Journal articles on the topic 'Aerosols Asia'
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1
Choi, Wonei, Hyeongwoo Kang, Dongho Shin, and Hanlim Lee. "Satellite-Based Aerosol Classification for Capital Cities in Asia Using a Random Forest Model." Remote Sensing 13, no. 13 (June 24, 2021): 2464. http://dx.doi.org/10.3390/rs13132464.
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Aerosol types in Asian capital cities were classified using a random forest (RF) satellite-based aerosol classification model during 2018–2020 in an investigation of the contributions of aerosol types, with or without Aerosol Robotic Network (AERONET) observations. In this study, we used the recently developed RF aerosol classification model to detect and classify aerosols into four types: pure dust, dust-dominated aerosols, strongly absorbing aerosols, and non-absorbing aerosols. Aerosol optical and microphysical properties for each aerosol type detected by the RF model were found to be reasonably consistent with those for typical aerosol types. In Asian capital cities, pollution-sourced aerosols, especially non-absorbing aerosols, were found to predominate, although Asian cities also tend to be seasonally affected by natural dust aerosols, particularly in East Asia (March–May) and South Asia (March–August). No specific seasonal effects on aerosol type were detected in Southeast Asia, where there was a predominance of non-absorbing aerosols. The aerosol types detected by the RF model were compared with those identified by other aerosol classification models. This study indicates that the satellite-based RF model may be used as an alternative in the absence of AERONET sites or observations.
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Zhu, Anbao, Haiming Xu, Jiechun Deng, Jing Ma, and Shuhui Li. "El Niño–Southern Oscillation (ENSO) effect on interannual variability in spring aerosols over East Asia." Atmospheric Chemistry and Physics 21, no. 8 (April 20, 2021): 5919–33. http://dx.doi.org/10.5194/acp-21-5919-2021.
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Abstract. Effects of the El Niño–Southern Oscillation (ENSO) on the interannual variability in spring aerosols over East Asia are investigated using the Modern Era Retrospective analysis for Research and Applications Version 2 (MERRA-2) reanalysis aerosol data. Results show that the ENSO has a crucial effect on the spring aerosols over mainland South East Asia, southern China, and the ocean south of Japan. The above-normal (below-normal) aerosols are found over these regions during the ensuing spring of El Niño (La Niña). In contrast to the local aerosol diffusion in winter, the ENSO affects East Asian aerosols in the following spring mainly via the modulation of upstream aerosol generation and transport processes. The underlying physical mechanism is that during the ensuing spring of El Niño (La Niña), the dry (wet) air and reduced (enhanced) precipitation are beneficial for the increase (reduction) in biomass burning activities over northern mainland South East Asia, resulting in more (fewer) carbonaceous aerosol emissions. On the other hand, the anomalous anticyclone (cyclone) over the north-western Pacific (WNP) associated with El Niño (La Niña) enhances (weakens) the low-level south-westerly wind from northern mainland South East Asia to southern Japan, which transports more (less) carbonaceous aerosol downstream. Anomalous precipitation plays a role in reducing aerosols over the source region, but its washout effect over the downstream region is limited. The ENSO's impact on the ensuing spring aerosols is mainly attributed to the eastern Pacific ENSO rather than the central Pacific ENSO.
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Xiong, Jie, Tianliang Zhao, Yongqing Bai, Yu Liu, and Yongxiang Han. "Simulation and Analyses of the Potential Impacts of Different Particle-Size Dust Aerosols Caused by the Qinghai-Tibet Plateau Desertification on East Asia." Sustainability 12, no. 8 (April 16, 2020): 3231. http://dx.doi.org/10.3390/su12083231.
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In this paper on the analysis of the vertical distribution of different-diameter dust aerosols and the potential impacts on East Asia, the sensitivity simulation tests of dust aerosols during 2002–03 were conducted by changing the underlying surface on the Qinghai-Tibet Plateau in the global atmospheric circulation model Community Atmosphere Model (CAM) 3.1. The results show that dust aerosol particles in East Asia are mainly distributed in the diameters of 0.64–5.12 μm. The high concentrations of dust aerosols are centered on the surface in the source areas and gradually raised during the eastward transport across East Asia, reaching a height of 4 km at 120° E. The small dust particles with diameters less than 1.28 μm are transported higher and farther driven by the midlatitude westerlies. The Qinghai-Tibet Plateau desertification leads to increasing concentrations of dust aerosols in all size bins and raisesthe transport height of dust aerosols in East Asia. The long-range transport in the East Asian troposphere is dominated by dust aerosols particles of diameters 0.64–2.56 μm, as well as a large contribution of dust aerosols with diameters larger than 1.28 μm.
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Jiang, X., M. C. Barth, C. Wiedinmyer, and S. T. Massie. "Influence of anthropogenic aerosols on the Asian monsoon: a case study using the WRF-Chem model." Atmospheric Chemistry and Physics Discussions 13, no. 8 (August 16, 2013): 21383–425. http://dx.doi.org/10.5194/acpd-13-21383-2013.
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Abstract. Aerosols, in particular those related to anthropogenic activities, including black carbon, organic carbon, and sulfate aerosols, have been found to affect the Asian monsoon through direct and indirect aerosol radiative forcing. In this work, we use the coupled regional Weather Research and Forecasting model with Chemistry (WRF-Chem) to understand how aerosol changes from local emission sources could modulate the Asian monsoon precipitation through aerosol direct and indirect radiative effects. Our modeling results with the consideration of the local emissions show an improvement in simulated monsoon precipitation, when compared to reanalysis data and satellite observations. Aerosols generally induce a reduction in pre-monsoon and monsoon precipitation in East Asia. Over the Indian region, local anthropogenic emissions tend to reduce precipitation in the source regions while slightly increasing precipitation outside of the emission source regions. The increase in precipitation corresponds to a decrease in the cloud base level or lifting condensation level. Analysis of vertical cloud properties suggests that the increased cloud droplet number and prolonged cloud lifetime/reduced precipitation efficiency due to the local aerosol emissions are responsible for the precipitation reduction over East Asia. Aerosols from local emissions also play a very important role in the simulated surface temperature, radiation, and monsoon circulations.
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Tian, Pengfei, Lei Zhang, Jianmin Ma, Kai Tang, Lili Xu, Yuan Wang, Xianjie Cao, et al. "Radiative absorption enhancement of dust mixed with anthropogenic pollution over East Asia." Atmospheric Chemistry and Physics 18, no. 11 (June 4, 2018): 7815–25. http://dx.doi.org/10.5194/acp-18-7815-2018.
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Abstract. The particle mixing state plays a significant yet poorly quantified role in aerosol radiative forcing, especially for the mixing of dust (mineral absorbing) and anthropogenic pollution (black carbon absorbing) over East Asia. We have investigated the absorption enhancement of mixed-type aerosols over East Asia by using the Aerosol Robotic Network observations and radiative transfer model calculations. The mixed-type aerosols exhibit significantly enhanced absorbing ability than the corresponding unmixed dust and anthropogenic aerosols, as revealed in the spectral behavior of absorbing aerosol optical depth, single scattering albedo, and imaginary refractive index. The aerosol radiative efficiencies for the dust, mixed-type, and anthropogenic aerosols are −101.0, −112.9, and −98.3 Wm-2τ-1 at the bottom of the atmosphere (BOA); −42.3, −22.5, and −39.8 Wm-2τ-1 at the top of the atmosphere (TOA); and 58.7, 90.3, and 58.5 Wm-2τ-1 in the atmosphere (ATM), respectively. The BOA cooling and ATM heating efficiencies of the mixed-type aerosols are significantly higher than those of the unmixed aerosol types over the East Asia region, resulting in atmospheric stabilization. In addition, the mixed-type aerosols correspond to a lower TOA cooling efficiency, indicating that the cooling effect by the corresponding individual aerosol components is partially counteracted. We conclude that the interaction between dust and anthropogenic pollution not only represents a viable aerosol formation pathway but also results in unfavorable dispersion conditions, both exacerbating the regional air pollution in East Asia. Our results highlight the necessity to accurately account for the mixing state of aerosols in atmospheric models over East Asia in order to better understand the formation mechanism for regional air pollution and to assess its impacts on human health, weather, and climate.
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Hu, Zhiyuan, Jianping Huang, Chun Zhao, Yuanyuan Ma, Qinjian Jin, Yun Qian, L. Ruby Leung, Jianrong Bi, and Jianmin Ma. "Trans-Pacific transport and evolution of aerosols: spatiotemporal characteristics and source contributions." Atmospheric Chemistry and Physics 19, no. 19 (October 10, 2019): 12709–30. http://dx.doi.org/10.5194/acp-19-12709-2019.
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Abstract. Aerosols in the middle and upper troposphere have a long enough lifetime for trans-Pacific transport from East Asia to North America to influence air quality on the west coast of the United States (US). Here, we conduct quasi-global simulations (180∘ W–180∘ E and 70∘ S–75∘ N) from 2010 to 2014 using an updated version of WRF-Chem (Weather Research and Forecasting model fully coupled with chemistry) to analyze the spatiotemporal characteristics and source contributions of trans-Pacific aerosol transport. We find that trans-Pacific total aerosols have a maximum mass concentration (about 15 µg m−3) in the boreal spring with a peak between 3 and 4 km above the surface around 40∘ N. Sea salt and dust dominate the total aerosol mass concentration below 1 km and above 4 km, respectively. About 80.8 Tg of total aerosols (48.7 Tg of dust) are exported annually from East Asia, of which 26.7 Tg of aerosols (13.4 Tg of dust) reach the west coast of the US. Dust contributions from four desert regions in the Northern Hemisphere are analyzed using a tracer-tagging technique. About 4.9, 3.9, and 4.5 Tg year−1 of dust aerosol emitted from north Africa, the Middle East and central Asia, and East Asia, respectively, can be transported to the west coast of the US. The trans-Pacific aerosols dominate the column-integrated aerosol mass (∼65.5 %) and number concentration (∼80 %) over western North America. Radiation budget analysis shows that the inflow aerosols could contribute about 86.4 % (−2.91 W m−2) at the surface, 85.5 % (+1.36 W m−2) in the atmosphere, and 87.1 % (−1.55 W m−2) at the top of atmosphere to total aerosol radiative effect over western North America. However, near the surface in central and eastern North America, aerosols are mainly derived from local emissions, and the radiative effect of imported aerosols decreases rapidly. This study motivates further investigations of the potential impacts of trans-Pacific aerosols from East Asia on regional air quality and the hydrological cycle in North America.
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Maki, Teruya, Shogo Furumoto, Yuya Asahi, Kevin C. Lee, Koichi Watanabe, Kazuma Aoki, Masataka Murakami, et al. "Long-range-transported bioaerosols captured in snow cover on Mount Tateyama, Japan: impacts of Asian-dust events on airborne bacterial dynamics relating to ice-nucleation activities." Atmospheric Chemistry and Physics 18, no. 11 (June 8, 2018): 8155–71. http://dx.doi.org/10.5194/acp-18-8155-2018.
