Journal articles on the topic 'Atmospheric dust transport'
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1
Schepanski, Kerstin, Marc Mallet, Bernd Heinold, and Max Ulrich. "North African dust transport toward the western Mediterranean basin: atmospheric controls on dust source activation and transport pathways during June–July 2013." Atmospheric Chemistry and Physics 16, no. 22 (November 15, 2016): 14147–68. http://dx.doi.org/10.5194/acp-16-14147-2016.
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Abstract. Dust transported from north African source region toward the Mediterranean basin and Europe is a ubiquitous phenomenon in the Mediterranean region. Winds formed by large-scale pressure gradients foster dust entrainment into the atmosphere over north African dust source regions and advection of dust downwind. The constellation of centers of high and low pressure determines wind speed and direction, and thus the chance for dust emission over northern Africa and transport toward the Mediterranean. We present characteristics of the atmospheric dust life cycle determining dust transport toward the Mediterranean basin with focus on the ChArMEx (Chemistry-Aerosol Mediterranean Experiment) special observation period in June and July 2013 using the atmosphere–dust model COSMO-MUSCAT (COSMO: COnsortium for Small-scale MOdeling; MUSCAT: MUltiScale Chemistry Aerosol Transport Model). Modes of atmospheric circulation are identified from empirical orthogonal function (EOF) analysis of the geopotential height at 850 hPa and compared to EOFs calculated from 1979–2015 ERA-Interim reanalysis. Two different phases are identified from the first EOF, which in total explain 45 % of the variance. They are characterized by the propagation of the subtropical ridge into the Mediterranean basin, the position of the Saharan heat low and the predominant Iberian heat low, and discussed illustrating a dipole pattern for enhanced (reduced) dust emission fluxes, stronger (weaker) meridional dust transport, and consequent increased (decreased) atmospheric dust concentrations and deposition fluxes. In the event of a predominant high-pressure zone over the western and central Mediterranean (positive phase), a hot spot in dust emission flux is evident over the Grand Erg Occidental, and a reduced level of atmospheric dust loading occurs over the western Mediterranean basin. The meridional transport in northward direction is reduced due to prevailing northerly winds. In case of a predominant heat low trough linking the Iberian and the Saharan heat low (negative phase), meridional dust transport toward the western Mediterranean is increased due to prevailing southerly winds resulting in an enhanced atmospheric dust loading over the western Mediterranean. Altogether, results from this study illustrate the relevance of knowing dust source location and characteristics in concert with atmospheric circulation. The study elaborates on the question of the variability of summertime dust transport toward the Mediterranean and Europe with regard to atmospheric circulation conditions controlling dust emission and transport routes of Saharan dust, exemplarily for the 2-month period of June–July 2013. Ultimately, outcomes from this study contribute to the understanding of the variance in dust transport into a populated region.
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Toth III, Joseph R., Siddharth Rajupet, Henry Squire, Blaire Volbers, Jùn Zhou, Li Xie, R. Mohan Sankaran, and Daniel J. Lacks. "Electrostatic forces alter particle size distributions in atmospheric dust." Atmospheric Chemistry and Physics 20, no. 5 (March 17, 2020): 3181–90. http://dx.doi.org/10.5194/acp-20-3181-2020.
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Abstract. Large amounts of dust are lofted into the atmosphere from arid regions of the world before being transported up to thousands of kilometers. This atmospheric dust interacts with solar radiation and causes changes in the climate, with larger-sized particles having a heating effect, and smaller-sized particles having a cooling effect. Previous studies on the long-range transport of dust have found larger particles than expected, without a model to explain their transport. Here, we investigate the effect of electric fields on lofted airborne dust by blowing sand through a vertically oriented electric field, and characterizing the size distribution as a function of height. We also model this system, considering the gravitational, drag, and electrostatic forces on particles, to understand the effects of the electric field. Our results indicate that electric fields keep particles suspended at higher elevations and enrich the concentration of larger particles at higher elevations. We extend our model from the small-scale system to long-range atmospheric dust transport to develop insights into the effects of electric fields on size distributions of lofted dust in the atmosphere. We show that the presence of electric fields and the resulting electrostatic force on charged particles can help explain the transport of unexpectedly large particles and cause the size distribution to become more uniform as a function of elevation. Thus, our experimental and modeling results indicate that electrostatic forces may in some cases be relevant regarding the effect of atmospheric dust on the climate.
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Heavens, Nicholas G., David M. Kass, James H. Shirley, Sylvain Piqueux, and Bruce A. Cantor. "An Observational Overview of Dusty Deep Convection in Martian Dust Storms." Journal of the Atmospheric Sciences 76, no. 11 (October 16, 2019): 3299–326. http://dx.doi.org/10.1175/jas-d-19-0042.1.
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Abstract Deep convection, as used in meteorology, refers to the rapid ascent of air parcels in Earth’s troposphere driven by the buoyancy generated by phase change in water. Deep convection undergirds some of Earth’s most important and violent weather phenomena and is responsible for many aspects of the observed distribution of energy, momentum, and constituents (particularly water) in Earth’s atmosphere. Deep convection driven by buoyancy generated by the radiative heating of atmospheric dust may be similarly important in the atmosphere of Mars but lacks a systematic description. Here we propose a comprehensive framework for this phenomenon of dusty deep convection (DDC) that is supported by energetic calculations and observations of the vertical dust distribution and exemplary dusty deep convective structures within local, regional, and global dust storm activity. In this framework, DDC is distinct from a spectrum of weaker dusty convective activity because DDC originates from preexisting or concurrently forming mesoscale circulations that generate high surface dust fluxes, oppose large-scale horizontal advective–diffusive processes, and are thus able to maintain higher dust concentrations than typically simulated. DDC takes two distinctive forms. Mesoscale circulations that form near Mars’s highest volcanoes in dust storms of all scales can transport dust to the base of the upper atmosphere in as little as 2 h. In the second distinctive form, mesoscale circulations at low elevations within regional and global dust storm activity generate freely convecting streamers of dust that are sheared into the middle atmosphere over the diurnal cycle.
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Banks, Jamie R., Anja Hünerbein, Bernd Heinold, Helen E. Brindley, Hartwig Deneke, and Kerstin Schepanski. "The sensitivity of the colour of dust in MSG-SEVIRI Desert Dust infrared composite imagery to surface and atmospheric conditions." Atmospheric Chemistry and Physics 19, no. 10 (May 23, 2019): 6893–911. http://dx.doi.org/10.5194/acp-19-6893-2019.
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Abstract. Infrared “Desert Dust” composite imagery taken by the Spinning Enhanced Visible and InfraRed Imager (SEVIRI), onboard the Meteosat Second Generation (MSG) series of satellites above the equatorial East Atlantic, has been widely used for more than a decade to identify and track the presence of dust storms from and over the Sahara Desert, the Middle East, and southern Africa. Dust is characterised by distinctive pink colours in the Desert Dust false-colour imagery; however, the precise colour is influenced by numerous environmental properties, such as the surface thermal emissivity and skin temperature, the atmospheric water vapour content, the quantity and height of dust in the atmosphere, and the infrared optical properties of the dust itself. For this paper, simulations of SEVIRI infrared measurements and imagery have been performed using a modelling system, which combines dust concentrations simulated by the aerosol transport model COSMO-MUSCAT (COSMO: COnsortium for Small-scale MOdelling; MUSCAT: MUltiScale Chemistry Aerosol Transport Model) with radiative transfer simulations from the RTTOV (Radiative Transfer for TOVS) model. Investigating the sensitivity of the synthetic infrared imagery to the environmental properties over a 6-month summertime period from 2011 to 2013, it is confirmed that water vapour is a major control on the apparent colour of dust, obscuring its presence when the moisture content is high. Of the three SEVIRI channels used in the imagery (8.7, 10.8, and 12.0 µm), the channel at 10.8 µm has the highest atmospheric transmittance and is therefore the most sensitive to the surface skin temperature. A direct consequence of this sensitivity is that the background desert surface exhibits a strong diurnal cycle in colour, with light blue colours possible during the day and purple hues prevalent at night. In dusty scenes, the clearest pink colours arise from high-altitude dust in dry atmospheres. Elevated dust influences the dust colour primarily by reducing the contrast in atmospheric transmittance above the dust layer between the SEVIRI channels at 10.8 and 12.0 µm, thereby boosting red and pink colours in the imagery. Hence, the higher the dust altitude, the higher the threshold column moisture needed for dust to be obscured in the imagery: for a sample of dust simulated to have an aerosol optical depth (AOD) at 550 nm of 2–3 at an altitude of 3–4 km, the characteristic colour of the dust may only be impaired when the total column water vapour is particularly moist (⪆39 mm). Meanwhile, dust close to the surface (altitude <1 km) is only likely to be apparent when the atmosphere is particularly dry and when the surface is particularly hot, requiring column moisture ⪅13 mm and skin temperatures ⪆314 K, and is highly unlikely to be apparent when the skin temperature is ⪅300 K. Such low-altitude dust will regularly be almost invisible within the imagery, since it will usually be beneath much of the atmospheric water vapour column. It is clear that the interpretation of satellite-derived dust imagery is greatly aided by knowledge of the background environment.
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Takahashi, Y., M. Higashi, T. Furukawa, and S. Mitsunobu. "Change of iron species and iron solubility in Asian dust during the long-range transport from western China to Japan." Atmospheric Chemistry and Physics Discussions 11, no. 7 (July 8, 2011): 19545–80. http://dx.doi.org/10.5194/acpd-11-19545-2011.
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Abstract. In the North Pacific, transport and deposition of mineral dust from Asia appear to be one of major sources of iron which can regulate growth of phytoplankton in the ocean. In this process, it is essential to identify chemical species of iron contained in Asian dust, because bioavailability of iron in the ocean is strongly influenced by the solubility of iron, which in turn is dependent on iron species in the dust. Here, we report that clay minerals (illite and chlorite) in the dusts near the source (western China) are transformed into ferrihydrite by atmospheric chemical processes during their long-range transport to eastern China and Japan based on the speciation by X-ray absorption fine structure (XAFS) and other methods such as X-ray diffraction and chemical extraction. Moreover, it was found that iron in the dust after the transport becomes more soluble in our leaching experiments conducted for 24 h compared with those for initial dusts possibly due to the formation of ferrihydrite in the atmosphere. Our findings suggested that ferrihydrite secondarily formed during the transport is an important source of soluble iron species, which can be more soluble than clay minerals initially contained in the mineral dust such as illite and chlorite.
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Grogan, Dustin F. P., and Terrence R. Nathan. "Passive versus Active Transport of Saharan Dust Aerosols by African Easterly Waves." Atmosphere 12, no. 11 (November 16, 2021): 1509. http://dx.doi.org/10.3390/atmos12111509.
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Theory and modeling are combined to reveal the physical and dynamical processes that control Saharan dust transport by amplifying African easterly waves (AEWs). Two cases are examined: active transport, in which the dust is radiatively coupled to the circulation; passive transport, in which the dust is radiatively decoupled from the circulation. The theory is built around a dust conservation equation for dust-coupled AEWs in zonal-mean African easterly jets. The theory predicts that, for both the passive and active cases, the dust transports will be largest where the zonal-mean dust gradients are maximized on an AEW critical surface. Whether the dust transports are largest for the radiatively passive or radiatively active case depends on the growth rate of the AEWs, which is modulated by the dust heating. The theoretical predictions are confirmed via experiments carried out with the Weather Research and Forecasting model, which is coupled to a dust conservation equation. The experiments show that the meridional dust transports dominate in the passive case, while the vertical dust transports dominate in the active case.
