Thematische Bibliographien / Anode Li

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Auswahl der wissenschaftlichen Literatur zum Thema „Anode Li“

Autor: Grafiati

Veröffentlicht am 25. Mai 2024

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Zeitschriftenartikel zum Thema "Anode Li"

Su, Yu-Sheng, Kuang-Che Hsiao, Pedaballi Sireesha und Jen-Yen Huang. „Lithium Silicates in Anode Materials for Li-Ion and Li Metal Batteries“. Batteries 8, Nr. 1 (04.01.2022): 2. http://dx.doi.org/10.3390/batteries8010002.

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The structural and interfacial stability of silicon-based and lithium metal anode materials is essential to their battery performance. Scientists are looking for a better inactive material to buffer strong volume change and suppress unwanted surface reactions of these anodes during cycling. Lithium silicates formed in situ during the formation cycle of silicon monoxide anode not only manage anode swelling but also avoid undesired interfacial interactions, contributing to the successful commercialization of silicon monoxide anode materials. Additionally, lithium silicates have been further utilized in the design of advanced silicon and lithium metal anodes, and the results have shown significant promise in the past few years. In this review article, we summarize the structures, electrochemical properties, and formation conditions of lithium silicates. Their applications in advanced silicon and lithium metal anode materials are also introduced.

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Yang, Chunpeng, Lei Zhang, Boyang Liu, Shaomao Xu, Tanner Hamann, Dennis McOwen, Jiaqi Dai et al. „Continuous plating/stripping behavior of solid-state lithium metal anode in a 3D ion-conductive framework“. Proceedings of the National Academy of Sciences 115, Nr. 15 (26.03.2018): 3770–75. http://dx.doi.org/10.1073/pnas.1719758115.

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The increasing demands for efficient and clean energy-storage systems have spurred the development of Li metal batteries, which possess attractively high energy densities. For practical application of Li metal batteries, it is vital to resolve the intrinsic problems of Li metal anodes, i.e., the formation of Li dendrites, interfacial instability, and huge volume changes during cycling. Utilization of solid-state electrolytes for Li metal anodes is a promising approach to address those issues. In this study, we use a 3D garnet-type ion-conductive framework as a host for the Li metal anode and study the plating and stripping behaviors of the Li metal anode within the solid ion-conductive host. We show that with a solid-state ion-conductive framework and a planar current collector at the bottom, Li is plated from the bottom and rises during deposition, away from the separator layer and free from electrolyte penetration and short circuit. Owing to the solid-state deposition property, Li grows smoothly in the pores of the garnet host without forming Li dendrites. The dendrite-free deposition and continuous rise/fall of Li metal during plating/stripping in the 3D ion-conductive host promise a safe and durable Li metal anode. The solid-state Li anode shows stable cycling at 0.5 mA cm−2 for 300 h with a small overpotential, showing a significant improvement compared with reported Li anodes with ceramic electrolytes. By fundamentally eliminating the dendrite issue, the solid Li metal anode shows a great potential to build safe and reliable Li metal batteries.

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Park, Se Hwan, Dayoung Jun, Gyu Hyeon Lee, Seong Gyu Lee, Ji Eun Jung und Yun Jung Lee. „Designing the 3D Porous Anode Based on Pore Size Dependent Li Deposition Behavior for Reversible Li Metal-Free Solid-State-Batteries“. ECS Meeting Abstracts MA2022-02, Nr. 4 (09.10.2022): 470. http://dx.doi.org/10.1149/ma2022-024470mtgabs.

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Li metal-based all-solid-state batteries (ASSBs) can potentially combine the high energy of Li metal anodes and the safety of ASSBs. Among Li metal-based ASSBs, lithium-free or anodeless ASSBs are considered optimal battery configurations because of their higher energy density and economic advantages attributed to the absence of Li metal during the battery assembly process. Despite the extensive interest in Li-free ASSBs, they continue to suffer from low Coulombic efficiency and poor cycle performance. One reason for this inferior performance is the unstable interface between the current collector and solid electrolyte (SE), which can eventually lead to inhomogeneous Li deposition, dendritic Li growth, and internal short circuits. Various approaches including 3D porous anodes have been proposed to control the Li deposition behavior and improve the reversibility of anodeless ASSBs; however, there is no clarity on the mechanism and conditions for determining the Li deposition behavior in this emerging system. In this study, we systematically investigate the Li deposition behavior depending on the pore size of 3D anode and successfully demonstrate the strategy to obtain a highly reversible 3D porous anode for Li-free ASSBs. We found that more Li deposits could be accommodated within the pores of the anode with a smaller pore size using stacked Ni particles as the Li-hosting porous anode; this implies that the Li movement into the anode occurs via diffusional Coble creep. We proposed the modification of the Ni surface with carbon coating and Ag nanoparticle decoration (Ni_C_Ag particles) to further improve the Li storage capacity of the Ni-based 3D anode and, thereby, secure the interfacial contact between the 3D Ni anode and SE. The resulting Ni_C_Ag 3D anode successfully accommodated the entire Li deposit of 2 mAh cm−2 within the porous architecture without the separation of the anode/SE interface. We clarified the improved Li storage capacity of the Ni_C_Ag anode as follows. (1) C and especially Ag electrochemically react with Li ions above 0 V; thus, Li ions can be transported to 3D Ni_C_Ag porous anode before Li deposition at the SE/anode interface at < 0 V. Further, the high Li ion diffusion coefficient of lithiated carbon and Li-Ag alloy can further reduce Li ions within the pores of the 3D anode; therefore, Li deposition can occur within the porous 3D Ni anode. (2) Lithiophilic C and Ag facilitated the movement of Li via diffusional Coble creep. In particular, Ag with solid solubility in Li (Li(Ag)) can significantly enhance Li adatom mobility because of the identical structure of Li(Ag) with pure Li. (3) Li(Ag) is widely known to lower the energy barrier for Li nucleation. With the significantly reduced nucleation overpotential and interfacial resistance, the Ni_C_Ag anode showed high reversibility in Li deposition and stripping. The Ni_C_Ag anode could be cycled for more than 60 and 100 cycles with Li3PS4 and Li6PS5Cl0.5Br0.5 SE in half cells with a capacity limit of 2 mAh cm−2 and a current density of 0.5 mA cm− 2maintaining the CE of 97.9% and 96.9 %, respectively. Further, the synergistic effects of the stable anode/SE interface and reduced nucleation energy barrier enable stable NCM full-cell cycling at a room temperature of 30 °C. The NCM811 cathode/Ni_C_Ag anode full cell in the Li-free configuration showed an initial areal discharge capacity of 2 mAh cm−2, and it operated stably with a CE of 99.47% for 100 cycles. Figure 1