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Abstract. The westerly wind travelling at high altitudes over eastern Asia transports aerosols from the Asian deserts and urban areas to downwind areas such as Japan. These long-range-transported aerosols include not only mineral particles but also microbial particles (bioaerosols), that impact the ice-cloud formation processes as ice nuclei. However, the detailed relations of airborne bacterial dynamics to ice nucleation in high-elevation aerosols have not been investigated. Here, we used the aerosol particles captured in the snow cover at altitudes of 2450 m on Mt Tateyama to investigate sequential changes in the ice-nucleation activities and bacterial communities in aerosols and elucidate the relationships between the two processes. After stratification of the snow layers formed on the walls of a snow pit on Mt Tateyama, snow samples, including aerosol particles, were collected from 70 layers at the lower (winter accumulation) and upper (spring accumulation) parts of the snow wall. The aerosols recorded in the lower parts mainly came from Siberia (Russia), northern Asia and the Sea of Japan, whereas those in the upper parts showed an increase in Asian dust particles originating from the desert regions and industrial coasts of Asia. The snow samples exhibited high levels of ice nucleation corresponding to the increase in Asian dust particles. Amplicon sequencing analysis using 16S rRNA genes revealed that the bacterial communities in the snow samples predominately included plant associated and marine bacteria (phyla Proteobacteria) during winter, whereas during spring, when dust events arrived frequently, the majority were terrestrial bacteria of phyla Actinobacteria and Firmicutes. The relative abundances of Firmicutes (Bacilli) showed a significant positive relationship with the ice nucleation in snow samples. Presumably, Asian dust events change the airborne bacterial communities over Mt Tateyama and carry terrestrial bacterial populations, which possibly induce ice-nucleation activities, thereby indirectly impacting climate change.
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Park, R. S., S. J. Lee, S. K. Shin, and C. H. Song. "Contribution of ammonium nitrate to aerosol optical depth and direct radiative forcing by aerosols over East Asia." Atmospheric Chemistry and Physics Discussions 13, no. 7 (July 20, 2013): 19193–235. http://dx.doi.org/10.5194/acpd-13-19193-2013.
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Abstract. This study focused on the contribution of ammonium nitrate (NH4NO3) to aerosol optical depth (AOD) and direct radiative forcing (DRF) by aerosols over an East Asian domain. In order to evaluate the contribution, CTM-estimated AOD was combined with satellite-retrieved AOD, utilizing a data assimilation technique, over East Asia for the entire year of 2006. Using the assimilated AOD and CTM-estimated aerosol optical properties, the DRF by aerosols was estimated over East Asia via a radiative transfer model (RTM). Both assimilated AOD and estimated DRF values showed relatively good agreements with AOD and DRF by aerosols from AERONET. Based on these results, the contributions of NH4NO3 to AOD and DRF by aerosols (ΦAOD and ΦDRF) were estimated for four seasons of 2006 over East Asia. Both ΦAOD and ΦDRF showed seasonal variations over East Asia within the ranges between 4.7% (summer) and 31.3% (winter) and between 4.7% (summer) and 30.7% (winter), respectively, under clear-sky conditions, showing annual average contributions of 15.6% and 15.3%. Under all-sky conditions, ΦDRF varied between 3.6% (summer) and 24.5% (winter), showing annual average contribution of 12.1% over East Asia. These annual average contributions of NH4NO3 to AOD and DRF are almost comparable to the annual average mass fractions of NH4NO3 to PM2.5 and PM10 (17.0% and 14.0%, respectively). ΦAOD and ΦDRF were even larger in the locations where NH3 and NOx emission rates are strong like the Central East China (CEC) region and Sichuan basin. For example, under clear-sky conditions, both ΦAOD and ΦDRF over the CEC region range between 6.9% (summer) and 47.9% (winter) and between 6.7% (summer) and 47.5% (winter), respectively. Based on this analysis, it was concluded that both ΦDRF and ΦDRF cannot be ignored in East Asian air quality and radiative forcing studies, particularly during winter.
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Park, R. S., S. Lee, S. K. Shin, and C. H. Song. "Contribution of ammonium nitrate to aerosol optical depth and direct radiative forcing by aerosols over East Asia." Atmospheric Chemistry and Physics 14, no. 4 (February 27, 2014): 2185–201. http://dx.doi.org/10.5194/acp-14-2185-2014.
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Abstract. This study focused on the contribution of ammonium nitrate (NH4NO3) to aerosol optical depth (AOD) and direct radiative forcing (DRF) by aerosols over an East Asian domain. In order to evaluate the contribution, chemistry-transport model (CTM)-estimated AOD was combined with satellite-retrieved AOD, utilizing a data assimilation technique, over East Asia for the entire year of 2006. Using the assimilated AOD and CTM-estimated aerosol optical properties, the DRF by aerosols was estimated over East Asia via a radiative transfer model (RTM). Both assimilated AOD and estimated DRF values showed relatively good agreements with AOD and DRF by aerosols from AERONET. Based on these results, the contributions of NH4NO3 to AOD and DRF by aerosols (ΦAOD and ΦDRF) were estimated for the four seasons of 2006 over East Asia. Both ΦAOD and ΦDRF showed seasonal variations over East Asia within the ranges between 4.7% (summer) and 31.3% (winter) and between 4.7% (summer) and 30.7% (winter), respectively, under clear-sky conditions, showing annual average contributions of 15.6% and 15.3%. Under all-sky conditions, ΦDRF varied between 3.6% (summer) and 24.5% (winter), showing annual average contribution of 12.1% over East Asia. These annual average contributions of NH4NO3 to AOD and DRF are almost comparable to the annual average mass fractions of NH4NO3 in PM2.5 and PM10 (17.0% and 14.0%, respectively). ΦAOD and ΦDRF were even larger in the locations where NH3 and NOx emission rates are strong, such as the central East China (CEC) region and Sichuan Basin. For example, under clear-sky conditions, both ΦAOD and ΦDRF over the CEC region range between 6.9% (summer) and 47.9% (winter) and between 6.7% (summer) and 47.5% (winter), respectively. Based on this analysis, it was concluded that both ΦAOD and ΦDRF cannot be ignored in East Asian air quality and radiative forcing studies, particularly during winter.
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Liu, Yushan, and Bingqi Yi. "Aerosols over East and South Asia: Type Identification, Optical Properties, and Implications for Radiative Forcing." Remote Sensing 14, no. 9 (April 25, 2022): 2058. http://dx.doi.org/10.3390/rs14092058.
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Identification of aerosol types has long been a difficult problem over East and South Asia due to various limitations. In this study, we use 2-dimensional (2-D) and multi-dimensional Mahalanobis distance (MD) clustering algorithms to identify aerosol characteristics based on the data from the Aerosol Robotic Network from March 1998 to February 2018 over the South and East Asian region (10°N~50°N, 70°E~135°E). The single scattering albedo (SSA), absorption Angstrom exponent (AAE), extinction Angstrom exponent (EAE), real index of refraction (RRI), and imaginary index of refraction (IRI) are utilized for classification of aerosols. Sub-regions with similar background conditions over East and South Asia are identified by hierarchical clustering algorithm to illustrate distinctive meteorological states in different areas. The East and South Asian aerosols are found to have distinct regional and seasonal features relating to the meteorological conditions, land cover, and industrial infrastructure. It is found that the proportions of dust aerosol are the highest in spring at the SACOL site and in summer at the sites near the Northern Indo-Gangetic Plain area. In spring, biomass-burning aerosols are dominant over the central Indo-China Peninsula area. The aerosol characteristics at coastal sites are also analyzed and compared with previous results. The 2-D clustering method is useful when limited aerosol parameters are available, but the results are highly dependent on the sets of parameters used for identification. Comparatively, the MD method, which considers multiple aerosol parameters, could provide more comprehensive classification of aerosol types. It is estimated that only about 50% of the data samples that are identifiable by the MD method could be classified by the 2-D methods, and a lot of undetermined data samples could be mis-classified by the 2-D methods. The aerosol radiative forcing (ARF) and the aerosol radiative forcing efficiency (ARFE) of various aerosol types at the top and the bottom of the atmosphere (TOA and BOA) are determined based on the MD aerosol classification. The dust aerosols are found to have the largest ARF at the TOA (−36 W/m2), followed by the urban/industrial aerosols and biomass-burning aerosols. The ARFE of biomass-burning aerosols at the BOA (−165 W/m2/AOD550nm) is the strongest among those of the other aerosol types. The comparison of the results by MD and 2-D methods shows that the differences in ARF and ARFE are generally within 10%. Our results indicate the importance of aerosol type classification in accurately attributing the radiative contributions of different aerosol components.
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Liu, Yushan, and Bingqi Yi. "Aerosols over East and South Asia: Type Identification, Optical Properties, and Implications for Radiative Forcing." Remote Sensing 14, no. 9 (April 25, 2022): 2058. http://dx.doi.org/10.3390/rs14092058.
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Identification of aerosol types has long been a difficult problem over East and South Asia due to various limitations. In this study, we use 2-dimensional (2-D) and multi-dimensional Mahalanobis distance (MD) clustering algorithms to identify aerosol characteristics based on the data from the Aerosol Robotic Network from March 1998 to February 2018 over the South and East Asian region (10°N~50°N, 70°E~135°E). The single scattering albedo (SSA), absorption Angstrom exponent (AAE), extinction Angstrom exponent (EAE), real index of refraction (RRI), and imaginary index of refraction (IRI) are utilized for classification of aerosols. Sub-regions with similar background conditions over East and South Asia are identified by hierarchical clustering algorithm to illustrate distinctive meteorological states in different areas. The East and South Asian aerosols are found to have distinct regional and seasonal features relating to the meteorological conditions, land cover, and industrial infrastructure. It is found that the proportions of dust aerosol are the highest in spring at the SACOL site and in summer at the sites near the Northern Indo-Gangetic Plain area. In spring, biomass-burning aerosols are dominant over the central Indo-China Peninsula area. The aerosol characteristics at coastal sites are also analyzed and compared with previous results. The 2-D clustering method is useful when limited aerosol parameters are available, but the results are highly dependent on the sets of parameters used for identification. Comparatively, the MD method, which considers multiple aerosol parameters, could provide more comprehensive classification of aerosol types. It is estimated that only about 50% of the data samples that are identifiable by the MD method could be classified by the 2-D methods, and a lot of undetermined data samples could be mis-classified by the 2-D methods. The aerosol radiative forcing (ARF) and the aerosol radiative forcing efficiency (ARFE) of various aerosol types at the top and the bottom of the atmosphere (TOA and BOA) are determined based on the MD aerosol classification. The dust aerosols are found to have the largest ARF at the TOA (−36 W/m2), followed by the urban/industrial aerosols and biomass-burning aerosols. The ARFE of biomass-burning aerosols at the BOA (−165 W/m2/AOD550nm) is the strongest among those of the other aerosol types. The comparison of the results by MD and 2-D methods shows that the differences in ARF and ARFE are generally within 10%. Our results indicate the importance of aerosol type classification in accurately attributing the radiative contributions of different aerosol components.
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Mehta, M., N. Singh, M. Mittal, and M. Gumber. "ON VERTICAL DISTRIBUTION OF MAJOR AEROSOL TYPES OVER DIFFERENT PARTS OF ASIA." ISPRS - International Archives of the Photogrammetry, Remote Sensing and Spatial Information Sciences XLII-5 (November 19, 2018): 553–55. http://dx.doi.org/10.5194/isprs-archives-xlii-5-553-2018.