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Liu, Z., D. Liu, J. Huang, M. Vaughan, I. Uno, N. Sugimoto, C. Kittaka, et al. "Airborne dust distributions over the Tibetan Plateau and surrounding areas derived from the first year of CALIPSO lidar observations." Atmospheric Chemistry and Physics 8, no. 16 (August 29, 2008): 5045–60. http://dx.doi.org/10.5194/acp-8-5045-2008.
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Abstract. Using an analysis of the first full year of CALIPSO lidar measurements, this paper derives unprecedented, altitude-resolved seasonal distributions of desert dust transported over the Tibetan Plateau (TP) and the surrounding areas. The CALIPSO lidar observations include numerous large dust plumes over the northern slope and eastern part of the TP, with the largest number of dust events occurring in the spring of 2007, and some layers being lofted to altitudes of 11–12 km. Generation of the Tibetan airborne dusts appears to be largely associated with source regions to the north and on the eastern part of the plateau. Examination of the CALIPSO time history reveals an "airborne dust corridor" due to the eastward transport of dusts originating primarily in these source areas. This corridor extends from west to east and shows a seasonality largely modulated by the TP through its dynamical and thermal forcing on the atmospheric flows. On the southern side, desert dust particles originate predominately in Northwest India and Pakistan. The dust transport occurs primarily in dry seasons around the TP western and southern slopes and dust particles become mixed with local polluted aerosols. No significant amount of dust appears to be transported over the Himalayas. Extensive forward trajectory simulations are also conducted to confirm the dust transport pattern from the nearby sources observed by the CALIPSO lidar. Comparisons with the OMI and MODIS measurements show the unique capability of the CALIPSO lidar to provide unambiguous, altitude-resolved dust measurements.
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Schepanski, Kerstin, Bernd Heinold, and Ina Tegen. "Harmattan, Saharan heat low, and West African monsoon circulation: modulations on the Saharan dust outflow towards the North Atlantic." Atmospheric Chemistry and Physics 17, no. 17 (September 1, 2017): 10223–43. http://dx.doi.org/10.5194/acp-17-10223-2017.
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Abstract. The outflow of dust from the northern African continent towards the North Atlantic is stimulated by the atmospheric circulation over North Africa, which modulates the spatio-temporal distribution of dust source activation and consequently the entrainment of mineral dust into the boundary layer, as well as the transport of dust out of the source regions. The atmospheric circulation over the North African dust source regions, predominantly the Sahara and the Sahel, is characterized by three major circulation regimes: (1) the harmattan (trade winds), (2) the Saharan heat low (SHL), and (3) the West African monsoon circulation. The strength of the individual regimes controls the Saharan dust outflow by affecting the spatio-temporal distribution of dust emission, transport pathways, and deposition fluxes.This study aims at investigating the atmospheric circulation pattern over North Africa with regard to its role favouring dust emission and dust export towards the tropical North Atlantic. The focus of the study is on summer 2013 (June to August), during which the SALTRACE (Saharan Aerosol Long-range TRansport and Aerosol-Cloud interaction Experiment) field campaign also took place. It involves satellite observations by the Spinning Enhanced Visible and InfraRed Imager (SEVIRI) flying on board the geostationary Meteosat Second Generation (MSG) satellite, which are analysed and used to infer a data set of active dust sources. The spatio-temporal distribution of dust source activation frequencies (DSAFs) allows for linking the diurnal cycle of dust source activations to dominant meteorological controls on dust emission. In summer, Saharan dust source activations clearly differ from dust source activations over the Sahel regarding the time of day when dust emission begins. The Sahara is dominated by morning dust source activations predominantly driven by the breakdown of the nocturnal low-level jet. In contrast, dust source activations in the Sahel are predominantly activated during the second half of the day, when downdrafts associated with deep moist convection are the major atmospheric driver. Complementary to the satellite-based analysis on dust source activations and implications from their diurnal cycle, simulations on atmosphere and dust life cycle were performed using the mesoscale atmosphere–dust model system COSMO-MUSCAT (COSMO: COnsortium for Small-scale MOdelling; MUSCAT: MUltiScale Chemistry Aerosol Transport Model). Fields from this simulation were analysed regarding the variability of the harmattan, the Saharan heat low, and the monsoon circulation as well as their impact on the variability of the Saharan dust outflow towards the North Atlantic. This study illustrates the complexity of the interaction among the three major circulation regimes and their modulation of the North African dust outflow. Enhanced westward dust fluxes frequently appear following a phase characterized by a deep SHL. Ultimately, findings from this study contribute to the quantification of the interannual variability of the atmospheric dust burden.
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Osada, K., S. Ura, M. Kagawa, M. Mikami, T. Y. Tanaka, S. Matoba, K. Aoki, et al. "Wet and dry deposition of mineral dust particles in Japan: factors related to temporal variation and spatial distribution." Atmospheric Chemistry and Physics 14, no. 2 (January 29, 2014): 1107–21. http://dx.doi.org/10.5194/acp-14-1107-2014.
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Abstract. Recent ground networks and satellite remote-sensing observations have provided useful data related to spatial and vertical distributions of mineral dust particles in the atmosphere. However, measurements of temporal variations and spatial distributions of mineral dust deposition fluxes are limited in terms of their duration, location, and processes of deposition. To ascertain temporal variations and spatial distributions of mineral dust deposition using wet and dry processes, weekly deposition samples were obtained at Sapporo, Toyama, Nagoya, Tottori, Fukuoka, and Cape Hedo (Okinawa) in Japan during October 2008–December 2010 using automatic wet and dry separating samplers. Mineral dust weights in water-insoluble residue were estimated from Fe contents measured using an X-ray fluorescence analyser. Wet and dry deposition fluxes of mineral dusts were both high in spring and low in summer, showing similar seasonal variations to frequency of aeolian dust events (Kosa) in Japan. For wet deposition, highest and lowest annual dust fluxes were found at Toyama (9.6 g m−2 yr−1) and at Cape Hedo (1.7 g m−2 yr−1) as average values in 2009 and 2010. Higher wet deposition fluxes were observed at Toyama and Tottori, where frequent precipitation (> 60% days per month) was observed during dusty seasons. For dry deposition among Toyama, Tottori, Fukuoka, and Cape Hedo, the highest and lowest annual dust fluxes were found respectively at Fukuoka (5.2 g m−2 yr−1) and at Cape Hedo (2.0 g m−2 yr−1) as average values in 2009 and 2010. The average ratio of wet and dry deposition fluxes was the highest at Toyama (3.3) and the lowest at Hedo (0.82), showing a larger contribution of the dry process at western sites, probably because of the distance from desert source regions and because of the effectiveness of the wet process in the dusty season. Size distributions of refractory dust particles were obtained using four-stage filtration: > 20, > 10, > 5, and > 1 μm diameter. Weight fractions of the sum of > 20 μm and 10–20 μm (giant fraction) were higher than 50% for most of the event samples. Irrespective of the deposition type, the giant dust fractions generally decreased with increasing distance from the source area, suggesting the selective depletion of larger giant particles during atmospheric transport. Based on temporal variations of PMc (2.5 < D < 10 μm), ground-based lidar, backward air trajectories, and vertical profiles of potential temperatures, transport processes of dust particles are discussed for events with high-deposition and low-deposition flux with high PMc. Low dry dust depositions with high PMc concentrations were observed under stronger (5 K km−1) stratification of potential temperature with thinner and lower (< 2 km) dust distributions because the PMc fraction of dust particles only survived after depletion of giant dust particles by rapid gravitational settling at the time they reach Japan. In contrast, transport through a thicker (> 2 km) dust layer with weak vertical gradient of potential temperature carry more giant dust particles to Japan. Because giant dust particles are an important mass fraction of dust accumulation, especially in the North Pacific, which is known as a high-nutrient, low-chlorophyll (HNLC) region, the transport height and fraction of giant dust particles are important factors for studying dust budgets in the atmosphere and their role in biogeochemical cycles.
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Voss, Kara K., Amato T. Evan, Kimbery A. Prather, and F. Martin Ralph. "Dusty Atmospheric Rivers: Characteristics and Origins." Journal of Climate 33, no. 22 (November 15, 2020): 9749–62. http://dx.doi.org/10.1175/jcli-d-20-0059.1.
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AbstractAtmospheric rivers (AR) are narrow bands of strong horizontal transport of water vapor in the midlatitudes that can cause extreme precipitation, which contributes to beneficial water supply and sometimes flooding. The precipitation productivity of an AR is affected by microphysical processes, including the influence of aerosols. Earlier case studies have shown that some ARs over the North Pacific Ocean contain dust from Africa and Asia that can strongly influence precipitation by acting as ice nuclei. This paper explores how commonly dust and ARs occur together, or in close proximity. A “dust score” is introduced to characterize the dustiness of the environment associated with ARs by using satellite-based observations. This method is applied to days on which one or more ARs made landfall along the west coast of the United States between 2001 and 2018. The dust score is used to describe the seasonality and year-to-year variability of dusty-environment ARs. Dusty ARs occur primarily in the early spring (March–April), and dust is preferentially found within the warm sector of AR-associated extratropical cyclones and is also enhanced in the cold sector. Year-to-year variability in dust score is dependent more on year-to-year variability in dust than on the frequency of AR days. This year-to-year variability is also strongly related to correlations between the frequency of ARs and the dustiness of the northeastern Pacific, motivating additional investigation into potential dynamical association between dust and ARs.
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O'Sullivan, Debbie, Franco Marenco, Claire L. Ryder, Yaswant Pradhan, Zak Kipling, Ben Johnson, Angela Benedetti, et al. "Models transport Saharan dust too low in the atmosphere: a comparison of the MetUM and CAMS forecasts with observations." Atmospheric Chemistry and Physics 20, no. 21 (November 5, 2020): 12955–82. http://dx.doi.org/10.5194/acp-20-12955-2020.
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Abstract. We investigate the dust forecasts from two operational global atmospheric models in comparison with in situ and remote sensing measurements obtained during the AERosol properties – Dust (AER-D) field campaign. Airborne elastic backscatter lidar measurements were performed on board the Facility for Airborne Atmospheric Measurements during August 2015 over the eastern Atlantic, and they permitted us to characterise the dust vertical distribution in detail, offering insights on transport from the Sahara. They were complemented with airborne in situ measurements of dust size distribution and optical properties, as well as datasets from the Cloud–Aerosol Transport System (CATS) spaceborne lidar and the Moderate Resolution Imaging Spectroradiometer (MODIS). We compare the airborne and spaceborne datasets to operational predictions obtained from the Met Office Unified Model (MetUM) and the Copernicus Atmosphere Monitoring Service (CAMS). The dust aerosol optical depth predictions from the models are generally in agreement with the observations but display a low bias. However, the predicted vertical distribution places the dust lower in the atmosphere than highlighted in our observations. This is particularly noticeable for the MetUM, which does not transport coarse dust high enough in the atmosphere or far enough away from the source. We also found that both model forecasts underpredict coarse-mode dust and at times overpredict fine-mode dust, but as they are fine-tuned to represent the observed optical depth, the fine mode is set to compensate for the underestimation of the coarse mode. As aerosol–cloud interactions are dependent on particle numbers rather than on the optical properties, this behaviour is likely to affect their correct representation. This leads us to propose an augmentation of the set of aerosol observations available on a global scale for constraining models, with a better focus on the vertical distribution and on the particle size distribution. Mineral dust is a major component of the climate system; therefore, it is important to work towards improving how models reproduce its properties and transport mechanisms.