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Bao, Wurigumula, und Ying Shirley Meng. „(Invited) Development and Application of Titration Gas Chromatography in Elucidating the Behavior of Anode in Lithium Batteries“. ECS Meeting Abstracts MA2023-01, Nr. 2 (28.08.2023): 633. http://dx.doi.org/10.1149/ma2023-012633mtgabs.

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The accelerated transition to renewable energy systems worldwide has triggered increasing interest in energy storage technologies, especially in lithium batteries. Accurate diagnosis and understanding of the batteries degradation mechanism are essential. Titration Gas Chromatography (TGC) has been developed to quantitively understand the anode. The inactive Li in the cycled anode can be categorized into two kinds: 1) trapped Li0 (such as trapped lithiated graphite (LixC6), Li0, and lithium silicon alloy (LixSi)) and 2) solid electrolyte interphase (SEI) Li+. Noted that only trapped Li0 can react with the protic solvent to generate the hydrogen (H2), while SEI (Li+) does not1. Therefore, the H2 gas quantification can be correlated to the trapped Li0 as the foundation mechanism of TGC. With the optimal solvent selection, we successfully applied TGC to investigated: 1) the degradation behavior of Si-based anode materials2, 3; 2) corrosion effects on electrochemically deposited Li metal anode4; 3) the cycling behavior of Gr anode; 4) Li inventory quantification in practical Li metal battery5. We demonstrate the various application of TGC techniques in quantitatively examining the Li inventory changes of the anode. Beyond that, the results can provide unique insights into identifying the critical bottlenecks that facilitate battery performance development. References: Fang, C.; Li, J.; Zhang, M.; Zhang, Y.; Yang, F.; Lee, J. Z.; Lee, M. H.; Alvarado, J.; Schroeder, M. A.; Yang, Y.; Lu, B.; Williams, N.; Ceja, M.; Yang, L.; Cai, M.; Gu, J.; Xu, K.; Wang, X.; Meng, Y. S., Quantifying inactive lithium in lithium metal batteries. Nature 2019, 572 (7770), 511-515. Bao, W.; Fang, C.; Cheng, D.; Zhang, Y.; Lu, B.; Tan, D. H.; Shimizu, R.; Sreenarayanan, B.; Bai, S.; Li, W., Quantifying lithium loss in amorphous silicon thin-film anodes via titration-gas chromatography. Cell Reports Physical Science 2021, 2 (10), 100597. Sreenarayanan, B.; Tan, D. H.; Bai, S.; Li, W.; Bao, W.; Meng, Y. S., Quantification of lithium inventory loss in micro silicon anode via titration-gas chromatography. Journal of Power Sources 2022, 531, 231327. Lu, B.; Li, W.; Cheng, D.; Bhamwala, B.; Ceja, M.; Bao, W.; Fang, C.; Meng, Y. S., Suppressing chemical corrosions of lithium metal anodes. Advanced Energy Materials 2022, 2202012. Deng, W.; Yin, X.; Bao, W.; Zhou, X.; Hu, Z.; He, B.; Qiu, B.; Meng, Y. S.; Liu, Z., Quantification of reversible and irreversible lithium in practical lithium-metal batteries. Nature Energy 2022, 7 (11), 1031-1041.

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Wang, Hansen, Yayuan Liu, Yuzhang Li und Yi Cui. „Lithium Metal Anode Materials Design: Interphase and Host“. Electrochemical Energy Reviews 2, Nr. 4 (12.10.2019): 509–17. http://dx.doi.org/10.1007/s41918-019-00054-2.

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Abstract Li metal is the ultimate anode choice due to its highest theoretical capacity and lowest electrode potential, but it is far from practical applications with its poor cycle lifetime. Recent research progresses show that materials designs of interphase and host structures for Li metal are two effective ways addressing the key issues of Li metal anodes. Despite the exciting improvement on Li metal cycling capability, problems still exist with these methodologies, such as the deficient long-time cycling stability of interphase materials and the accelerated Li corrosion for high surface area three-dimensional composite Li anodes. As a result, Coulombic efficiency of Li metal is still not sufficient for full-cell cycling. In the near future, an interphase protected three-dimensional composite Li metal anode, combined with high performance novel electrolytes might be the ultimate solution. Besides, nanoscale characterization technologies are also vital for guiding future Li metal anode designs. Graphic Abstract

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Gabrisch, H., R. Yazami und B. Fultz. „Lattice defects in LiCoO2“. Microscopy and Microanalysis 7, S2 (August 2001): 518–19. http://dx.doi.org/10.1017/s143192760002866x.

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Rechargeable Lithium ion batteries are widely used as portable power source in communication and computer technology, prospective uses include medical implantable devices and electric vehicles. The safety and cycle life of Li ion batteries is improved over that of batteries containing metallic lithium anodes because the insertion of Li between the crystal layers of both electrodes was proved to be safer than the electroplating of Li onto a metallic Lithium anode. in Li-ion batteries, the charge transport is governed by the oscillation of Li ions between anode and cathode. They are sometimes called “rocking-chair“ batteries. The most common materials for these batteries are lithiated carbons for anodes, and transition metal oxides (LixCoO2) as cathodes.LixCoO2 has an ordered rhombohedral Rm structure consisting of alternating layers of Co-O-Li-O-Co. The capacity and energy density of the batteries is limited by the amount of Li that can be stored in the anode and cathode materials.

