophyll Qy bands, our results reveal additional pathways of energy relaxation on the higher-lying excited states involving the S2 energy levels of carotenoids, including ultrafast carotenoid-to-chlorophyll energy transfer on 90-150 fs timescales.
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HASHIMOTO, Hideki, Tokutake SASHIMA, Kazuhiro YANAGI, and Masayuki YOSHIZAWA. "Ultrafast Relaxation Processes of Photosynthetic Carotenoids." Review of Laser Engineering 32, no. 11 (2004): 701–10. http://dx.doi.org/10.2184/lsj.32.701.

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Kosumi, Daisuke, Takayuki Kajikawa, Kazuhiko Sakaguchi, Shigeo Katsumura, and Hideki Hashimoto. "Excited state properties of β-carotene analogs incorporating a lactone ring." Physical Chemistry Chemical Physics 19, no. 4 (2017): 3000–3009. http://dx.doi.org/10.1039/c6cp06828f.

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Miki, Takeshi, Tiago Buckup, Marie S. Krause, June Southall, Richard J. Cogdell, and Marcus Motzkus. "Vibronic coupling in the excited-states of carotenoids." Physical Chemistry Chemical Physics 18, no. 16 (2016): 11443–53. http://dx.doi.org/10.1039/c5cp07542d.

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The ultrafast femtochemistry of carotenoids is governed by the interaction between electronic excited states, which has been explained by the relaxation dynamics within a few hundred femtoseconds from the lowest optically allowed excited state S2to the optically dark state S1.
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Hashimoto, Hideki, Mitsuru Sugisaki, and Masayuki Yoshizawa. "Ultrafast time-resolved vibrational spectroscopies of carotenoids in photosynthesis." Biochimica et Biophysica Acta (BBA) - Bioenergetics 1847, no. 1 (January 2015): 69–78. http://dx.doi.org/10.1016/j.bbabio.2014.09.001.

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Tamura, Hiroyuki, and Hiroshi Ishikita. "Quenching of Singlet Oxygen by Carotenoids via Ultrafast Superexchange Dynamics." Journal of Physical Chemistry A 124, no. 25 (June 2, 2020): 5081–88. http://dx.doi.org/10.1021/acs.jpca.0c02228.

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Niedzwiedzki, Dariusz M., Daniel J. Sandberg, Hong Cong, Megan N. Sandberg, George N. Gibson, Robert R. Birge, and Harry A. Frank. "Ultrafast time-resolved absorption spectroscopy of geometric isomers of carotenoids." Chemical Physics 357, no. 1-3 (February 2009): 4–16. http://dx.doi.org/10.1016/j.chemphys.2008.07.011.

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Lee, Sebok, Terry Park, Jaebeom Lee, and Yoonsoo Pang. "Ultrafast Electron Injection from the S2 State of Carotenoids into TiO2 Nanoparticles." Journal of Nanoscience and Nanotechnology 17, no. 4 (April 1, 2017): 2685–89. http://dx.doi.org/10.1166/jnn.2017.13369.

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Romero, Elisabet, Ivo H. M. van Stokkum, Jan P. Dekker, and Rienk van Grondelle. "Ultrafast carotenoid band shifts correlated with Chlz excited states in the photosystem II reaction center: are the carotenoids involved in energy transfer?" Physical Chemistry Chemical Physics 13, no. 13 (2011): 5573. http://dx.doi.org/10.1039/c0cp02896g.

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Niedzwiedzki, Dariusz, Jeremy F. Koscielecki, Hong Cong, James O. Sullivan, George N. Gibson, Robert R. Birge, and Harry A. Frank. "Ultrafast Dynamics and Excited State Spectra of Open-Chain Carotenoids at Room and Low Temperatures." Journal of Physical Chemistry B 111, no. 21 (May 2007): 5984–98. http://dx.doi.org/10.1021/jp070500f.

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Dissertations / Theses on the topic "Carotenoids, Ultrafast"

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Singh, Asmita. "Illuminating the ultrafast excited state dynamics of protein-bound carotenoids in plants." Diss., University of Pretoria, 2017. http://hdl.handle.net/2263/63170.