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Ben-Ami, Y., I. Koren, O. Altaratz, A. Kostinski, and Y. Lehahn. "Discernible rhythm in the spatio/temporal distributions of transatlantic dust." Atmospheric Chemistry and Physics 12, no. 5 (March 1, 2012): 2253–62. http://dx.doi.org/10.5194/acp-12-2253-2012.
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Abstract. The differences in North African dust emission regions and transport routes, between the boreal winter and summer, are thoroughly documented. Here we re-examine the spatial and temporal characteristics of dust transport over the tropical and subtropical North Atlantic Ocean, using 10 yr of satellite data, in order to better characterize the different dust transport periods. We see a robust annual triplet: a discernible rhythm of "transatlantic dust weather". The proposed annual partition is composed of two heavy loading periods, associated here with a northern-route period and southern-route period, and one light-loading period, accompanied by unusually low average optical depth of dust. The two dusty periods are quite different in character: their duration, transport routes, characteristic aerosol loading and frequency of pronounced dust episodes. The southern-route period lasts ~4 months. It is characterized by a relatively steady southern positioning, low frequency of dust events, low background values and high variance in dust loading. The northern-route period lasts ~6.5 months and is associated with a steady drift northward of ~0.1 latitude day−1, reaching ~1500 km north of the southern-route. The northern period is characterized by higher frequency of dust events, higher (and variable) background and smaller variance in dust loading. It is less episodic than the southern period. Transitions between the periods are brief. Separation between the southern and northern periods is marked by northward latitudinal shift in dust transport and by moderate reduction in the overall dust loading. The second transition, between the northern and southern periods, commences with an abrupt reduction in dust loading and rapid shift southward of ~0.2 latitude day−1, and ~1300 km in total. Based on cross-correlation analyses, we attribute the observed rhythm to the contrast between the northwestern and southern Saharan dust source spatial distributions. Despite the vast difference in areas, the Bodélé Depression, located in Chad, appears to modulate transatlantic dust patterns about half the time.
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Eguchi, K., I. Uno, K. Yumimoto, T. Takemura, A. Shimizu, N. Sugimoto, and Z. Liu. "Trans-pacific dust transport: integrated analysis of NASA/CALIPSO and a global aerosol transport model." Atmospheric Chemistry and Physics 9, no. 9 (May 14, 2009): 3137–45. http://dx.doi.org/10.5194/acp-9-3137-2009.
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Abstract. Detailed 3-D structures of Trans-Pacific Asian dust transport occurring during 5–15 May 2007 were investigated using the NASA/CALIOP vertical-resolved measurements and a three-dimensional aerosol model (SPRINTARS). Both CALIOP and SPRINTARS dust extinctions showed a good agreement along the way of the transport from the dust source regions across North Pacific into North America. A vertically two-layered dust distribution was observed over the northeastern Pacific and North America. The lower dust layer originated from a dust storm generated in the Gobi Desert on 5 May. It was transported at an altitude of around 4 km MSL and has mixed with Asian anthropogenic air pollutants during the course of transport. The upper dust layer mainly originated from a dust storm that occurred in the Taklimakan Desert 2–3 days after the Gobi dust storm generation. The upper dust cloud was transported in higher altitudes above the major clouds layer during the Trans-Pacific transport. It therefore has remained unmixed with the Asian air pollutants and almost unaffected by wet removal. The decay of its concentration level was small (only one-half after its long-distance transport crossing the Pacific). Our dust budget analysis revealed that the Asian dust flux passing through the longitude plane of 140° E was 2.1 Tg, and one third of that arrived North America. The cases analyzed in this study revealed that, while the Gobi Desert is an important source that can contribute to the long-range dust transport, the Taklimakan Desert appears to be another important source that can contribute to the dust transport occurring particularly at high altitudes.
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Takahashi, Y., M. Higashi, T. Furukawa, and S. Mitsunobu. "Change of iron species and iron solubility in Asian dust during the long-range transport from western China to Japan." Atmospheric Chemistry and Physics 11, no. 21 (November 11, 2011): 11237–52. http://dx.doi.org/10.5194/acp-11-11237-2011.
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Abstract. In the North Pacific, transport and deposition of mineral dust from Asia appear to be one of major sources of iron which can regulate growth of phytoplankton in the ocean. In this process, it is essential to identify chemical species of iron contained in Asian dust, because bioavailability of iron in the ocean is strongly influenced by the solubility of iron, which in turn is dependent on iron species in the dust. Here, we report that clay minerals (illite and chlorite) in the dusts near the source collected at Aksu (western China) can be transformed into ferrihydrite by atmospheric chemical processes during their long-range transport to eastern China (Qingdao) and Japan (Tsukuba) based on the speciation by X-ray absorption fine structure (XAFS) and other methods such as X-ray diffraction and chemical extraction. As a result, Fe molar ratio in Aksu (illite : chlorite : ferrihydrite = 70 : 25 : 5) was changed to that in Tsukuba (illite : chlorite : ferrihydrite = 65 : 10 : 25). Moreover, leaching experiments were conducted to study the change of iron solubility. It was found that the iron solubility for the dust in Tsukuba (soluble iron fraction: 11.8 % and 1.10 % for synthetic rain water and seawater, respectively) was larger than that in Aksu (4.1 % and 0.28 %, respectively), showing that iron in the dust after the transport becomes more soluble possibly due to the formation of ferrihydrite in the atmosphere. Our findings suggested that secondary formation of ferrihydrite during the transport should be considered as one of important processes in evaluating the supply of soluble iron to seawater.
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Xu, Chao, Yaoming Ma, Kun Yang, and Chao You. "Tibetan Plateau Impacts on Global Dust Transport in the Upper Troposphere." Journal of Climate 31, no. 12 (June 2018): 4745–56. http://dx.doi.org/10.1175/jcli-d-17-0313.1.
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Dust is a major component of atmospheric aerosol worldwide, greatly affecting regional and global climate. In this study dust aerosol optical depth (DAOD) and dust mass fluxes (DMF) were evaluated at different altitudes using measurements by the Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) and ERA-Interim data from March through May (MAM) for the period 2007–16. Significantly higher upper-tropospheric (above ~8 km) dust loads and DMF downstream of the Tibetan Plateau (TP) relative to those over other major dust sources of the Northern Hemisphere were found during spring. A DMF magnitude of 1010 g integrated across a 2°-latitude segment during spring was estimated downstream of the TP in the upper troposphere. A dust belt can be clearly seen at altitudes higher than 6 km over the downwind direction of the TP at latitudes of around 30°–40°N, crossing the Pacific Ocean and extending to North America during spring. A pathway for transporting dust aerosols into the upper troposphere is proposed, as follows. Dust is uplifted to the midtroposphere over the source regions; then, frequent, deep, dry convection prevailing over the TP during spring can cause convective overshooting that uplifts the dust aerosols to the upper troposphere. The TP thus acts as a channel for transporting dust from the lower atmosphere to the upper troposphere, enabling the long-range zonal transport of dust around the Northern Hemisphere.
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Wu, Na, Yongxiao Ge, Jilili Abuduwaili, Gulnura Issanova, and Galymzhan Saparov. "Insights into Variations and Potential Long-Range Transport of Atmospheric Aerosols from the Aral Sea Basin in Central Asia." Remote Sensing 14, no. 13 (July 3, 2022): 3201. http://dx.doi.org/10.3390/rs14133201.
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The dramatic shrinkage of the Aral Sea in the past decades has inevitably led to an environmental calamity. Existing knowledge on the variations and potential transport of atmospheric aerosols from the Aral Sea Basin (ASB) is limited. To bridge this knowledge gap, this study tried to identify the variations and long-range transport of atmospheric aerosols from the ASB in recent years. The Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model and Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) data were used to gain new insight into the types, variation and long-range transport of atmospheric aerosols from the ASB. The results showed five types of tropospheric aerosols and one type of stratospheric aerosol were observed over the ASB. Polluted dust and dust were the dominant subtypes through the year. Sulfate/other was the only stratospheric aerosol detected. The occurrence frequency of aerosols over the ASB showed obvious seasonal variation. Maximum occurrence frequency of dust appeared in spring (MAM) and that of polluted dust peaked in summer (JJA). The monthly occurrence frequency of dust and polluted dust exhibited unimodal distribution. Polluted dust and dust were distributed over wide ranges from 1 km to 5 km vertically. The multi-year average thickness of polluted dust and dust layers was around 1.3 km. Their potential long-range transport in different directions mainly impacts Uzbekistan, Turkmenistan, Kazakhstan and eastern Iran, and may reach as far as the Caucasus region, part of China, Mongolia and Russia. Combining aerosol lidar, atmospheric climate models and geochemical methods is strongly suggested to gain clarity on the variations and long-range transport of atmospheric aerosols from the Aral Sea Basin.
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Park, Sung-Bin, Jeong-A. Cho, Sang Seo Park, Ja-Ho Koo, and Yun Gon Lee. "A Possible Linkage between Dust Frequency and the Siberian High in March over Northeast Asia." Atmosphere 12, no. 2 (January 29, 2021): 176. http://dx.doi.org/10.3390/atmos12020176.
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Spring dust frequency in northeast Asia has been investigated using various approaches to understand the mechanisms of dust emission and transport. However, little attention has been paid to the linkage between dust activity and the Siberian High (SH), particularly when the SH pressure system is highly variable. In this study, we characterize the possible physical mechanisms of dust emission and transport associated with the Siberian High Intensity (SHI) and Siberian High Position Index (SHPI) in March using 18 years of ground-based observations and reanalysis data. We found that when the SHI was strong and the SH’s center was farther east (“Strong–East period”), surface and atmospheric temperatures were cooler than when the SHI was weak and the SH’s center was farther west (“Weak-West period”), due to anomalous anticyclonic pressure and strong easterlies. As a result, a reduction in the meridional temperature gradient in the lower atmosphere suppressed dust emission and transport, due to stagnant atmospheric conditions. This anomalous anticyclonic pressure in the Strong-East case seems to reduce the development of extratropical cyclones (ETC) in northeast Asia, leading to a less effective dust transport. A case study with composite analysis also showed a similar physical mechanism: stagnant air accompanying weakened westerlies in the Strong-East period suppressed dust transport to South Korea. Our findings reveal that the intensity and position of the SH can be utilized to identify spring transboundary air pollutants in northeast Asia.
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Boose, Yvonne, André Welti, James Atkinson, Fabiola Ramelli, Anja Danielczok, Heinz G. Bingemer, Michael Plötze, Berko Sierau, Zamin A. Kanji, and Ulrike Lohmann. "Heterogeneous ice nucleation on dust particles sourced from nine deserts worldwide – Part 1: Immersion freezing." Atmospheric Chemistry and Physics 16, no. 23 (December 6, 2016): 15075–95. http://dx.doi.org/10.5194/acp-16-15075-2016.