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Fluegel, Marius, Karsten Richter, Margret Wohlfahrt-Mehrens und Thomas Waldmann. „Detection of Li Deposition on Si/Graphite Anodes from Commercial Li-Ion Cells - a Post-Mortem GD-OES Depth Profiling Study“. ECS Meeting Abstracts MA2022-02, Nr. 3 (09.10.2022): 239. http://dx.doi.org/10.1149/ma2022-023239mtgabs.

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A new semi-quantitative method based on Post-Mortem glow discharge optical emission spectroscopy (GD-OES) depth profiling was developed to detect Li deposition on Si/graphite anodes. By means of the detected amounts of Li, Si and O in the GD-OES depth profiles, a corridor is determined, in which the minimum amount of Li deposition is found. Three different commercially available 18650 cell types containing Si/graphite as anode active material were acquired to evaluate the newly developed method. Those three cell types were initially characterized in detail by means of SEM/EDX, GD-OES, ICP-OES, and Hg porosimetry regarding their cell chemistry and electrode properties. One cell type was a high-power cell due to its high anode porosity and low anode coating thickness. The other two cell types were high-energy cells, which have thick anode coatings and low porosities. We aged the cells at 45 °C until their SOH was 80% and analysed the aging behaviour using SEM, DVA, GD-OES, and in coin half-cells. GD-OES depth profiling revealed that no Li plating occurs during cycling aging at 45 °C. Contrary to this, Li plating was detected on the anodes of all three cell types by the new GD-OES method after the high-power cell was aged at -20 °C and the high-energy cells were aged to 0 °C. Cells, which were previously aged at 45 °C until 80% SOH have afterwards been cycled under the same conditions, which led to Li plating in the fresh cells. Cell types exhibiting predominantly loss of anode active material (LAAM) as aging mechanism during the first aging at 45 °C, still suffered from Li plating during the second aging. However, if the main aging mechanism during the initial aging was loss of cyclable Li inventory (LLI), the cells did show a significantly reduced tendency for Li plating, even though the same conditions caused Li plating in the fresh cells. Analysis of the aged anodes using coin half-cells revealed that the loss of anode material was caused by the deactivation of Si anode material. SEM images of the anode cross-section indicate that the deactivation is most likely mainly induced by the formation of a thick film surrounding the Si particles. In combination with complementary methods like SEM, ICP-OES, and coin half-cell analysis, the newly developed GD-OES method yields in profound understanding of the aging behaviour of state-of-the-art Li-ion cells contain Si/graphite anodes. Figure 1

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Dasgupta, Neil P. „(Invited) Interfacial Dynamics of Anode-Free Solid-State Batteries“. ECS Meeting Abstracts MA2022-02, Nr. 4 (09.10.2022): 482. http://dx.doi.org/10.1149/ma2022-024482mtgabs.

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There is significant interest in solid-state batteries (SSBs) as an alternative to traditional Li-ion batteries, as they can potentially eliminate the flammable liquid electrolyte and enable Li-metal anodes. However, manufacturing of SSBs with Li metal anodes poses a significant challenge, owing to the highly reactive nature of Li metal. Therefore, there has been a recent increase in interest in “anode-free” configurations, where the Li metal anode is formed in situ using the pre-existing inventory in the cathode. In addition to manufacturing considerations, anode-free configurations also enhance energy density compared to batteries with excess Li metal in the anode. However, compared to pre-formed Li metal/solid electrolyte interfaces, the nucleation, growth, and stripping of Li metal in anode-free SSBs has not been widely studied, and poses unique electro-chemo-mechanical phenomena. To probe the dynamic interfacial evolution of anode-free SSBs, in this study, I will present results using a complimentary set of in situ/operando methodologies. First, I will describe the morphological evolution of Li nucleation and growth at garnet LLZO solid electrolytes, using a newly developed platform for operando 3-D video microscopy [1]. In particular, the influence of mechanical stresses on both the thermodynamic and kinetic properties of Li will be discussed, and unique electrochemical signatures of anode-free plating will described. A mechanistic framework for these electro-chemo-mechanics will be presented, which results in design rules for improving the homogeneity of Li plating during anode formation. To compliment this morphological information, I will also present results using operando x-ray photoelectron spectroscopy (XPS) on sulfide solid electrolytes. This allows for direct observation of SEI formation during in situ anode formation. In particular, we observe a transition in reaction pathways from SEI formation to nucleation of Li metal, which is a function of both the charging protocol and the presence of interlayer coatings [2-3]. Finally, these results will be compared and contrasted to anode-free Li plating in liquid electrolytes, and a discussion will be presented on how to optimize plating morphology and reversibility. [1] E. Kazyak, M. Wang, K. Lee, S. Yadavalli, A. J. Sanchez, M. D. Thouless, J. Sakamoto, N. P. Dasgupta, Submitted (2022). [2] A. L. Davis, R. Garcia-Mendez, K. N. Wood, E. Kazyak, K.-H. Chen, G. Teeter, J. Sakamoto, N. P. Dasgupta, J. Mater. Chem. A 8, 6291 (2020). [3] A. L. Davis, E. Kazyak, D. W. Liao, K. N. Wood, N. P. Dasgupta, J. Electrochem. Soc. 168, 070557 (2021).

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Zhao, Nahong, Lijun Fu, Lichun Yang, Tao Zhang, Gaojun Wang, Yuping Wu und Teunis van Ree. „Nanostructured anode materials for Li-ion batteries“. Pure and Applied Chemistry 80, Nr. 11 (01.01.2008): 2283–95. http://dx.doi.org/10.1351/pac200880112283.

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This paper focuses on the latest progress in the preparation of a series of nanostructured anode materials in our laboratory and their electrochemical properties for Li-ion batteries. These anode materials include core-shell structured Si nanocomposites, TiO2 nanocomposites, novel MoO2 anode material, and carbon nanotube (CNT)-coated SnO2 nanowires (NWs). The substantial advantages of these nanostructured anodes provide greatly improved electrochemical performance including high capacity, better cycling behavior, and rate capability.