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Global energy demands have escalated over the past few decades, creating a necessity for alternative energy sources. Solar technologies inspired by the primary solar energy storing process known on earth, photosynthesis, have subsequently gained popularity. The natural photosynthetic apparatus comprises a network of membrane-bound pigment-protein complexes, with the main plant light-harvesting complex (LHCII) consisting of chlorophyll (Chl) and carotenoid (Car) pigments. Electronic excitation energy transfer (ET) of the harvested energy takes place amongst these pigments on ultrafast timescales. This energy is funnelled towards a photosynthetic reaction centre where charge separation is achieved, creating a Biobattery, which powers the subsequent manufacture of energy-rich chemical compounds for photosynthetic activity. Transient absorption pump-probe spectroscopy has proven to be a useful technique for monitoring the evolution of the excited state dynamics, such as electronic transitions and excitation ET amongst Car and Chl pigments of LHCII trimers isolated from spinach leaves. This method was utilized to probe samples excited under four different conditions: at pump excitation wavelengths (𝜆𝑒𝑥) of 489 nm (preferentially exciting Cars Lutein1 and Neoxanthin) and 506 nm (targeting Cars Lutein2 and Violaxanthin), each with an intensity of either 800 nJ/pulse (relatively high) or 500 nJ/pulse (comparatively low). A global analysis was applied to each dataset using the robust, open-source Glotaran software, from which three kinetic decay lifetimes for the various processes were extracted. General spectral observations encompassed a negative pump ground state bleach (GSB) at each 𝜆𝑒𝑥; negative Chl b and Chl a GSBs, superimposed with negative stimulated emission (SE) signals; and a positive excited state absorption (ESA) band. The first lifetime of a few picoseconds corresponded mainly to Car-S2 depopulation, resulting either from energy relaxation towards Car-S1, or ET to Chls. Small, but distinct Chl b signals of less than 3 mOD were also detected on this timescale. The second lifetime, which is between 10 and 12 ps, was characteristic to the Lutein Car-S1 lifetime, mainly depicting Car-S1 ET to Chl a. The third lifetime, which extended from ~200 ps to the nanosecond timescale, was attributed to Chl a fluorescence. The 𝜆𝑒𝑥 of 489 nm directly excites the Chl Soret region, whilst excitation at 506 nm shows a pump intensity-dependence. Laser pulse photon density values were ~1014 photons·cm-2·pulse-1 for these datasets. Singlet-singlet annihilation calculations performed on the samples excited at 506 nm provided low annihilation probabilities of 9.0% and 11.5% for a low and high pump intensity, respectively, limiting the possibility of sample photobleaching. Optimization and redevelopment of the experimental setup significantly improved both the data quality and various recorded parameters, concluding that pump-probe spectroscopy was successful on the prepared LHCII trimers. Results acquired and calculations performed correlated with literature, where minimal changes were noticed in the timescales and ET pathways. The robustness of plant systems was confirmed through both excitation-wavelength and intensity dependence. This work paves the way for advanced studies on the role Cars play in non-photochemical quenching (NPQ), a self-protection mechanism of plants against over-illumination; and for the tailoring of artificial light-harvesting antennas based on research conducted on their natural counterparts.
Globale energievereistes het oor die afgelope paar dekades toegeneem, wat die ontwikkeling van alternatiewe energiebronne noodsaaklik maak. Sontegnologieë, geïnspireer deur die primêre sonenergiebergingsproses op aarde, fotosintese, het daarom gewild geword. Die natuurlike fotosintetiese apparaat bestaan uit 'n netwerk van membraangebonde pigment-proteïenkomplekse, met die hoof ligversamelingskompleks in plante (LHCII) wat bestaan uit chlorofil- (Chl) en karotenoïed- (Car) pigmente. Die energie wat deur die pigmente geabsorbeer word, word tussen elektroniese opgewekte toestande op verskillende pigmente op ultravinnige tydskale oorgedra. Hierdie energie word na ʼn fotosintetiese reaksiesentrum gekanaliseer, waar 'n ladingskeiding geïnduseer word en 'n Biobattery sodoende geskep word. Die energie wat in dié battery gestoor is, word gebruik om energieryke chemiese verbindings te vervaardig — wat as brandstof vir die plant dien om sy lewensfunksies te verrig. Tydopgeloste-absorpsie-pomp-tasting-spektroskopie is 'n nuttige tegniek om die dinamika tussen opgewekte toestande te volg. ‘n Voorbeeld van sulke dinamika is die elektroniese opwekking en energie-oordrag tussen die Car- en Chl-pigmente van geïsoleerde LHCII-trimere in spinasieblare. Hierdie metode is gebruik om monsters onder vier verskillende toestande te ondersoek by pompgolflengtes (𝜆𝑒𝑥) van 489 nm (waar hoofsaaklik die Cars Luteïne1 en Neoksantine opgewek word) en 506 nm (vir Cars Luteïne2 en Violaksantine), en pompenergieë van ‘n relatief hoë 800 nJ/puls, of 500 nJ/puls vir elke golflengte.
Dissertation (MSc)--University of Pretoria, 2017.
National Research Foundation (NRF)
Physics
MSc
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Miki, Takeshi [Verfasser], and Marcus [Akademischer Betreuer] Motzkus. "Third- and Fifth-order Nonlinear Time-resolved Spectroscopies for Ultrafast Molecular Dynamics in Carotenoids / Takeshi Miki ; Betreuer: Marcus Motzkus." Heidelberg : Universitätsbibliothek Heidelberg, 2017. http://d-nb.info/1180986385/34.