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Abstract. Desert dust is one of the most abundant ice nucleating particle types in the atmosphere. Traditionally, clay minerals were assumed to determine the ice nucleation ability of desert dust and constituted the focus of ice nucleation studies over several decades. Recently some feldspar species were identified to be ice active at much higher temperatures than clay minerals, redirecting studies to investigate the contribution of feldspar to ice nucleation on desert dust. However, so far no study has shown the atmospheric relevance of this mineral phase.For this study four dust samples were collected after airborne transport in the troposphere from the Sahara to different locations (Crete, the Peloponnese, Canary Islands, and the Sinai Peninsula). Additionally, 11 dust samples were collected from the surface from nine of the biggest deserts worldwide. The samples were used to study the ice nucleation behavior specific to different desert dusts. Furthermore, we investigated how representative surface-collected dust is for the atmosphere by comparing to the ice nucleation activity of the airborne samples. We used the IMCA-ZINC setup to form droplets on single aerosol particles which were subsequently exposed to temperatures between 233 and 250 K. Dust particles were collected in parallel on filters for offline cold-stage ice nucleation experiments at 253–263 K. To help the interpretation of the ice nucleation experiments the mineralogical composition of the dusts was investigated. We find that a higher ice nucleation activity in a given sample at 253 K can be attributed to the K-feldspar content present in this sample, whereas at temperatures between 238 and 245 K it is attributed to the sum of feldspar and quartz content present. A high clay content, in contrast, is associated with lower ice nucleation activity. This confirms the importance of feldspar above 250 K and the role of quartz and feldspars determining the ice nucleation activities at lower temperatures as found by earlier studies for monomineral dusts. The airborne samples show on average a lower ice nucleation activity than the surface-collected ones. Furthermore, we find that under certain conditions milling can lead to a decrease in the ice nucleation ability of polymineral samples due to the different hardness and cleavage of individual mineral phases causing an increase of minerals with low ice nucleation ability in the atmospherically relevant size fraction. Comparison of our data set to an existing desert dust parameterization confirms its applicability for climate models. Our results suggest that for an improved prediction of the ice nucleation ability of desert dust in the atmosphere, the modeling of emission and atmospheric transport of the feldspar and quartz mineral phases would be key, while other minerals are only of minor importance.
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Doganay, H., D. Akcali, T. Goktaş, K. Çaglar, D. Erbas, C. Saydam, and H. Bolay. "African Dust-Laden Atmospheric Conditions Activate the Trigeminovascular System." Cephalalgia 29, no. 10 (October 2009): 1059–68. http://dx.doi.org/10.1111/j.1468-2982.2008.01839.x.
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It has been recently noticed that dust originating from deserts can be transported to other continents by the atmosphere and has an adverse effect on public health, such as increased asthma attacks. Dust originating from the Saharan Desert could initiate a series of reactions upon contact with cloud water and results in the formation of reduced iron (Fe2+), oxalate and various basic amino acids. We aimed to evaluate whether the simulation of Saharan dust-containing atmospheric conditions could trigger the trigeminovascular system. Freely moving rats incubated within simulated atmospheric conditions containing (i) Saharan dust, (ii) Co60 gamma ray-treated Saharan dust (sterilized) and (iii) dust-free air, were investigated for the presence of c-fos expression in trigeminal nucleus caudalis (TNC) and for NOx (nitrate+nitrite) levels in blood samples. Atmospheric samples were analysed for microorganisms. Saharan dust-containing atmospheric conditions induced c-fos expression in nociceptive neurons within TNC. The number of c-fos+ neurons in superficial lamina of TNC was significantly higher in the Saharan dust group (32.9 ± 5.3, P = 0.0001) compared with dust-free air (11.02 ± 2.7) or Co60-treated Saharan dust groups (15.01 ± 2.4). An increase in NOx levels was detected in blood samples of rats exposed to Saharan dust-containing atmosphere. This study has revealed an unknown environmental factor as a possible trigger for headache. It is the first time that transport of Saharan dust with the atmospheric air stream has been documented to be able to trigger the trigeminovascular system in animals. Further studies are needed to explore the mechanisms and molecules that mediate the nociceptive effect and to guide new treatment strategies.
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Vogel, Bernhard, Corinna Hoose, Heike Vogel, and Christoph Kottmeier. "A model of dust transport applied to the Dead Sea Area." Meteorologische Zeitschrift 15, no. 6 (December 20, 2006): 611–24. http://dx.doi.org/10.1127/0941-2948/2006/0168.
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Groot Zwaaftink, Christine D., Ólafur Arnalds, Pavla Dagsson-Waldhauserova, Sabine Eckhardt, Joseph M. Prospero, and Andreas Stohl. "Temporal and spatial variability of Icelandic dust emissions and atmospheric transport." Atmospheric Chemistry and Physics 17, no. 17 (September 14, 2017): 10865–78. http://dx.doi.org/10.5194/acp-17-10865-2017.
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Abstract. Icelandic dust sources are known to be highly active, yet there exist few model simulations of Icelandic dust that could be used to assess its impacts on the environment. We here present estimates of dust emission and transport in Iceland over 27 years (1990–2016) based on FLEXDUST and FLEXPART simulations and meteorological re-analysis data. Simulations for the year 2012 based on high-resolution operational meteorological analyses are used for model evaluation based on PM2. 5 and PM10 observations in Iceland. For stations in Reykjavik, we find that the spring period is well predicted by the model, while dust events in late fall and early winter are overpredicted. Six years of dust concentrations observed at Stórhöfði (Heimaey) show that the model predicts concentrations of the same order of magnitude as observations and timing of modelled and observed dust peaks agrees well. Average annual dust emission is 4.3 ± 0.8 Tg during the 27 years of simulation. Fifty percent of all dust from Iceland is on average emitted in just 25 days of the year, demonstrating the importance of a few strong events for annual total dust emissions. Annual dust emission as well as transport patterns correlate only weakly to the North Atlantic Oscillation. Deposition amounts in remote regions (Svalbard and Greenland) vary from year to year. Only limited dust amounts reach the upper Greenland Ice Sheet, but considerable dust amounts are deposited on Icelandic glaciers and can impact melt rates there. Approximately 34 % of the annual dust emission is deposited in Iceland itself. Most dust (58 %), however, is deposited in the ocean and may strongly influence marine ecosystems.
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Sudarchikova, N., U. Mikolajewicz, C. Timmreck, D. O'Donnell, G. Schurgers, D. Sein, and K. Zhang. "Dust deposition in Antarctica in glacial and interglacial climate conditions: a modelling study." Climate of the Past Discussions 10, no. 5 (September 10, 2014): 3715–53. http://dx.doi.org/10.5194/cpd-10-3715-2014.
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Abstract. The mineral dust cycle responds to climate variations and plays an important role in the climate system by affecting the radiative balance of the atmosphere and modifying biogeochemistry. Polar ice cores provide a unique information about deposition of aeolian dust particles transported over long distance. These cores are a paleoclimate proxy archive of climate variability thousands of years ago. The current study is a first attempt to simulate past interglacial dust cycles with a global aerosol-climate model ECHAM5-HAM. The results are used to explain the dust deposition changes in Antarctica in terms of quantitative contribution of different processes, such as emission, atmospheric transport and precipitation, which will help to interpret paleodata from Antarctic ice cores. The investigated periods include four interglacial time-slices such as the pre-industrial control (CTRL), mid-Holocene (6000 yr BP), last glacial inception (115 000 yr BP) and Eemian (126 000 yr BP). One glacial time interval, which is Last Glacial Maximum (LGM) (21 000 yr BP) was simulated as well as to be a reference test for the model. Results suggest an increase of mineral dust deposition globally, and in Antarctica, in the past interglacial periods relative to the pre-industrial CTRL simulation. Approximately two thirds of the increase in the mid-Holocene and Eemian is attributed to enhanced Southern Hemisphere dust emissions. Slightly strengthened transport efficiency causes the remaining one third of the increase in dust deposition. The moderate change of dust deposition in Antarctica in the last glacial inception period is caused by the slightly stronger poleward atmospheric transport efficiency compared to the pre-industrial. Maximum dust deposition in Antarctica was simulated for the glacial period. LGM dust deposition in Antarctica is substantially increased due to 2.6 times higher Southern Hemisphere dust emissions, two times stronger atmospheric transport towards Antarctica, and 30% weaker precipitation over the Southern Ocean. The model is able to reproduce the order of magnitude of dust deposition globally and in Antarctica for the pre-industrial and LGM climates.
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Sudarchikova, N., U. Mikolajewicz, C. Timmreck, D. O'Donnell, G. Schurgers, D. Sein, and K. Zhang. "Modelling of mineral dust for interglacial and glacial climate conditions with a focus on Antarctica." Climate of the Past 11, no. 5 (May 19, 2015): 765–79. http://dx.doi.org/10.5194/cp-11-765-2015.
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Abstract. The mineral dust cycle responds to climate variations and plays an important role in the climate system by affecting the radiative balance of the atmosphere and modifying biogeochemistry. Polar ice cores provide unique information about deposition of aeolian dust particles transported over long distances. These cores are a palaeoclimate proxy archive of climate variability thousands of years ago. The current study is a first attempt to simulate past interglacial dust cycles with a global aerosol–climate model ECHAM5-HAM. The results are used to explain the dust deposition changes in Antarctica in terms of quantitative contribution of different processes, such as emission, atmospheric transport and precipitation, which will help to interpret palaeodata from Antarctic ice cores. The investigated periods include four interglacial time slices: the pre-industrial control (CTRL), mid-Holocene (6000 yr BP; hereafter referred to as "6 kyr"), last glacial inception (115 000 yr BP; hereafter "115 kyr") and Eemian (126 000 yr BP; hereafter "126 kyr"). One glacial time interval, the Last Glacial Maximum (LGM) (21 000 yr BP; hereafter "21 kyr"), was simulated as well to be a reference test for the model. Results suggest an increase in mineral dust deposition globally, and in Antarctica, in the past interglacial periods relative to the pre-industrial CTRL simulation. Approximately two-thirds of the increase in the mid-Holocene and Eemian is attributed to enhanced Southern Hemisphere dust emissions. Slightly strengthened transport efficiency causes the remaining one-third of the increase in dust deposition. The moderate change in dust deposition in Antarctica in the last glacial inception period is caused by the slightly stronger poleward atmospheric transport efficiency compared to the pre-industrial. Maximum dust deposition in Antarctica was simulated for the glacial period. LGM dust deposition in Antarctica is substantially increased due to 2.6 times higher Southern Hemisphere dust emissions, 2 times stronger atmospheric transport towards Antarctica, and 30% weaker precipitation over the Southern Ocean. The model is able to reproduce the order of magnitude of dust deposition globally and in Antarctica for the pre-industrial and LGM climates.
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Yu, Yan, Olga V. Kalashnikova, Michael J. Garay, and Michael Notaro. "Climatology of Asian dust activation and transport potential based on MISR satellite observations and trajectory analysis." Atmospheric Chemistry and Physics 19, no. 1 (January 11, 2019): 363–78. http://dx.doi.org/10.5194/acp-19-363-2019.
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Abstract. Asian dust, primarily emitted from the Taklamakan and Gobi deserts, has been reported to reach remote destinations, such as North America. However, the relative contribution of the Taklamakan and Gobi deserts to dust loadings through long-range transport remains unaddressed in any observational study. Here, the climatology of Asian dust activation and potential for transport is investigated using stereo observations of dust sources from the Multi-angle Imaging SpectroRadiometer (MISR) instrument combined with observation-initiated trajectory modeling. MISR-derived dust plume top height and dust plume motion vectors confirm the peak of dust activation and transport potential in spring over the Gobi Desert and in both spring and summer over the Taklamakan Desert. The long-range trajectory patterns of Asian dust, including the influence on North America through trans-Pacific transport, are assessed using extensive forward trajectories initiated by MISR dust plume observations. The trajectory analysis reveals latitude-dependent spread of dust trajectories from the Taklamakan and Gobi deserts, with Taklamakan dust dominantly affecting to the south of 50∘ N and Gobi dust primarily affecting to the north of 50∘ N in North America. The Asian dust activation and transport potential exhibit substantial seasonal and interannual variability, motivating future studies on the potential drivers.