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Meng, Shirley. „Understanding Li Nucleation and Growth“. ECS Meeting Abstracts MA2023-01, Nr. 22 (28.08.2023): 1580. http://dx.doi.org/10.1149/ma2023-01221580mtgabs.

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Lithium metal anode has been widely studied for next generation lithium metal batteries. Its chemical, electrochemical and mechanical properties are unique as lithium is the lightest metal in the planet earth. In this talk, I will use some of the advanced modeling and characterization methods to probe and understand the lithium metal anode in a rechargeable battery. The tools we developed here will be also useful for other reactive metal anodes such as sodium and zinc.

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Dissertationen zum Thema "Anode Li"

Cen, Yinjie. „Si/C Nanocomposites for Li-ion Battery Anode“. Digital WPI, 2017. https://digitalcommons.wpi.edu/etd-dissertations/468.

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The demand for high performance Lithium-ion batteries (LIBs) is increasing due to widespread use of portable devices and electric vehicles. Silicon (Si) is one of the most attractive candidate anode materials for the next generation LIBs because of its high theoretical capacity (3,578 mAh/g) and low operation potential (~0.4 V vs Li+/Li). However, the high volume change (>300%) during Lithium ion insertion/extraction leads to poor cycle life. The goal of this work is to improve the electrochemical performance of Si/C composite anode in LIBs. Two strategies have been employed: to explore spatial arrangement in micro-sized Si and to use Si/graphene nanocomposites. A unique branched microsized Si with carbon coating was made and demonstrated promising electrochemical performance with a high active material loading ratio of 2 mg/cm2, large initial discharge capacity of 3,153 mAh/g and good capacity retention of 1,133 mAh/g at the 100th cycle at 1/4C current rate. Exploring the spatial structure of microsized Si with its advantages of low cost, easy dispersion, and immediate compatibility with the prevailing electrode manufacturing technology, may indicate a practical approach for high energy density, large-scale Si anode manufacturing. For Si/Graphene nanocomposites, the impact of particle size, surface treatment and graphene quality were investigated. It was found that the electrochemical performance of Si/Graphene anode was improved by surface treatment and use of graphene with large surface area and high defect density. The 100 nm Si/Graphene nanocomposites presented the initial capacity of 2,737 mAh/g and good cycling performance with a capacity of 1,563 mAh/g after 100 cycles at 1/2C current rate. The findings provided helpful insights for design of different types of graphene nanocomposite anodes.

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Gullbrekken, Øystein. „Thermal characterisation of anode materials for Li-ion batteries“. Thesis, Norges teknisk-naturvitenskapelige universitet, Institutt for materialteknologi, 2012. http://urn.kb.se/resolve?urn=urn:nbn:no:ntnu:diva-19224.

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Coin cells with lithium and graphite electrodes were assembled using different combinations of graphite material and electrolyte. Specifically, three commercially available graphite materials and five electrolyte compositions were studied. The cells were discharge-charge cycled with varying parameters in order to determine the performance of the graphite materials and electrolytes. Particularly, a temperature chamber was employed to cycle some cells at temperatures between 0 and 40°C to find the significance of the electrolyte composition and graphite material on the cell performance at these temperatures. The cycled cells were disassembled and samples from the graphite electrode soaked with electrolyte were prepared for thermal analysis, specifically differential scanning calorimetry (DSC). The thermal stability of the graphite electrodes and the influence from the graphite and electrolyte properties and the cycling parameters were analysed. In order to facilitate the interpretation of the results from discharge-charge cycling at different temperatures, DSC analysis from -80 to +50°C was performed on the pure electrolytes.Confirming previous studies, it was found that both the thermal stability and cycling performance were highly influenced by the properties of a solid electrolyte interphase (SEI), situated between the graphite surface and the electrolyte and formed during cycling. The three graphites were good substrates for stable SEI formation, exhibited by high thermal stability after being cycled at room temperature. After cycling with a temperature program, subjecting the cells to temperatures between 0 and 40°C, the thermal stability was generally reduced. This was attributed to increased SEI formation. The properties of both the electrolyte and graphite influenced the SEI and consequent thermal stability, though in different ways.The cell capacity was considerably reduced upon cycling at lower temperatures, such as 10 and 0°C. The results indicate that the electrolyte properties, particularly the viscosity and resulting conductivity, played the most important role in determining the cell performance. Low viscosity electrolyte components should be utilised, maintaining the electrolyte conductivity even at reduced temperatures. The graphite properties did not influence the cell performance at the temperatures studied. Advice is given on which electrolyte components should be avoided to build Li-ion cells performing acceptably at temperatures from 0 to 40°C.

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FUGATTINI, Silvio. „Binder-free porous germanium anode for Li-ion batteries“. Doctoral thesis, Università degli studi di Ferrara, 2019. http://hdl.handle.net/11392/2488081.

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To develop high energy density lithium ion batteries, the use of new electrode materials is required. Germanium is among the possible alternatives to the most commonly used anode, graphite (372 mAh/g), thanks to its four-times higher theoretical gravimetric capacity (1600 mAh/g). Here is presented a two-step method to produce a binder-free porous germanium anode, depositing the semiconductor on metallic substrates by means of Plasma Enhanced Chemical Vapour Deposition (PECVD) and subsequently performing an electrochemical etching with hydrofluoric acid to create a porous structure. The Ge-based electrode attained a capacity of 1250 mAh/g at a current rate of 1C (1C=1600 mA/g) and retained a stable capacity above 1100 mAh/g for more than 1000 cycles tested at different C-rates up to 5C. Both deposition and etching techniques are scalable for industrial production, whose fields of application could be aerospace or medical applications, due to the high cost of germanium as a raw material.
Per sviluppare batterie agli ioni di litio ad alta densità energetica, è necessario l’utilizzo di nuovi materiali elettrodici. Il germanio è una delle possibili alternative all’anodo più comunemente impiegato, la grafite (372 mAh/g), grazie alla sua capacità gravimetrica teorica quattro volte maggiore (1600 mAh/g). In questo lavoro viene presentato un processo in due fasi per realizzare un anodo in germanio poroso privo di legante (binder), realizzando film di semiconduttore su substrati metallici mediante deposizione chimica da fase vapore assisitita da plasma (PECVD) ed effettuando successivamente un attacco elettrochimico con acido fluoridrico per creare una struttura porosa. L’elettrodo in germanio poroso ha raggiunto una capacità di 1250 mAh/g ad una velocità di carica/scarica pari ad 1C (1C = 1600 mA/g) mantenendo, inoltre, una capacità stabilmente superiore a 1100 mAh/g per più di 1000 cicli a diversi C-rate fino a 5C. Sia la tecnica di deposizione che quella di attacco chimico sono scalabili per la produzione industriale, i cui possibili campi di applicazione sono il settore aerospaziale o medico, a causa dell’elevato costo del germanio come materia prima.