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RAGNONI, ELENA. "Excited state dynamics of carbonyl carotenoids investigated by ultrafast vibrational and electronic spectroscopies." Doctoral thesis, 2015. http://hdl.handle.net/2158/1003628.

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Carbonyl carotenoids, mostly present in marinae algae and dinoflagellates of deep waters, are well-known light-harvesting pigments, which absorb the green-blue wavelengths of the scattered sunlight and efficiently transfer energy to nearby chlorophylls in antenna complexes. In recent years, carbonyl carotenoids have been largely investigated as interesting dyes for organic photovoltaic devises. Due to the presence of a conjugated electron-withdrawing group to the polyene chain, absorption wavelengths and lifetime of photo-excited states show to be sensitive to the polarity of the surrounding. An intra-molecular charge transfer (ICT) state is generally invoked, whose nature and mechanism of formation have not been clarified yet. In this PhD thesis, I focus the attention on the photo-physics and photo-dynamics properties of two carbonyl carotenoids, Peridinin and the all trans-beta-apo-8’-carotenal, dissolved in several solvents, differing for both polarity and polarizability, and exciting the sample at different excitation wavelengths. By means of 3rd and 5th order non-linear spectroscopies, both in the infrared and in the visible region, I identify excited state vibrational marker bands of the ICT state, whose evolution suggests a strong mixing in the ionic and covalent character of the low-lying excited state. With the support of calculations, no evidences of a further electronic excited state in between the covalent S1(2Ag-) state and the ionic S2(1Bu+) state are found. Two relaxation pathways are finally presented for carbonyl carotenoids in non-polar and polar solvents: while in non-polar solvents the S2-S1 energy gap results in no differences with respect to non-carbonyl carotenoids, a strong mixing of the two low-lying states occurs in both strongly and moderately polar environments. In the latter case, also the solvent polarizability effect is evident and can be rationalized in terms of a dynamical stabilization of slightly distorted molecules, favorited by a solvent rearrangement. The presence in polar solution of slightly distorted molecules, and thus the removal from the Franck-Condon geometry along with relaxation, is further confirmed by the wavelength excitation dependence observed: exciting on the very red-tail of the absorption spectrum, in fact, a subpopulation of slightly distorted molecules is photo-selected and directly excited to the low-lying charge transfer state.
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CHÁBERA, Pavel. "Excited state dynamics of carotenoids in solution and proteins." Doctoral thesis, 2010. http://www.nusl.cz/ntk/nusl-53736.

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Time resolved spectroscopy is one of the crucial methods used to study processes on molecular level in biological systems. It is useful especially for monitoring fast processes that take a place in photosynthetic apparatus of photosynthetic organisms, such as electron and energy transfer. The integral parts of photosynthetic apparatus are carotenoids, whose role in the photosynthetic apparatus is not as well explored as it is for chlorophylls. It was proved that carotenoids actively participate in energy transfer processes in photosynthetic antennas. They have a crucial role in protection against excess energy damage. They are also electron donors in both antennas and reaction centers. The fact that photo-physical properties of carotenoids are much different from properties of others organic pigments, complicates studies of their functions in photosynthesis as well as in other biological systems. This thesis employs advanced methods of femtosecond spectroscopy to obtain more information about carotenoid functions in some biological systems and in solution with special focus on carotenoids containing carbonyl group.
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Ostroumov, Evgeny E. [Verfasser]. "Ultrafast relaxation dynamics of carotenoid excited states / vorgelegt von Evgeny Evgenievich Ostroumov." 2010. http://d-nb.info/1008199877/34.