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<p><strong>Abstract.</strong> Asia, being the largest continent, both in its size and population is affected by different types of atmospheric aerosols. Also, owing to different local emissions/sources along with the long range transport mechanisms, there is a large variability in the distribution of different types of aerosols across the continent. Not only the effects are pertinent to the regional and global climate system, but the loadings also affect human health. Though there have been studies in the past focussing on columnar distribution of aerosol types over Asian region at continental and regional scales, studies focussed on regional vertical distribution of major aerosol types over different regions of Asia need attention. This paper presents the decadal (2007&ndash;16) vertical distribution of major aerosol components, i.e., dust, polluted dust and smoke over different parts of Asia as seen from the space-borne lidar, i.e., Cloud Aerosol Lidar with Orthogonal Polarisation (CALIOP) onboard Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO). Such a study can be useful in capacity building focussed on aerosol variability through remote sensing techniques.</p>
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Gao, Chao, Aijun Xiu, Xuelei Zhang, Qingqing Tong, Hongmei Zhao, Shichun Zhang, Guangyi Yang, and Mengduo Zhang. "Two-way coupled meteorology and air quality models in Asia: a systematic review and meta-analysis of impacts of aerosol feedbacks on meteorology and air quality." Atmospheric Chemistry and Physics 22, no. 8 (April 22, 2022): 5265–329. http://dx.doi.org/10.5194/acp-22-5265-2022.
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Abstract. Atmospheric aerosols can exert an influence on meteorology and air quality through aerosol–radiation interaction (ARI) and aerosol–cloud interaction (ACI), and this two-way feedback has been studied by applying two-way coupled meteorology and air quality models. As one of the regions with the highest aerosol loading in the world, Asia has attracted many researchers to investigate the aerosol effects with several two-way coupled models (WRF-Chem, WRF-CMAQ, GRAPES-CUACE, WRF-NAQPMS, and GATOR-GCMOM) over the last decade. This paper attempts to offer a bibliographic analysis regarding the current status of applications of two-way coupled models in Asia, related research focuses, model performances, and the effects of ARI and/or ACI on meteorology and air quality. There were a total of 160 peer-reviewed articles published between 2010 and 2019 in Asia meeting the inclusion criteria, with more than 79 % of papers involving the WRF-Chem model. The number of relevant publications has an upward trend annually, and East Asia, India, and China, as well as the North China Plain are the most studied areas. The effects of ARI and both ARI and ACI induced by natural aerosols (particularly mineral dust) and anthropogenic aerosols (bulk aerosols, different chemical compositions, and aerosols from different sources) are widely investigated in Asia. Through the meta-analysis of surface meteorological and air quality variables simulated by two-way coupled models, the model performance affected by aerosol feedbacks depends on different variables, simulation time lengths, selection of two-way coupled models, and study areas. Future research perspectives with respect to the development, improvement, application, and evaluation of two-way coupled meteorology and air quality models are proposed.
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Yang, Hong, Jinhui Xu, Wai-Shing Wu, Chun Hong Wan, and Jian Zhen Yu. "Chemical Characterization of Water-Soluble Organic Aerosols at Jeju Island Collected During ACE-Asia." Environmental Chemistry 1, no. 1 (2004): 13. http://dx.doi.org/10.1071/en04006.
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Environmental Context. Atmospheric aerosols — particles suspended in the atmosphere — are responsible for many phenomena, including formation of cloud condensation nuclei and degradation of regional visibility. Water-soluble organic carbon (WSOC) components make up a significant fraction of the aerosols' carbon mass, and have consequently received increasing attention from researchers. The chemical composition of the WSOC fraction, and thus their sources and effects, are not well known. This study focusses on WSOC from samples collected in South Korea as part of ACE-Asia (Asia-Pacific Regional Aerosol Characterization Experiment), a large international collaboration including Asia, the USA, Europe and Australia. Abstract.During the Asia-Pacific Regional Aerosol Characterization Experiment (ACE-Asia) intensive field campaign, aerosol samples of less than 2.5 μm diameter were collected at Jeju Island, South Korea, for chemical characterization of the water-soluble organic carbon (WSOC) fraction. The WSOC fraction had an average mass concentration of roughly half of that of sulfate and accounted for about two-thirds of the organic carbon mass. Thirty individual water-soluble organic compounds, belonging to the classes of mono- and di-carboxylic acids, aliphatic amines, and amino acids, were identified, accounting for 14% of the WSOC on a carbon basis. Oxalic acid was the most abundant single component. An additional 3% of the WSOC was estimated to be monomeric carbohydrates. Thermal analysis of the aerosol’s water extracts indicated that a significant fraction (~50%) of WSOC was thermally recalcitrant, possibly consisting of polymeric materials.
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Persad, Geeta G., David J. Paynter, Yi Ming, and V. Ramaswamy. "Competing Atmospheric and Surface-Driven Impacts of Absorbing Aerosols on the East Asian Summertime Climate." Journal of Climate 30, no. 22 (November 2017): 8929–49. http://dx.doi.org/10.1175/jcli-d-16-0860.1.
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East Asia has some of the largest concentrations of absorbing aerosols globally, and these, along with the region’s scattering aerosols, have both reduced the amount of solar radiation reaching Earth’s surface regionally (solar dimming) and increased shortwave absorption within the atmosphere, particularly during the peak months of the East Asian summer monsoon (EASM). This study analyzes how atmospheric absorption and surface solar dimming compete in driving the response of regional summertime climate to anthropogenic aerosols, which dominates, and why—issues of particular importance for predicting how East Asian climate will respond to projected changes in absorbing and scattering aerosol emissions in the future. These questions are probed in a state-of-the-art general circulation model using a combination of realistic and novel idealized aerosol perturbations that allow analysis of the relative influence of absorbing aerosols’ atmospheric and surface-driven impacts on regional circulation and climate. Results show that even purely absorption-driven dimming decreases EASM precipitation by cooling the land surface, counteracting climatological land–sea contrast and reducing ascending atmospheric motion and onshore winds, despite the associated positive top-of-the-atmosphere regional radiative forcing. Absorption-driven atmospheric heating does partially offset the precipitation and surface evaporation reduction from surface dimming, but the overall response to aerosol absorption more closely resembles the response to its surface dimming than to its atmospheric heating. These findings provide a novel decomposition of absorbing aerosol’s impacts on regional climate and demonstrate that the response cannot be expected to follow the sign of absorption’s top-of-the-atmosphere or even atmospheric radiative perturbation.
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Chavan, Prashant, Suvarna Fadnavis, Tanusri Chakroborty, Christopher E. Sioris, Sabine Griessbach, and Rolf Müller. "The outflow of Asian biomass burning carbonaceous aerosol into the upper troposphere and lower stratosphere in spring: radiative effects seen in a global model." Atmospheric Chemistry and Physics 21, no. 18 (September 28, 2021): 14371–84. http://dx.doi.org/10.5194/acp-21-14371-2021.
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Abstract. Biomass burning (BB) over Asia is a strong source of carbonaceous aerosols during spring. From ECHAM6–HAMMOZ model simulations and satellite observations, we show that there is an outflow of Asian BB carbonaceous aerosols into the upper troposphere and lower stratosphere (UTLS) (black carbon: 0.1 to 6 ng m−3 and organic carbon: 0.2 to 10 ng m−3) during the spring season. The model simulations show that the greatest transport of BB carbonaceous aerosols into the UTLS occurs from the Indochina and East Asia region by deep convection over the Malay Peninsula and Indonesia. The increase in BB carbonaceous aerosols enhances atmospheric heating by 0.001 to 0.02 K d−1 in the UTLS. The aerosol-induced heating and circulation changes increase the water vapor mixing ratios in the upper troposphere (by 20–80 ppmv) and in the lowermost stratosphere (by 0.02–0.3 ppmv) over the tropics. Once in the lower stratosphere, water vapor is further transported to the South Pole by the lowermost branch of the Brewer–Dobson circulation. These aerosols enhance the in-atmosphere radiative forcing (0.68±0.25 to 5.30±0.37 W m−2), exacerbating atmospheric warming, but produce a cooling effect on climate (top of the atmosphere – TOA: -2.38±0.12 to -7.08±0.72 W m−2). The model simulations also show that Asian carbonaceous aerosols are transported to the Arctic in the troposphere. The maximum enhancement in aerosol extinction is seen at 400 hPa (by 0.0093 km−1) and associated heating rates at 300 hPa (by 0.032 K d−1) in the Arctic.
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Cheng, Yueming, Tie Dai, Jiming Li, and Guangyu Shi. "Measurement Report: Determination of aerosol vertical features on different timescales over East Asia based on CATS aerosol products." Atmospheric Chemistry and Physics 20, no. 23 (December 10, 2020): 15307–22. http://dx.doi.org/10.5194/acp-20-15307-2020.
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Abstract. The Cloud-Aerosol Transport System (CATS) lidar, on board the International Space Station (ISS), provides a new opportunity for studying aerosol vertical distributions, especially the diurnal variations, from space observations. In this study, we investigate the seasonal variations and diurnal cycles in the vertical aerosol extinction coefficients (AECs) over East Asia by taking advantage of 32 months of continuous and uniform aerosol measurements from the CATS lidar. Over the Tibetan Plateau, a belt of AECs at approximately 6 km between 30 and 38∘ N persistently exists in all seasons with an obvious seasonal variation. In summer, the aerosols at 6 km are identified as a mixture of both anthropogenic aerosols transported from India and coarse dust particles from Asian dust sources. In addition, the high AECs up to 8 km in summer over the Tibetan Plateau are caused by smoke aerosols from thermal dynamic processes. In fall and winter, the northern slope of the plateau is continuously influenced by both dust aerosols and polluted aerosols transported upslope from cities located at lower elevations in northwestern Asia. The diurnal variation in AECs in North China is mainly related to the diurnal variations in the transported dust and local polluted aerosols. Below 2 km, the AEC profiles in North China at 06:00 and 12:00 CST (China standard time) are significantly higher than those at 00:00 and 18:00 CST, reaching a maximum at midday. The aerosol vertical profiles over the Tarim Desert region in summer have obvious diurnal variations, and the AECs at 12:00 and 18:00 CST are significantly higher than those at 00:00 and 06:00 CST, which are induced by the strong diurnal variations in near-surface wind speeds. In addition, the peak in the AEC profiles has a significant seasonal variation, which is mainly determined by the boundary layer height.
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Nee, Janbai. "Asian Dust properties investigated by multi-instruments." E3S Web of Conferences 99 (2019): 02003. http://dx.doi.org/10.1051/e3sconf/20199902003.
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Dust and many types of aerosols are major pollutants significantly affecting the environment in the East Asia. To identify and classify various types of aerosols is a challenge. In Taiwan and nearby areas, Asian Dust mainly arrive in spring with an average of about 5 dust storms each year. They usually come with some other aerosol sources, therefore it is important to identify these aerosols and their properties. In this paper, we report studying of dust aerosols by using several ground-based and remote sensing measurements. The AERONET data is used to find optical properties of aerosols in 2008-2012. The lidar observations can investigate further properties and atmospheric processes for specific dust events, including observations of aerosol-cloud interactions. These combined with model or space observations can help us to understand long range dust particles transported to distant areas and their interaction with weather systems. A real time case of observation of dust-cloud interaction is provided.