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Janíček, Zdeněk. „Stabilita katodového materiálu pro LI-ion akumulátory“. Master's thesis, Vysoké učení technické v Brně. Fakulta elektrotechniky a komunikačních technologií, 2014. http://www.nusl.cz/ntk/nusl-220974.

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This diploma thesis focuses on study of positive electrode materials for Li-Ion batteries. Our aim are intercalation materials whose are really perspective materials whose are widely used in this case. The theoretical part of my thesis focus on basic study of Li-ion batteries and their parameters. We studied charging and discharging processes. AFM and SEM were used as additional techniques for study LiCoO2 a Li0,975K0,025CoO2. We tested lifetime and stability of electrode as a perspective material for electrode for Li-ion batteries.

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Buiel, Edward. „Lithium insertion in hard carbon anode materials for Li-ion batteries“. Thesis, National Library of Canada = Bibliothèque nationale du Canada, 1998. http://www.collectionscanada.ca/obj/s4/f2/dsk2/tape15/PQDD_0013/NQ36573.pdf.

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Mayo, Martin. „Ab initio anode materials discovery for Li- and Na-ion batteries“. Thesis, University of Cambridge, 2018. https://www.repository.cam.ac.uk/handle/1810/270545.

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This thesis uses first principles techniques, mainly the ab initio random structure searching method (AIRSS), to study anode materials for lithium- and sodium- ion batteries (LIBs and NIBs, respectively). Initial work relates to a theoretical structure prediction study of the lithium and sodium phosphide systems in the context of phosphorus anodes as candidates for LIBs and NIBs. The work reveals new Li-P and Na-P phases, some of which can be used to better interpret previous experimental results. By combining AIRSS searches with a high-throughput screening search from structures in the Inorganic Crystal Structure Database (ICSD), regions in the phase diagram are correlated to different ionic motifs and NMR chemical shielding is predicted from first principles. An electronic structure analysis of the Li-P and Na-P compounds is performed and its implication on the anode performance is discussed. The study is concluded by exploring the addition of aluminium dopants to the Li-P compounds to improve the electronic conductivity of the system. The following work deals with a study of tin anodes for NIBs. The structure prediction study yields a variety of new phases; of particular interest is a new NaSn$_2$ phase predicted by AIRSS. This phase plays a crucial role in understanding the alloying mechanism of high-capacity tin anodes, work which was done in collaboration with experimental colleagues. Our predicted theoretical voltages give excellent agreement with the experimental electrochemical cycling curve. First principles molecular dynamics is used to propose an amorphous Na$_1$Sn$_1$ model which, in addition to the newly derived NaSn$_2$ phase, provides help in revealing the electrochemical processes. In the subsequent work, we study Li-Sn and Li-Sb intermetallics in the context of alloy anodes for LIBs. A rich phase diagram of Li-Sn is present, exhibiting a variety of new phases. The calculated voltages show excellent agreement with previously reported cycling measurements and a consistent structural evolution of Li-Sn phases as Li concentration increases is revealed. The study concluded by calculating NMR parameters on the hexagonal- and cubic-Li$_3$Sb phases which shed light on the interpretation of reported experimental data. We conclude with a structure prediction study of the pseudobinary Li-FeS$_2$ system, where FeS$_2$ is considered as a potential high-capacity electrochemical energy storage system. Our first principles calculations of intermediate structures help to elucidate the mechanism of charge storage observed by our experimental collaborators via $\textit{in operando}$ studies.

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Hapuarachchi, Sashini Neushika Sue. „Fabrication and characterization of silicon based electrodes for Li-ion batteries“. Thesis, Queensland University of Technology, 2021. https://eprints.qut.edu.au/207430/1/Sashini_Hapuarachchi_Thesis.pdf.

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This thesis presents the synthesis and characterization of silicon electrodes to address critical challenges in development of high capacity Li-ion batteries. Failure mechanisms of silicon electrodes are investigated at different material length scales and effective strategies are proposed to overcome them, which will benefit in developing high performance next-generation rechargeable Li-ion batteries.

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Vallachira, Warriam Sasikumar Pradeep. „Study of Silicon Oxycarbide(SiOC) as Anode Materials for Li-ion Batteries“. Doctoral thesis, Università degli studi di Trento, 2013. https://hdl.handle.net/11572/368129.