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Book chapters on the topic "Carotenoids, Ultrafast"

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Cerullo, Giulio, Dario Polli, Guglielmo Lanzani, Sandro De Silvestri, H. Hashimoto, and Richard Cogdell. "Energy relaxation of carotenoids in solution and in LH2 complexes studied with sub-10-fs temporal resolution." In Ultrafast Phenomena XIII, 628–30. Berlin, Heidelberg: Springer Berlin Heidelberg, 2003. http://dx.doi.org/10.1007/978-3-642-59319-2_194.

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Walla, P. J., P. A. Linden, and G. R. Fleming. "Fs-transient Absorption and Fluorescence Upconversion after Two-Photon Excitation of Carotenoids in Solution and in LHC II." In Ultrafast Phenomena XII, 671–73. Berlin, Heidelberg: Springer Berlin Heidelberg, 2001. http://dx.doi.org/10.1007/978-3-642-56546-5_199.

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Papagiannakis, Emmanouil, Ivo H. M. van Stokkum, Rienk van Grondelle, Mikas Vengris, Leonas Valkunas, Richard J. Cogdell, and Delmar S. Larsen. "Decomposing the Excited State Dynamics of Carotenoids in Light Harvesting Complexes and Dissecting Pulse Structures from Optimal Control Experiments." In Ultrafast Phenomena XV, 474–76. Berlin, Heidelberg: Springer Berlin Heidelberg, 2007. http://dx.doi.org/10.1007/978-3-540-68781-8_153.

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Gradinaru, C. C., I. H. M. van Stokkum, R. van Grondelle, and H. van Amerongen. "Ultrafast Absorption Changes of the Lhcii Carotenoids upon Selective Excitation of the Chlorophylls." In Photosynthesis: Mechanisms and Effects, 277–80. Dordrecht: Springer Netherlands, 1998. http://dx.doi.org/10.1007/978-94-011-3953-3_64.

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Miki, T., Tiago Buckup, M. Marek, R. J. Cogdell, and Marcus Motzkus. "Ultrafast Interaction of Dark and Bright Electronic States in Open-Chain Carotenoids Investigated by Pump-DFWM." In Springer Proceedings in Physics, 440–43. Cham: Springer International Publishing, 2015. http://dx.doi.org/10.1007/978-3-319-13242-6_107.

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Lin, Su, Evaldas Katilius, and Neal W. Woodbury. "Carotenoid Excited State Kinetics in Bacterial RCs with the Primary Electron Donor Oxidized." In Ultrafast Phenomena XV, 528–30. Berlin, Heidelberg: Springer Berlin Heidelberg, 2007. http://dx.doi.org/10.1007/978-3-540-68781-8_171.

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Polívka, Tomáš, Donatas Zigmantas, Jennifer L. Herek, James A. Bautista, Harry A. Frank, and Villy Sundström. "Direct observation of the S1 level of the carotenoid spheroidene using near-infrared femtosecond spectroscopy." In Ultrafast Phenomena XII, 668–70. Berlin, Heidelberg: Springer Berlin Heidelberg, 2001. http://dx.doi.org/10.1007/978-3-642-56546-5_198.

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Polívka, Tomáš, and Villy Sundström. "Carotenoid Excited States-Photophysics, Ultrafast Dynamics and Photosynthetic Functions." In Frontiers of Optical Spectroscopy, 187–219. Dordrecht: Springer Netherlands, 2005. http://dx.doi.org/10.1007/1-4020-2751-6_5.

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Herek, J. L., T. Polivka, T. Pullerits, R. J. Cogdell, C. N. Hunter, and V. SundströM. "Ultrafast Carotenoid Band Shifts Probe Structure and Dynamics in Photosynthesis." In Photosynthesis: Mechanisms and Effects, 37–40. Dordrecht: Springer Netherlands, 1998. http://dx.doi.org/10.1007/978-94-011-3953-3_8.

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Akimoto, Seiji, Makio Yokono, Michiya Higuchi, Akio Murakami, Shinichi Takaichi, and Mamoru Mimuro. "Ultrafast Relaxation Dynamics of a Keto-Carotenoid, Siphonaxanthin, Probed by Time-Resolved Fluorescence." In Photosynthesis. Energy from the Sun, 319–22. Dordrecht: Springer Netherlands, 2008. http://dx.doi.org/10.1007/978-1-4020-6709-9_72.