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Gao, Yiman, Bingliang Zhuang, Tijian Wang, Huimin Chen, Shu Li, Wen Wei, Huijuan Lin, and Mengmeng Li. "Climatic–Environmental Effects of Aerosols and Their Sensitivity to Aerosol Mixing States in East Asia in Winter." Remote Sensing 14, no. 15 (July 23, 2022): 3539. http://dx.doi.org/10.3390/rs14153539.
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To establish the direct climatic and environmental effect of anthropogenic aerosols in East Asia in winter under external, internal, and partial internal mixing (EM, IM and PIM) states, a well-developed regional climate–chemical model RegCCMS is used by carrying out sensitive numerical simulations. Different aerosol mixing states yield different aerosol optical and radiative properties. The regional averaged EM aerosol single scattering albedo is approximately 1.4 times that of IM. The average aerosol effective radiative forcing in the atmosphere ranges from −0.35 to +1.40 W/m2 with increasing internal mixed aerosols. Due to the absorption of black carbon aerosol, lower air temperatures are increased, which likely weakens the EAWM circulations and makes the atmospheric boundary more stable. Consequently, substantial accumulations of aerosols further appear in most regions of China. This type of interaction will be intensified when more aerosols are internally mixed. Overall, the aerosol mixing states may be important for regional air pollution and climate change assessments. The different aerosol mixing states in East Asia in winter will result in a variation from 0.04 to 0.11 K for the averaged lower air temperature anomaly and from approximately 0.45 to 2.98 μg/m3 for the aerosol loading anomaly, respectively, due to the different mixing aerosols.
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Zhang, Hongyue, Siyu Chen, Nanxuan Jiang, Xin Wang, Xiaorui Zhang, Jian Liu, Zhou Zang, et al. "Differences in Sulfate Aerosol Radiative Forcing between the Daytime and Nighttime over East Asia Using the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) Model." Atmosphere 9, no. 11 (November 13, 2018): 441. http://dx.doi.org/10.3390/atmos9110441.
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The effect of aerosols is an important indicator of climate change. Sulfate aerosols, as the major scattering aerosols, which have attracted more and more attention in recent years. The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) were utilized to investigate the spatial distribution of sulfate aerosols and their radiative forcing characteristics over East Asia in 2010. Results showed that sulfate aerosols were mainly distributed over eastern China (24–43° N, 101–126° E), especially in the Sichuan Basin. The concentration of sulfate aerosols decreased with increasing altitude over East Asia. It also exhibited obvious seasonal variations, where the largest range of sulfate aerosol concentrations was found in summer, with a maximum of 2.4 μg kg−1 over eastern China. Although sulfate aerosol concentrations varied slightly during day and night, there was still a significantly difference in the sulfate aerosol radiative forcing. Specifically, the magnitude of the direct radiative forcing induced by sulfate aerosols at the surface was approximately −3.02 W m−2 in the daytime, while that was +0.24 W m−2 in the nighttime. This asymmetric change that was caused by the radiative forcing of sulfate aerosols between day and night would have significant impacts on climate change at the regional scale.
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Sun, Jie, Kaihua Ding, Zulong Lai, and Haijun Huang. "Global and Regional Variations and Main Drivers of Aerosol Loadings over Land during 1980–2018." Remote Sensing 14, no. 4 (February 11, 2022): 859. http://dx.doi.org/10.3390/rs14040859.
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Aerosol particles originated from anthropogenic emissions, volcanic eruptions, biomass burning, and fossil combustion emissions, and their radiative effect is one of the most uncertain factors in climate change. Meanwhile, aerosol particles in fine particle size could also cause irreversible effects on the human respiratory system. This study attempted to analyse the spatial and temporal variations of global aerosol optical depth (AOD, 550 nm) during 1980–2018 using MERRA-2 aerosol reanalysis products and to investigate the effects of natural/anthropogenic emissions of different types of aerosols on AOD values. The results show that the global annual mean AOD values kept high levels with significant fluctuations during 1980–1995 and showed a consistent decreasing and less volatile trend after 1995. Spatially, the AOD values are relatively higher in the Northern Hemisphere than in the Southern Hemisphere, especially in North Africa (0.329), Northern India (0.235), and Eastern China (0.347), because of the intensive natural/anthropogenic aerosol emissions there. The sulphate-based aerosols emitted by biomass burning and anthropogenic emissions are the main types of aerosols worldwide, especially in densely populated and industrialized regions such as East Asia and Europe. Dust aerosols are also the main aerosol type in desert areas. For example, the AOD and AODP values for the Sahara Desert are 0.3178 and 75.32%, respectively. Both black carbon aerosols (BC) and organic carbon aerosols (OC) are primary or secondary from carbon emissions of fossil fuels, biomass burning, and open burning. Thus, the regions with high BC and OC aerosol loadings are mainly located in densely populated or vegetated areas such as East Asia, South Asia, and Central Africa. Sea salt aerosols are mainly found in coastline areas along the warm current pathway. This study could help relevant researchers in the fields of atmospheric science, environmental protection, air pollution, and ecological environment to understand the global spatial–temporal variations and main driving factors of aerosol loadings.
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Penning de Vries, M. J. M., S. Beirle, and T. Wagner. "UV Aerosol Indices from SCIAMACHY: introducing the SCattering Index (SCI)." Atmospheric Chemistry and Physics 9, no. 24 (December 21, 2009): 9555–67. http://dx.doi.org/10.5194/acp-9-9555-2009.
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Abstract. The Absorbing Aerosol Index (AAI) is a useful tool for detecting aerosols that absorb UV radiation – especially in cases where other aerosol retrievals fail, such as over bright surfaces (e.g. desert) and in the presence of clouds. The AAI does not, however, consider contributions from scattering (hardly absorbing) aerosols and clouds: they cause negative AAI values and are usually disregarded. In this paper, we demonstrate the use of the AAI's negative counterpart, the SCattering Index (SCI) to detect scattering aerosols. Consideration of the full UV Aerosol Index scale is of importance if the Aerosol Index is to be used for the quantification of aerosol absorption in the future. Maps of seasonally averaged SCI show significantly enhanced values in summer in Southeast USA and Southeast Asia, pointing to a high production of scattering aerosols (presumably mainly sulphate aerosols and secondary organic aerosols) in this season. The application of a cloud filter makes the presence of scattering aerosols even more clear. Radiative transfer calculations were performed to investigate the sensitivity of AAI and SCI to cloud parameters, and it is demonstrated that clouds cause significant SCI, in some special cases even small AAI values. The results from cloud modelling imply that cloud effects need to be taken into account when AAI and SCI are used in a quantitative manner. The paper concludes with a comparison of aerosol parameters from AERONET and our Aerosol Indices (AAI and SCI) from SCIAMACHY, where reasonable agreement was found for six AERONET stations in Southeast USA, Southeast Asia, and Africa. These findings corroborate the suitability of SCI as a tool to detect scattering aerosols.
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Luan, Y., and L. Jaeglé. "Composite study of aerosol export events from East Asia and North America." Atmospheric Chemistry and Physics Discussions 12, no. 8 (August 28, 2012): 21977–2022. http://dx.doi.org/10.5194/acpd-12-21977-2012.
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Abstract. We use satellite observations of aerosol optical depth (AOD) from the Moderate Resolution Imaging Spectrometer (MODIS) together with the GEOS-Chem global chemical transport model to contrast export of aerosols from East Asia and North America during 2004–2010. The GEOS-Chem model reproduces the spatial distribution and temporal variations of Asian aerosol outflow generally well, although a low bias (−30%) is found in the model fine mode AOD. We use the model to identify 244 aerosol pollution export events from E. Asia and 251 export events from N. America over our 7-yr study period. When these events are composited by season, we find that the AOD in the outflow is enhanced by 50–100% relative to seasonal mean values. The composite Asian plume splits into one branch going poleward towards the Arctic, with the other crossing the Pacific in 6–8 days. A fraction of the aerosols is trapped in the subtropical Pacific High. The N. American plume travels to the northeast Atlantic, reaching Europe after 4–5 days. Part of the composite plume turns anticyclonically in the Azores High, where it slowly decays. Both the Asian and N. American export events are favored by a dipole structure in sea-level pressure anomalies, associated with mid-latitude cyclone activity over the respective source regions. The observed AOD in the E. Asian outflow exhibits stronger seasonality, with a spring maximum, than the N. American outflow, with a weak summer maximum. The large spring AOD in the Asian outflow is the result of enhanced sulfate and dust aerosol concentrations, but is also due to a larger export efficiency of sulfate and SO2 from the Asian boundary layer relative to the N. American boundary layer. While the N. American sulfate outflow is mostly found in the lower troposphere (1–3 km altitude), the Asian sulfate outflow occurs at higher altitudes (2–6 km). In the Asian outflow 42–59% of the sulfate column is present above 2 km altitude, with only 24–35% in the N. American outflow. We link this to the factor of 2–5 lower precipitation in the warm conveyor belts (WCB) of midlatitude cyclones over E. Asia compared to N. America. This relative lack of precipitation makes Asian WCB very efficient for injecting aerosols in the middle troposphere.
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Park, Soon-Ung, and Jeong Hoon Cho. "Air Quality in East Asia during the heavy haze event period of 10 to 15 January 2013." International Journal of Energy and Environment 15 (March 24, 2021): 1–9. http://dx.doi.org/10.46300/91012.2021.15.1.
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A prolonged heavy haze event that has caused for the Environmental Protection Bureau (EPB) in Beijing to take emergency measures for the protection of the public health and the reduction of air pollution damages in China has been analyzed with the use of the Aerosol modeling System (AMS) to identify causes of this event. It is found that the heavy haze event is associated with high aerosols and water droplets concentrations. These high aerosol concentrations are mainly composed of anthropogenic aerosols, especially secondary inorganic aerosols formed by gas-to-particle conversion of gaseous pollutants in the eastern part of China whereas those in the northeastern parts of China are composed of the mixture of the anthropogenic aerosols and the Asian dust aerosol originated from the dust source regions of northern China and Mongolia. These high aerosol concentrations are found to be subsequently transported to the downwind regions of the Korean Peninsula and Japan causing a prolonged haze event there. It is also found that the Asian dust aerosol originated from northern China and Mongolia and the anthropogenic aerosols produced by chemical reactions of pollutants in the high emissions region of eastern China can cause significantly adverse environmental impacts in the whole Asian region by increased atmospheric aerosol loadings that may cause respiration diseases and visibility reduction and by excess deposition of aerosols causing adverse impacts on terrestrial and marine eco-systems.
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Herbert, Ross, Laura J. Wilcox, Manoj Joshi, Ellie Highwood, and Dave Frame. "Nonlinear response of Asian summer monsoon precipitation to emission reductions in South and East Asia." Environmental Research Letters 17, no. 1 (December 22, 2021): 014005. http://dx.doi.org/10.1088/1748-9326/ac3b19.