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The principal object of this thesis is the investigation of silicon oxycarbide (SiOC) ceramics as anode material for Li-ion batteries. The investigated materials are prepared by cross linking commercial polymer siloxanes via hydrosylilation reactions or hybrid alkoxide precursors via sol-gel. The cross linked polymer networks are then converted in to ceramic materials by a pyrolysis process in controlled argon atmosphere at 800-1300 Â°C. In details the influence of carbon content on lithium storage properties is addressed for SiOC with the same O/Si atomic ratio of about 1. Detailed structural characterization studies are performed using complementary techniques which aim correlating the electrochemical behavior with the microstructure of the SiOC anodes. Results suggest that SiOC anodes behave as a composite material consisting of a disordered silicon oxycarbide phase having a very high first insertion capacity of ca 1300 mAh g-1 and a free C phase. However, the charge irreversibly trapped into the amorphous silicon oxycarbide network is also high. In consequence the maximum reversible lithium storage capacity of 650 mAh g-1 is measured on high-C content SiOCs with the ratio between amorphous silicon oxycarbide and the free C phase of ï ¾ 1:1. The high carbon content SiOC shows also an excellent cycling stability and performance at high charging/discharging rate with the stable capacity at 2C rate being around 200 mAh g-1. Increasing the pyrolysis temperature has an opposite effect on the low-C and high-C materials: for the latter one the reversible capacity decreases following a known trend while the former shows an increase of xi the reversible capacity which has never been observed before for similar materials. The influence of pyrolysis atmosphere on lithium storage capacity is investigated as well. It is found that pyrolysis in Ar/H2 mixtures, compared to the treatment under pure Ar, results into a decrease of the concentration of C dangling bonds as revealed by electron spin resonance (ESR) measurements. The sample prepared under Ar/H2 mixture shows an excellent cycling stability with an increase in the specific capacity of about 150 mAh g-1 compared to its analogues pyrolysed in pure argon atmosphere. In order to study the role of porosity towards the lithium storage properties, a comparison of dense and porous materials obtained using same starting precursors is made. Porous SiOC ceramics are prepared by HF etching of the SiOC ceramics. HF etching removes a part of the amorphous silica phase from SiOC nanostructure leaving a porous structure. Porous ceramics with surface areas up to 640 m2 g-1 is obtained. The electrochemical charging/discharging results indicate that the porosity can help to increase the lithium storage capacity and it also leads to an enhanced cycling stability. This work demonstrates clearly that silicon oxycarbide (SiOC) ceramics present excellent electrochemical properties to be applied as a promising anode material for lithium storage applications.

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Vallachira, Warriam Sasikumar Pradeep Pradeep. „Study of Silicon Oxycarbide(SiOC) as Anode Materials for Li-ion Batteries“. Doctoral thesis, University of Trento, 2013. http://eprints-phd.biblio.unitn.it/1112/1/PhD_Thesis_Vallachira_Pradeep.pdf.

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The principal object of this thesis is the investigation of silicon oxycarbide (SiOC) ceramics as anode material for Li-ion batteries. The investigated materials are prepared by cross linking commercial polymer siloxanes via hydrosylilation reactions or hybrid alkoxide precursors via sol-gel. The cross linked polymer networks are then converted in to ceramic materials by a pyrolysis process in controlled argon atmosphere at 800-1300 °C. In details the influence of carbon content on lithium storage properties is addressed for SiOC with the same O/Si atomic ratio of about 1. Detailed structural characterization studies are performed using complementary techniques which aim correlating the electrochemical behavior with the microstructure of the SiOC anodes. Results suggest that SiOC anodes behave as a composite material consisting of a disordered silicon oxycarbide phase having a very high first insertion capacity of ca 1300 mAh g-1 and a free C phase. However, the charge irreversibly trapped into the amorphous silicon oxycarbide network is also high. In consequence the maximum reversible lithium storage capacity of 650 mAh g-1 is measured on high-C content SiOCs with the ratio between amorphous silicon oxycarbide and the free C phase of  1:1. The high carbon content SiOC shows also an excellent cycling stability and performance at high charging/discharging rate with the stable capacity at 2C rate being around 200 mAh g-1. Increasing the pyrolysis temperature has an opposite effect on the low-C and high-C materials: for the latter one the reversible capacity decreases following a known trend while the former shows an increase of xi the reversible capacity which has never been observed before for similar materials. The influence of pyrolysis atmosphere on lithium storage capacity is investigated as well. It is found that pyrolysis in Ar/H2 mixtures, compared to the treatment under pure Ar, results into a decrease of the concentration of C dangling bonds as revealed by electron spin resonance (ESR) measurements. The sample prepared under Ar/H2 mixture shows an excellent cycling stability with an increase in the specific capacity of about 150 mAh g-1 compared to its analogues pyrolysed in pure argon atmosphere. In order to study the role of porosity towards the lithium storage properties, a comparison of dense and porous materials obtained using same starting precursors is made. Porous SiOC ceramics are prepared by HF etching of the SiOC ceramics. HF etching removes a part of the amorphous silica phase from SiOC nanostructure leaving a porous structure. Porous ceramics with surface areas up to 640 m2 g-1 is obtained. The electrochemical charging/discharging results indicate that the porosity can help to increase the lithium storage capacity and it also leads to an enhanced cycling stability. This work demonstrates clearly that silicon oxycarbide (SiOC) ceramics present excellent electrochemical properties to be applied as a promising anode material for lithium storage applications.

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VERSACI, DANIELE. „Materials for high energy Li-ion and post Li-ion batteries“. Doctoral thesis, Politecnico di Torino, 2021. http://hdl.handle.net/11583/2896992.

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Bücher zum Thema "Anode Li"

Mogensen, Mogens. Kinetics of LiCl Film Formation on Li Anodes in SOCl2. Roskilde, Denmark: Riso National Laboratory, 1987.

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Buchteile zum Thema "Anode Li"

Hassan, Afaq, Saima Nazir, M. Sagir, Tausif Ahmad und M. B. Tahir. „Metallic Li Anode: An Introduction“. In Lithium-Sulfur Batteries: Key Parameters, Recent Advances, Challenges and Applications, 169–86. Singapore: Springer Nature Singapore, 2024. http://dx.doi.org/10.1007/978-981-99-2796-8_10.

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Hien Nguyen, Thi Dieu, Hai Duong Pham, Shih-Yang Lin, Ngoc Thanh Thuy Tran und Ming-Fa Lin. „Fundamental Properties of Li+-Based Battery Anode“. In Lithium-Ion Batteries and Solar Cells, 59–77. First edition. | Boca Raton, FL : CRC Press/ Taylor & Francis Group, LLC, 2021.: CRC Press, 2020. http://dx.doi.org/10.1201/9781003138327-4.