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Dai, Guangyao, Kangwen Sun, Xiaoye Wang, Songhua Wu, Xiangying E, Qi Liu, and Bingyi Liu. "Dust transport and advection measurement with spaceborne lidars ALADIN and CALIOP and model reanalysis data." Atmospheric Chemistry and Physics 22, no. 12 (June 20, 2022): 7975–93. http://dx.doi.org/10.5194/acp-22-7975-2022.
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Abstract. In this paper, a long-term large-scale Saharan dust transport event which occurred between 14 and 27 June 2020 is tracked with the spaceborne lidars ALADIN (Atmospheric Laser Doppler Instrument) and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) together with ECMWF (European Centre for Medium-Range Forecasts) and HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory model) analysis. We evaluate the performance of ALADIN and CALIOP on the observations of dust optical properties and wind fields and explore the possibility of tracking the dust events and calculating the dust mass advection with the combination of satellite and model data. The dust plumes are identified with the AIRS/Aqua Dust Score Index and with the vertical feature mask product from CALIOP. The emission, dispersion, transport and deposition of the dust event are monitored using the data from AIRS/Aqua, CALIOP and HYSPLIT. With the quasi-synchronized observations by ALADIN and CALIOP, combined with the wind field and relative humidity, the dust advection values are calculated. From this study, it is found that the dust event generated on 14 and 15 June 2020 from the Sahara in North Africa dispersed and moved westward over the Atlantic Ocean, finally being deposited in the western Atlantic Ocean, the Americas and the Caribbean Sea. During the transport and deposition processes, the dust plumes are trapped in the northeasterly trade-wind zone between latitudes of 5∘ and 30∘ N and altitudes of 0 and 6 km. Aeolus provided the observations of the dynamics of this dust transport event in the Saharan Air Layer (SAL). From the measurement results on 19 June 2020, the dust plumes are captured quasi-simultaneously over the emission region (Western Sahara), the transport region (middle Atlantic) and the deposition region (western Atlantic) individually, which indicates that the dust plume area over the Atlantic on the morning of this day is quite enormous and that this dust transport event is massive and extensive. The quasi-synchronization observation results of 15, 16, 19, 24 and 27 June by ALADIN and CALIOP during the entire transport process show good agreement with the Dust Score Index data and the HYSPLIT trajectories, which indicates that the transport process of the same dust event is tracked by ALADIN and CALIOP, verifies that the dust transport spent around 2 weeks from the emission to the deposition and achieved the respective observations of this dust event's emission phase, development phase, transport phase, descent phase and deposition phase. Finally, the advection values for different dust parts and heights on 19 June and on the entire transport routine during transportation are computed. On 19 June, the mean dust advection values are about 1.91±1.21 mg m−2 s−1 over the emission region, 1.38±1.28 mg m−2 s−1 over the transport region and 0.75±0.68mgm-2s-1 over the deposition region. In the whole lifetime of the dust event, the mean dust advection values were about 1.51±1.03mgm-2s-1 on 15 June 2020, 2.19±1.72mgm-2s-1 on 16 June 2020, 1.38±1.28mgm-2s-1 on 19 June 2020, 1.60±1.08mgm-2s-1 on 24 June 2020 and 1.03±0.60mgm-2s-1 on 27 June 2020. During the dust development stage, the mean advection values gradually increased and reached their maximum on 16 June with the enhancement of the dust event. Then, the mean advection values decreased during the transport and the deposition of the dust over the Atlantic Ocean, the Americas and the Caribbean Sea.
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Abdelkader, Mohamed, Swen Metzger, Benedikt Steil, Klaus Klingmüller, Holger Tost, Andrea Pozzer, Georgiy Stenchikov, Leonard Barrie, and Jos Lelieveld. "Sensitivity of transatlantic dust transport to chemical aging and related atmospheric processes." Atmospheric Chemistry and Physics 17, no. 6 (March 20, 2017): 3799–821. http://dx.doi.org/10.5194/acp-17-3799-2017.
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Abstract. We present a sensitivity study on transatlantic dust transport, a process which has many implications for the atmosphere, the ocean and the climate. We investigate the impact of key processes that control the dust outflow, i.e., the emission flux, convection schemes and the chemical aging of mineral dust, by using the EMAC model following Abdelkader et al. (2015). To characterize the dust outflow over the Atlantic Ocean, we distinguish two geographic zones: (i) dust interactions within the Intertropical Convergence Zone (ITCZ), or the dust–ITCZ interaction zone (DIZ), and (ii) the adjacent dust transport over the Atlantic Ocean (DTA) zone. In the latter zone, the dust loading shows a steep and linear gradient westward over the Atlantic Ocean since particle sedimentation is the dominant removal process, whereas in the DIZ zone aerosol–cloud interactions, wet deposition and scavenging processes determine the extent of the dust outflow. Generally, the EMAC simulated dust compares well with CALIPSO observations; however, our reference model configuration tends to overestimate the dust extinction at a lower elevation and underestimates it at a higher elevation. The aerosol optical depth (AOD) over the Caribbean responds to the dust emission flux only when the emitted dust mass is significantly increased over the source region in Africa by a factor of 10. These findings point to the dominant role of dust removal (especially wet deposition) in transatlantic dust transport. Experiments with different convection schemes have indeed revealed that the transatlantic dust transport is more sensitive to the convection scheme than to the dust emission flux parameterization. To study the impact of dust chemical aging, we focus on a major dust outflow in July 2009. We use the calcium cation as a proxy for the overall chemical reactive dust fraction and consider the uptake of major inorganic acids (i.e., H2SO4, HNO3 and HCl) and their anions, i.e., sulfate (SO42−), bisulfate (HSO4−), nitrate (NO3−) and chloride (Cl−), on the surface of mineral particles. The subsequent neutralization reactions with the calcium cation form various salt compounds that cause the uptake of water vapor from the atmosphere, i.e., through the chemical aging of dust particles leading to an increase of 0.15 in the AOD under subsaturated conditions (July 2009 monthly mean). As a result of the radiative feedback on surface winds, dust emissions increased regionally. On the other hand, the aged dust particles, compared to the non-aged particles, are more efficiently removed by both wet and dry deposition due to the increased hygroscopicity and particle size (mainly due to water uptake). The enhanced removal of aged particles decreases the dust burden and lifetime, which indirectly reduces the dust AOD by 0.05 (monthly mean). Both processes can be significant (major dust outflow, July 2009), but the net effect depends on the region and level of dust chemical aging.
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Nowottnick, E., P. Colarco, A. da Silva, D. Hlavka, and M. McGill. "The fate of saharan dust across the atlantic and implications for a central american dust barrier." Atmospheric Chemistry and Physics 11, no. 16 (August 18, 2011): 8415–31. http://dx.doi.org/10.5194/acp-11-8415-2011.
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Abstract. Saharan dust was observed over the Caribbean basin during the summer 2007 NASA Tropical Composition, Cloud, and Climate Coupling (TC4) field experiment. Airborne Cloud Physics Lidar (CPL) and satellite observations from MODIS suggest a barrier to dust transport across Central America into the eastern Pacific. We use the NASA GEOS-5 atmospheric transport model with online aerosol tracers to perform simulations of the TC4 time period in order to understand the nature of this barrier. Our simulations are driven by the Modern Era Retrospective-Analysis for Research and Applications (MERRA) meteorological analyses. Compared to observations from MODIS and CALIOP, GEOS-5 reproduces the observed location and magnitude of observed dust events, but our baseline simulation does not develop as strong a barrier to dust transport across Central America as observations suggest. Analysis of the dust transport dynamics and loss processes suggest that while both mechanisms play a role in defining the dust transport barrier, loss processes by wet removal of dust are about twice as important as transport. Sensitivity analyses with our model showed that the dust barrier would not exist without convective scavenging over the Caribbean. The best agreement between our model and the observations was obtained when dust wet removal was parameterized to be more aggressive, treating the dust as we do hydrophilic aerosols.
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Abbasi, Sajjad, Mahrooz Rezaei, Farnaz Ahmadi, and Andrew Turner. "Atmospheric transport of microplastics during a dust storm." Chemosphere 292 (April 2022): 133456. http://dx.doi.org/10.1016/j.chemosphere.2021.133456.
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Perfumo, Amedea, and Roger Marchant. "Global transport of thermophilic bacteria in atmospheric dust." Environmental Microbiology Reports 2, no. 2 (April 2010): 333–39. http://dx.doi.org/10.1111/j.1758-2229.2010.00143.x.
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Zhao, T. L., S. L. Gong, X. Y. Zhang, and D. A. Jaffe. "Asian dust storm influence on North American ambient PM levels: observational evidence and controlling factors." Atmospheric Chemistry and Physics 8, no. 10 (May 22, 2008): 2717–28. http://dx.doi.org/10.5194/acp-8-2717-2008.
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Abstract. New observational evidence of the trans-Pacific transport of Asian dust and its contribution to the ambient particulate matter (PM) levels in North America was revealed, based on the interannual variations between Asian dust storms and the ambient PM levels in western North America from year 2000 to 2006. A high correlation was found between them with an R2 value of 0.83. From analysis of the differences in the correlation between 2005 and 2006, three factors explain the variation of trans-Pacific transport and influences of Asian dust storms on PM levels in western North America. These were identified by modeling results and the re-analysis data. They were 1) Strength of frontal cyclones from Mongolia to north eastern China: The frontal cyclones in East Asia not only bring strong cold air outbreaks, generating dust storms in East Asia, but also lift Asian dust into westerly winds of the free troposphere for trans-Pacific transport; 2) Pattern of transport pathway over the North Pacific: The circulation patterns of westerlies over the North Pacific govern the trans-Pacific transport pattern. Strong zonal airflow of the westerly jet in the free troposphere over the North Pacific favor significant trans-Pacific transport of Asian dust; 3) Variation of precipitation in the North Pacific: The scavenging of Asian dust particles by precipitation is a major process of dust removal on the trans-Pacific transport pathway. Therefore, variation of precipitation in the North Pacific could affect trans-Pacific transport of Asian dust.
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Zhao, Xiaoxi, Kan Huang, Joshua S. Fu, and Sabur F. Abdullaev. "Long-range transport of Asian dust to the Arctic: identification of transport pathways, evolution of aerosol optical properties, and impact assessment on surface albedo changes." Atmospheric Chemistry and Physics 22, no. 15 (August 15, 2022): 10389–407. http://dx.doi.org/10.5194/acp-22-10389-2022.
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Abstract. Airborne dust is one of the most important natural aerosols; it has various environmental impacts on air quality, ocean fertilization, and the global climate change. Asian dust, representing one of the major dust sources in the world, has been widely studied due to its long-range transport capability. However, its transport to the Arctic has been less investigated. In this study, two typical transport routes were identified based on the recorded dust events in China during 2011–2015. Accordingly, two specific Asian dust long-range transport events were selected and compared, i.e., one observed at Barrow, Alaska (traveled mostly over lands within 6–7 d), and the other one observed at Alert, Canada (traveled mostly over oceans within 7–8 d). The transport routes of the two dust events had been cross-validated by using air mass trajectory modeling, meteorology reanalysis data, ground-based aerosol columnar and profiling observations, and spaceborne remote sensing. It was found that different transport routes to the Arctic had divergent effects on the evolution of aerosol properties, revealing different mixing extents between dust, anthropogenic particles, smoke, and sea salts. Based on the Snow, Ice, and Aerosol Radiative (SNICAR) model, the albedo simulation indicated that dust and elemental carbon together reduced the surface albedo by 0.35 % to 2.63 % compared to the pure snow condition. This study implied that the dust long-range transport from China to the Arctic was ubiquitous and may be a potential contributor to the Arctic regional climate.