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Abstract Anthropogenic aerosols over South and East Asia currently have a stronger impact on the Asian summer monsoon (ASM) than greenhouse gas emissions, yet projected aerosol emission changes in these regions are subject to considerable uncertainties such as timescale, location, or emission type. We use a circulation/climate model with idealised aerosol distributions to demonstrate that the sum of ASM responses to aerosol emission reductions in each region is very different to the response to simultaneous reductions in both regions, implying the ASM response to aerosol emissions reductions is highly nonlinear. The phenomenon is independent of whether aerosols are scattering or absorbing, and results from interaction of induced atmospheric circulation changes. The nonlinearity from interactions between aerosol forcing from different regions represents a new source of uncertainty in projections of ASM changes over the next 30–40 years, and may limit the utility of country-dependent aerosol trajectories when considering their Asia-wide effects, though we recommend further work to establish whether the nonlinearity is buffered by other drivers. To understand likely changes in the ASM due to aerosol reductions, countries will need to accurately take account of emissions reductions from across the wider region, rather than approximating them using simple scenarios and emulators. The nonlinearity in the response to forcing therefore presents a regional public goods issue for countries affected by the ASM, as the costs and benefits of aerosol emissions reductions are not internalised; in fact, forcings from different countries such as India and China work jointly to determine outcomes across the region.
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Deng, Jiechun, Leying Zhang, Jing Ma, and Dorina Chyi. "Modulated Responses of East Asian Winter Climate to Anthropogenic Aerosols by Urban Cover in Eastern China." Atmosphere 12, no. 4 (April 9, 2021): 471. http://dx.doi.org/10.3390/atmos12040471.
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The increasing anthropogenic aerosols (AAs) over East Asia have caused significant regional climate responses, but the role of urban land-use changes which occur simultaneously, in altering these AA-induced changes, is not well understood. Here, the modulation of the AAs’ effect on the East Asian winter (November–January) climate by the urban cover in eastern China was investigated using the Community Atmosphere Model version 5.1 coupled with the Community Land Model version 4. Results show that the winter sulfate aerosol burden is higher from central eastern China to southern Japan in the case with the presence of urban cover than in the case without it, resulting from urban-induced circulation changes. Such aerosol changes markedly increase the cloud fraction and precipitation over northern China and the adjacent ocean to the east, especially convection activities around southern Japan. This leads to a cooling effect near the surface over northern China and in the mid-upper troposphere to the east due to aerosol direct and indirect effects. The resulting circulation responses act to shift the mid-tropospheric East Asian trough southward and the upper-level East Asian westerly jet-stream as well, further supporting the surface changes. These winter climate responses to the urban-modulated aerosols can largely offset or even reverse those to the AAs forcing without the urban cover in the model, especially in northern East Asia. This study highlights the need to consider the modulating role of urban land-use changes in assessing the AAs’ climatic effect over East Asia and other regions.
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Yang, Q., C. M. Bitz, and S. J. Doherty. "Offsetting effects of aerosols on Arctic and global climate in the late 20th century." Atmospheric Chemistry and Physics Discussions 13, no. 11 (November 27, 2013): 30929–43. http://dx.doi.org/10.5194/acpd-13-30929-2013.
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Abstract. We examine the impacts of atmospheric aerosols on Arctic and global climate using a series of 20th century transient simulations from Community Climate System Model version 4 (CCSM4). We focus on the response of surface air temperature to the direct radiative forcing driven by changes in sulfate and black carbon (BC) concentrations from 1975 to 2005 and we also examine the response to sulfate, BC, and organic carbon aerosols varying at once. The direct forcing from sulfate dominates the aerosol climate effect. Globally averaged, all three aerosols produce a cooling trend of 0.015 K decade−1 during the period 1975–2005. In the Arctic, surface air temperature has large spatial variations in response to changes in aerosol concentrations. Over the European Arctic, aerosols induce about 0.6 K decade−1 warming which is about 1.8 K warming over the 30 yr period. This warming is triggered mainly by the reduction in sulfate and BC emissions over Europe since the 1970s and is reinforced by sea ice loss and a strengthening in atmospheric northward heat transport. Over the Siberian and North American Arctic, surface air temperature is likely influenced primarily by changes in aerosol emissions from Asia. An increase in sulfate emissions over Asia induces a large cooling while an increase in BC over Asia causes a significant warming.
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Luan, Y., and L. Jaeglé. "Composite study of aerosol export events from East Asia and North America." Atmospheric Chemistry and Physics 13, no. 3 (February 1, 2013): 1221–42. http://dx.doi.org/10.5194/acp-13-1221-2013.
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Abstract. We use satellite observations of aerosol optical depth (AOD) from the Moderate Resolution Imaging Spectrometer (MODIS) together with the GEOS-Chem global chemical transport model to contrast export of aerosols from East Asia and North America during 2004–2010. The GEOS-Chem model reproduces the spatial distribution and temporal variations of Asian aerosol outflow generally well, although a low bias (−30%) is found in the model fine mode AOD, particularly during summer. We use the model to identify 244 aerosol pollution export events from E. Asia and 251 export events from N. America over our 7-year study period. When these events are composited by season, we find that the AOD in the outflow is enhanced by 50–100% relative to seasonal mean values. The composite Asian plume splits into one branch going poleward to the Arctic in 3–4 days, with the other crossing the Pacific Ocean in 6–8 days. A fraction of the aerosols is trapped in the subtropical Pacific High during spring and summer. The N. American plume travels to the northeast Atlantic, reaching Europe after 4–5 days. Part of the composite plume turns anticyclonically in the Azores High, where it slowly decays. Both the Asian and N. American export events are favored by a dipole structure in sea-level pressure anomalies, associated with mid-latitude cyclone activity over the respective source regions. This dipole structure during outflow events is a strong feature for all seasons except summer, when convection becomes more important. The observed AOD in the E. Asian outflow exhibits stronger seasonality, with a spring maximum, than the N. American outflow, with a broad spring/summer maximum. The large spring AOD in the Asian outflow is the result of enhanced sulfate and dust aerosol concentrations, but is also due to a larger export efficiency of sulfate and SO2 from the Asian boundary layer relative to the N. American boundary layer. While the N. American sulfate outflow is mostly found in the lower troposphere (1–3 km altitude), the Asian sulfate outflow occurs at higher altitudes (2–6 km). In the Asian outflow 42–59% of the sulfate column is present above 2 km altitude, with only 24–35% in the N. American outflow. We link this to the factor of 2–5 lower precipitation in the warm conveyor belts (WCB) of midlatitude cyclones over E. Asia compared to N. America. This relative lack of precipitation makes Asian WCB very efficient for injecting aerosols in the middle troposphere.
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Wang, Sheng-Hsiang, Heng-Wai Lei, Shantanu Kumar Pani, Hsiang-Yu Huang, Neng-Huei Lin, Ellsworth J. Welton, Shuenn-Chin Chang, and Yueh-Chen Wang. "Determination of Lidar Ratio for Major Aerosol Types over Western North Pacific Based on Long-Term MPLNET Data." Remote Sensing 12, no. 17 (August 26, 2020): 2769. http://dx.doi.org/10.3390/rs12172769.
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East Asia is the most complex region in the world for aerosol studies, as it encounters a lot of varieties of aerosols, and aerosol classification can be a challenge in this region. In the present study, we focused on the relationship between aerosol types and aerosol optical properties. We analyzed the long-term (2005–2012) data of vertical profiles of aerosol extinction coefficients, lidar ratio (Sp), and other aerosol optical properties obtained from a NASA Micro-Pulse Lidar Network and Aerosol Robotic Network site in northern Taiwan, which frequently receives Asian continental outflows. Based on aerosol extinction vertical profiles, the profiles were classified into two types: type 1 (single-layer structure) and type 2 (two-layer structure). Fall season (October–November) was the prevailing season for the Type 1, whereas type 2 mainly happened in spring (March–April). In type 1, air masses normally originated from three regional sectors, i.e., Asia continental (AC), Pacific Ocean (PO), and Southeast Asia (SA). The mean Sp values were 39 ± 17 sr, 30 ± 12 sr, and 38 ± 18 sr for the AC, PO, and SA sectors, respectively. The Sp results suggested that aerosols from the AC sector contained dust and anthropogenic particles, and aerosols from the PO sector were most likely sea salts. We further combined the EPA dust event database and backward trajectory analysis for type 2. Results showed that Sp was 41 ± 14 sr and 53 ± 21 sr for dust storm and biomass-burning events, respectively. The Sp for biomass-burning events in type 2 showed two peaks patterns. The first peak occurred within range of 30–50 sr corresponding to urban pollutant, and the second peak occurred within range of 60–80 sr in relation to biomass burning. Finally, our study summarized the Sp values for four major aerosol types over northern Taiwan, viz., urban (42 ± 18 sr), dust (34 ± 6 sr), biomass-burning (69 ± 12 sr), and oceanic (30 ± 12 sr). Our findings provide useful references for aerosol classification and air pollution identification over the western North Pacific.
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Bollasina, Massimo, Sumant Nigam, and K.-M. Lau. "Absorbing Aerosols and Summer Monsoon Evolution over South Asia: An Observational Portrayal." Journal of Climate 21, no. 13 (July 1, 2008): 3221–39. http://dx.doi.org/10.1175/2007jcli2094.1.
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Abstract The South Asian haze builds up from December to May, is mostly of anthropogenic origin, and absorbs part of the solar radiation. The influence of interannual variations of absorbing aerosols over the Indo-Gangetic Plain in May on the Indian summer monsoon is characterized by means of an observational analysis. Insight into how the aerosol impact is generated is also provided. It is shown that anomalous aerosol loading in late spring leads to remarkable and large-scale variations in the monsoon evolution. Excessive aerosols in May lead to reduced cloud amount and precipitation, increased surface shortwave radiation, and land surface warming. The June (and July) monsoon anomaly associated with excessive May aerosols is of opposite sign over much of the subcontinent (although with a different pattern) with respect to May. The monsoon strengthens in June (and July). The analysis suggests that the significant large-scale aerosol influence on monsoon circulation and hydroclimate is mediated by the heating of the land surface, pursuant to reduced cloudiness and precipitation in May. The finding of the significant role of the land surface in the realization of the aerosol impact is somewhat novel.
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Penning de Vries, M., S. Beirle, and T. Wagner. "UV aerosol indices from SCIAMACHY: introducing the SCattering Index (SCI)." Atmospheric Chemistry and Physics Discussions 9, no. 3 (June 19, 2009): 13569–92. http://dx.doi.org/10.5194/acpd-9-13569-2009.
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Abstract. The Absorbing Aerosol Index (AAI) is a useful tool for detecting aerosols that absorb UV radiation – especially in cases where other aerosol retrievals fail, such as over bright surfaces (e.g. desert) and in the presence of clouds. The AAI does not, however, consider contributions from "scattering" (hardly absorbing) aerosols and clouds: they cause negative AAI values and are usually discarded. In this paper, we demonstrate the use of the AAI's negative counterpart, the SCattering Index (SCI) to detect "scattering" aerosols. Maps of seasonally averaged SCI show significantly enhanced values in summer in Southeast USA and Southeast Asia, pointing to high production of "scattering" aerosols (presumably mainly sulphate aerosols and organic aerosols) in this season. The application of a cloud filter makes the presence of "scattering" aerosols even more clear. In a comparison of AOT from AERONET and our Aerosol Indices from SCIAMACHY, good agreement was found for two AERONET stations in Southeast USA, and two stations in Africa. This fact confirms the suitability of SCI as a tool to detect "scattering" aerosols. The combination of the UV Aerosol Indices AAI and SCI provides the unique possibility to characterise absorbing properties of aerosols from space. Accurate knowledge about aerosol absorption is crucial for the correct determination of the contribution of aerosols to the radiative budget.