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Samaras, I., L. Tsiakiris, S. Kokkou, O. Valassiades und Th Karakostas. „Li-Si System Studies as Possible Anode For Li-Ion Batteries“. In New Trends in Intercalation Compounds for Energy Storage, 597–600. Dordrecht: Springer Netherlands, 2002. http://dx.doi.org/10.1007/978-94-010-0389-6_55.

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Pribat, Didier. „Silicon nanowires for Li-based battery anode applications“. In Silicon Nanomaterials Sourcebook, 455–74. Boca Raton, FL: CRC Press, Taylor & Francis Group, [2017] | Series: Series in materials science and engineering: CRC Press, 2017. http://dx.doi.org/10.4324/9781315153544-23.

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Kim, Chan, und Morinobu Endo. „Anode Performance of the Li-Ion Secondary Battery“. In Design and Control of Structure of Advanced Carbon Materials for Enhanced Performance, 255–75. Dordrecht: Springer Netherlands, 2001. http://dx.doi.org/10.1007/978-94-010-1013-9_15.

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Tsurumaki, Akiko, Sergio Brutti, Giorgia Greco und Maria Assunta Navarra. „Closed Battery Systems“. In The Materials Research Society Series, 173–211. Cham: Springer International Publishing, 2024. http://dx.doi.org/10.1007/978-3-031-48359-2_10.

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AbstractBattery technologies are expected to strongly contribute to the global energy storage industry and market. Among the several promising battery technologies, Li-metal batteries, all-solid-state Li batteries, and beyond-lithium systems are discussed in this chapter. Li metal represents a key anode material for boosting the energy density of batteries, but the formation of Li dendrites limits a safe and stable function of the system. The use of solid-state electrolytes allows a safer battery operation, by limiting the electrolyte flammability and dendrite formation, yet the performance is insufficient because of slower kinetics of the lithium ion. Possible solutions against these critical problems, especially through the discovery of new materials, are here discussed. Moreover, other innovative technologies based on Na, Ca, and Mg, so-called beyond-lithium batteries, are presented. Insights into these emerging battery systems, as well as a series of issues that came up with the replacement of lithium, are described in this chapter. Focus is particularly placed on development of battery materials with different perspectives, including performance, stability, and sustainability.

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Kang, Chiwon, Indranil Lahiri, Rangasamy Baskaran, Mansoo Choi, Won-Gi Kim, Yang-Kook Sun und Wonbong Choi. „3D Multiwall Carbon Nanotubes (MWCNTs) for Li-Ion Battery Anode“. In Supplemental Proceedings, 35–41. Hoboken, NJ, USA: John Wiley & Sons, Inc., 2012. http://dx.doi.org/10.1002/9781118357002.ch5.

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Nguyen-Huu, T., und Q. Le-Minh. „Stress Analysis of Silicon-Based Anode in Li-Ion Battery“. In Proceedings of the International Conference on Advances in Computational Mechanics 2017, 95–104. Singapore: Springer Singapore, 2018. http://dx.doi.org/10.1007/978-981-10-7149-2_7.

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Wang, Heng, Bing Li und Zuxin Zhao. „Electrodeposited Si-Al Thin Film as Anode for Li Ion Batteries“. In TMS 2014: 143rd Annual Meeting & Exhibition, 891–97. Cham: Springer International Publishing, 2014. http://dx.doi.org/10.1007/978-3-319-48237-8_105.

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Wang, Heng, Bing Li und Zuxin Zhao. „Electrodeposited Si-Al Thin Film as Anode for Li Ion Batteries“. In TMS 2014 Supplemental Proceedings, 891–97. Hoboken, NJ, USA: John Wiley & Sons, Inc., 2014. http://dx.doi.org/10.1002/9781118889879.ch105.

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Konferenzberichte zum Thema "Anode Li"

Hess, Robert, Jeff Britt, Joshua Stewart und Mark Niedzwiecki. „Use of a High Energy-Dense Li Anode Cell for an eVTOL Application“. In Vertical Flight Society 76th Annual Forum & Technology Display. The Vertical Flight Society, 2020. http://dx.doi.org/10.4050/f-0076-2020-16406.

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Electric vertical take-off and landing (eVTOL) aircraft require sufficient electric energy to complete their missions and sufficient electric power for hover conditions (including standard and degraded modes of operation). When using current battery technology, the energy storage system constitutes a significant portion of the vehicle mass, thereby significantly limiting vehicle performance. Advanced cell technologies using solid lithium (Li) anode technology have the potential to increase energy density as compared to traditional cell-based on graphite anodes. Efforts to develop battery solutions using Li anode technology for an eVTOL application demonstrate reduced battery weight while achieving near-term performance objectives.

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Liu, Teng, Xiao-Guang Yang und Chao-Yang Wang. „Discovery and Development of a Fast Charging Li-Ion Battery“. In ASME 2018 International Mechanical Engineering Congress and Exposition. American Society of Mechanical Engineers, 2018. http://dx.doi.org/10.1115/imece2018-87661.

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Enabling fast charging of Li-ion batteries (LiB) is essential for mainstream adoption of electric vehicles (EVs). A critical challenge to fast charging is lithium plating, which can lead to drastic capacity loss and safety risks. Fundamentally, fast charging is restricted by anode surface reaction kinetics, lithium diffusion in anode solid particles and Li+ diffusion and conduction in electrolyte. In this work, we present an analysis of the contributions of these different physicochemical processes to the total overpotential during fast charging, using an electrochemical-thermal (ECT) coupled model. Special attention is paid to the effect of increasing electrode thickness, a common approach for raising energy density of EV cells, on fast charging capability. It is found that lithium plating is more prone to occur in thicker anodes due to larger electrolyte transport resistance. Furthermore, we present a novel approach of thermal stimulation to enable 10-minutes (6C rate) fast charging of an EV cell with 170Wh/kg energy density.

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Wu, James J., und William R. Bennett. „Fundamental investigation of Si anode in Li-Ion cells“. In 2012 IEEE Energytech. IEEE, 2012. http://dx.doi.org/10.1109/energytech.2012.6304667.