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Worthy, Soleil E., Anand Kumar, Yu Xi, Jingwei Yun, Jessie Chen, Cuishan Xu, Victoria E. Irish, Pierre Amato, and Allan K. Bertram. "The effect of (NH<sub>4</sub>)<sub>2</sub>SO<sub>4</sub> on the freezing properties of non-mineral dust ice-nucleating substances of atmospheric relevance." Atmospheric Chemistry and Physics 21, no. 19 (October 4, 2021): 14631–48. http://dx.doi.org/10.5194/acp-21-14631-2021.
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Abstract. A wide range of materials including mineral dust, soil dust, and bioaerosols have been shown to act as ice nuclei in the atmosphere. During atmospheric transport, these materials can become coated with inorganic and organic solutes which may impact their ability to nucleate ice. While a number of studies have investigated the impact of solutes at low concentrations on ice nucleation by mineral dusts, very few studies have examined their impact on non-mineral dust ice nuclei. We studied the effect of dilute (NH4)2SO4 solutions (0.05 M) on immersion freezing of a variety of non-mineral dust ice-nucleating substances (INSs) including bacteria, fungi, sea ice diatom exudates, sea surface microlayer substances, and humic substances using the droplet-freezing technique. We also studied the effect of (NH4)2SO4 solutions (0.05 M) on the immersion freezing of several types of mineral dust particles for comparison purposes. (NH4)2SO4 had no effect on the median freezing temperature (ΔT50) of 9 of the 10 non-mineral dust materials tested. There was a small but statistically significant decrease in ΔT50 (−0.43 ± 0.19 ∘C) for the bacteria Xanthomonas campestris in the presence of (NH4)2SO4 compared to pure water. Conversely, (NH4)2SO4 increased the median freezing temperature of four different mineral dusts (potassium-rich feldspar, Arizona Test Dust, kaolinite, montmorillonite) by 3 to 9 ∘C and increased the ice nucleation active site density per gram of material (nm(T)) by a factor of ∼ 10 to ∼ 30. This significant difference in the response of mineral dust and non-mineral dust ice-nucleating substances when exposed to (NH4)2SO4 suggests that they nucleate ice and/or interact with (NH4)2SO4 via different mechanisms. This difference suggests that the relative importance of mineral dust to non-mineral dust particles for ice nucleation in mixed-phase clouds could potentially increase as these particles become coated with (NH4)2SO4 in the atmosphere. This difference also suggests that the addition of (NH4)2SO4 (0.05 M) to atmospheric samples of unknown composition could potentially be used as an indicator or assay for the presence of mineral dust ice nuclei, although additional studies are still needed as a function of INS concentration to confirm the same trends are observed for different INS concentrations than those used here. A comparison with results in the literature does suggest that our results may be applicable to a range of mineral dust and non-mineral dust INS concentrations.
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Schepanski, K., I. Tegen, and A. Macke. "Saharan dust transport and deposition towards the tropical northern Atlantic." Atmospheric Chemistry and Physics 9, no. 4 (February 16, 2009): 1173–89. http://dx.doi.org/10.5194/acp-9-1173-2009.
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Abstract. We present a study of Saharan dust export towards the tropical North Atlantic using the regional dust emission, transport and deposition model LM-MUSCAT. Horizontal and vertical distribution of dust optical thickness, concentration, and dry and wet deposition rates are used to describe seasonality of dust export and deposition towards the eastern Atlantic for three typical months in different seasons. Deposition rates strongly depend on the vertical dust distribution, which differs with seasons. Furthermore the contribution of dust originating from the Bodélé Depression to Saharan dust over the Atlantic is investigated. A maximum contribution of Bodélé dust transported towards the Cape Verde Islands is evident in winter when the Bodélé source area is most active and dominant with regard to activation frequency and dust emission. Limitations of using satellite retrievals to estimate dust deposition are highlighted.
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Nickovic, S., A. Vukovic, M. Vujadinovic, V. Djurdjevic, and G. Pejanovic. "Technical Note: High-resolution mineralogical database of dust-productive soils for atmospheric dust modeling." Atmospheric Chemistry and Physics 12, no. 2 (January 18, 2012): 845–55. http://dx.doi.org/10.5194/acp-12-845-2012.
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Abstract. Dust storms and associated mineral aerosol transport are driven primarily by meso- and synoptic-scale atmospheric processes. It is therefore essential that the dust aerosol process and background atmospheric conditions that drive dust emissions and atmospheric transport are represented with sufficiently well-resolved spatial and temporal features. The effects of airborne dust interactions with the environment determine the mineral composition of dust particles. The fractions of various minerals in aerosol are determined by the mineral composition of arid soils; therefore, a high-resolution specification of the mineral and physical properties of dust sources is needed. Several current dust atmospheric models simulate and predict the evolution of dust concentrations; however, in most cases, these models do not consider the fractions of minerals in the dust. The accumulated knowledge about the impacts of the mineral composition in dust on weather and climate processes emphasizes the importance of including minerals in modeling systems. Accordingly, in this study, we developed a global dataset consisting of the mineral composition of the current potentially dust-producing soils. In our study, we (a) mapped mineral data to a high-resolution 30 s grid, (b) included several mineral-carrying soil types in dust-productive regions that were not considered in previous studies, and (c) included phosphorus.
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Yuan, Tiangang, Siyu Chen, Jianping Huang, Dongyou Wu, Hui Lu, Guolong Zhang, Xiaojun Ma, Ziqi Chen, Yuan Luo, and Xiaohui Ma. "Influence of Dynamic and Thermal Forcing on the Meridional Transport of Taklimakan Desert Dust in Spring and Summer." Journal of Climate 32, no. 3 (February 2019): 749–67. http://dx.doi.org/10.1175/jcli-d-18-0361.1.
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The Weather Research and Forecasting Model coupled with chemistry (WRF-Chem) associated with in situ measurements and satellite retrievals was used to investigate the meridional transport of Taklimakan Desert (TD) dust, especially in summer. Both satellite observations and simulations reveal that TD dust particles accumulate over the Tibetan Plateau (TP) and the Tianshan Mountains in summer, resulting in higher dust concentration up to 85 μg m−3 here. The proportions of meridional transport of TD dust in summer increase up to 30% of the total output dust over the TD. Further, the impacts of thermal and dynamic forcing on the meridional transport of TD dust to the TP and Tianshan Mountains are investigated based on composite analysis and numerical modeling. It is found that the weakness of the westerly jet over East Asia significantly decreases the eastward transport of TD dust. More TD dust particles lifted to higher altitude reach up to 8 km induced by the enhanced sensible heating in summer. Under the influence of the northerly airflow over the TD regions, the TD dust particles are strengthened southward and transported to the northern slope of the TP through topographic forcing. Moreover, the cyclonic circulation raises dust particles to higher altitude over the TP. It can further intensify the TP heat source by direct radiative forcing of dust aerosols, which may have a positive feedback to the southward transport of TD dust. This research provides confidence for the investigation of the role of TP dust with regard to the radiation balance and hydrological cycle over East Asia.
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Yumimoto, K., K. Eguchi, I. Uno, T. Takemura, Z. Liu, A. Shimizu, and N. Sugimoto. "An elevated large-scale dust veil from the Taklimakan Desert: Intercontinental transport and three-dimensional structure as captured by CALIPSO and regional and global models." Atmospheric Chemistry and Physics 9, no. 21 (November 11, 2009): 8545–58. http://dx.doi.org/10.5194/acp-9-8545-2009.
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Abstract. An intense dust storm occurred during 19–20 May 2007 over the Taklimakan Desert in northwestern China. Over the following days, the space-borne lidar CALIOP tracked an optically thin, highly elevated, horizontally extensive dust veil that was transported intercontinentally over eastern Asia, the Pacific Ocean, North America, and the Atlantic Ocean. A global aerosol transport model (SPRINTARS) simulated the dust veil quite well and provided a three-dimensional view of the intercontinental dust transport. The SPRINTARS simulation revealed that the dust veil traveled at 4–10 km altitudes with a thickness of 1–4 km along the isentropic surface between 310 and 340 K. The transport speed was about 1500 km/day. The estimated dust amount exported to the Pacific was 30.8 Gg, of which 65% was deposited in the Pacific and 18% was transported to the North Atlantic. These results imply that dust veils can fertilize open oceans, add to background dust, and affect the radiative budget at high altitudes through scattering and absorption. The injection mechanism that lifts dust particles into the free atmosphere is important for understanding the formation of the dust veil and subsequent long-range transport. We used a regional dust transport model (RC4) to analyze the dust emission and injection over the source region. The RC4 analysis revealed that strong northeasterly surface winds associated with low pressures invaded the Taklimakan Desert through the eastern corridor. These winds then formed strong upslope wind along the high, steep mountainsides of the Tibetan Plateau and blew large amounts of dust into the air. The updraft lifted the dust particles farther into the upper troposphere (about 9 km above mean sea level, MSL), where westerlies are generally present. The unusual terrain surrounding the Taklimakan Desert played a key role in the injection of dust to the upper troposphere to form the dust veil.
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Denjean, C., F. Cassola, A. Mazzino, S. Triquet, S. Chevaillier, N. Grand, T. Bourrianne, et al. "Size distribution and optical properties of mineral dust aerosols transported in the western Mediterranean." Atmospheric Chemistry and Physics 16, no. 2 (February 1, 2016): 1081–104. http://dx.doi.org/10.5194/acp-16-1081-2016.
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Abstract. This study presents in situ aircraft measurements of Saharan mineral dust transported over the western Mediterranean basin in June–July 2013 during the ChArMEx/ADRIMED (the Chemistry-Aerosol Mediterranean Experiment/Aerosol Direct Radiative Impact on the regional climate in the MEDiterranean region) airborne campaign. Dust events differing in terms of source region (Algeria, Tunisia and Morocco), time of transport (1–5 days) and height of transport were sampled. Mineral dust were transported above the marine boundary layer, which conversely was dominated by pollution and marine aerosols. The dust vertical structure was extremely variable and characterized by either a single layer or a more complex and stratified structure with layers originating from different source regions. Mixing of mineral dust with pollution particles was observed depending on the height of transport of the dust layers. Dust layers carried a higher concentration of pollution particles below 3 km above sea level (a.s.l.) than above 3 km a.s.l., resulting in a scattering Ångström exponent up to 2.2 below 3 km a.s.l. However, the optical properties of the dust plumes remained practically unchanged with respect to values previously measured over source regions, regardless of the altitude. Moderate absorption of light by the dust plumes was observed with values of aerosol single scattering albedo at 530 nm ranging from 0.90 to 1.00. Concurrent calculations from the aerosol chemical composition revealed a negligible contribution of pollution particles to the absorption properties of the dust plumes that was due to a low contribution of refractory black carbon in regards to the fraction of dust and sulfate particles. This suggests that, even in the presence of moderate pollution, likely a persistent feature in the Mediterranean, the optical properties of the dust plumes could be assumed similar to those of native dust in radiative transfer simulations, modelling studies and satellite retrievals over the Mediterranean. Measurements also showed that the coarse mode of mineral dust was conserved even after 5 days of transport in the Mediterranean, which contrasts with the gravitational depletion of large particles observed during the transport of dust plumes over the Atlantic. Simulations with the WRF mesoscale meteorological model highlighted a strong vertical turbulence within the dust layers that could prevent deposition of large particles during their atmospheric transport. This has important implications for the dust radiative effects due to surface dimming, atmospheric heating and cloud formation. The results presented here add to the observational data set necessary for evaluating the role of mineral dust on the regional climate and rainfall patterns in the western Mediterranean basin and understanding their atmospheric transport at global scale.