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Kim, Maeng-Ki, William K. M. Lau, Mian Chin, Kyu-Myong Kim, Y. C. Sud, and Greg K. Walker. "Atmospheric Teleconnection over Eurasia Induced by Aerosol Radiative Forcing during Boreal Spring." Journal of Climate 19, no. 18 (September 15, 2006): 4700–4718. http://dx.doi.org/10.1175/jcli3871.1.
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Abstract The direct effects of aerosols on global and regional climate during boreal spring are investigated based on numerical simulations with the NASA Global Modeling and Assimilation Office finite-volume general circulation model (fvGCM) with Microphyics of Clouds with the Relaxed–Arakawa Schubert Scheme (McRAS), using aerosol forcing functions derived from the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The authors find that anomalous atmospheric heat sources induced by absorbing aerosols (dust and black carbon) excite a planetary-scale teleconnection pattern in sea level pressure, temperature, and geopotential height spanning North Africa through Eurasia to the North Pacific. Surface cooling due to direct effects of aerosols is found in the vicinity and downstream of the aerosol source regions, that is, South Asia, East Asia, and northern and western Africa. Significant atmospheric heating is found in regions with large loading of dust (over northern Africa and the Middle East) and black carbon (over Southeast Asia). Paradoxically, the most pronounced feature in aerosol-induced surface temperature is an east–west dipole anomaly with strong cooling over the Caspian Sea and warming over central and northeastern Asia, where aerosol concentrations are low. Analyses of circulation anomalies show that the dipole anomaly is a part of an atmospheric teleconnection pattern driven by atmospheric heating anomalies induced by absorbing aerosols in the source regions, but the influence was conveyed globally through barotropic energy dispersion and sustained by feedback processes associated with the regional circulations. The surface temperature signature associated with the aerosol-induced teleconnection bears striking resemblance to the spatial pattern of observed long-term trend in surface temperature over Eurasia. Additionally, the boreal spring wave train pattern is similar to that reported by Fukutomi et al. associated with the boreal summer precipitation seesaw between eastern and western Siberia. The results of this study raise the possibility that global aerosol forcing during boreal spring may play an important role in spawning atmospheric teleconnections that affect regional and global climates.
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Chang, Chiao-Wei, Wei-Ting Chen, and Yi-Chun Chen. "Susceptibility of East Asian Marine Warm Clouds to Aerosols in Winter and Spring from Co-Located A-Train Satellite Observations." Remote Sensing 13, no. 24 (December 20, 2021): 5179. http://dx.doi.org/10.3390/rs13245179.
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We constructed the A-Train co-located aerosol and marine warm cloud data from 2006 to 2010 winter and spring over East Asia and investigated the sensitivities of single-layer warm cloud properties to aerosols under different precipitation statuses and environmental regimes. The near-surface stability (NSS), modulated by cold air on top of a warm surface, and the estimated inversion strength (EIS) controlled by the subsidence are critical environmental parameters affecting the marine warm cloud structure over East Asia and, thus, the aerosols–cloud interactions. Based on our analysis, precipitating clouds revealed higher cloud susceptibility to aerosols as compared to non-precipitating clouds. The cloud liquid water path (LWP) increased with aerosols for precipitating clouds, yet decreased with aerosols for non-precipitating clouds, consistent with previous studies. For precipitating clouds, the cloud LWP and albedo increased more under higher NSS as unstable air promotes more moisture flux from the ocean. Under stronger EIS, the cloud albedo response to aerosols was lower than that under weaker EIS, indicating that stronger subsidence weakens the cloud susceptibility due to more entrainment drying. Our study suggests that the critical environmental factors governing the aerosol–cloud interactions may vary for different oceanic regions, depending on the thermodynamic conditions.
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Guo, Cui, Yao Zhou, Hongyan Zhou, Chang Su, and Liangliang Kong. "Aerosol Nutrients and Their Biological Influence on the Northwest Pacific Ocean (NWPO) and Its Marginal Seas." Biology 11, no. 6 (May 30, 2022): 842. http://dx.doi.org/10.3390/biology11060842.
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Atmospheric deposition is recognized as a significant source of nutrients in the surface ocean. The East Asia region is among the largest sources of aerosol emissions in the world, due to its large industrial, agricultural, and energy production. Thus, East Asian aerosols contain a large proportion of anthropogenic particles that are characterized by small size, complex composition, and high nutrient dissolution, resulting in important influences on marine microbes and biogeochemical cycles in the downwind areas of the northwest Pacific Ocean (NWPO). By using remote sensing, modeling, and incubation experimental methods, enhanced primary production due to the East Asian aerosol input has been observed in the NWPO, with subsequent promotion and inhibition impacts on different phytoplankton taxa. Changes of bacterial activity and diversity also occur in response to aerosol input. The impact of East Asian aerosol loadings is closely related to the amount and composition of the aerosol deposition as well as the hydrological condition of the receiving seawater. Here, we review the current state of knowledge on the atmospheric nutrients and the effects of the East Asian aerosols on microbes in the NWPO region. Future research perspectives are also proposed.
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Su, Hui, Jonathan H. Jiang, Xiaohong Liu, Joyce E. Penner, William G. Read, Steven Massie, Mark R. Schoeberl, Peter Colarco, Nathaniel J. Livesey, and Michelle L. Santee. "Observed Increase of TTL Temperature and Water Vapor in Polluted Clouds over Asia." Journal of Climate 24, no. 11 (June 1, 2011): 2728–36. http://dx.doi.org/10.1175/2010jcli3749.1.
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Abstract Satellite observations are analyzed to examine the correlations between aerosols and the tropical tropopause layer (TTL) temperature and water vapor. This study focuses on two regions, both of which are important pathways for the mass transport from the troposphere to the stratosphere and over which Asian pollution prevails: South and East Asia during boreal summer and the Maritime Continent during boreal winter. Using the upper-tropospheric carbon monoxide measurements from the Aura Microwave Limb Sounder as a proxy of aerosols to classify ice clouds as polluted or clean, the authors find that polluted clouds have a smaller ice effective radius and a higher temperature and specific humidity near the tropopause than clean clouds. The increase in water vapor appears to be related to the increase in temperature, as a result of increased aerosols. Meteorological differences between the clouds cannot explain the differences in temperature and water vapor for the polluted and clean clouds. The authors hypothesize that aerosol semidirect radiative heating and/or changes in cirrus radiative heating, resulting from aerosol microphysical effects on clouds, may contribute to the increased TTL temperature and thus increased water vapor in the polluted clouds.
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Proestakis, Emmanouil, Vassilis Amiridis, Eleni Marinou, Aristeidis K. Georgoulias, Stavros Solomos, Stelios Kazadzis, Julien Chimot, et al. "Nine-year spatial and temporal evolution of desert dust aerosols over South and East Asia as revealed by CALIOP." Atmospheric Chemistry and Physics 18, no. 2 (February 1, 2018): 1337–62. http://dx.doi.org/10.5194/acp-18-1337-2018.
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Abstract. We present a 3-D climatology of the desert dust distribution over South and East Asia derived using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) data. To distinguish desert dust from total aerosol load we apply a methodology developed in the framework of EARLINET (European Aerosol Research Lidar Network). The method involves the use of the particle linear depolarization ratio and updated lidar ratio values suitable for Asian dust, applied to multiyear CALIPSO observations (January 2007–December 2015). The resulting dust product provides information on the horizontal and vertical distribution of dust aerosols over South and East Asia along with the seasonal transition of dust transport pathways. Persistent high D_AOD (dust aerosol optical depth) values at 532 nm, of the order of 0.6, are present over the arid and semi-arid desert regions. Dust aerosol transport (range, height and intensity) is subject to high seasonality, with the highest values observed during spring for northern China (Taklimakan and Gobi deserts) and during summer over the Indian subcontinent (Thar Desert). Additionally, we decompose the CALIPSO AOD (aerosol optical depth) into dust and non-dust aerosol components to reveal the non-dust AOD over the highly industrialized and densely populated regions of South and East Asia, where the non-dust aerosols yield AOD values of the order of 0.5. Furthermore, the CALIPSO-based short-term AOD and D_AOD time series and trends between January 2007 and December 2015 are calculated over South and East Asia and over selected subregions. Positive trends are observed over northwest and east China and the Indian subcontinent, whereas over southeast China trends are mostly negative. The calculated AOD trends agree well with the trends derived from Aqua MODIS (Moderate Resolution Imaging Spectroradiometer), although significant differences are observed over specific regions.
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Yang, Q., C. M. Bitz, and S. J. Doherty. "Offsetting effects of aerosols on Arctic and global climate in the late 20th century." Atmospheric Chemistry and Physics 14, no. 8 (April 22, 2014): 3969–75. http://dx.doi.org/10.5194/acp-14-3969-2014.
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Abstract. We examine the impacts of atmospheric aerosols on Arctic and global climate using a series of 20th century transient simulations from Community Climate System Model version 4 (CCSM4). We focus on the response of surface air temperature to the direct radiative forcing driven by changes in sulfate and black carbon (BC) concentrations from 1975 to 2005 and we also examine the response to changes in sulfate, BC, and organic carbon (OC) aerosols collectively. The direct forcing from sulfate dominates the aerosol climate effect. Globally averaged, simultaneous changes in all three aerosols produce a cooling trend of 0.015 K decade−1 during the period 1975–2005. In the Arctic, surface air temperature has large spatial variations in response to changes in aerosol concentrations. Over the European Arctic, aerosols induce about 0.6 K decade−1 warming, which is about 1.8 K warming over the 30-year period. This warming is triggered mainly by the reduction in sulfate and BC emissions over Europe since the 1970s and is reinforced by sea ice loss and a strengthening in atmospheric northward heat transport. Changes in sulfate concentrations account for about two thirds of the warming and BC for the remaining one third. Over the Siberian and North American Arctic, surface air temperature is likely influenced by changes in aerosol concentrations over Asia. An increase in sulfate optical depth over Asia induces a large cooling while an increase in BC over Asia causes a significant warming.
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Zhou, Wei, Weiqi Xu, Hwajin Kim, Qi Zhang, Pingqing Fu, Douglas R. Worsnop, and Yele Sun. "A review of aerosol chemistry in Asia: insights from aerosol mass spectrometer measurements." Environmental Science: Processes & Impacts 22, no. 8 (2020): 1616–53. http://dx.doi.org/10.1039/d0em00212g.
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Aerosol mass spectrometer has been widely deployed in Asia for real-time characterization of aerosol chemistry, and has significantly improved our understanding of the sources, properties, and formation processes of aerosols in a complex environment.
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Kim, Ah-Hyun, Seong Soo Yum, Dong Yeong Chang, and Minsu Park. "Optimization of the sulfate aerosol hygroscopicity parameter in WRF-Chem." Geoscientific Model Development 14, no. 1 (January 15, 2021): 259–73. http://dx.doi.org/10.5194/gmd-14-259-2021.