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Li, Hong, Lihong Shi, Wei Lu, Xuejie Huang und Liquan Chen. „Nanosized alloy-based anode materials for Li ion batteries“. In Proceedings of the 7th Asian Conference. WORLD SCIENTIFIC, 2000. http://dx.doi.org/10.1142/9789812791979_0052.

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Sharma, N., K. M. Shaju, G. V. Subba Rao und B. V. R. Chowdari. „CaSnO3: a high capacity anode material for Li-ion batteries“. In Proceedings of the 8th Asian Conference. WORLD SCIENTIFIC, 2002. http://dx.doi.org/10.1142/9789812776259_0011.

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Purwanto, Agus, Endah Dyartanti, Inayati, Wahyudi Sutopo und Muhammad Nizam. „Synthesis of titania for anode material of Li-Ion battery“. In 2013 Joint International Conference on Rural Information & Communication Technology and Electric-Vehicle Technology (rICT & ICeV-T). IEEE, 2013. http://dx.doi.org/10.1109/rict-icevt.2013.6741524.

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Gavrilin, Ilya, Timofey Savchuk, Alexey Dronov und Tatiana Kulova. „TiO2 nanotubular arrays as anode materials for li-ion batteries“. In 2017 IEEE Conference of Russian Young Researchers in Electrical and Electronic Engineering (EIConRus). IEEE, 2017. http://dx.doi.org/10.1109/eiconrus.2017.7910830.

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Lou, Xiong Wen (David). „Metal Oxide based Nanostructured Anode Materials for Li-ion Batteries“. In 14th Asia Pacific Confederation of Chemical Engineering Congress. Singapore: Research Publishing Services, 2012. http://dx.doi.org/10.3850/978-981-07-1445-1_543.

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Arro, Christian, Assem Mohamed und Nasr Bensalah. „Germanium Oxide/germanium/ reduced Graphene (GeO2/Ge/r-GO) Hybrid Composite Anodes for Lithium-ion Batteries: Effect of Ge loading on Electrochemical Performance“. In Qatar University Annual Research Forum & Exhibition. Qatar University Press, 2021. http://dx.doi.org/10.29117/quarfe.2021.0065.

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Hybrid composites between Germanium (Ge) and carbonaceous materials are promising anode materials for Li-ion batteries (LIBs). The mitigation of reduced cycling ability and rate capability allows for the unhindered benefit of higher capacities in Ge-based anodes. Here, the effect of Ge mass loading on the electrochemical performance of GeO2/Ge/r-GO composites was evaluated as LIBs anode. GeO2/Ge/r-GO composites were synthesized by controlled microwave radiation of ball-milled Ge and sonicated dispersion of graphene oxide (GO). The composite anode at Ge 25% showed greatest cycling retention with 91% after 100 cycles and an average specific capacity of 300 mAh/g (1600 mAh/g Ge). At 75% Ge mass loading the anode suffered with limited cycling retention of 57.5% at the cost of greater specific capacities. The composite at 50% Ge attained advantageous characteristics of both composites with a stable cycling performance of 71.4% after 50 cycles and an average specific capacity of 400 mAh/g (1067 mAh/g Ge). These findings can be used to shape high-energy Ge-based anodes and guide future development in energy storage.

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Idrissi, Siham, Zineb Edfouf, Omar Benabdallah, Abdelfettah Lallaoui und Fouzia Cherkaoui El Moursli. „Tin Phosphite SnHPO3 a New Anode Material for Li-ion Batteries“. In 2018 6th International Renewable and Sustainable Energy Conference (IRSEC). IEEE, 2018. http://dx.doi.org/10.1109/irsec.2018.8702926.

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Berichte der Organisationen zum Thema "Anode Li"

Lake, Carla. High performance anode for advanced Li batteries. Office of Scientific and Technical Information (OSTI), November 2015. http://dx.doi.org/10.2172/1224711.

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B. Fultz. Anode Materials for Rechargeable Li-Ion Batteries. Office of Scientific and Technical Information (OSTI), Januar 2001. http://dx.doi.org/10.2172/773359.

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Herle, Subra, und Ajey Joshi. Advanced Anode Manufacturing through Ultra-Thin Li Deposition. Office of Scientific and Technical Information (OSTI), April 2024. http://dx.doi.org/10.2172/2341379.

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White, Ralph E., und Branko N. Popov. Synthesis, Characterization and Testing of Novel Anode and Cathode Materials for Li-Ion Batteries. Office of Scientific and Technical Information (OSTI), Oktober 2002. http://dx.doi.org/10.2172/900477.

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Dr. Malgorzata Gulbinska. Composit, Nanoparticle-Based Anode material for Li-ion Batteries Applied in Hybrid Electric (HEV's). Office of Scientific and Technical Information (OSTI), August 2009. http://dx.doi.org/10.2172/962928.

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Gross, M. E., E. S. Mast, J. P. Lemmon und R. L. Pearson III. Development of an Anode Stabilization Layer for High Energy Li-S Cells for Electric Vehicles. Office of Scientific and Technical Information (OSTI), März 2012. http://dx.doi.org/10.2172/1038137.

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Gratz, Eric. Recovery of High Value Anode Materials for a Closed Loop Li-ion Battery Recycling Process (Final Report). Office of Scientific and Technical Information (OSTI), April 2020. http://dx.doi.org/10.2172/1614871.

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Visco, Steven J. Advanced Lithium Anodes for Li/Air and Li/Water Batteries. Fort Belvoir, VA: Defense Technical Information Center, Oktober 2005. http://dx.doi.org/10.21236/ada441240.

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WANG, DONGHAI, und TIEN DUONG. Electrochemically Responsive Self-Formed Li-ion Conductors for High Performance Li Metal Anodes. Office of Scientific and Technical Information (OSTI), Dezember 2019. http://dx.doi.org/10.2172/1579536.

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Mikhaylik, Yuriy. Protection of Lithium (Li) Anodes Using Dual Phase Electrolytes. Office of Scientific and Technical Information (OSTI), September 2014. http://dx.doi.org/10.2172/1368169.

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