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Nickovic, S., A. Vukovic, M. Vujadinovic, V. Djurdjevic, and G. Pejanovic. "Technical Note: Minerals in dust productive soils – impacts and global distribution." Atmospheric Chemistry and Physics Discussions 11, no. 9 (September 20, 2011): 26009–34. http://dx.doi.org/10.5194/acpd-11-26009-2011.
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Abstract. Dust storms and associated mineral aerosol transport are mainly driven by meso and synoptic scale atmospheric processes. It is therefore essential that the dust aerosol process and background atmospheric conditions that drive the dust emission and atmospheric transport be represented with sufficiently well resolved spatial and temporal features. Effects of airborne dust interactions with the environment are determent by the mineral composition of dust particles. Fractions of various minerals in the aerosol are determined by the mineral composition of arid soils, therefore high-resolution specification of mineral and physical properties of dust sources is needed as well. Most current dust atmospheric models simulate/predict the evolution of dust concentration but in most cases they do not consider fractions of minerals in dust. Accumulated knowledge on impacts of mineral composition in dust on weather and climate processes emphasizes the importance of considering minerals in modelling systems. Following such needs, in this study we developed a global dataset on mineral composition of potentially dust productive soils. In our study (a) we mapped mineral data into a high-resolution 30-s grid, (b) we included mineral carrying soil types in dust productive regions that were not considered in previous studies, and (c) included phosphorus having in mind their importance for terrestrial and marine nutrition processes.
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Varga, G., J. Kovács, and G. Újvári. "Late Pleistocene variations of the background aeolian dust concentration in the Carpathian Basin: an estimate using decomposition of grain-size distribution curves of loess deposits." Netherlands Journal of Geosciences - Geologie en Mijnbouw 91, no. 1-2 (September 2013): 159–71. http://dx.doi.org/10.1017/s0016774600001566.
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AbstractAeolian dust deposits can be considered as one of the most important archives of past climatic changes. Alternating loess and paleosol strata display variations of the dust load in the Pleistocene atmosphere. By using the observations of recent dust storms, we are able to employ Late Pleistocene stratigraphic datasets (with accurate chronological framework) and detailed granulometric data for making conclusions on the atmospheric dust load in the past. Age-depths models, created from the absolute age data and stratigraphic interpretation, allow us to calculate sedimentation rates and dust fluxes, while grain-size specifies the dry-deposition velocity, i.e. the atmospheric residence time of mineral particles. Thus, the dust concentration can be expressed as the quotient of the dust flux and gravitational settling velocity. Recent observations helped to clarify the mechanisms behind aeolian sedimentation and the physical background of this process has nowadays been well established. Based on these two, main contrasting sedimentary modes of dust transport and deposition can be recognised: the short suspension episodes of the coarse (silt and very fine sand) fraction and the long-range transport of a fine (clay and fine silt) component. Using parametric curve fitting the basic statistical properties of these two sediment populations can be revealed for Pleistocene aeolian dust deposits, as it has been done for loess in Hungary. As we do not have adequate information on the magnitude and frequency of the Pleistocene dust storms, conclusions could only be made on the magnitude of continuous background dust load. The dust concentration can be set in the range between 1100 and 2750 μg/m3. These values are mostly higher than modern dust concentrations, even in arid regions. Another interesting proxy of past atmospheric conditions could be the visibility, being proportional to the dust concentration. According to the known empirical dust concentration – visibility equations, its value is around 6.5 to 26 kilometres.
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Prospero, Joseph M., Anthony C. Delany, Audrey C. Delany, and Toby N. Carlson. "The Discovery of African Dust Transport to the Western Hemisphere and the Saharan Air Layer: A History." Bulletin of the American Meteorological Society 102, no. 6 (June 2021): E1239—E1260. http://dx.doi.org/10.1175/bams-d-19-0309.1.
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AbstractThere is great interest in wind-borne mineral dust because of the role that dust plays in climate by modulating solar radiation and cloud properties. Today, much research focuses on North Africa because it is Earth’s largest and most persistently active dust source. Moreover, this region is expected to be greatly impacted by climate change, which would affect dust emission rates. Interest in dust was stimulated over 50 years ago when it was discovered that African dust was frequently transported across the Atlantic in great quantities. Here we report on the initial discovery of African dust in the Caribbean Basin. We show that there were three independent “first” discoveries of African dust in the 1950s through the 1960s. In each case, the discoverers were not seeking dust but, rather, they had other research objectives. The meteorological context of African dust transport was first elucidated in 1969 with the characterization of the Saharan air layer (SAL) and its role in effecting the efficient transport of African dust over great distances to the Western Hemisphere. The link between dust transport and African climate was established in the 1970s and 1980s when dust transport to the Caribbean increased greatly following the onset of severe drought in the Sahel. Here we chronicle these events and show how they contributed to our current state of knowledge.
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Johnson, M. S., N. Meskhidze, V. P. Kiliyanpilakkil, and S. Gassó. "Understanding the transport of Patagonian dust and its influence on marine biological activity in the South Atlantic Ocean." Atmospheric Chemistry and Physics 11, no. 6 (March 17, 2011): 2487–502. http://dx.doi.org/10.5194/acp-11-2487-2011.
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Abstract. The supply of bioavailable iron to the high-nitrate low-chlorophyll (HNLC) waters of the Southern Ocean through atmospheric pathways could stimulate phytoplankton blooms and have major implications for the global carbon cycle. In this study, model results and remotely-sensed data are analyzed to examine the horizontal and vertical transport pathways of Patagonian dust and quantify the effect of iron-laden mineral dust deposition on marine biological productivity in the surface waters of the South Atlantic Ocean (SAO). Model simulations for the atmospheric transport and deposition of mineral dust and bioavailable iron are carried out for two large dust outbreaks originated at the source regions of northern Patagonia during the austral summer of 2009. Model-simulated horizontal and vertical transport pathways of Patagonian dust plumes are in reasonable agreement with remotely-sensed data. Simulations indicate that the synoptic meteorological patterns of high and low pressure systems are largely accountable for dust transport trajectories over the SAO. According to model results and retrievals from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO), synoptic flows caused by opposing pressure systems (a high pressure system located to the east or north-east of a low pressure system) elevate the South American dust plumes well above the marine boundary layer. Under such conditions, the bulk concentration of mineral dust can quickly be transported around the low pressure system in a clockwise manner, follow the southeasterly advection pathway, and reach the HNLC waters of the SAO and Antarctica in ~3–4 days after emission from the source regions of northern Patagonia. Two different mechanisms for dust-iron mobilization into a bioavailable form are considered in this study. A global 3-D chemical transport model (GEOS-Chem), implemented with an iron dissolution scheme, is employed to estimate the atmospheric fluxes of soluble iron, while a dust/biota assessment tool (Boyd et al., 2010) is applied to evaluate the amount of bioavailable iron formed through the slow and sustained leaching of dust in the ocean mixed layer. The effect of iron-laden mineral dust supply on surface ocean biomass is investigated by comparing predicted surface chlorophyll-a concentration ([Chl-a]) to remotely-sensed data. As the dust transport episodes examined here represent large summertime outflows of mineral dust from South American continental sources, this study suggests that (1) atmospheric fluxes of mineral dust from Patagonia are not likely to be the major source of bioavailable iron to ocean regions characterized by high primary productivity; (2) even if Patagonian dust plumes may not cause visible algae blooms, they could still influence background [Chl-a] in the South Atlantic sector of the Southern Ocean.
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Bory, A., F. Dulac, C. Moulin, I. Chiapello, P. P. Newton, W. Guelle, C. E. Lambert, and G. Bergametti. "Atmospheric and oceanic dust fluxes in the northeastern tropical Atlantic Ocean: how close a coupling?" Annales Geophysicae 20, no. 12 (December 31, 2002): 2067–76. http://dx.doi.org/10.5194/angeo-20-2067-2002.
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Abstract. Atmospheric inputs to the ocean of dust originating from Africa are compared with downward dust flux in the oceanic water column. Atmospheric fluxes were estimated using remote-sensing-derived dust optical thickness and parameters from a transport/deposition model (TM2z). Oceanic fluxes were measured directly over/in two regions of contrasting primary productivity of the northeastern tropical Atlantic (one mesotrophic and one oligotrophic, located at about 500 and 1500 km off Mauritania) underlying the offshore dust plume. In both regions, estimates of annual atmospheric dust inputs to the ocean surface are lower than, but of the same order of magnitude as, oceanic fluxes (49.5 and 8.8 mg.m-2 .d-1 in the mesotrophic and oligotrophic regions). Part of this mismatch may reflect both a general flaw in the dust grain size distribution used in transport models, which likely underestimates large particles, and/or lateral advection to each region of dustier surface waters from upstream, where dust deposition is higher. Higher-frequency temporal coupling between atmospheric and oceanic fluxes seems to be primary-productivity dependent, as hypothesized in previously reported studies.Key words. Atmospheric composition and structure (aerosols and particles; geochemical cycles) Oceanography: biological and chemical (geochemistry)
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Zhao, T. L., S. L. Gong, X. Y. Zhang, J.-P. Blanchet, I. G. McKendry, and Z. J. Zhou. "A Simulated Climatology of Asian Dust Aerosol and Its Trans-Pacific Transport. Part I: Mean Climate and Validation." Journal of Climate 19, no. 1 (January 1, 2006): 88–103. http://dx.doi.org/10.1175/jcli3605.1.
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Abstract The Northern Aerosol Regional Climate Model (NARCM) was used to construct a 44-yr climatology of spring Asian dust aerosol emission, column loading, deposition, trans-Pacific transport routes, and budgets during 1960–2003. Comparisons with available ground dust observations and Total Ozone Mapping Spectrometer (TOMS) Aerosol Index (AI) measurements verified that NARCM captured most of the climatological characteristics of the spatial and temporal distributions, as well as the interannual and daily variations of Asian dust aerosol during those 44 yr. Results demonstrated again that the deserts in Mongolia and in western and northern China (mainly the Taklimakan and Badain Juran, respectively) were the major sources of Asian dust aerosol in East Asia. The dust storms in spring occurred most frequently from early April to early May with a daily averaged dust emission (diameter d < 41 μm) of 1.58 Mt in April and 1.36 Mt in May. Asian dust aerosol contributed most of the dust aerosol loading in the troposphere over the midlatitude regions from East Asia to western North America during springtime. Climatologically, dry deposition was a dominant dust removal process near the source areas, while the removal of dust particles by precipitation was the major process over the trans-Pacific transport pathway (where wet deposition exceeded dry deposition up to a factor of 20). The regional transport of Asian dust aerosol over the Asian subcontinent was entrained to an elevation of <3 km. The frontal cyclone in Mongolia and northern China uplifted dust aerosol in the free troposphere for trans-Pacific transport. Trans-Pacific dust transport peaked between 3 and 10 km in the troposphere along a zonal transport axis around 40°N. Based on the 44-yr-averaged dust budgets for the modeling domain from East Asia to western North America, it was estimated that of the average spring dust aerosol (diameter d < 41 μm) emission of ∼120 Mt from Asian source regions, about 51% was redeposited onto the source regions, 21% was deposited onto nondesert regions within the Asian subcontinent, and 26% was exported from the Asian subcontinent to the Pacific Ocean. In total, 16% of Asian dust aerosol emission was deposited into the North Pacific, while ∼3% of Asian dust aerosol was carried to the North American continent via trans-Pacific transport.