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Abstract. A new sulfate aerosol hygroscopicity parameter (κSO4) parameterization is suggested that is capable of considering the two major sulfate aerosols, H2SO4 and (NH4)2SO4, using the molar ratio of ammonium to sulfate (R). An alternative κSO4 parameterization method is also suggested that utilizes typical geographical distribution patterns of sulfate and ammonium, which can be used when ammonium data are not available for model calculation. Using the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem), the impacts of different κSO4 parameterizations on cloud microphysical properties and cloud radiative effects in East Asia are examined. Comparisons with the observational data obtained from an aircraft field campaign suggest that the new κSO4 parameterizations simulate more reliable aerosol and cloud condensation nuclei concentrations, especially over the sea in East Asia, than the original κSO4 parameterization in WRF-Chem that assumes sulfate aerosols as (NH4)2SO4 only. With the new κSO4 parameterizations, the simulated cloud microphysical properties and precipitation became significantly different, resulting in a greater cloud albedo effect of about −1.5 W m−2 in East Asia than that with the original κSO4 parameterization. The new κSO4 parameterizations are simple and readily applicable to numerical studies investigating the impact of sulfate aerosols in aerosol–cloud interactions without additional computational expense.
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Shin, Sung-Kyun, Matthias Tesche, Youngmin Noh, and Detlef Müller. "Aerosol-type classification based on AERONET version 3 inversion products." Atmospheric Measurement Techniques 12, no. 7 (July 11, 2019): 3789–803. http://dx.doi.org/10.5194/amt-12-3789-2019.
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Abstract. This study proposes an aerosol-type classification based on the particle linear depolarization ratio (PLDR) and single-scattering albedo (SSA) provided in the AErosol RObotic NETwork (AERONET) version 3 level 2.0 inversion product. We compare our aerosol-type classification with an earlier method that uses fine-mode fraction (FMF) and SSA. Our new method allows for a refined classification of mineral dust that occurs as a mixture with other absorbing aerosols: pure dust (PD), dust-dominated mixed plume (DDM), and pollutant-dominated mixed plume (PDM). We test the aerosol classification at AERONET sites in East Asia that are frequently affected by mixtures of Asian dust and biomass-burning smoke or anthropogenic pollution. We find that East Asia is strongly affected by pollution particles with high occurrence frequencies of 50 % to 67 %. The distribution and types of pollution particles vary with location and season. The frequency of PD and dusty aerosol mixture (DDM+PDM) is slightly lower (34 % to 49 %) than pollution-dominated mixtures. Pure dust particles have been detected in only 1 % of observations. This suggests that East Asian dust plumes generally exist in a mixture with pollution aerosols rather than in pure form. In this study, we have also considered data from selected AERONET sites that are representative of anthropogenic pollution, biomass-burning smoke, and mineral dust. We find that average aerosol properties obtained for aerosol types in our PLDR–SSA-based classification agree reasonably well with those obtained at AERONET sites representative for different aerosol types.
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Liu, Xiaodong, Libin Yan, Ping Yang, Zhi-Yong Yin, and Gerald R. North. "Influence of Indian Summer Monsoon on Aerosol Loading in East Asia." Journal of Applied Meteorology and Climatology 50, no. 3 (March 1, 2011): 523–33. http://dx.doi.org/10.1175/2010jamc2414.1.
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Abstract The spatial and temporal variations of aerosol loading over eastern Asia specified in terms of the aerosol optical depth (AOD) at the 550-nm wavelength during July are examined in conjunction with the intensity of the Indian summer monsoon. AOD derived from Moderate Resolution Imaging Spectroradiometer (MODIS) observations, gridded reanalyses, and ground-based measurements are used in the analysis. Two contrasting years, 2002 and 2003, which represent weak and active Indian summer monsoon events, respectively, are selected for the study, with a focus on an eastern Asian southern subregion (SR; 23°–32°N, 105°–120°E) and an eastern Asian northern subregion (NR; 35°–44°N, 115°–130°E). It is shown that the interannual variation of July mean wind intensity is a major factor in regulating the midsummer spatial pattern of aerosols over eastern Asia when the Indian monsoon index is anomalously large. The AOD anomalies in the NR and SR are positive and negative, respectively, during an active monsoon year, whereas the opposite is observed during a weak monsoon year. The variation patterns of less cloudy-day visibility, observed at four meteorological stations in the SR and NR subregions, also show spatial–temporal aerosol variability evident in the MODIS AOD data. Relative to the case of a weak monsoon year, meridional winds and convection are stronger and more clouds and precipitation are observed in the NR subregion during the active monsoon year. The opposite pattern is observed in the SR subregion. The spatial–temporal variation pattern of aerosols over eastern Asia illustrates the nonnegligible role of transport and dispersal mechanisms associated with the Indian summer monsoon in the region.
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Lee, K. H., and Y. J. Kim. "Satellite remote sensing of Asian aerosols: a case study of clean, polluted, and Asian dust storm days." Atmospheric Measurement Techniques 3, no. 6 (December 20, 2010): 1771–84. http://dx.doi.org/10.5194/amt-3-1771-2010.
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Abstract. In East Asia, satellite observation is important because aerosols from natural and anthropogenic sources have been recognized as a major source of regional and global air pollution. However, retrieving aerosols properties from satellite observations over land can be difficult because of the surface reflection, complex aerosol composition, and aerosol absorption. In this study, a new aerosol retrieval method called as the Moderate Resolution Imaging Spectroradiometer (MODIS) satellite aerosol retrieval (MSTAR) was developed and applied to three different aerosol event cases over East Asia. MSTAR uses a separation technique that can distinguish aerosol reflectance from top-of-atmosphere (TOA) reflectance. The aerosol optical thickness (AOT) was determined by comparing this aerosol reflectance with pre-calculated values. Three case studies show how the methodology identifies discrepancies between measured and calculated values to retrieve more accurate AOT. The comparison between MODIS and the Aerosol Robotic Network (AERONET) showed improvement using the suggested methodology with the cluster-based look-up-tables (LUTs) (linear slope = 0.94, R = 0.92) than using operational MODIS collection 5 aerosol products (linear slope = 0.78, R = 0.87). In conclusion, the suggested methodology is shown to work well with aerosol models acquired by statistical clustering of the observation data in East Asia.
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Kunwar, Bhagawati, and Kimitaka Kawamura. "Seasonal distributions and sources of low molecular weight dicarboxylic acids, ω-oxocarboxylic acids, pyruvic acid, α-dicarbonyls and fatty acids in ambient aerosols from subtropical Okinawa in the western Pacific Rim." Environmental Chemistry 11, no. 6 (2014): 673. http://dx.doi.org/10.1071/en14097.
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Environmental context Water-soluble dicarboxylic acids and related compounds are ubiquitous in atmospheric aerosols. They are abundantly emitted from Asian countries and transported to the Pacific Ocean. During the long-range transport, photochemical processing modifies organic aerosols. We conducted a 1-year observation of diacids and related compounds at Okinawa Island, an outflow region of the Asian Continent, to clarify their sources and photochemical aging. Abstract Ambient aerosol samples were collected for 1 year at Okinawa Island, Japan, and were analysed for water-soluble dicarboxylic acids, oxoacids, α-dicarbonyls and fatty acids to better understand biogenic v. anthropogenic sources and the formation–transformation of organic aerosols during long-range atmospheric transport. Here, we report seasonal variations of diacids and related compounds in Okinawa. We found a predominance of oxalic acid (C2) followed by malonic (C3) and succinic (C4) acid. Total diacids and oxoacids maximised in spring when air masses originated from the Asian Continent with westerly winds. In contrast, phthalic acid (Ph), a tracer of anthropogenic sources, peaked in winter. We found an increased C3/C4 ratio in summer, suggesting an enhanced photochemical aging of organic aerosols. The average ratio of total diacid-C/total carbon (TC) (5.4%) is higher than that (3.1%) from the East China Sea, suggesting that Okinawa aerosols are more aged than East Asian aerosols but less aged compared to those from the remote Pacific including tropics (8.8%). Biogenic short-chain fatty acids and azelaic acid (C9), the latter is a specific oxidation product of unsaturated fatty acids, maximised in summer, whereas higher plant-derived long-chain fatty acids maximised in spring. This study demonstrates that the ambient aerosols in Okinawa are strongly influenced by the Asian outflow in winter and spring and by biogenic organic matter in summer and spring. Enhanced contribution of oxalic acid to aerosol TC in spring suggests that Okinawa organic aerosols are mainly produced in East Asia and photochemically transformed during the transport.
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Zhai, Shixian, Daniel J. Jacob, Jared F. Brewer, Ke Li, Jonathan M. Moch, Jhoon Kim, Seoyoung Lee, et al. "Relating geostationary satellite measurements of aerosol optical depth (AOD) over East Asia to fine particulate matter (PM<sub>2.5</sub>): insights from the KORUS-AQ aircraft campaign and GEOS-Chem model simulations." Atmospheric Chemistry and Physics 21, no. 22 (November 18, 2021): 16775–91. http://dx.doi.org/10.5194/acp-21-16775-2021.
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Abstract. Geostationary satellite measurements of aerosol optical depth (AOD) over East Asia from the Geostationary Ocean Color Imager (GOCI) and Advanced Himawari Imager (AHI) instruments can augment surface monitoring of fine particulate matter (PM2.5) air quality, but this requires better understanding of the AOD–PM2.5 relationship. Here we use the GEOS-Chem chemical transport model to analyze the critical variables determining the AOD–PM2.5 relationship over East Asia by simulation of observations from satellite, aircraft, and ground-based datasets. This includes the detailed vertical aerosol profiling over South Korea from the KORUS-AQ aircraft campaign (May–June 2016) with concurrent ground-based PM2.5 composition, PM10, and AERONET AOD measurements. The KORUS-AQ data show that 550 nm AOD is mainly contributed by sulfate–nitrate–ammonium (SNA) and organic aerosols in the planetary boundary layer (PBL), despite large dust concentrations in the free troposphere, reflecting the optically effective size and high hygroscopicity of the PBL aerosols. We updated SNA and organic aerosol size distributions in GEOS-Chem to represent aerosol optical properties over East Asia by using in situ measurements of particle size distributions from KORUS-AQ. We find that SNA and organic aerosols over East Asia have larger size (number median radius of 0.11 µm with geometric standard deviation of 1.4) and 20 % larger mass extinction efficiency as compared to aerosols over North America (default setting in GEOS-Chem). Although GEOS-Chem is successful in reproducing the KORUS-AQ vertical profiles of aerosol mass, its ability to link AOD to PM2.5 is limited by under-accounting of coarse PM and by a large overestimate of nighttime PM2.5 nitrate. The GOCI–AHI AOD data over East Asia in different seasons show agreement with AERONET AODs and a spatial distribution consistent with surface PM2.5 network data. The AOD observations over North China show a summer maximum and winter minimum, opposite in phase to surface PM2.5. This is due to low PBL depths compounded by high residential coal emissions in winter and high relative humidity (RH) in summer. Seasonality of AOD and PM2.5 over South Korea is much weaker, reflecting weaker variation in PBL depth and lack of residential coal emissions.