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Conference papers on the topic "Carotenoids, Ultrafast"

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Davis, J. A., E. Cannon, L. V. Dao, P. Hannaford, K. A. Nugent, and H. M. Quiney. "Coherent Effects in Carotenoids." In International Conference on Ultrafast Phenomena. Washington, D.C.: OSA, 2010. http://dx.doi.org/10.1364/up.2010.thb3.

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Buckup, Tiago, Marie S. Marek, and Marcus Motzkus. "New Insights into the Excited State Relaxation Network of Carotenoids." In International Conference on Ultrafast Phenomena. Washington, D.C.: OSA, 2010. http://dx.doi.org/10.1364/up.2010.the16.

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Kosumi, D., M. Komukai, K. Yanagi, H. Hashimoto, and M. Yoshizawa. "Excitation energy dependence of ultrafast phenomena in all-trans-carotenoids." In International Quantum Electronics Conference, 2005. IEEE, 2005. http://dx.doi.org/10.1109/iqec.2005.1560969.

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Miki, T., T. Buckup, M. Marek, R. J. Cogdell, and M. Motzkus. "Ultrafast Interaction of Dark and Bright Electronic States in Open-Chain Carotenoids Investigated by Pump-DFWM." In International Conference on Ultrafast Phenomena. Washington, D.C.: OSA, 2014. http://dx.doi.org/10.1364/up.2014.08.tue.c.3.

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Gosztola, David, Hiroko Yamada, and Michael R. Wasielewski. "Picosecond Laser Induced Electric Field Modulation of Carotenoid Absorption Bands." In International Conference on Ultrafast Phenomena. Washington, D.C.: Optica Publishing Group, 1994. http://dx.doi.org/10.1364/up.1994.wc.17.

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Observation of band shifts in the absorption spectra of in vivo carotenoids has been attributed to electric field effects generated by membrane potentials. This electrochromism is related to what is known as the Stark effect, a term which is used to describe the effect of an applied electric field on many physical processes. Previous in vitro studies of how electric fields effect the absorption spectra of molecules all have relied on applying the perturbing electric field by using external electrodes around a dielectric spacer containing the molecule to be studied. The maximum applied field in these examples has been between 0.5 MV/cm and 3 MV/cm. These electric field intensities are of the same magnitude as those thought to be present across the membranes studied in the in vivo experiments.
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Cerullo, G., D. Polli, G. Lanzani, S. De Silvestri, R. J. Cogdell, and H. Hashimoto. "Energy relaxation of carotenoids in solution and in LH2 complexes studied with sub-10-fs temporal resolution." In International Conference on Ultrafast Phenomena. Washington, D.C.: OSA, 2002. http://dx.doi.org/10.1364/up.2002.wd39.

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Walla, P. J., P. A. Linden, and G. R. Fleming. "Fs-transient Absorption and Fluorescence Upconversion after Two-Photon Excitation of Carotenoids in Solution and in LHC II." In International Conference on Ultrafast Phenomena. Washington, D.C.: OSA, 2000. http://dx.doi.org/10.1364/up.2000.tuf51.

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Papagiannais, Emmanouil, Ivo H. M. van Stokkum, Rienk van Grondelle, Mikas Vengris, Leonas Valkunas, Richard J. Cogdell, and Delmar S. Larsen. "Decomposing the Excited State Dynamics of Carotenoids in Light Harvesting Complexes and Dissecting Pulse Structures from Optimal Control Experiments." In International Conference on Ultrafast Phenomena. Washington, D.C.: OSA, 2006. http://dx.doi.org/10.1364/up.2006.tua4.

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Yoshizawa, Masayuki, and Hideki Hashimoto. "Ultrafast dynamics in a series of carotenoids investigated by time-resolved stimulated Raman spectroscopy." In Optical Science and Technology, SPIE's 48th Annual Meeting, edited by Mark G. Kuzyk, Manfred Eich, and Robert A. Norwood. SPIE, 2003. http://dx.doi.org/10.1117/12.503934.

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Kosumi, D., S. Maruta, T. Kusumoto, R. Fujii, M. Sugisaki, M. Iha, H. A. Frank, and H. Hashimoto. "Excitation Energy Dependence of the S1 and ICT State Dynamics in Marine Carotenoids Studied by Femtosecond One- and Two-Photon Pump-Probe Spectroscopy." In International Conference on Ultrafast Phenomena. Washington, D.C.: OSA, 2010. http://dx.doi.org/10.1364/up.2010.me14.

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