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Bonasoni, P., P. Cristofanelli, F. Calzolari, U. Bonafè, F. Evangelisti, A. Stohl, S. Zauli Sajani, R. van Dingenen, T. Colombo, and Y. Balkanski. "Aerosol-ozone correlations during dust transport episodes." Atmospheric Chemistry and Physics 4, no. 5 (August 3, 2004): 1201–15. http://dx.doi.org/10.5194/acp-4-1201-2004.
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Abstract. Its location in the Mediterranean region and its physical characteristics render Mt. Cimone (44°11′ N, 10°42′ E), the highest peak of the Italian northern Apennines (2165 m asl), particularly suitable to study the transport of air masses from the north African desert area to Europe. During these northward transports 12 dust events were registered in measurements of the aerosol concentration at the station during the period June–December 2000, allowing the study of the impact of mineral dust transports on free tropospheric ozone concentrations, which were also measured at Mt. Cimone. Three-dimensional backward trajectories were used to determine the air mass origin, while TOMS Aerosol Index data for the Mt. Cimone area were used to confirm the presence of absorbing aerosol over the measurement site. A trajectory statistical analysis allowed identifying the main source areas of ozone and aerosols. The analysis of these back trajectories showed that central Europe and north and central Italy are the major pollution source areas for ozone and fine aerosol, whereas the north African desert regions were the most important source areas for coarse aerosol and low ozone concentrations. During dust events, the Mt. Cimone mean volume concentration for coarse particles was 6.18 µm3/cm3 compared to 0.63 µm3/cm3 in dust-free conditions, while the ozone concentrations were 4% to 21% lower than the monthly mean background values. Our observations show that surface ozone concentrations were lower than the background values in air masses coming from north Africa, and when these air masses were also rich in coarse particles, the lowest ozone values were registered. Moreover, preliminary results on the possible impact of the dust events on PM10 and ozone values measured in Italian urban and rural areas showed that during the greater number of the considered dust events, significant PM10 increases and ozone decreases have occurred in the Po valley.
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Ha, Raegyung, Amarjargal Baatar, and Yongjae Yu. "Identification of atmospheric transport and dispersion of Asian dust storms." Natural Hazards and Earth System Sciences 17, no. 8 (August 29, 2017): 1425–35. http://dx.doi.org/10.5194/nhess-17-1425-2017.
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Abstract. Backward trajectories of individual Asian dust storm (ADS) events were calculated using the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) at four representative stations in Korea. A total of 743 ADS events and associated 2229 (endings of altitudes at 1000, 1500, and 2000 m per ADS event) backward trajectories from four stations were traced from January 2003 to August 2015. Regardless of the locations of the observed stations and the threshold time divide, a recent increase in the ADS occurrence rate was statistically significant with a 99.9 % confidence limit. Winter and spring were high-occurrence seasons for the ADS, while it rarely occurred in summer. Angular distributions of dust transport indicated a dominance of northwesterly wind, as more than two-thirds of ADS events are azimuthally confined from 290 to 340°. In addition, there is a tendency for stronger PM10 dust air concentration to be from the northwest. We found a strong inverse correlation between the number of days with ADS events and cumulative PM10 dust air concentration, indicating that the total amount of cumulative PM10 discharge was rather constant over time. If so, relatively shorter transport distances and a more continental dust passage over the Shandong peninsular would yield less PM10 in a shorter transport path but with a stronger concentration.
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Huang, Huilin, Yun Qian, Ye Liu, Cenlin He, Jianyu Zheng, Zhibo Zhang, and Antonis Gkikas. "Where does the dust deposited over the Sierra Nevada snow come from?" Atmospheric Chemistry and Physics 22, no. 23 (December 7, 2022): 15469–88. http://dx.doi.org/10.5194/acp-22-15469-2022.
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Abstract. Mineral dust contributes up to one-half of surface aerosol loading in spring over the southwestern United States, posing an environmental challenge that threatens human health and the ecosystem. Using self-organizing map (SOM) analysis with dust deposition and flux data from WRF-Chem and Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2), we identify four typical dust transport patterns across the Sierra Nevada, associated with the mesoscale winds, Sierra barrier jet (SBJ), North Pacific High (NPH), and long-range cross-Pacific westerlies, respectively. We find that dust emitted from the Central Valley is persistently transported eastward, while dust from the Mojave Desert and Great Basin influences the Sierra Nevada during mesoscale transport occurring mostly in winter and early spring. Asian dust reaching the mountain range comes either from the west through straight isobars (cross-Pacific transport) or from the north in the presence of the NPH. Extensive dust depositions are found on the west slope of the mountain, contributed by Central Valley emissions and cross-Pacific remote transport. In particular, the SBJ-related transport produces deposition through landfalling atmospheric rivers, whose frequency might increase in a warming climate.
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Vaughan, M., C. Trepte, C. Hostetler, and D. Winker. "Airborne dust distributions over the Tibetan Plateau and surrounding areas derived from the first year of CALIPSO lidar observations." Atmospheric Chemistry and Physics Discussions 8, no. 2 (March 25, 2008): 5957–77. http://dx.doi.org/10.5194/acpd-8-5957-2008.
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Abstract. Airborne dust is a major environmental hazard in Asia. Using an analysis of the first full year of CALIPSO lidar measurements, this paper derives unprecedented, altitude-resolved seasonal distributions of desert dust transported over the Tibetan Plateau (TP) and the surrounding areas. The CALIPSO lidar observations include numerous large dust plumes over the northern slope and eastern part of the TP, with the largest number of dust events occurring in the spring of 2007, and some layers being lofted to altitudes of 10 km and higher. Generation of the Tibetan airborne dusts appears to be largely associated with source regions to the north and on the eastern part of the plateau. Examination of the CALIPSO time history reveals an "airborne dust corridor" due to the eastward transport of dusts originating primarily in these source areas. This corridor extends from west to east and shows a seasonality largely modulated by the TP through its dynamical and thermal forcing on the atmospheric flows. On the southern side, desert dust particles originate predominately in North India and Pakistan. The dust transport occurs primarily in dry seasons around the TP western and southern slopes and dust particles become mixed with local polluted aerosols. No significant amount of dust appears to be transported over the Himalayas. Extensive forward trajectory simulations are also conducted to confirm the dust transport pattern from the nearby sources observed by the CALIPSO lidar.
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Aili, Aishajiang, Hailiang Xu, Tursun Kasim, and Abudumijiti Abulikemu. "Origin and Transport Pathway of Dust Storm and Its Contribution to Particulate Air Pollution in Northeast Edge of Taklimakan Desert, China." Atmosphere 12, no. 1 (January 14, 2021): 113. http://dx.doi.org/10.3390/atmos12010113.
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The Taklimakan Desert in Northwest China is the major source of dust storms in China. The northeast edge of this desert is a typical arid area which houses a fragile oasis eco-environment. Frequent dust storms cause harmful effects on the oasis ecosystem and negative impacts on agriculture, transportation, and human health. In this study, the major source region, transport pathway, and the potential contribution of dust storms to particulate air pollution were identified by using both trajectory analysis and monitoring data. To assess the source regions of dust storms, 48 h backward trajectories of air masses arriving at the Bugur (Luntai) County, which is located at the northeast edge of Taklimakan Desert, China on the dusty season (spring) and non-dusty month (August, representing non-dusty season) in the period of 1999–2013, were determined using Hybrid Single Particle Lagrangian Integrated Trajectory model version 4 (HYSPLIT 4). The trajectories were categorized by k-means clustering into 5 clusters (1a–5a) in the dusty season and 2 clusters (1b and 2b) in the non-dusty season, which show distinct features in terms of the trajectory origins and the entry direction to the site. Daily levels of three air pollutants measured at a station located in Bugur County were analyzed by using Potential Source Contribution Function (PSCF) for each air mass cluster in dusty season. The results showed that TSP is the major pollutant, with an average concentration of 612 µg/m3, as compared to SO2 (23 µg/m3) and NO2 (32 µg/m3) in the dusty season. All pollutants were increased with the dust weather intensity, i.e., from suspended dust to dust storms. High levels of SO2 and NO2 were mostly associated with cluster 1a and cluster 5a which had trajectories passing over the anthropogenic source regions, while high TSP was mainly observed in cluster 4a, which has a longer pathway over the shifting sand desert area. Thus, on strong dust storm days, not only higher TSP but also higher SO2 and NO2 levels were observed as compared to normal days. The results of this study could be useful to forecast the potential occurrence of dust storms based on meteorological data. Research focusing on this dust-storm-prone region will help to understand the possible causes for the changes in the dust storm frequency and intensity, which can provide the basis for mitigation of the negative effects on human health and the environment.
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Xiong, Jie, Tianliang Zhao, Yongqing Bai, Yu Liu, and Yongxiang Han. "Simulation and Analyses of the Potential Impacts of Different Particle-Size Dust Aerosols Caused by the Qinghai-Tibet Plateau Desertification on East Asia." Sustainability 12, no. 8 (April 16, 2020): 3231. http://dx.doi.org/10.3390/su12083231.
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In this paper on the analysis of the vertical distribution of different-diameter dust aerosols and the potential impacts on East Asia, the sensitivity simulation tests of dust aerosols during 2002–03 were conducted by changing the underlying surface on the Qinghai-Tibet Plateau in the global atmospheric circulation model Community Atmosphere Model (CAM) 3.1. The results show that dust aerosol particles in East Asia are mainly distributed in the diameters of 0.64–5.12 μm. The high concentrations of dust aerosols are centered on the surface in the source areas and gradually raised during the eastward transport across East Asia, reaching a height of 4 km at 120° E. The small dust particles with diameters less than 1.28 μm are transported higher and farther driven by the midlatitude westerlies. The Qinghai-Tibet Plateau desertification leads to increasing concentrations of dust aerosols in all size bins and raisesthe transport height of dust aerosols in East Asia. The long-range transport in the East Asian troposphere is dominated by dust aerosols particles of diameters 0.64–2.56 μm, as well as a large contribution of dust aerosols with diameters larger than 1.28 μm.
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Banerjee, Priyanka, S. K. Satheesh, K. Krishna Moorthy, Ravi S. Nanjundiah, and Vijayakumar S. Nair. "Long-Range Transport of Mineral Dust to the Northeast Indian Ocean: Regional versus Remote Sources and the Implications." Journal of Climate 32, no. 5 (February 5, 2019): 1525–49. http://dx.doi.org/10.1175/jcli-d-18-0403.1.
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Abstract Synergizing satellite remote sensing data with vertical profiles of atmospheric thermodynamics and regional climate model simulations, we investigate the relative importance, transport pathways, and seasonality of contribution of dust from regional (Thar Desert and adjoining arid regions) and remote (southwest Asia and northeast Africa) sources over the northeast Indian Ocean [i.e., the Bay of Bengal (BOB)]. We show that while over the northern BOB dust from the regional sources contribute more than 50% to the total dust load during the southwest monsoon period (June–September), interestingly; the remote dust sources dominate rest of the year. On the other hand, over the southern BOB, dust transported from the remote-source regions dominate throughout the year. During June, the dry elevated layer (at altitudes between 850 and 700 hPa) of dust, transported across the Indo-Gangetic Plain to the northern BOB, arises primarily from the Thar Desert. Dust from remote sources in the far west reaches the southern BOB after traversing over and around the southern Indian Peninsula. Since dust from these distinct source regions have different mineral composition (hence optical properties) and undergo distinct changes during atmospheric transport, it is important to understand source-specific dust contribution and transport pathways to address dust–climate feedback.