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Nair, Vijayakumar Sivadasan, Filippo Giorgi, and Usha Keshav Hasyagar. "Amplification of South Asian haze by water vapour–aerosol interactions." Atmospheric Chemistry and Physics 20, no. 22 (November 28, 2020): 14457–71. http://dx.doi.org/10.5194/acp-20-14457-2020.
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Abstract. Air pollution and wintertime fog over South Asia is a major concern due to its significant implications for air quality, visibility and health. Using a regional climate model coupled with chemistry, we assess the contribution of the hygroscopic growth of aerosols (ambient–dry) to the total aerosol optical depth and demonstrate that the increased surface cooling due to the hygroscopic effects of aerosols further increases the humidity in the boundary layer and thus enhances the confinement of pollutants through aerosol–boundary layer interactions. This positive feedback mechanism plays an important role in the prevalence of wintertime fog and poor air quality conditions over South Asia, where water vapour contributes more than half of the aerosol optical depth. The aerosol–boundary layer interactions lead to moistening of the boundary layer and drying of the free troposphere, which amplifies the long-term trend in relative humidity over the Indo-Gangetic Plain during winter. Hence, the aerosol–water vapour interaction plays a decisive role in the formation and maintenance of the wintertime fog conditions over South Asia, which needs to be considered for planning mitigation strategies.
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Lee, Hsiang-He, Rotem Z. Bar-Or, and Chien Wang. "Biomass burning aerosols and the low-visibility events in Southeast Asia." Atmospheric Chemistry and Physics 17, no. 2 (January 23, 2017): 965–80. http://dx.doi.org/10.5194/acp-17-965-2017.
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Abstract. Fires including peatland burning in Southeast Asia have become a major concern to the general public as well as governments in the region. This is because aerosols emitted from such fires can cause persistent haze events under certain weather conditions in downwind locations, degrading visibility and causing human health issues. In order to improve our understanding of the spatiotemporal coverage and influence of biomass burning aerosols in Southeast Asia, we have used surface visibility and particulate matter concentration observations, supplemented by decade-long (2003 to 2014) simulations using the Weather Research and Forecasting (WRF) model with a fire aerosol module, driven by high-resolution biomass burning emission inventories. We find that in the past decade, fire aerosols are responsible for nearly all events with very low visibility (< 7 km). Fire aerosols alone are also responsible for a substantial fraction of low-visibility events (visibility < 10 km) in the major metropolitan areas of Southeast Asia: up to 39 % in Bangkok, 36 % in Kuala Lumpur, and 34 % in Singapore. Biomass burning in mainland Southeast Asia accounts for the largest contribution to total fire-produced PM2.5 in Bangkok (99 %), while biomass burning in Sumatra is a major contributor to fire-produced PM2.5 in Kuala Lumpur (50 %) and Singapore (41 %). To examine the general situation across the region, we have further defined and derived a new integrated metric for 50 cities of the Association of Southeast Asian Nations (ASEAN): the haze exposure day (HED), which measures the annual exposure days of these cities to low visibility (< 10 km) caused by particulate matter pollution. It is shown that HEDs have increased steadily in the past decade across cities with both high and low populations. Fire events alone are found to be responsible for up to about half of the total HEDs. Our results suggest that in order to improve the overall air quality in Southeast Asia, mitigation policies targeting both biomass burning and fossil fuel burning sources need to be implemented.
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Jung, J., Y. J. Kim, K. Y. Lee, M. G. -Cayetano, T. Batmunkh, J. H. Koo, and J. Kim. "Spectral optical properties of long-range transport Asian dust and pollution aerosols over Northeast Asia in 2007 and 2008." Atmospheric Chemistry and Physics Discussions 10, no. 2 (February 1, 2010): 2397–444. http://dx.doi.org/10.5194/acpd-10-2397-2010.
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Abstract. As a part of the IGAC (International Global Atmospheric Chemistry) Mega-cities program, aerosol physical and optical properties were continuously measured from March 2007 to March 2008 at an urban site (37.57° N, 126.94° E) in Seoul, Korea. Spectral optical properties of long-range transported Asian dust and pollution aerosols have been investigated based on the year long measurement data. Optically measured black carbon/thermally measured elemental carbon (BC/EC) ratio showed clear monthly variation with high values in summer and low values in winter mainly due to the enhancement of light attenuation by the internal mixing of EC. Novel approach has been suggested to retrieve the spectral light absorption coefficient (babs) from Aethalometer raw data by using BC/EC ratio. Mass absorption efficiency, σabs(=babs/EC) at 550 nm at the measurement site was determined to be 9.0±1.3, 8.9±1.5, 9.5±2.0, and 10.3±1.7 m2 g−1 in spring, summer, fall, and winter, respectively with an annual mean of 9.4±1.8 m2 g−1. Threshold values to classify severe haze events were suggested in this study. Increasing trend of aerosol single scattering albedo (SSA) with wavelength was observed during Asian dust events while little spectral dependence of SSA was observed during long-range transport pollution (LTP) events. Satellite aerosol optical thickness (AOT) and Hysplit air mass backward trajectory analyses as well as chemical analysis were performed to characterize the dependence of spectral optical properties on aerosol type. Results from this study can provide useful information for studies on regional air quality and aerosol's effects on climate change.
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Jung, J., Y. J. Kim, K. Y. Lee, M. G. -Cayetano, T. Batmunkh, J. H. Koo, and J. Kim. "Spectral optical properties of long-range transport Asian dust and pollution aerosols over Northeast Asia in 2007 and 2008." Atmospheric Chemistry and Physics 10, no. 12 (June 21, 2010): 5391–408. http://dx.doi.org/10.5194/acp-10-5391-2010.
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Abstract. As a part of the IGAC (International Global Atmospheric Chemistry) Mega-cities program, aerosol physical and optical properties were continuously measured from March 2007 to March 2008 at an urban site (37.57° N, 126.94° E) in Seoul, Korea. Spectral optical properties of long-range transported Asian dust and pollution aerosols have been investigated based on the year long measurement data. Optically measured black carbon/thermally measured elemental carbon (BC/EC) ratio showed clear monthly variation with high values in summer and low values in winter mainly due to the enhancement of light attenuation by the internal mixing of EC. Novel approach has been suggested to retrieve the spectral light absorption coefficient (babs) from Aethalometer raw data by using BC/EC ratio. Mass absorption efficiency, σabs (=babs/EC) at 550 nm was determined to be 9.0±1.3, 8.9±1.5, 9.5±2.0, and 10.3±1.7 m2 g−1 in spring, summer, fall, and winter, respectively with an annual mean of 9.4±1.8 m2 g−1. Threshold values to classify severe haze events were suggested in this study. Increasing trend of aerosol single scattering albedo (SSA) with wavelength was observed during Asian dust events while little spectral dependence of SSA was observed during long-range transport pollution (LTP) events. Satellite aerosol optical thickness (AOT) and Hysplit air mass backward trajectory analyses as well as chemical analysis were performed to characterize the dependence of spectral optical properties on aerosol type. Results from this study can provide useful information for studies on regional air quality and aerosol's effects on climate change.
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Wu, Na, Yongxiao Ge, Jilili Abuduwaili, Gulnura Issanova, and Galymzhan Saparov. "Insights into Variations and Potential Long-Range Transport of Atmospheric Aerosols from the Aral Sea Basin in Central Asia." Remote Sensing 14, no. 13 (July 3, 2022): 3201. http://dx.doi.org/10.3390/rs14133201.
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The dramatic shrinkage of the Aral Sea in the past decades has inevitably led to an environmental calamity. Existing knowledge on the variations and potential transport of atmospheric aerosols from the Aral Sea Basin (ASB) is limited. To bridge this knowledge gap, this study tried to identify the variations and long-range transport of atmospheric aerosols from the ASB in recent years. The Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model and Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) data were used to gain new insight into the types, variation and long-range transport of atmospheric aerosols from the ASB. The results showed five types of tropospheric aerosols and one type of stratospheric aerosol were observed over the ASB. Polluted dust and dust were the dominant subtypes through the year. Sulfate/other was the only stratospheric aerosol detected. The occurrence frequency of aerosols over the ASB showed obvious seasonal variation. Maximum occurrence frequency of dust appeared in spring (MAM) and that of polluted dust peaked in summer (JJA). The monthly occurrence frequency of dust and polluted dust exhibited unimodal distribution. Polluted dust and dust were distributed over wide ranges from 1 km to 5 km vertically. The multi-year average thickness of polluted dust and dust layers was around 1.3 km. Their potential long-range transport in different directions mainly impacts Uzbekistan, Turkmenistan, Kazakhstan and eastern Iran, and may reach as far as the Caucasus region, part of China, Mongolia and Russia. Combining aerosol lidar, atmospheric climate models and geochemical methods is strongly suggested to gain clarity on the variations and long-range transport of atmospheric aerosols from the Aral Sea Basin.
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Pan, X., M. Chin, R. Gautam, H. Bian, D. Kim, P. R. Colarco, T. L. Diehl, et al. "A multi-model evaluation of aerosols over South Asia: Common problems and possible causes." Atmospheric Chemistry and Physics Discussions 14, no. 13 (July 22, 2014): 19095–147. http://dx.doi.org/10.5194/acpd-14-19095-2014.
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Abstract. Atmospheric pollution over South Asia attracts special attention due to its effects on regional climate, the water cycle, and human health. These effects are potentially growing owing to rising trends of anthropogenic aerosol emissions found there. In this study, the spatio-temporal aerosol distributions over South Asia from 7 global models, for the period of 2000–2007, are evaluated systematically against aerosol retrievals of NASA satellite sensors and ground-based measurements. Overall, substantial underestimations of aerosol loading over South Asia are found systematically in 6 out of 7 models. Averaged over the entire South Asia, the annual mean Aerosol Optical Depth (AOD) is underestimated by a range of 18–45 % across models compared to MISR, which is the lowest bound among various satellite AOD retrievals (from MISR, SeaWiFS, MODIS Aqua and Terra). In particular at Kanpur located in northern India, AOD is underestimated even more by a factor of 4, and annual mean Aerosol Absorption Optical Depth (AAOD) is underestimated by about a factor of 2 in comparison with AERONET, during the post-monsoon and the wintertime periods (i.e. October–January) when agricultural waste burning and anthropogenic emissions dominate. The largest model underestimation of aerosol loading occurs in the lowest boundary layer (from surface to 2 km) based on the comparisons with aerosol extinction vertical distribution from CALIPSO. The possible causes for the common problems of model aerosol underestimation over south Asia are identified here, which are suggested as the following. During the winter, not only the columnar aerosol loading in models, but also surface concentrations of all aerosol components (sulfate, nitrate, organic aerosol and black carbon) are found lower than observations (ISRO-GBP, ICARB and CALIPSO), indicating that anthropogenic emissions, especially biofuel, are likely underestimated in this season. Nitrate, a major component of aerosols in South Asia, is either not considered in 4 out of 7 models or significantly lower than observations in other 2 models. Surprisingly, the near-surface relative humidity in these models is found significantly lower than observations in the winter, resulting in suppression of the hygroscopic growth of soluble aerosols and formations of sulfate and nitrate, and thereby underestimation of AOD. During the post-monsoon season, the deficiency of agricultural waste burning emissions in GFED2 biomass burning emission inventory, used by the models, partly contributes to the model underestimation of aerosol loading over South Asia in burning seasons.